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The groove density mismatching of compression gratings, an often-neglected key issue, can induce significant spatiotemporal aberrations especially for super-intense femtosecond lasers. We mainly investigate the angular chirp and the consequent degradation of the effective focused intensity introduced by the groove density mismatching of compression gratings in ultra-intense femtosecond lasers. The results indicate that the tolerances of grating groove density mismatching will rapidly decrease with the beam aperture or spectral bandwidth increases. For our 100PW laser under construction, the grating groove density mismatching should be as small as 0.001 gr/mm if the drop of effective focused intensity has to be controlled below 15%. More importantly, new angular chirp compensation schemes are proposed for both double-grating and four-grating compressors. This work reveals the importance of groove density matching of compression gratings, and can provide helpful guidelines for the design of ultra-intense femtosecond lasers.

In quest of achieving compact and economic PW-level Ti:Sapphire (Ti:sa) lasers with a sub-15 fs pulse duration, a modified hybrid amplification scheme, which combines the optical parametric chirped pulse amplifier (OPCPA) and the chirped pulse amplifier (CPA), is presented and numerically investigated in this paper. The key characteristic of this scheme is that the conventional Ti:sa regenerative amplifier and preamplifier are replaced by a dual-crystal OPCPA front-end, which is spectrally matched with the upstream seed source and the downstream Ti:sa amplifiers and, therefore, can realize a broader spectrum. Moreover, some useful laser techniques are also applied to suppress the spectral gain narrowing and redshift in the Ti:sa CPA chain and to control the residual dispersion in the laser system. This way, fewer amplification stages and pump lasers are required to reach PW-level peak power compared with traditional all-CPA Ti:sa lasers. Numerical results indicate that pulse energy and spectral bandwidth can reach up to ∼22 J and ∼125 nm at full width at half maximum (FWHM), respectively, only by employing three-stage amplifiers. After compression, PW-level lasers with a ∼13.3 fs pulse duration are expected. This work can offer a promising route for the development of compact and economic PW-level Ti:sa lasers.

A single-shot measurement of electron emittance was experimentally accomplished using a focused transfer line with a dipole. The betatron phase of electrons based on laser wakefield acceleration (LWFA) is energy dependent owing to the coupling of the longitudinal acceleration field and the transverse focusing (defocusing) field in the bubble. The phase space presents slice information after phase compensation relative to the center energy. Fitting the transverse size of the electron beam at different energy slices in the energy spectrum measured 0.27 mm mrad in the experiment. The diagnosis of slice emittance facilitates local electron quality manipulation, which is important for the development of LWFA-based free electron lasers. The quasi-3D particle-in-cell simulations matched the experimental results and analysis well.

The delay-shift of the pre-pulse may mislead the determination of its origination and cause problems for the temporal contrast improvement of high-peak-power lasers, especially when the corresponding post-pulse is beyond the time window of the measurement device. In this work, an empirical formula is proposed to predict the delay-shift of pre-pulses for the first time. The empirical formula shows that the delay-shift is proportional to the square of the post-pulse’s initial delay, and also the ratio of the third-order dispersion to the group delay dispersion’s square, which intuitively reveals the main cause for the delay-shift and may provide a convenient routing for identifying the real sources of pre-pulses in both chirped-pulse amplification (CPA) and optical parametric chirped-pulse amplification (OPCPA) systems. The empirical formula agrees well with the experimental results both in the CPA and the OPCPA systems. Besides, a numerical simulation is also carried out to further verify the empirical formula.

The focusing quality of high peak power lasers plays a crucial role in laser wakefield electron acceleration investigations. We report here an improvement in the focusing quality of the SULF-1PW laser beamline, planning to drive and generate 5~10 GeV electron beams. After the wavefront correction in vacuum with an adaptive optical system and the focusing with an f/56 off-axis parabolic mirror, near-diffraction-limited focal spots with a size of 52 × 54 μm2 at full width at half maximum are achieved, and the enclosed energy inside this size is ~36.6%. Consequently, the focused intensity of ~1.66 × 1019 W/cm2 can be achieved at 1 PW peak power. Moreover, we also examine the wavefront stability in air and vacuum, respectively. From the statistical analysis of 1900 shots of successive laser pulses at 1 Hz, we identify the wavefront fluctuation resulting from air turbulence and the better correction capacity in vacuum. This work demonstrates the importance and necessity of wavefront correction in vacuum for high peak power lasers.

