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141 result(s) for "Amann, Markus"
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Electrically tunable nonlinear polaritonic metasurface
Nonlinear polaritonic metasurfaces created by the coupling of intersubband nonlinearities in semiconductor heterostructures with optical modes in nanoresonators have recently demonstrated efficient frequency mixings at very low pumping intensities of the order of a few tens of kilowatts per square centimetre. In these subwavelength structures, the efficiency, spectral bandwidth and local nonlinear phase of wave mixing do not depend on phase matching but only on the nonlinear response of the constituent meta-atoms. We exploit this property to demonstrate an electrically tunable nonlinear metasurface that combines a plasmonic nanocavity and a quantum-engineered semiconductor heterostructure, in which the magnitude and phase of the local nonlinear responses are controlled by a bias voltage through the quantum-confined Stark effect. We demonstrate spectral tuning, dynamic intensity modulation and dynamic beam manipulation for second-harmonic generation. Our work suggests a route for electrically reconfigurable flat nonlinear optical elements with versatile functionalities.By coupling plasmonic resonators with a semiconductor heterostructure, researchers control the nonlinear response by a bias voltage, thereby enabling spectral tuning, dynamic intensity modulation and dynamic beam manipulation for second-harmonic generation.
Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions
Multiple-quantum-well semiconductors can provide one of the largest known nonlinear material responses, which is, however, geometrically limited to light beams polarized perpendicular to the semiconductor layers; by coupling a plasmonic metasurface to the semiconductor heterostructure, this limitation can be lifted, opening a new path towards ultrathin planarized components with large nonlinear response. A new angle on nonlinear optics Multiple-quantum-well semiconductor heterostructures have been engineered to generate useful nonlinear optical responses that far exceed those of traditional nonlinear optical materials. But their range of applicability is geometrically limited as they require that the incident light be polarized perpendicular to the semiconductor layers. Jongwon Lee et al . now show that, by coupling a plasmonic metasurface to the semiconductor heterostructure, this geometrical limitation can be removed, thereby lifting the orientation restrictions on the use of these nonlinear optical elements. Intersubband transitions in n-doped multi-quantum-well semiconductor heterostructures make it possible to engineer one of the largest known nonlinear optical responses in condensed matter systems—but this nonlinear response is limited to light with electric field polarized normal to the semiconductor layers 1 , 2 , 3 , 4 , 5 , 6 , 7 . In a different context, plasmonic metasurfaces (thin conductor–dielectric composite materials) have been proposed as a way of strongly enhancing light–matter interaction and realizing ultrathin planarized devices with exotic wave properties 8 , 9 , 10 , 11 . Here we propose and experimentally realize metasurfaces with a record-high nonlinear response based on the coupling of electromagnetic modes in plasmonic metasurfaces with quantum-engineered electronic intersubband transitions in semiconductor heterostructures. We show that it is possible to engineer almost any element of the nonlinear susceptibility tensor of these structures, and we experimentally verify this concept by realizing a 400-nm-thick metasurface with nonlinear susceptibility of greater than 5 × 10 4 picometres per volt for second harmonic generation at a wavelength of about 8 micrometres under normal incidence. This susceptibility is many orders of magnitude larger than any second-order nonlinear response in optical metasurfaces measured so far 12 , 13 , 14 , 15 . The proposed structures can act as ultrathin highly nonlinear optical elements that enable efficient frequency mixing with relaxed phase-matching conditions, ideal for realizing broadband frequency up- and down-conversions, phase conjugation and all-optical control and tunability over a surface.
The 2020 report of The Lancet Countdown on health and climate change: responding to converging crises
For the Chinese, French, German, and Spanish translations of the abstract see Supplementary Materials section.TRANSLATIONSFor the Chinese, French, German, and Spanish translations of the abstract see Supplementary Materials section.
The 2018 report of the Lancet Countdown on health and climate change: shaping the health of nations for centuries to come
The report draws on world-class expertise from climate scientists, ecologists, mathematicians, geographers, engineers, energy, food, livestock, and transport experts, economists, social and political scientists, public health professionals, and doctors. The Lancet Countdown's work builds on decades of research in this field, and was first proposed in the 2015 Lancet Commission on health and climate change,1 which documented the human impacts of climate change and provided ten global recommendations to respond to this public health emergency and secure the public health benefits available (panel 1). The following four key messages derive from the Lancet Countdown's 2018 report Present day changes in heat waves, labour capacity, vector-borne disease, and food security provide early warning of the compounded and overwhelming impact on public health that are expected if temperatures continue to rise. Correspondingly, global subsidies for fossil fuels continued to decrease, and carbon pricing only covers 13·1% of global greenhouse-gas emissions, a number that is expected to increase to more than 20% when planned legislation in China is implemented in late 2018 (indicators 4.6 and 4.7).
