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In the summer of 2017, huge wildfires in the British Columbia region (Canada) led to the injection of a remarkably high concentration of biomass burning aerosol in the atmosphere. These aerosol masses reached the city of Naples, Italy, at the end of August 2017, where they were characterized by means of a multiwavelength lidar and a sun–sky–lunar photometer. Here we report on the optical and microphysical properties of this aerosol in an intriguing condition, occurring on 4 September 2017, which is characterized by an interesting multi-layered vertical distribution of the aerosol. The Lidar profiles highlighted the presence of four aerosol layers, with two located in the lower troposphere and the other two at stratospheric altitudes. A rather thorough characterization of the biomass burning aerosol was carried out. The aerosol depolarization ratio showed an increasing dependence on the altitude with averaged values of 2–4% for the tropospheric layers, which are indicative of almost spherical smoke particles, and larger values in the stratospheric layers, suggestive of aspheric particles. Lidar-derived size distributions were retrieved for the first three aerosol layers, highlighting a higher particle concentration in the fine-mode fraction for the layers observed at higher altitudes. A dominance of fine particles in the atmosphere (fine-mode fraction > 0.8) with low absorption properties (absorption AOD < 0.0025 and SSA > 0.97) was also observed over the whole atmospheric column by sun photometer data. The space-resolved results provided by the lidar data are consistent with the columnar features retrieved by the AERONET sun photometer, thus evidencing the reliability and capability of lidar characterization of atmospheric aerosol in a very interesting condition of multiple aerosol layers originating from Canadian fires overpassing the observation station.

The aerosol properties of Mount Etna’s passive degassing plume and its short-term processes and radiative impact were studied in detail during the EPL-RADIO campaigns (summer 2016–2017), using a synergistic combination of observations and radiative transfer modelling. Summit observations show extremely high particulate matter concentrations. Using portable photometers, the first mapping of small-scale (within ∼ 20 km from the degassing craters) spatial variability of the average size and coarse-to-fine burden proportion of volcanic aerosols is obtained. A substantial variability of the plume properties is found at these spatial scales, revealing that processes (e.g. new particle formation and/or coarse aerosols sedimentation) are at play, which are not represented with current regional scale modelling and satellite observations. Statistically significant progressively smaller particles and decreasing coarse-to-fine particles burden proportion are found along plume dispersion. Vertical structures of typical passive degassing plumes are also obtained using observations from a fixed LiDAR station constrained with quasi-simultaneous photometric observations. These observations are used as input to radiative transfer calculations, to obtain the shortwave top of the atmosphere (TOA) and surface radiative effect of the plume. For a plume with an ultraviolet aerosol optical depth of 0.12–0.14, daily average radiative forcings of - 4.5 and - 7.0 W/m 2 , at TOA and surface, are found at a fixed location ∼ 7 km downwind the degassing craters. This is the first available estimation in the literature of the local radiative impact of a passive degassing volcanic plume.

Lockdown measures applied in the aftermath of the COVID-19 pandemic spread to Italy in the period March 13 th –May 4 th strongly limited the social and industrial activities with consequent effects on the air pollution. Here we report a study on the influence of the lockdown measures on the air quality in the city of Naples (Italy). The comparison of the levels of various gaseous pollutants (C 6 H 6 , CO, NO 2 and SO 2 ) and particulate matter (PM 10 , PM 2.5 , PM 1 ) at ground level as well as of atmospheric aerosol properties registered by remote sensing techniques during the lockdown period with the values observed in the earlier months and during the same period of the previous year is used to gain interesting information on the environmental impact of the human activities. Our findings show a rather significant reduction of the pollution due to NO 2 (49–62%) in urban as well as in green suburban area, while CO and SO 2 showed a more important reduction in urban or industrial districts of the city (50–58% and 70%, respectively). Particulate matter at ground level is also affected but to a more limited extent (29–49%). Nevertheless, characterization of atmospheric aerosol columnar properties suggests an interesting variation of its composition. The observed features have been associated to the strong meteorological interference from Saharan Dust in the Mediterranean area also affecting the city of Naples.

