Explore the vast range of titles available.

This review article summarizes the emerging field of quantum nonlinear optics. Three major approaches to generate optical nonlinearities based on cavity quantum electrodynamics, atomic ensembles with large Kerr nonlinearities and strong atomic interactions are reviewed. Applications of quantum nonlinear optics and many-body physics with strongly interacting photons are also discussed. The realization of strong interactions between individual photons is a long-standing goal of both fundamental and technological significance. Scientists have known for over half a century that light fields can interact inside nonlinear optical media, but the nonlinearity of conventional materials is negligible at the light powers associated with individual photons. Nevertheless, remarkable advances in quantum optics have recently culminated in the demonstration of several methods for generating optical nonlinearities at the level of individual photons. Systems exhibiting strong photon–photon interactions enable a number of unique applications, including quantum-by-quantum control of light fields, single-photon switches and transistors, all-optical deterministic quantum logic, and the realization of strongly correlated states of light and matter.

The properties of coupled emitters can differ dramatically from those of their individual constituents. Canonical examples include sub- and super-radiance, wherein the decay rate of a collective excitation is reduced or enhanced due to correlated interactions with the environment. Here, we systematically study the properties of collective excitations for regularly spaced arrays of quantum emitters coupled to a one-dimensional waveguide. We find that, for low excitation numbers, the modal properties are well-characterized by spin waves with a definite wavevector. Moreover, the decay rate of the most subradiant modes obeys a universal scaling with a cubic suppression in the number of emitters. Multi-excitation subradiant eigenstates can be built from fermionic combinations of single excitation eigenstates; such 'fermionization' results in multiple excitations that spatially repel one another. We put forward a method to efficiently create and measure such subradiant states, which can be realized with superconducting qubits. These measurement protocols probe both real-space correlations (using on-site dispersive readout) and temporal correlations in the emitted field (using photon correlation techniques).

We theoretically study the few- and many-body dynamics of photons in chiral waveguides. In particular, we examine pulse propagation through an ensemble ofNtwo-level systems chirally coupled to a waveguide. We show that the system supports correlated multiphoton bound states, which have a well-defined photon numbernand propagate through the system with a group delay scaling as1/n2. This has the interesting consequence that, during propagation, an incident coherent-state pulse breaks up into different bound-state components that can become spatially separated at the output in a sufficiently long system. For sufficiently many photons and sufficiently short systems, we show that linear combinations ofn-body bound states recover the well-known phenomenon of mean-field solitons in self-induced transparency. Our work thus covers the entire spectrum from few-photon quantum propagation, to genuine quantum many-body (atom and photon) phenomena, and ultimately the quantum-to-classical transition. Finally, we demonstrate that the bound states can undergo elastic scattering with additional photons. Together, our results demonstrate that photon bound states are truly distinct physical objects emerging from the most elementary light-matter interaction between photons and two-level emitters. Our work opens the door to studying quantum many-body physics and soliton physics with photons in chiral waveguide QED.

Tailoring the interactions between quantum emitters and single photons constitutes one of the cornerstones of quantum optics. Coupling a quantum emitter to the band edge of a photonic crystal waveguide (PCW) provides a unique platform for tuning these interactions. In particular, the cross-over from propagating fields E ( x ) ∝ e ± i k x x outside the bandgap to localized fields E ( x ) ∝ e − κ x | x | within the bandgap should be accompanied by a transition from largely dissipative atom–atom interactions to a regime where dispersive atom–atom interactions are dominant. Here, we experimentally observe this transition by shifting the band edge frequency of the PCW relative to the D₁ line of atomic cesium for N̄ = 3.0 ± 0.5 atoms trapped along the PCW. Our results are the initial demonstration of this paradigm for coherent atom–atom interactions with low dissipation into the guided mode.

A powerful method to interface quantum light with matter is to propagate the light through an ensemble of atoms. Recently, a number of such interfaces have emerged, most prominently Rydberg ensembles, that enable strong nonlinear interactions between propagating photons. A largely open problem is whether these systems produce exotic many-body states of light and developing new tools to study propagation in the large photon number limit is highly desirable. Here we provide a method based on a “spin model” that maps quasi one-dimensional (1D) light propagation to the dynamics of an open 1D interacting spin system, where all photon correlations are obtained from those of the spins. The spin dynamics in turn are numerically solved using the toolbox of matrix product states. We apply this formalism to investigate vacuum induced transparency, wherein the different photon number components of a pulse propagate with number-dependent group velocity and separate at output. Numerical simulation of light propagation through 1D atomic systems in the many-body limit rapidly saturates hardware capabilities. Here, the authors tackle the problem by mapping the dynamics to an open 1D interacting spin system and solving it using the matrix product state ansatz.