Short-lived climate pollutant mitigation and the Sustainable Development Goals
The post-2015 development agenda is dominated by a set of Sustainable Development Goals (SDGs) that arose from the 2012 Rio+20 United Nations Conference on Sustainable Development. The 17 goals and 169 targets address diverse and intersecting aspects of human and environmental needs and challenges. Achieving the SDGs by 2030 requires implementing coordinated and concerted strategies and actions that minimize potential trade-offs and conflicts and maximize synergies to contribute to multiple SDGs. Measures to mitigate emissions of short-lived climate pollutants are an example of actions that contribute to multiple outcomes relevant to development. This Perspective highlights the interlinkages between these pollutants and the SDGs, and shows that implementing emissions reduction measures can contribute to achieving many of the SDGs. Many of the measures required to reduce emissions of short-lived climate pollutants contribute to achieving the sustainable development goals while complementing decarbonization efforts required to reduce long-term climate change.
Broadly tunable terahertz generation in mid-infrared quantum cascade lasers
Room temperature, broadly tunable, electrically pumped semiconductor sources in the terahertz spectral range, similar in operation simplicity to diode lasers, are highly desired for applications. An emerging technology in this area are sources based on intracavity difference-frequency generation in dual-wavelength mid-infrared quantum cascade lasers. Here we report terahertz quantum cascade laser sources based on an optimized non-collinear Cherenkov difference-frequency generation scheme that demonstrates dramatic improvements in performance. Devices emitting at 4 THz display a mid-infrared-to-terahertz conversion efficiency in excess of 0.6 mW W −2 and provide nearly 0.12 mW of peak power output. Devices emitting at 2 and 3 THz fabricated on the same chip display 0.09 and 0.4 mW W −2 conversion efficiencies at room temperature, respectively. High terahertz-generation efficiency and relaxed phase-matching conditions offered by the Cherenkov scheme allowed us to demonstrate, for the first time, an external-cavity terahertz quantum cascade laser source tunable between 1.70 and 5.25 THz. Compact, tunable terahertz sources are highly desired for sensing and imaging applications. Here Vijayraghavan et al . demonstrate room-temperature quantum cascade laser sources based on the non-linear optical conversion of mid-infrared light that provide a tunable output over a 3.5-THz bandwidth.
Technical opportunities to reduce global anthropogenic emissions of nitrous oxide
We describe a consistent framework developed to quantify current and future anthropogenic emissions of nitrous oxide and the available technical abatement options by source sector for 172 regions globally. About 65% of the current emissions derive from agricultural soils, 8% from waste, and 4% from the chemical industry. Low-cost abatement options are available in industry, wastewater, and agriculture, where they are limited to large industrial farms. We estimate that by 2030, emissions can be reduced by about 6% ±2% applying abatement options at a cost lower than 10 €/t CO2-eq. The largest abatement potential at higher marginal costs is available from agricultural soils, employing precision fertilizer application technology as well as chemical treatment of fertilizers to suppress conversion processes in soil (nitrification inhibitors). At marginal costs of up to 100 €/t CO2-eq, about 18% ±6% of baseline emissions can be removed and when considering all available options, the global abatement potential increases to about 26% ±9%. Due to expected future increase in activities driving nitrous oxide emissions, the limited technical abatement potential available means that even at full implementation of reduction measures by 2030, global emissions can be at most stabilized at the pre-2010 level. In order to achieve deeper reductions in emissions, considerable technological development will be required as well as non-technical options like adjusting human diets towards moderate animal protein consumption.