An innovative mobile lidar device, developed to monitor volcanic plumes during explosive eruptions at Mt. Etna (Italy) and to analyse the optical properties of volcanic particles, was upgraded in October 2023 with the aim of improving volcanic plume retrievals. The new configuration of the lidar allows it to obtain new data on both the optical and the microphysical properties of the atmospheric aerosol. In fact, after the upgrade, the lidar is able to measure three backscattering coefficients, two extinction coefficients and two depolarisation ratios in a configuration defined as “state-of-the-art lidar”, where properties such as particle size distribution and the refractive index can be derived. During the lidar implementation, we were able to test the system’s performance through specific calibration measurements. A comparison in an aerosol-free region (7.2–12 km) between lidar signals at 1064 nm, 532 nm and 355 nm and the corresponding pure molecular profiles showed a relative difference of <1% between them for all the wavelengths, highlighting the good dynamic of the signals. The overlap correction allowed us to reduce the underestimation of the backscattering coefficient from 50% to 10% below 450 m and 750 m at both 355 and 532 nm, respectively. The correct alignment between the laser beam and the receiver optical chain was tested using the signal received from the different quadrants of the telescope, and the relative differences between the four directions were comparable to zero, within the margin of error. Finally, the first measurement results are shown and compared with results obtained by other instruments, with the aim of proving the ability of the upgraded system to more precisely characterise aerosol optical and microphysical properties.

In January 2016, a measurement campaign was carried out by the China Meteorological Administration, the Beijing Research Institute of Telemetry, and the Physics Department of the University of Naples “Federico II” in the Yulong Naxi Autonomous County (China) at 3200 m above sea level to evaluate the air quality in the high mountains with the lidar technique. Here we report on an interesting event that occurred on 16 January between 12.00 and 00.00 UTC, when a striking aerosol stratification was observed on the site. Aerosol transport events are studied starting from lidar characterization of different aerosol masses. From lidar signals at 355 and 532 nm, integrated on 30 min, the aerosol characterization is done in terms of aerosol depolarization ratio with a spatial resolution of 60 m and color ratio; these parameters allow for highlighting a phenomenon of aerosol transport from the Tibetan plateau planetary boundary layer and from northern India. The initial layer is composed of a mixture of aerosols characterized by average values of the aerosol depolarization ratio and the color ratio of (30 ± 2)% and (0.9 ± 0.2), respectively, indicating a large non-spherical aerosol composition. Then, the deposition of this aerosol load ensues, and aerosols with such features are progressively observed at lower altitudes.

We report on the characterization of columnar aerosol optical and microphysical properties in the Naples Mediterranean area over a period of five years by the ground-based sun–sky–lunar photometer operating at our observational station in the frame of the AERONET network. Statistical and climatological analyses of daily mean values of aerosol optical depth at 440 nm (AOD440) and Ångström exponent at 440/870 nm (α440/870) allowed for highlighting their typical seasonal behavior. In particular, we observe higher mean values of the AOD440 during summer or spring, which are consistent with an increased frequency of both Saharan dust transport events and biomass burning episodes affecting the measurement area in these periods of the year. Conversely, α440/870 does not show any typical seasonal trend. In order to gain information on the different aerosol contributions along the atmospheric column, the frequency distributions of AOD440 and α440/870 were analyzed and fitted by a superposition of Gaussian functions. The most populated modes are centered at α440/870 = 1.26 ± 0.07 and AOD440 = 0.16 ± 0.01. These values are associated with continental polluted aerosol mixed with sea salt aerosol and correspond to the background conditions typically observed in clear atmospheric conditions. Daily size distributions averaged over each month highlight that the fine aerosol component always prevails over the coarse fraction, except for the few months in which Saharan dust events are particularly frequent. Finally, the mean value of the SSA at 440 nm resulted as 0.94 ± 0.05, while the refractive index real and imaginary part were 1.47 ± 0.07 and (6.5 ± 0.2) × 10−3, respectively. These values are in agreement with those observed in other Mediterranean sites located in Southern Italy, evidencing a rather characteristic feature of the geographical region.

During the summer of 2017, multiple huge fires occurred on Mount Vesuvius (Italy), dispersing a large quantity of ash in the surrounding area ensuing the burning of tens of hectares of Mediterranean scrub. The fires affected a very large area of the Vesuvius National Park and the smoke was driven by winds towards the city of Naples, causing daily peak values of particulate matter (PM) concentrations at ground level higher than the limit of the EU air quality directive. The smoke plume spreading over the area of Naples in this period was characterized by active (lidar) and passive (sun photometer) remote sensing as well as near-surface (optical particle counter) observational techniques. The measurements allowed us to follow both the PM variation at ground level and the vertical profile of fresh biomass burning aerosol as well as to analyze the optical and microphysical properties. The results evidenced the presence of a layer of fine mode aerosol with large mean values of optical depth (AOD > 0.25) and Ångstrom exponent (γ > 1.5) above the observational site. Moreover, the lidar ratio and aerosol linear depolarization obtained from the lidar observations were about 40 sr and 4%, respectively, consistent with the presence of biomass burning aerosol in the atmosphere.

