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Detectors based on liquid argon (LAr) often require surfaces that can shift vacuum ultraviolet (VUV) light and reflect the visible shifted light. For the LAr instrumentation of the LEGEND-200 neutrinoless double beta decay experiment, several square meters of wavelength-shifting reflectors (WLSR) were prepared: the reflector Tetratex® (TTX) was in-situ evaporated with the wavelength shifter tetraphenyl butadiene (TPB). For even larger detectors, TPB evaporation will be more challenging and plastic films of polyethylene naphthalate (PEN) are considered as an option to ease scalability. In this work, we first characterized the absorption (and reflectivity) of PEN, TPB (and TTX) films in response to visible light. We then measured TPB and PEN coupled to TTX in a LAr setup equipped with a VUV sensitive photomultiplier tube. The effective VUV photon yield in the setup was first measured using an absorbing reference sample, and the VUV reflectivity of TTX quantified. The characterization and simulation of the setup along with the measurements and modelling of the optical parameters of TPB, PEN and TTX allowed to estimate the absolute quantum efficiency (QE) of TPB and PEN in LAr (at 87K) for the first time: these were found to be above 67 and 49%, respectively (at 90% CL). These results provide relevant input for the optical simulations of experiments that use TPB in LAr, such as LEGEND-200, and for experiments that plan to use TPB or PEN to shift VUV scintillation light.

The DARWIN observatory is a proposed next-generation experiment with 40 tonnes of liquid xenon as an active target in a time projection chamber. To study challenges related to the construction and operation of a multi-tonne scale detector, we have designed and constructed a vertical, full-scale demonstrator for the DARWIN experiment at the University of Zurich. Here, we present the first results from a several-months run with 343 kg of xenon and electron drift lifetime and transport measurements with a 53 cm tall purity monitor immersed in the cryogenic liquid. After 88 days of continuous purification, the electron lifetime reached a value of ( 664 ± 23 ) μ s . We measured the drift velocity of electrons for electric fields in the range (25–75) V/cm, and found values consistent with previous measurements. We also calculated the longitudinal diffusion constant of the electron cloud in the same field range, and compared with previous data, as well as with predictions from an empirical model.

The Pauli Exclusion Principle (PEP) appears from fundamental symmetries in quantum field theories, but its physical origin is still to be understood. High-precision experimental searches for small PEP violations permit testing key assumptions of the Standard Model with high sensitivity. We report on a dedicated measurement with Gator, a low-background, high-purity germanium detector operated at the Laboratori Nazionali del Gran Sasso, aimed at testing PEP-violating atomic transitions in lead. The experimental technique, relying on forming a new symmetry state by introducing electrons into the pre-existing electron system through a direct current, satisfies the conditions of the Messiah-Greenberg superselection rule. No PEP violation has been observed, and an upper limit on the PEP violation probability of β 2 / 2 < 4.8 · 10 - 29 (90% CL) is set. This improves the previous constraint from a comparable measurement by more than one order of magnitude.

The Monument experiment measures ordinary muon capture (OMC) on isotopes relevant for neutrinoless double-beta ( [Formula omitted]) decay and nuclear astrophysics. OMC is a particularly attractive tool for improving the theoretical description of [Formula omitted] decay. It involves similar momentum transfers and allows testing the virtual transitions involved in [Formula omitted] decay against experimental data. During the 2021 campaign, Monument studied OMC on [Formula omitted]Se and [Formula omitted]Ba, the isotopes relevant for next-generation [Formula omitted] decay searches, like Legend and nEXO. The experimental setup has been designed to accurately extract the total and partial muon capture rates, which requires precise reconstruction of energies and time-dependent intensities of the OMC-related [Formula omitted] rays. The setup also includes a veto counter system to allow selecting a clean sample of OMC events. This work provides a detailed description of the Monument setup operated during the 2021 campaign, its two DAQ systems, calibration and analysis approaches, and summarises the achieved detector performance. Future improvements are also discussed.

