Explore the vast range of titles available.

The injection of sulfur dioxide (SO2) into the stratosphere and its subsequent oxidation to form sulfate aerosols after large volcanic eruptions can have profound effects on Earth's climate. The removal of volcanic SO2 in the stratosphere is thought to be driven by its gas-phase oxidation by the hydroxyl radical (OH); once oxidized, it goes on to form sulfate aerosols. However, it has also been suggested that heterogeneous oxidation on ash could also be important or even dominant, which would imply the faster removal of SO2 and thus the faster formation of aerosols, at least in ash-rich plumes. Additionally, recent work uses an assumed exponential fit to determine the total SO2 mass loading following large eruptions; the quality of this fit translates directly to the accuracy of the mass loading estimate. It is therefore of interest to examine how accurately the SO2 decay timescale can be determined from observations and to compare observations to models. Here we evaluate the SO2 decay timescale and its uncertainties following several significant eruptions using three different sets of satellite observations and compare these to the CESM2-WACCM6 model. We show that defining an accurate baseline against which a volcanic injection can be quantified increases the variability and uncertainty in the estimated decay timescale for some satellite datasets. While the typical decay timescale for SO2 is on the order of a few weeks to a month, we find that uncertainties across different altitudes and eruptions result in timescales that can vary by more than a factor of 2. This makes it difficult to attribute variations in the decay timescale to specific SO2-removal processes for the events examined.

Spaceborne measurements by NASA’s Orbiting Carbon Observatory-2 (OCO-2) at the kilometer scale reveal distinct structures of atmospheric carbon dioxide (CO 2 ) caused by known anthropogenic and natural point sources. OCO-2 transects across the Los Angeles megacity (USA) show that anthropogenic CO 2 enhancements peak over the urban core and decrease through suburban areas to rural background values more than ~100 kilometers away, varying seasonally from ~4.4 to 6.1 parts per million. A transect passing directly downwind of the persistent isolated natural CO 2 plume from Yasur volcano (Vanuatu) shows a narrow filament of enhanced CO 2 values (~3.4 parts per million), consistent with a CO 2 point source emitting 41.6 kilotons per day. These examples highlight the potential of the OCO-2 sensor, with its unprecedented resolution and sensitivity, to detect localized natural and anthropogenic CO 2 sources.

Severe haze is a major public health concern in China and India. Both countries rely heavily on coal for energy, and sulfur dioxide (SO 2 ) emitted from coal-fired power plants and industry is a major pollutant contributing to their air quality problems. Timely, accurate information on SO 2 sources is a required input to air quality models for pollution prediction and mitigation. However, such information has been difficult to obtain for these two countries, as fast-paced changes in economy and environmental regulations have often led to unforeseen emission changes. Here we use satellite observations to show that China and India are on opposite trajectories for sulfurous pollution. Since 2007, emissions in China have declined by 75% while those in India have increased by 50%. With these changes, India is now surpassing China as the world’s largest emitter of anthropogenic SO 2 . This finding, not predicted by emission scenarios, suggests effective SO 2 control in China and lack thereof in India. Despite this, haze remains severe in China, indicating the importance of reducing emissions of other pollutants. In India, ~33 million people now live in areas with substantial SO 2 pollution. Continued growth in emissions will adversely affect more people and further exacerbate morbidity and mortality.

Volcanoes are the main pathway to the surface for volatiles that are stored within the Earth. Carbon dioxide (CO 2 ) is of particular interest because of its potential for climate forcing. Understanding the balance of CO 2 that is transferred from the Earth’s surface to the Earth’s interior, hinges on accurate quantification of the long-term emissions of volcanic CO 2 to the atmosphere. Here we present an updated evaluation of the world’s volcanic CO 2 emissions that takes advantage of recent improvements in satellite-based monitoring of sulfur dioxide, the establishment of ground-based networks for semi-continuous CO 2 -SO 2 gas sensing and a new approach to estimate key volcanic gas parameters based on magma compositions. Our results reveal a global volcanic CO 2 flux of 51.3 ± 5.7 Tg CO 2 /y (11.7 × 10 11  mol CO 2 /y) for non-eruptive degassing and 1.8 ± 0.9 Tg/y for eruptive degassing during the period from 2005 to 2015. While lower than recent estimates, this global volcanic flux implies that a significant proportion of the surface-derived CO 2 subducted into the Earth’s mantle is either stored below the arc crust, is efficiently consumed by microbial activity before entering the deeper parts of the subduction system, or becomes recycled into the deep mantle to potentially form diamonds.

