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Nanostructured magnetic materials provide an efficient tool for light manipulation on sub-nanosecond and sub-micron scales, and allow for the observation of the novel effects which are fundamentally impossible in smooth films. For many cases of practical importance, it is vital to observe the magneto-optical intensity modulation in a dual-polarization regime. However, the nanostructures reported on up to date usually utilize a transverse Kerr effect and thus provide light modulation only for p-polarized light. We present a concept of a transparent magnetic metasurface to solve this problem, and demonstrate a novel mechanism for magneto-optical modulation. A 2D array of bismuth-substituted iron-garnet nanopillars on an ultrathin iron-garnet slab forms a metasurface supporting quasi-waveguide mode excitation. In contrast to plasmonic structures, the all-dielectric magnetic metasurface is shown to exhibit much higher transparency and superior quality-factor resonances, followed by a multifold increase in light intensity modulation. The existence of a wide variety of excited mode types allows for advanced light control: transmittance of both p- and s-polarized illumination becomes sensitive to the medium magnetization, something that is fundamentally impossible in smooth magnetic films. The proposed metasurface is very promising for sensing, magnetometry and light modulation applications. The authors fabricate and investigate the metasurface made of 2D iron-garnet subwavelength nanopillar array on a thin iron-garnet film. It exhibits high quality-factor resonances, leading to a multifold increase in light intensity modulation of the transmitted light with an advantage of P and S polarizations both sensitive to the medium magnetization.

All-optical magnetization reversal with femtosecond laser pulses facilitates the fastest and least dissipative magnetic recording, but writing magnetic bits with spatial resolution better than the wavelength of light has so far been seen as a major challenge. Here, we demonstrate that a single femtosecond laser pulse of wavelength 800 nm can be used to toggle the magnetization exclusively within one of two 10-nm thick magnetic nanolayers, separated by just 80 nm, without affecting the other one. The choice of the addressed layer is enabled by the excitation of a plasmon-polariton at a targeted interface of the nanostructure, and realized merely by rotating the polarization-axis of the linearly-polarized ultrashort optical pulse by 90°. Our results unveil a robust tool that can be deployed to reliably switch magnetization in targeted nanolayers of heterostructures, and paves the way to increasing the storage density of opto-magnetic recording by a factor of at least 2. The density of magnetic storage media is limited by the superparamagnetic limit when scaling down magnetic bits. Here, the authors open the way for stacked magnetic storage by using all-optical switching and addressing different magnetic layers by polarization-dependent excitation of plasmon-polaritons.

Plasmonics allows light to be localized on length scales much shorter than its wavelength, which makes it possible to integrate photonics and electronics on the nanoscale. Magneto-optical materials are appealing for applications in plasmonics because they open up the possibility of using external magnetic fields in plasmonic devices. Here, we fabricate a new magneto-optical material, a magnetoplasmonic crystal, that consists of a nanostructured noble-metal film on top of a ferromagnetic dielectric, and we demonstrate an enhanced Kerr effect with this material. Such magnetoplasmonic crystals could have applications in telecommunications, magnetic field sensing and all-optical magnetic data storage. A new magneto-optical material consisting of a nanostructured gold film on top of a ferromagnetic dielectric demonstrated significantly enhanced Faraday and Kerr effects.

The explosive development of quantum magnonics requires the consideration of several previously known effects from a new angle. In particular, taking into account the quantum behavior of magnons is essential at high excitations of the magnetic system, under the conditions of the so-called phenomenon of “foldover” (bi-stable) magnetic resonance. Previously, this effect was considered in the quasi-classical macrospin approximation. However, at large angles of magnetization precession, the magnon density exceeds the critical value for the formation of a magnon Bose condensate (mBEC). Naturally, this purely quantum phenomenon does not exist in the classical approximation. In addition, mBEC leads to superfluid transfer of magnetization, which suppresses the macroinhomogeneity of the samples. The experiments presented in the article show that quantum phenomena well describes the experimental results of nonlinear magnetic resonance in yttrium iron garnet. Thus, we remove the questions that arose earlier when considering this effect without taking into account quantum phenomena. This discovery paves the way for many quantum applications of supermagnonics, such as the magnetic Josephson effect, long-range spin transport, Q-bits, quantum logic, magnetic sensors, and others.