The XENON1T dark matter experiment aims to detect weakly interacting massive particles (WIMPs) through low-energy interactions with xenon atoms. To detect such a rare event necessitates the use of radiopure materials to minimize the number of background events within the expected WIMP signal region. In this paper we report the results of an extensive material radioassay campaign for the XENON1T experiment. Using gamma-ray spectroscopy and mass spectrometry techniques, systematic measurements of trace radioactive impurities in over one hundred samples within a wide range of materials were performed. The measured activities allowed for stringent selection and placement of materials during the detector construction phase and provided the input for XENON1T detection sensitivity estimates through Monte Carlo simulations.

The XENON1T experiment aims for the direct detection of dark matter in a detector filled with 3.3 tons of liquid xenon. In order to achieve the desired sensitivity, the background induced by radioactive decays inside the detector has to be sufficiently low. One major contributor is the β -emitter 85 Kr which is present in the xenon. For XENON1T a concentration of natural krypton in xenon nat Kr / Xe < 200 ppq   (parts per quadrillion,  1 ppq = 10 - 15 mol / mol ) is required. In this work, the design, construction and test of a novel cryogenic distillation column using the common McCabe–Thiele approach is described. The system demonstrated a krypton reduction factor of 6.4 · 10 5 with thermodynamic stability at process speeds above 3 kg/h. The resulting concentration of nat Kr / Xe < 26 ppq is the lowest ever achieved, almost one order of magnitude below the requirements for XENON1T and even sufficient for future dark matter experiments using liquid xenon, such as XENONnT and DARWIN.

For the first time, a small dual-phase (liquid/gas) xenon time projection chamber was equipped with a top array of silicon photomultipliers for light and charge readout. Here we describe the instrument in detail, as well as the data processing and the event position reconstruction algorithms. We obtain a spatial resolution of ∼ 1.5 mm in the horizontal plane. To characterise the detector performance, we show calibration data with internal 83 m Kr and 37 Ar sources, and we detail the production of the latter as well as its introduction into the system. We finally compare the observed light and charge yields down to electronic recoil energies of 2.82 keV to predictions based on NEST v2.0.

For the first time, a small dual-phase (liquid/gas) xenon time projection chamber was equipped with a top array of silicon photomultipliers for light and charge readout. Here we describe the instrument in detail, as well as the data processing and the event position reconstruction algorithms. We obtain a spatial resolution of [Formula omitted] in the horizontal plane. To characterise the detector performance, we show calibration data with internal [Formula omitted] and [Formula omitted] sources, and we detail the production of the latter as well as its introduction into the system. We finally compare the observed light and charge yields down to electronic recoil energies of [Formula omitted] to predictions based on NEST v2.0.

We correct an overestimation of the production rate of$$^{137}$$137 Xe in the DARWIN detector operated at LNGS. This formerly dominant intrinsic background source is now at a level similar to the irreducible background from solar$$^8$$8 B neutrinos, thus unproblematic at the LNGS depth. The projected half-life sensitivity for the neutrinoless double beta decay ($$0\\nu \\beta \\beta $$0 ν β β ) of$$^{136}$$136 Xe improves by$$22\\%$$22 % compared to the previously reported number and is now$$T^{0\\nu }_{1/2}= {3.0\\times 10^{27}} \\hbox { yr}$$T 1 / 2 0 ν = 3.0 × 10 27 yr (90% C.L.) after 10 years of DARWIN operation.

In this paper, we describe the XENON100 data analyses used to assess the target-intrinsic background sources radon ([InlineMediaObject not available: see fulltext.]), thoron ([InlineMediaObject not available: see fulltext.]) and krypton ([InlineMediaObject not available: see fulltext.]). We detail the event selections of high-energy alpha particles and decay-specific delayed coincidences. We derive distributions of the individual radionuclides inside the detector and quantify their abundances during the main three science runs of the experiment over a period of ∼4years, from January 2010 to January 2014. We compare our results to external measurements of radon emanation and krypton concentrations where we find good agreement. We report an observed reduction in concentrations of radon daughters that we attribute to the plating-out of charged ions on the negatively biased cathode.