It is interesting to observe that all optical materials with a positive refractive index have a value of index that is of order unity. Surprisingly, though, a deep understanding of the mechanisms that lead to this universal behavior seems to be lacking. Moreover, this observation is difficult to reconcile with the fact that a single isolated atom is known to have a giant optical response, as characterized by a resonant scattering cross section that far exceeds its physical size. Here, we theoretically and numerically investigate the evolution of the optical properties of an ensemble of ideal atoms as a function of density, starting from the dilute gas limit, including the effects of multiple scattering and near-field interactions. Interestingly, despite the giant response of an isolated atom, we find that the maximum index does not indefinitely grow with increasing density but rather reaches a limiting value ofn≈1.7. This limit arises purely from electrodynamics, as it occurs at densities far below those where chemical processes become important. We propose an explanation based upon strong-disorder renormalization group theory, in which the near-field interaction combined with random atomic positions results in an inhomogeneous broadening of atomic resonance frequencies. This mechanism ensures that, regardless of the physical atomic density, light at any given frequency only interacts with at most a few near-resonant atoms per cubic wavelength, thus limiting the maximum index attainable. Our work is a promising first step to understand the limits of the refractive index from a bottom-up, atomic physics perspective, and it also introduces the renormalization group as a powerful tool to understand the generally complex problem of multiple scattering of light overall.

Optical trapping is an indispensable tool in physics and the life sciences. However, there is a clear trade off between the size of a particle to be trapped, its spatial confinement, and the intensities required. This is due to the decrease in optical response of smaller particles and the diffraction limit that governs the spatial variation of optical fields. It is thus highly desirable to find techniques that surpass these bounds. Recently, a number of experiments using nanophotonic cavities have observed a qualitatively different trapping mechanism described as 'self-induced back-action trapping' (SIBA). In these systems, the particle motion couples to the resonance frequency of the cavity, which results in a strong interplay between the intra-cavity field intensity and the forces exerted. Here, we provide a theoretical description that for the first time captures the remarkable range of consequences. In particular, we show that SIBA can be exploited to yield dynamic reshaping of trap potentials, strongly sub-wavelength trap features, and significant reduction of intensities seen by the particle, which should have important implications for future trapping technologies.

Cold atoms coupled to photonic crystals constitute an exciting platform for exploring quantum many-body physics. For example, such systems offer the potential to realize strong photon-mediated forces between atoms, which depend on the atomic internal (spin) states, and where both the motional and spin degrees of freedom can exhibit long coherence times. An intriguing question then is whether exotic phases could arise, wherein crystalline or other spatial patterns and spin correlations are fundamentally tied together, an effect that is atypical in condensed matter systems. Here, we analyse one realistic model Hamiltonian in detail. We show that this previously unexplored system exhibits a rich phase diagram of emergent orders, including spatially dimerized spin-entangled pairs, a fluid of composite particles comprised of joint spin-phonon excitations, phonon-induced Néel ordering, and a fractional magnetization plateau associated with trimer formation. Cold atoms coupled to photonic crystals constitute a platform for exploring many-body physics. Here the authors study the effect of coupling between the atomic internal degrees of freedom and motion, showing that such systems can realize extreme spin-orbital coupling and uncover a rich phase diagram.

There has been rapid development of systems that yield strong interactions between freely propagating photons in one-dimension via controlled coupling to quantum emitters. This raises interesting possibilities such as quantum information processing with photons or quantum many-body states of light, but treating such systems generally remains a difficult task theoretically. Here, we describe a novel technique in which the dynamics and correlations of a few photons can be exactly calculated, based upon knowledge of the initial photonic state and the solution of the reduced effective dynamics of the quantum emitters alone. We show that this generalized 'input-output' formalism allows for a straightforward numerical implementation regardless of system details, such as emitter positions, external driving, and level structure. As a specific example, we apply our technique to show how atomic systems with infinite-range interactions and under conditions of electromagnetically induced transparency enable the selective transmission of correlated multi-photon states.

Realizing systems that support robust, controlled interactions between individual photons is an exciting frontier of nonlinear optics. To this end, one approach that has emerged recently is to leverage atomic interactions to create strong and spatially nonlocal interactions between photons. In particular, effective photonic interactions have been successfully created via interactions between atoms excited to Rydberg levels. Here, we investigate an alternative approach, in which atomic interactions arise via their common coupling to photonic crystal waveguides. This technique takes advantage of the ability to separately tailor the strength and range of interactions via the dispersion engineering of the structure itself, which can lead to qualitatively new types of phenomena. For example, much of the work on photon-photon interactions relies on the linear optical effect of electromagnetically induced transparency, in combination with the use of interactions to shift optical pulses into or out of the associated transparency window. Here, we identify a large new class of “correlated transparency windows,” in which photonic states of a certain number and shape selectively propagate through the system. Through this technique, we show that molecular bound states of photon pairs can be created.