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41 result(s) for "Foret, Gilles"
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The unintended consequence of SO2 and NO2 regulations over China: increase of ammonia levels and impact on PM2.5 concentrations
Air pollution reaching hazardous levels in many Chinese cities has been a major concern in China over the past decades. New policies have been applied to regulate anthropogenic pollutant emissions, leading to changes in atmospheric composition and in particulate matter (PM) production. Increasing levels of atmospheric ammonia columns have been observed by satellite during recent years. In particular, observations from the Infrared Atmospheric Sounding Interferometer (IASI) reveal an increase of these columns by 15 % and 65 % from 2011 to 2013 and 2015, respectively, over eastern China. In this paper we performed model simulations for 2011, 2013 and 2015 in order to understand the origin of this increase and to quantify the link between ammonia and the inorganic components of particles: NH4(p)+/SO4(p)2-/NO3(p)-. Interannual change of meteorology can be excluded as a reason: year 2015 meteorology leads to enhanced sulfate production over eastern China, which increases the ammonium and decreases the ammonia content, which is contrary to satellite observations. Reductions in SO2 and NOx emissions from 2011 to 2015 of 37.5 % and 21 % respectively, as constrained from satellite data, lead to decreased inorganic matter (by 14 % for NH4(p)++SO4(p)2-+NO3(p)-). This in turn leads to increased gaseous NH3(g) tropospheric columns by as much as 24 % and 49 % (sampled corresponding to IASI data availability) from 2011 to 2013 and 2015 respectively and thus can explain most of the observed increase.
An investigation on the origin of regional springtime ozone episodes in the western Mediterranean
For the identification of regional springtime ozone episodes, rural European Monitoring and Evaluation Programme (EMEP) ozone measurements from countries surrounding the western Mediterranean (Spain, France, Switzerland, Italy, Malta) have been examined with emphasis on periods of high ozone-mixing ratios, according to the variation of the daily afternoon (12:00–18:00) ozone values. For two selected high ozone episodes in April and May 2008, composite NCEP/NCAR reanalysis maps of various meteorological parameters and/or their anomalies (geopotential height, specific humidity, vertical wind velocity omega, vector wind speed and temperature) at various tropospheric pressure levels have been examined together with the corresponding satellite Infrared Atmospheric Sounding Interferometer (IASI) ozone measurements (at 3 and 10 km), CHIMERE simulations, vertical ozone soundings and HYSPLIT back trajectories. The observations show that high ozone values are detected in several countries simultaneously over several days. Also, the examined spring ozone episodes over the western Mediterranean and in central Europe are linked to synoptic meteorological conditions very similar to those recently observed in summertime ozone episodes over the eastern Mediterranean (Kalabokas et al., 2013, 2015; Doche et al., 2014), where the transport of tropospheric ozone-rich air masses through atmospheric subsidence significantly influences the boundary layer and surface ozone-mixing ratios. In particular, the geographic areas with observed tropospheric subsidence seem to be the transition regions between high-pressure and low-pressure systems. During the surface ozone episodes IASI satellite measurements show extended areas of high ozone in the lower- and upper-troposphere over the low-pressure system areas, adjacent to the anticyclones, which influence significantly the boundary layer and surface ozone-mixing ratios within the anticyclones by subsidence and advection in addition to the photochemically produced ozone there, resulting in exceedances of the 60 ppb standard.
Impacts of regional climate change on air quality projections and associated uncertainties
A 2-degree global warming is likely to affect the production, deposition, and transport of air pollutants, leading to impacts on air quality and health. In the present study we use an ensemble of four regional chemistry-transport models, driven by meteorological data from different climate models, to assess such changes and their uncertainties for PM2.5 and SOMO35. Changes and uncertainties are compared to the inter-model variability. We find that the impact of regional climate change on PM2.5, averaged over the model ensemble, ranges from −0.5 μg.m −3 to +1.3 μg.m −3 over Europe. It mainly results from changes in natural and biogenic emissions, such as desert dust, sea salt and biogenic VOCs. Statistically significant decreases in PM2.5 are found over southwestern Russia and Ukraine as well as an increase over Southern Spain. Modeled changes in summer ozone levels range from −1.7 to 1.6 ppbv. We find a smaller ensemble-mean evolution of SOMO35 as compared to inter-model variability. We also investigate the uncertainty due to inter-decadal variability and find that 10-year periods may not be sufficient to allow the detection of statistically significant change signals.