We present the first sulfur dioxide (SO2) retrievals from Tropospheric Emissions: Monitoring of Pollution (TEMPO), the first geostationary atmospheric composition sensor to cover North America, along with some potential applications of TEMPO SO2 data. We show that high resolution (∼10 km2) TEMPO measurements can be used to produce good quality SO2 retrievals with relatively small noise and biases. We demonstrate that hourly TEMPO data are useful for monitoring volcanic hazards, by providing frequent updates on the plume location and additional information on the plume height or winds. With the large number of measurements from TEMPO, it is also feasible to monitor diurnal changes in SO2 for relatively large sources such as the Cantarell oil field. We also show that high‐cadence TEMPO measurements allow estimates of SO2 degassing from Popocatépetl volcano on sub‐daily timescales. Overall, our results suggest that TEMPO can significantly enhance space‐based SO2 detection and monitoring over North America.

Fuego volcano (Guatemala) is one of the most active and hazardous volcanoes in the world. Its persistent activity generates lava flows, pyroclastic density currents (PDCs), and lahars that threaten the surrounding areas and produce frequent morphological change. Fuego’s eruption deposits are often rapidly eroded or remobilized by heavy rains and its constant activity and inaccessible terrain makes ground-based assessment of recent eruptive deposits very challenging. Earth-orbiting satellites can provide unique observations of volcanoes during eruptive activity, when ground-based techniques may be too hazardous, and also during inter-eruptive phases, but have typically been hindered by relatively low spatial and temporal resolution. Here, we use a new source of Earth observation data for volcano monitoring: high resolution (~3 m pixel size) images acquired from a constellation of over 150 CubeSats (‘Doves’) operated by Planet Labs Inc. The Planet Labs constellation provides high spatial resolution at high cadence (<1–72 h), permitting space-based tracking of volcanic activity with unprecedented detail. We show how PlanetScope images collected before, during, and after an eruption can be applied for mapping ash clouds, PDCs, lava flows, or the analysis of morphological change. We assess the utility of the PlanetScope data as a tool for volcano monitoring and rapid deposit mapping that could assist volcanic hazard mitigation efforts in Guatemala and other active volcanic regions.

We present a synthesis of diverse observations of the first recorded eruption of Nabro volcano, Eritrea, which began on 12 June 2011. While no monitoring of the volcano was in effect at the time, it has been possible to reconstruct the nature and evolution of the eruption through analysis of regional seismological and infrasound data and satellite remote sensing data, supplemented by petrological analysis of erupted products and brief field surveys. The event is notable for the comparative rarity of recorded historical eruptions in the region and of caldera systems in general, for the prodigious quantity of SO 2 emitted into the atmosphere and the significant human impacts that ensued notwithstanding the low population density of the Afar region. It is also relevant in understanding the broader magmatic and tectonic significance of the volcanic massif of which Nabro forms a part and which strikes obliquely to the principal rifting directions in the Red Sea and northern Afar. The whole-rock compositions of the erupted lavas and tephra range from trachybasaltic to trachybasaltic andesite, and crystal-hosted melt inclusions contain up to 3,000 ppm of sulphur by weight. The eruption was preceded by significant seismicity, detected by regional networks of sensors and accompanied by sustained tremor. Substantial infrasound was recorded at distances of hundreds to thousands of kilometres from the vent, beginning at the onset of the eruption and continuing for weeks. Analysis of ground deformation suggests the eruption was fed by a shallow, NW–SE-trending dike, which is consistent with field and satellite observations of vent distributions. Despite lack of prior planning and preparedness for volcanic events in the country, rapid coordination of the emergency response mitigated the human costs of the eruption.

