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This work reports on the first attempt to prepare bioderived polymer films by blending polylactic acid (PLA) and poly(dodecylene furanoate) (PDoF). This blend, containing 10 wt% PDoF, was filled with reduced graphene oxide (rGO) in variable weight fractions (from 0.25 to 2 phr), and the resulting nanocomposites were characterized to assess their microstructural, thermal, mechanical, optical, electrical, and gas barrier properties. The PLA/PDoF blend resulted as immiscible, and the addition of rGO, which preferentially segregated in the PDoF phase, resulted in smaller (from 2.6 to 1.6 µm) and more irregularly shaped PDoF domains and in a higher PLA/PDoF interfacial interaction, which suggests the role of rGO as a blend compatibilizer. rGO also increased PLA crystallinity, and this phenomenon was more pronounced when PDoF was also present, thus evidencing a synergism between PDoF and rGO in accelerating the crystallization kinetics of PLA. Dynamic mechanical thermal analysis (DMTA) showed that the glass transition of PDoF, observed at approx. 5 °C, shifted to a higher temperature upon rGO addition. The addition of 10 wt% PDoF in PLA increased the strain at break from 5.3% to 13.0% (+145%), and the addition of 0.25 phr of rGO increased the tensile strength from 35.6 MPa to 40.2 MPa (+13%), without significantly modifying the strain at break. Moreover, rGO decreased the electrical resistivity of the films, and the relatively high percolation threshold (between 1 and 2 phr) was probably linked to the low aspect ratio of rGO nanosheets and their preferential distribution inside PDoF domains. PDoF and rGO also modified the optical transparency of PLA, resulting in a continuous decrease in transmittance in the visible/NIR range. Finally, rGO strongly modified the gas barrier properties, with a remarkable decrease in diffusivity and permeability to gases such as O2, N2, and CO2. Overall, the presented results highlighted the positive and sometimes synergistic role of PDoF and rGO in tuning the thermomechanical and functional properties of PLA, with simultaneous enhancement of ductility, crystallization kinetics, and gas barrier performance, and these novel polymer nanocomposites could thus be promising for packaging applications.

Abstract The process of implantation and diffusion of positron in nanochanneled silicon crystals has been simulated in detail through the Monte Carlo technique. Our implantation simulations evidenced the fraction of empty volume inside the sample to be the decisive factor in the determination of the shape of the implantation profile, with the specific shape of the nanoscopic structure playing a marginal role for implantation processes with an energy above 3 keV. Moreover we observed that, due to the high density of surfaces inside of the silicon sample, the subsequent diffusion process is highly suppressed and that thermalized positrons reach the surface of a nanoscopic channel close to their implantation depth. Due to this suppression of the diffusion process, 60–80% of the positrons implanted at an energy comprised between 4 and 13 keV will reach, at thermal energy, the surface of a channel without escaping the sample or undergoing annihilation. Graphical abstract

Antihydrogen atoms with K or sub-K temperature are a powerful tool to precisely probe the validity of fundamental physics laws and the design of highly sensitive experiments needs antihydrogen with controllable and well defined conditions. We present here experimental results on the production of antihydrogen in a pulsed mode in which the time when 90% of the atoms are produced is known with an uncertainty of ~250 ns. The pulsed source is generated by the charge-exchange reaction between Rydberg positronium atoms—produced via the injection of a pulsed positron beam into a nanochanneled Si target, and excited by laser pulses—and antiprotons, trapped, cooled and manipulated in electromagnetic traps. The pulsed production enables the control of the antihydrogen temperature, the tunability of the Rydberg states, their de-excitation by pulsed lasers and the manipulation through electric field gradients. The production of pulsed antihydrogen is a major landmark in the AE ḡ IS experiment to perform direct measurements of the validity of the Weak Equivalence Principle for antimatter. Antihydrogen atoms are a unique type of antimatter that can be used to probe small violations of fundamental laws of physics. The authors present experimental results obtained with the AEgIS project at CERN for the production of antihydrogen atoms (Hbar) via charge exchange with laser excited positronium that allow for precise timing of Hbar production.

We describe a novel method to use a scintillating fiber detector similar to the Fast Annihilation Cryogenic Tracking (FACT) used at the antimatter experiment AEgIS to monitor the presence of ortho-positronium. A single scintillating fiber was coupled to a photomultiplier tube and irradiated by flashes of about \\(610^6\\) \\(511\\,keV\\) \\(\\)-rays produced by \\(10\\,ns\\) long positron pulses. The results were used to demonstrate the ability to track the creation and annihilation of ortho-positronium atoms over time in cryogenic and highly magnetic environments by using the FACT detector as a \"digital calorimeter\".

A powerful and robust control system is a crucial, often neglected, pillar of any modern, complex physics experiment that requires the management of a multitude of different devices and their precise time synchronisation. The AEgIS collaboration presents CIRCUS, a novel, autonomous control system optimised for time-critical experiments such as those at CERN's Antiproton Decelerator and, more broadly, in atomic and quantum physics research. Its setup is based on Sinara/ARTIQ and TALOS, integrating the ALPACA analysis pipeline, the last two developed entirely in AEgIS. It is suitable for strict synchronicity requirements and repeatable, automated operation of experiments, culminating in autonomous parameter optimisation via feedback from real-time data analysis. CIRCUS has been successfully deployed and tested in AEgIS; being experiment-agnostic and released open-source, other experiments can leverage its capabilities.