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Simultaneous Removal of NO.sub.x and Toluene on CuMnMgAl Layered Double Oxides
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Simultaneous Removal of NO.sub.x and Toluene on CuMnMgAl Layered Double Oxides
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Journal Article
Simultaneous Removal of NO.sub.x and Toluene on CuMnMgAl Layered Double Oxides
2024
Overview
In this study, pure phase Cu.sub.2.5Mn.sub.0.5MgAl precursor was synthesized by layered double hydroxides (LDHs) precursor template method. Subsequently, Cu.sub.2.5Mn.sub.0.5MgAl-LDH is calcined at 500, 600 and 700 â to obtain the corresponding layered double oxides (LDO) catalysts for simultaneous removal of NO.sub.x and toluene. The results show that Cu.sub.2.5Mn.sub.0.5MgAl-500 exhibits the best catalytic performance in both NO.sub.x reduction and toluene oxidation reactions and the conversion of NO.sub.x and toluene can reach 85% and 88% at 210 â, respectively. XRD, SEM, BET, NH.sub.3-TPD, H.sub.2-TPR, XPS and in situ DRIFT were applied to characterize the prepared catalysts. The obtained Cu.sub.2.5Mn.sub.0.5MgAl-500 has abundant acid sites, excellent redox capacity and the highest concentration of surface Mn.sup.4+ and Cu.sup.+ species, which are considered to be the main factors determining its excellent catalytic performance. In addition, Cu.sub.2.5Mn.sub.0.5MgAl-500 shows superior durability and good tolerance to H.sub.2O/SO.sub.2.
Publisher
Springer
Subject