Lidar observations are very useful to analyse dispersed volcanic clouds in the troposphere mainly because of their high range resolution, providing morphological as well as microphysical (size and mass) properties. In this work, we analyse the volcanic cloud of 18 May 2016 at Mt. Etna, in Italy, retrieved by polarimetric dual-wavelength Lidar measurements. We use the AMPLE (Aerosol Multi-Wavelength Polarization Lidar Experiment) system, located in Catania, about 25 km from the Etna summit craters, pointing at a thin volcanic cloud layer, clearly visible and dispersed from the summit craters at the altitude between 2 and 4 km and 6 and 7 km above the sea level. Both the backscattering and linear depolarization profiles at 355 nm (UV, ultraviolet) and 532 nm (VIS, visible) wavelengths, respectively, were obtained using different angles at 20°, 30°, 40° and 90°. The proposed approach inverts the Lidar measurements with a physically based inversion methodology named Volcanic Ash Lidar Retrieval (VALR), based on Maximum-Likelihood (ML). VALRML can provide estimates of volcanic ash mean size and mass concentration at a resolution of few tens of meters. We also compared those results with two methods: Single-variate Regression (SR) and Multi-variate Regression (MR). SR uses the backscattering coefficient or backscattering and depolarization coefficients of one wavelength (UV or VIS in our cases). The MR method uses the backscattering coefficient of both wavelengths (UV and VIS). In absence of in situ airborne validation data, the discrepancy among the different retrieval techniques is estimated with respect to the VALR ML algorithm. The VALR ML analysis provides ash concentrations between about 0.1 μg/m3 and 1 mg/m3 and particle mean sizes of 0.1 μm and 6 μm, respectively. Results show that, for the SR method differences are less than <10%, using the backscattering coefficient only and backscattering and depolarization coefficients. Moreover, we find differences of 20–30% respect to VALR ML, considering well-known parametric retrieval methods. VALR algorithms show how a physics-based inversion approaches can effectively exploit the spectral-polarimetric Lidar AMPLE capability.

Volcanic emissions are a well-known hazard that can have serious impacts on local populations and aviation operations. Whereas several remote sensing observations detect high-intensity explosive eruptions, few studies focus on low intensity and long-lasting volcanic emissions. In this work, we have managed to fully characterize those events by analyzing the volcanic plume produced on the last day of the 2018 Christmas eruption at Mt. Etna, in Italy. We combined data from a visible calibrated camera, a multi-wavelength elastic/Raman Lidar system, from SEVIRI (EUMETSAT-MSG) and MODIS (NASA-Terra/Aqua) satellites and, for the first time, data from an automatic sun-photometer of the aerosol robotic network (AERONET). Results show that the volcanic plume height, ranging between 4.5 and 6 km at the source, decreased by about 0.5 km after 25 km. Moreover, the volcanic plume was detectable by the satellites up to a distance of about 400 km and contained very fine particles with a mean effective radius of about 7 µm. In some time intervals, volcanic ash mass concentration values were around the aviation safety thresholds of 2 × 10−3 g m−3. Of note, Lidar observations show two main stratifications of about 0.25 km, which were not observed at the volcanic source. The presence of the double stratification could have important implications on satellite retrievals, which usually consider only one plume layer. This work gives new details on the main features of volcanic plumes produced during low intensity and long-lasting volcanic plume emissions.

A lidar for aerosol monitoring with conventional optical design can provide good quality signals from several hundred meters up to tens of kilometres above the ground, but the aerosol load is mainly contained (up to 80%) in the planetary boundary layer that can have a height of only hundreds of meters above the ground level. Therefore, the measurement of the complete aerosol extinction profile is generally a very difficult challenge. In this paper, we proposed an optical design of lidar systems able of producing signals starting from a few tens of meters above the ground. The overlap profiles obtained from an optimized lidar was compared with ray tracing simulations and further conventional lidar apparatuses.