A comparative risk assessment of burden of disease and injury attributable to 67 risk factors and risk factor clusters in 21 regions, 1990–2010: a systematic analysis for the Global Burden of Disease Study 2010
Quantification of the disease burden caused by different risks informs prevention by providing an account of health loss different to that provided by a disease-by-disease analysis. No complete revision of global disease burden caused by risk factors has been done since a comparative risk assessment in 2000, and no previous analysis has assessed changes in burden attributable to risk factors over time. We estimated deaths and disability-adjusted life years (DALYs; sum of years lived with disability [YLD] and years of life lost [YLL]) attributable to the independent effects of 67 risk factors and clusters of risk factors for 21 regions in 1990 and 2010. We estimated exposure distributions for each year, region, sex, and age group, and relative risks per unit of exposure by systematically reviewing and synthesising published and unpublished data. We used these estimates, together with estimates of cause-specific deaths and DALYs from the Global Burden of Disease Study 2010, to calculate the burden attributable to each risk factor exposure compared with the theoretical-minimum-risk exposure. We incorporated uncertainty in disease burden, relative risks, and exposures into our estimates of attributable burden. In 2010, the three leading risk factors for global disease burden were high blood pressure (7·0% [95% uncertainty interval 6·2–7·7] of global DALYs), tobacco smoking including second-hand smoke (6·3% [5·5–7·0]), and household air pollution from solid fuels (4·3% [3·4–5·3]). In 1990, the leading risks were childhood underweight (7·9% [6·8–9·4]), household air pollution from solid fuels (HAP; 6·8% [5·5–8·0]), and tobacco smoking including second-hand smoke (6·1% [5·4–6·8]). Dietary risk factors and physical inactivity collectively accounted for 10·0% (95% UI 9·2–10·8) of global DALYs in 2010, with the most prominent dietary risks being diets low in fruits and those high in sodium. Several risks that primarily affect childhood communicable diseases, including unimproved water and sanitation and childhood micronutrient deficiencies, fell in rank between 1990 and 2010, with unimproved water and sanitation accounting for 0·9% (0·4–1·6) of global DALYs in 2010. However, in most of sub-Saharan Africa childhood underweight, HAP, and non-exclusive and discontinued breastfeeding were the leading risks in 2010, while HAP was the leading risk in south Asia. The leading risk factor in Eastern Europe, Andean Latin America, and southern sub-Saharan Africa in 2010 was alcohol use; in most of Asia, most of Latin America, North Africa and Middle East, and central Europe it was high blood pressure. Despite declines, tobacco smoking including second-hand smoke remained the leading risk in high-income north America and western Europe. High body-mass index has increased globally and it is the leading risk in Australasia and southern Latin America, and also ranks high in other high-income regions, North Africa and Middle East, and Oceania. Worldwide, the contribution of different risk factors to disease burden has changed substantially, with a shift away from risks for communicable diseases in children towards those for non-communicable diseases in adults. These changes are related to the ageing population, decreased mortality among children younger than 5 years, changes in cause-of-death composition, and changes in risk factor exposures. New evidence has led to changes in the magnitude of key risks including unimproved water and sanitation, vitamin A and zinc deficiencies, and ambient particulate matter pollution. The extent to which the epidemiological shift has occurred and what the leading risks currently are varies greatly across regions. In much of sub-Saharan Africa, the leading risks are still those associated with poverty and those that affect children. Bill & Melinda Gates Foundation.
Decomposing Air Pollutant Emissions in Asia: Determinants and Projections
High levels of air pollution pose an urgent social and public health challenge in many Asian regions. This study evaluates the role of key factors that determined the changes in emission levels in China, India and Japan over the past 25 years. While emissions of air pollutants have been declining in Japan since the 1990s, China and India have experienced a rapid growth in pollution levels in recent years. Around 2005, control measures for sulfur emissions started to deliver expected reductions in China, followed by cuts in nitrogen oxides ten years later. Despite recent policy interventions, growing emission trends in India persist. A decomposition analysis of emission-driving factors indicates that emission levels would have been at least two-times higher without the improvements in energy intensity and efficiency, combined with end-of-pipe measures. Due to the continuous reliance on fossil fuels, the abatement effect of a cleaner fuel mix was in most cases significantly smaller than other factors. A reassessment of emission projections developed in the past suggests a decisive impact of energy and environmental policies. It is expected that targeted legislative instruments will play a dominant role in achieving future air-quality goals in Asia.
Simultaneously Mitigating Near-Term Climate Change and Improving Human Health and Food Security
Tropospheric ozone and black carbon (BC) contribute to both degraded air quality and global warming. We considered ~400 emission control measures to reduce these pollutants by using current technology and experience. We identified 14 measures targeting methane and BC emissions that reduce projected global mean warming ~0.5°C by 2050. This strategy avoids 0.7 to 4.7 million annual premature deaths from outdoor air pollution and increases annual crop yields by 30 to 135 million metric tons due to ozone reductions in 2030 and beyond. Benefits of methane emissions reductions are valued at $700 to $5000 per metric ton, which is well above typical marginal abatement costs (less than $250). The selected controls target different sources and influence climate on shorter time scales than those of carbon dioxide-reduction measures. Implementing both substantially reduces the risks of crossing the 2°C threshold.