Air Quality Degradation by Mineral Dust over Beijing, Chengdu and Shanghai Chinese Megacities
Air pollution in Chinese megacities has reached extremely hazardous levels, and human activities are responsible for the emission or production of large amounts of particulate matter (PM). In addition to PM from anthropogenic sources, natural phenomena, such as dust storms over Asian deserts, may also emit large amounts of PM, which lead episodically to poor air quality over Chinese megacities. In this paper, we quantify the degradation of air quality by dust over Beijing, Chengdu and Shanghai megacities using the three dimensions (3D) chemistry transport model CHIMERE, which simulates dust emission and transport online. In the first part of our work, we evaluate dust emissions using Moderate Resolution Imaging Spectroradiometer (MODIS) and Infrared Atmospheric Sounding Interferometer (IASI) satellite observations of aerosol optical depth, respectively, in the visible and the thermal infrared over source areas. PM simulations were also evaluated compared to surface monitoring stations. Then, mineral dust emissions and their impacts on particle composition of several Chinese megacities were analyzed. Dust emissions and transport over China were simulated during three years (2011, 2013 and 2015). Annual dust contributions to the PM 10 budget over Beijing, Chengdu and Shanghai were evaluated respectively as 6.6%, 9.5% and 9.3%. Dust outbreaks largely contribute to poor air quality events during springtime. Indeed it was found that dust significantly contribute for 22%, 52% and 43% of spring PM 10 events (for Beijing, Chengdu and Shanghai respectively).
Understanding the Simulated Ammonia Increasing Trend from 2008 to 2015 over Europe with CHIMERE and Comparison with IASI Observations
The objective of this study is to assess and understand the NH3 recent trends and to identify the key components driving its concentrations. We have simulated the seasonal cycle, the interannual variability, and the trends in NH3 vertical column densities (VCD) from 2008 to 2015 over Europe, with the CHIMERE regional chemistry–transport model. We have also confronted the simulations against the Infrared Atmospheric Sounding Interferometer (IASI) satellite observations. IASI often shows a strong maximum in summer in addition to the spring peak, whereas CHIMERE only shows a slight peak in summer some years. This result could point to a misrepresentation of the temporal profile of the NH3 emissions, i.e., to missing emission sources during summertime either due to more than expected fertilizer use or to increased volatilization under warmer conditions. The simulated NH3 VCDs present an increasing trend over continental Europe (+2.7 ± 1.0 %/yr) but also at the national scale for Spain, Germany, UK, France, and Poland. Sensitivity tests indicate that these simulated positive trends are mainly due to (i) the trends in NH3 emissions, found heterogeneous in the EMEP NH3 emissions with strong disparities depending on the country, and (ii) the negative trends in NOx and SOx emissions. The impact of reductions in NO2 and SO2 emissions on NH3 concentrations should therefore be taken into account in future policies. This simulated NH3 VCD increase at the European scale is confirmed by IASI-v3R satellite observations in spring and summer, when ammonia emissions strongly contribute to the annual budget in accordance with crop requirements. Nevertheless, there are remaining differences about the significance and magnitude between the simulated and observed trends at the national scale, and it warrants further investigation.
Experimental Testing of Passive Linear TMD for Postural Tremor Attenuation
Research interest to provide a mechanical solution for involuntary tremors is increasing due to the severe side effects caused by the medications used to lessen its symptoms. This paper deals with the design of a cantilever-type tuned mass damper (TMD) used to prove the effectiveness of passive controllers in reducing the involuntary tremor’s vibrational signals transmitted by the muscles to the hand segment. TMD is tested on an experimental arm, reflecting the flexion-extension motion of the wrist, excited by a mechanical shaker with the measured tremor signal of a patient with essential tremor. The designed TMD provides a new operational frequency for each position of the screw fixed to its beam. Modal damping ratios are also calculated using different methods for each position. The effectiveness of the TMD is quantified by measurements using a vibrometer and inertial measurement unit. Three TMDs, representing 15.7% total mass ratio, cause a reduction of 29% for the acceleration, 69% for the velocity, 79% for the displacement, 67% for the angular velocity, and 82% for the angular displacement signals. These encouraging results will allow the improvement of the design of the passive controller in the form of a wearable bracelet suitable for daily life.
Calculation of dynamic responses of railway sleepers on a nonlinear foundation
The safety of a passing train depends on different factors, of which one of the most important is the behavior of the foundation. Therefore, the effects of the nonlinearity of ballast on the dynamic responses of the railway track are a key research interest. In this paper, a new model of railway sleepers posed on a nonlinear foundation has been developed. By coupling the finite element method (FEM) of the sleeper with an analytical model of the periodically supported beam model, the dynamic equation of the sleeper is developed. On the other hand, by considering a periodic series of moving loads, this equation can be transformed to a forced nonlinear oscillation. Iteration procedures have been built to calculate the periodic solution. This method has demonstrated a good convergence of results by comparison with the analytical solution in the linear case. The influence of the nonlinear foundation has been investigated by two examples: cubic-nonlinear and bi-linear foundations. The parametric studies demonstrate that numerical results converge with a small number of iterations.