The separation of volcanic ash and sulfur dioxide (SO2) gas is sometimes observed during volcanic eruptions. The exact conditions under which separation occurs are not fully understood but the phenomenon is of importance because of the effects volcanic emissions have on aviation, on the environment, and on the earth's radiation balance. The eruption of Grímsvötn, a subglacial volcano under the Vatnajökull glacier in Iceland during 21–28 May 2011 produced one of the most spectacular examples of ash and SO2 separation, which led to errors in the forecasting of ash in the atmosphere over northern Europe. Satellite data from several sources coupled with meteorological wind data and photographic evidence suggest that the eruption column was unable to sustain itself, resulting in a large deposition of ash, which left a low-level ash-rich atmospheric plume moving southwards and then eastwards towards the southern Scandinavian coast and a high-level predominantly SO2 plume travelling northwards and then spreading eastwards and westwards. Here we provide observational and modelling perspectives on the separation of ash and SO2 and present quantitative estimates of the masses of ash and SO2 that erupted, the directions of transport, and the likely impacts. We hypothesise that a partial column collapse or “sloughing” fed with ash from pyroclastic density currents (PDCs) occurred during the early stage of the eruption, leading to an ash-laden gravity intrusion that was swept southwards, separated from the main column. Our model suggests that water-mediated aggregation caused enhanced ash removal because of the plentiful supply of source water from melted glacial ice and from entrained atmospheric water. The analysis also suggests that ash and SO2 should be treated with separate source terms, leading to improvements in forecasting the movement of both types of emissions.

The Stratospheric Sulfur and its Role in Climate (SSiRC) Interactive Stratospheric Aerosol Model Intercomparison Project (ISA-MIP) explores uncertainties in the processes that connect volcanic emission of sulfur gas species and the radiative forcing associated with the resulting enhancement of the stratospheric aerosol layer. The central aim of ISA-MIP is to constrain and improve interactive stratospheric aerosol models and reduce uncertainties in the stratospheric aerosol forcing by comparing results of standardized model experiments with a range of observations. In this paper we present four co-ordinated inter-model experiments designed to investigate key processes which influence the formation and temporal development of stratospheric aerosol in different time periods of the observational record. The Background (BG) experiment will focus on microphysics and transport processes under volcanically quiescent conditions, when the stratospheric aerosol is controlled by the transport of aerosols and their precursors from the troposphere to the stratosphere. The Transient Aerosol Record (TAR) experiment will explore the role of small- to moderate-magnitude volcanic eruptions, anthropogenic sulfur emissions, and transport processes over the period 1998–2012 and their role in the warming hiatus. Two further experiments will investigate the stratospheric sulfate aerosol evolution after major volcanic eruptions. The Historical Eruptions SO2 Emission Assessment (HErSEA) experiment will focus on the uncertainty in the initial emission of recent large-magnitude volcanic eruptions, while the Pinatubo Emulation in Multiple models (PoEMS) experiment will provide a comprehensive uncertainty analysis of the radiative forcing from the 1991 Mt Pinatubo eruption.

Satellite measurements of volcanic sulfur dioxide (SO₂) emissions can provide critical information for aviation hazard mitigation, particularly when ash detection techniques fail. Recent developments in space-based SO₂ monitoring are discussed, focusing on daily, global ultraviolet (UV) measurements by the Ozone Monitoring Instrument (OMI) on NASA's Aura satellite. OMI's high sensitivity to SO₂ permits long-range tracking of volcanic clouds in the upper troposphere and lower stratosphere (UTLS) and accurate mapping of their perimeters to facilitate avoidance. Examples from 2006 to 2007 include eruptions of Soufriere Hills (Montserrat), Rabaul (Papua New Guinea), Nyamuragira (DR Congo), and Jebel at Tair (Yemen). A tendency for some volcanic clouds to occupy the jet stream suggests an increased threat to aircraft that exploit this phenomenon. Synergy between NASA A-Train sensors such as OMI and the Atmospheric Infrared Sounder (AIRS) on the Aqua satellite can provide critical information on volcanic cloud altitude. OMI and AIRS SO₂ data products are being produced in near real-time for distribution to Volcanic Ash Advisory Centers (VAACs) via a NOAA website. Operational issues arising from these improved SO₂ measurements include the reliability of SO₂ as proxy for co-erupted ash, the duration of VAAC advisories for long-lived volcanic clouds, and the potential effects of elevated concentrations of SO₂ and sulfate aerosol in ash-poor clouds on aircraft and avionics (including cumulative effects after multiple inadvertent transits through dilute clouds). Further research is required in these areas. Aviation community assistance is sought through continued reporting of sulfurous odors or other indications of diffuse volcanic cloud encounters, in order to validate the satellite retrievals.