Optical tools are promising for spin-wave generation because of the possibilities of ultrafast manipulation and local excitation. However, a single laser pulse can inject spin waves (SWs) only with a broad frequency spectrum, resulting in short propagation distances and low wave amplitudes. Here, we excite a magnetic garnet film by a train of fs-laser pulses with a 1-GHz repetition rate so that the pulse separation is shorter than the decay time of magnetic modes, which allows us to achieve a collective impact on the magnetization and establish a quasistationary source of spin waves, namely, a coherent accumulation of magnons (“magnon cloud”). This approach has several appealing features: (i) The magnon source is tunable, (ii) the SW amplitude can be significantly enhanced, (iii) the SW spectrum is quite narrow, providing long-distance propagation, (iv) the periodic pumping results in an almost constant-in-time SW amplitude for the distances larger than 20μm away from the source, and (v) the SW emission shows pronounced directionality. These results expand the capabilities of ultrafast coherent optical control of magnetization and pave the way for applications in data processing, including the quantum regime. The quasistationary magnon accumulation might also be of interest for applications in magnon Bose-Einstein condensates.

Ferrimagnetic rare-earth substituted metal alloys GdFeCo were shown to exhibit the phenomenon of all-optical magnetization switching via femtosecond laser pulses. All-optical magnetization switching has been comprehensively investigated in out-of-plane magnetized GdFeCo films; however, the films with the in-plane magnetic anisotropy have not yet been studied in detail. We report experimental observations of the magnetization switching of in-plane magnetized GdFeCo films by means of the femtosecond laser pulses in the presence of a small magnetic field of about 40 µT. The switching effect has a threshold both in the applied magnetic field and in the light intensity.

Magneto-optical effects in ferrimagnetic or ferromagnetic materials are usually too weak for potential applications. The transverse magneto-optical Kerr effect (TMOKE) in ferromagnetic films is typically on the order of 0.1%. Here, we demonstrate experimentally the enhancement of TMOKE due to the interaction of particle plasmons in gold nanowires with a photonic waveguide consisting of magneto-optical material, where hybrid waveguide-plasmon polaritons are excited. We achieve a large TMOKE that modulates the transmitted light intensity by 1.5%, accompanied by high transparency of the system. Our concept may lead to novel devices of miniaturized photonic circuits and switches, which are controllable by an external magnetic field.

Currently spin waves are considered for computation and data processing as an alternative to charge currents. Generation of spin waves by ultrashort laser pulses provides several important advances with respect to conventional approaches using microwaves. In particular, focused laser spot works as a point source for spin waves and allows for directional control of spin waves and switching between their different types. For further progress in this direction it is important to manipulate with the spectrum of the optically generated spin waves. Here we tackle this problem by launching spin waves by a sequence of femtosecond laser pulses with pulse interval much shorter than the relaxation time of the magnetization oscillations. This leads to the cumulative phenomenon and allows us to generate magnons in a specific narrow range of wavenumbers. The wavelength of spin waves can be tuned from 15 μm to hundreds of microns by sweeping the external magnetic field by only 10 Oe or by slight variation of the pulse repetition rate. Our findings expand the capabilities of the optical spin pump-probe technique and provide a new method for the spin wave generation and control.

Here we propose a magnetophotonic structure for the layer-selective magnetization switching with femtosecond laser pulses of different wavelengths. It is based on a chirped magnetophotonic crystal (MPC) containing magnetic GdFeCo and nonmagnetic dielectric layers. At each operating wavelength the laser pulses heat up to necessary level only one GdFeCo layer that leads to its magnetization reversal without any impact on the magnetization of the other layers. Moreover, magneto-optical reading of the MPC magnetization state is discussed. Lateral dimensions of the considered MPC can be made small enough to operate as a unit cell for data storage.

Optical impact on the spin system in a magnetically ordered medium provides a unique possibility for local manipulation of magnetization at subpicosecond time scales. One of the mechanisms of the optical manipulation is related to the inverse Faraday effect (IFE). Usually the IFE is observed in crystals and magnetic films on a substrate. Here we demonstrate the IFE induced by fs-laser pulses in the magnetic film inside the magnetophotonic microcavity. Spectral dependence of the IFE on the laser pulse wavelength in the band gap of the magnetophotonic microcavity has a sharp peak leading to a significant enhancement of the IFE. This phenomenon is explained by strong confinement of the electromagnetic energy within the magnetic film. Calculated near field distribution of the IFE effective magnetic field indicates its subwavelength localization within 30 nm along the film thickness. These excited volumes can be shifted along the sample depth via e.g. changing frequency of the laser pulses. The obtained results open a way for ultrafast optical control of magnetization at subwavelength scales.