Paris air quality monitoring for the 2024 Olympics and Paralympics: focus on air pollutants and pollen
BackgroundExposure to air pollution can affect the health of individuals with respiratory disease, but may also impede the health and performance of athletes. This is potentially relevant for people travelling to and competing in the Olympic and Paralympic Games (OPG) in Paris. We describe anticipated air quality in Paris based on historical monitoring data and describe the impact of the process on the development of monitoring strategies for future international sporting events.MethodsAir pollutant data for July to September 2020–2023 and pollen data for 2015–2022 were provided by Airparif (particulate matter (PM2.5), nitrogen dioxide (NO2) and ozone (O3)) and RNSA stations in the Paris region. Airparif’s street-level numerical modelling provided spatial data for the OPG venues.ResultsThe maximum daily mean PM2.5 was 11±6 µg/m3 at traffic stations, below the WHO recommended daily air quality threshold (AQT). Daily NO2 concentrations ranged from 5±3 µg/m3 in rural areas to 17±14 µgm3 in urban areas. Near traffic stations, this rose to 40±24 µg/m3 exceeding the WHO AQT. Both peaked around 06:00 and 20:00 UTC (coordinated universal time). The ambient O3 level exceeded the AQT on 20 days per month and peaked at 14:00 UTC. The main allergenic taxa from June to September was Poaceae (ie, grass pollen variety).ConclusionAir pollutant levels are expected to be within accepted air quality thresholds at the Paris OPG. However, O3 concentrations may be significantly raised in very hot and clear conditions and grass pollen levels will be high, prompting a need to consider and manage this risk in susceptible individuals.
Aerosol optical depth climatology from the high-resolution MAIAC product over Europe: differences between major European cities and their surrounding environments
The aerosol optical depth (AOD) is a derived measurement useful to investigate the aerosol load and its distribution at different spatio-temporal scales. In this work we use long-term (2000–2021) MAIAC (Multi-Angle Implementation of Atmospheric Correction) retrievals with 1 km resolution to investigate the climatological AOD variability and trends at different scales in Europe: a continental (30–60∘ N, 20∘ W–40∘ E), a regional (100 × 100 km2) and an urban–local scale (3 × 3 km2). The AOD climatology at the continental scale shows the highest values during summer (JJA) and the lowest during winter (DJF) seasons. Regional and urban–local scales are investigated for 21 cities in Europe, including capitals and large urban agglomerations. Analyses show AOD average (550 nm) values between 0.06 and 0.16 at the urban–local scale while also displaying a strong north–south gradient. This gradient corresponds to a similar one in the European background, with higher AOD being located over the Po Valley, the Mediterranean Basin and eastern Europe. Average enhancements of the local with respect to regional AOD of 57 %, 55 %, 39 % and 32 % are found for large metropolitan centers such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions. Negative average deviations are observed for other cities, such as Amsterdam (−17 %) and Brussels (−6 %), indicating higher regional background signal and suggesting a heterogeneous aerosol spatial distribution that conceals the urban–local signal. Finally, negative statistically significant AOD trends for the entire European continent are observed. A stronger decrease rate at the regional scale with respect to the local scale occurs for most of the cities under investigation.
Paris air quality monitoring for the 2024 Olympics and Paralympics: focus on air pollutants and pollen
Background Exposure to air pollution can affect the health of individuals with respiratory disease, but may also impede the health and performance of athletes. This is potentially relevant for people travelling to and competing in the Olympic and Paralympic Games (OPG) in Paris. We describe anticipated air quality in Paris based on historical monitoring data and describe the impact of the process on the development of monitoring strategies for future international sporting events. Methods Air pollutant data for July to September 2020–2023 and pollen data for 2015–2022 were provided by Airparif (particulate matter (PM 2.5 ), nitrogen dioxide (NO 2 ) and ozone (O 3 )) and RNSA stations in the Paris region. Airparif’s street-level numerical modelling provided spatial data for the OPG venues. Results The maximum daily mean PM 2.5 was 11±6 µg/m 3 at traffic stations, below the WHO recommended daily air quality threshold (AQT). Daily NO 2 concentrations ranged from 5±3 µg/m 3 in rural areas to 17±14 µgm 3 in urban areas. Near traffic stations, this rose to 40±24 µg/m 3 exceeding the WHO AQT. Both peaked around 06:00 and 20:00 UTC (coordinated universal time). The ambient O 3 level exceeded the AQT on 20 days per month and peaked at 14:00 UTC. The main allergenic taxa from June to September was Poaceae (ie, grass pollen variety). Conclusion Air pollutant levels are expected to be within accepted air quality thresholds at the Paris OPG. However, O 3 concentrations may be significantly raised in very hot and clear conditions and grass pollen levels will be high, prompting a need to consider and manage this risk in susceptible individuals.