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Superstrong, superstiff, and conductive alginate hydrogels
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Journal Article
Superstrong, superstiff, and conductive alginate hydrogels
2022
Overview
For the practical use of synthetic hydrogels as artificial biological tissues, flexible electronics, and conductive membranes, achieving requirements for specific mechanical properties is one of the most prominent issues. Here, we demonstrate superstrong, superstiff, and conductive alginate hydrogels with densely interconnecting networks implemented via simple reconstructing processes, consisting of anisotropic densification of pre-gel and a subsequent ionic crosslinking with rehydration. The reconstructed hydrogel exhibits broad ranges of exceptional tensile strengths (8–57 MPa) and elastic moduli (94–1,290 MPa) depending on crosslinking ions. This hydrogel can hold sufficient cations (e.g., Li
+
) within its gel matrix without compromising the mechanical performance and exhibits high ionic conductivity enough to be utilized as a gel electrolyte membrane. Further, this strategy can be applied to prepare mechanically outstanding, ionic-/electrical-conductive hydrogels by incorporating conducting polymer within the hydrogel matrix. Such hydrogels are easily laminated with strong interfacial adhesion by superficial de- and re-crosslinking processes, and the resulting layered hydrogel can act as a stable gel electrolyte membrane for an aqueous supercapacitor.
Specific mechanical properties are one of the most important issues for application of synthetic hydrogels as biological tissue, flexible electronics or in conductive membranes. Here, the authors demonstrate that a reconstruction process consisting of anisotropic densification of pre-gel and subsequent ionic crosslinking and rehydration leads to strong, stiff, and conductive alginate hydrogels with densely interconnecting networks.
Publisher
Nature Publishing Group UK,Nature Publishing Group,Nature Portfolio
Subject