The picosecond optical parametric chirped pulse amplifier (ps-OPCPA) with double BBO arrangement can support the ultrabroad spectrum even under a relatively long pump pulse duration (∼100 ps). In this work, five-wave-coupled equations taking into consideration different phase matching conditions between the parametric superfluorescence (PSF) and the signal are proposed to investigate the temporal contrast in ps-OPCPA schemes. Both the temporal contrast and the amplified spectrum are numerically analyzed in double BBO arrangements with four phase matching conditions. Numerical results show that the high temporal contrast and ultrabroad spectrum can be simultaneously realized by choosing the proper phase matching geometry in a double BBO arrangement. The numerical investigation here relaxes the requirement of very short pump pulses in ps-OPCPA, which can provide beneficial guidance for the design and construction of ps-OPCPA.

In this paper, we report a nonlinear optical parametric amplifier featuring high conversion efficiency, high temporal contrast and ultra-broadband spectrum simultaneously, based on the dual-crystal scheme. By removing the idler pulse between two crystals and optimizing the phase-matching geometry, the effective conversion efficiency can be enhanced to ∼ 40%, and the spectral bandwidth of the amplified pulse can reach 210 nm. Moreover, the degradation of temporal contrast due to the backconversion in dual-crystal scheme is avoided by optimizing two crystals’ thickness. The measured contrast ratio is 10 - 10 , which is almost the same as that of the single-crystal scheme. The energy stability and the beam profile in both dual crystal and single-crystal scheme are also compared. This work can provide very meaningful guideline for the design of high-peak-power OPCPA.

The misalignment of the gratings in pulse compressor can introduce residual angular chirp and finally result in a reduction of focused intensity, especially for high peak power femtosecond laser systems with large beam size and broadband spectrum. In this work, we study the angular chirp produced by grating misalignment in different dimensions and comprehensively investigate the various effects on the deterioration of the spatiotemporal characteristics of focused beam. Moreover, two representative ultra-high peak power femtosecond laser systems, featuring with 10 PW peak power/500 mm beam diameter/100 nm spectral width and 50 PW peak power/640 mm beam diameter/200 nm spectral width, are studied. For a drop of effective focused intensity smaller than 10%, the numerical results show that the misalignment of gratings must be kept below ~ 2 μrad and ~ 1 μrad for aforesaid 10 PW and 50 PW lasers, respectively. This work provides meaningful guidelines for the design and construction of the grating compressors in ultra-high peak power femtosecond laser systems.

We report dispersion management based on a mismatched-grating compressor for a 100 PW level laser, which utilizes optical parametric chirped pulse amplification and also features large chirped pulse duration and an ultra-broadband spectrum. The numerical calculation indicates that amplified pulses with 4 ns chirped pulse duration and 210 nm spectral bandwidth can be directly compressed to sub-13 fs, which is close to the Fourier-transform limit (FTL). More importantly, the tolerances of the mismatched-grating compressor to the misalignment of the stretcher, the error of the desired grating groove density and the variation of material dispersion are comprehensively analyzed, which is crucially important for its practical application. The results demonstrate that good tolerances and near-FTL compressed pulses can be achieved simultaneously, just by keeping a balance between the residual second-, third- and fourth-order dispersions in the laser system. This work can offer a meaningful guideline for the design and construction of 100 PW level lasers.

To improve pulse contrast in chirped pulse amplification petawatt laser systems, the regenerative amplifier is substituted with a multipass amplifier at the Shanghai Superintense Ultrafast Laser Facility (SULF). To reduce the consequent angular dispersion of the broadband spectrum, a double-grating stretcher is established in the SULF front end. A grating compressor is set up for the 10-PW front end to obtain 20-TW output. An accurate adjustment method of grating attitude (angular position) is presented, which references the direction of gravity, improving dispersion management and focusing ability of the beam. After a pulse passes the front end compressor, its duration and phase in the frequency domain are measured, and the duration can be continuously compressed to <24 fs.