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"Chen, Xiangyu"
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A Review of Contact Electrification at Diversified Interfaces and Related Applications on Triboelectric Nanogenerator
by
Chen, Xiangyu
,
Hu, Jun
,
Iwamoto, Mitsumasa
in
Charge transfer
,
Electrification
,
Energy harvesting
2024
HighlightsThe distinctive characteristics, underlying mechanisms, diverse range of selected materials, and modification methods of contact electrification (CE) at various interfaces are summarized and comparatively analyzed, offering valuable guidance for future investigations of triboelectric nanogenerator (TENG) at different interfaces.This review gives a detailed insight into the unique applications of TENG relying on different interfacial electrification.The challenges and development prospects of TENGs based on CE are discussed.The triboelectric nanogenerator (TENG) can effectively collect energy based on contact electrification (CE) at diverse interfaces, including solid–solid, liquid–solid, liquid–liquid, gas–solid, and gas–liquid. This enables energy harvesting from sources such as water, wind, and sound. In this review, we provide an overview of the coexistence of electron and ion transfer in the CE process. We elucidate the diverse dominant mechanisms observed at different interfaces and emphasize the interconnectedness and complementary nature of interface studies. The review also offers a comprehensive summary of the factors influencing charge transfer and the advancements in interfacial modification techniques. Additionally, we highlight the wide range of applications stemming from the distinctive characteristics of charge transfer at various interfaces. Finally, this review elucidates the future opportunities and challenges that interface CE may encounter. We anticipate that this review can offer valuable insights for future research on interface CE and facilitate the continued development and industrialization of TENG.
Journal Article
Neutrophil membrane-coated nanoparticles inhibit synovial inflammation and alleviate joint damage in inflammatory arthritis
2018
Rheumatoid arthritis is a common chronic inflammatory disorder and a major cause of disability. Despite the progress made with recent clinical use of anti-cytokine biologics, the response rate of rheumatoid arthritis treatment remains unsatisfactory, owing largely to the complexity of cytokine interactions and the multiplicity of cytokine targets. Here, we show a nanoparticle-based broad-spectrum anti-inflammatory strategy for rheumatoid arthritis management. By fusing neutrophil membrane onto polymeric cores, we prepare neutrophil membrane-coated nanoparticles that inherit the antigenic exterior and associated membrane functions of the source cells, which makes them ideal decoys of neutrophil-targeted biological molecules. It is shown that these nanoparticles can neutralize proinflammatory cytokines, suppress synovial inflammation, target deep into the cartilage matrix, and provide strong chondroprotection against joint damage. In a mouse model of collagen-induced arthritis and a human transgenic mouse model of arthritis, the neutrophil membrane-coated nanoparticles show significant therapeutic efficacy by ameliorating joint damage and suppressing overall arthritis severity.
Journal Article
Triboelectric sensor with ultra-wide linear range based on water-containing elastomer and ion-rich interface
by
Chen, Xiangyu
,
Liu, Zhaoqi
,
Hu, Jun
in
639/301/1005/1007
,
639/4077/4072/4062
,
Contact pressure
2024
The incompatibility of the high sensitivity and wide linear range still restricts the further development of active sensors. Here we report a triboelectric pressure sensor based on water-containing triboelectric elastomer with gradient-based microchannels. Tiny amount of liquid is injected into the triboelectric elastomer and the pressure-induced water bridges can modulate the built-in electric field of the sensor, which enhance the signal linearity near the compression limit. Moreover, it has been found that liquid-solid contact electrification can be enhanced by triggering selective ionic transfer, while the prepared ion-rich interface in the microchannels boosts the sensitivity of the sensor. Hence, an ultra-wide linear range (5 kPa–1240 kPa) with a sensitivity of 0.023 V kPa
−1
can be achieved, which is so far the widest linear range of active sensors to our knowledge. Our work can promote the practical application of triboelectric sensors and provide new insights for other sensory devices.
The incompatibility between high sensitivity and a wide linear range has hindered the development of sensors. Here, the authors propose a pressure sensor that combines a water-containing triboelectric elastomer with gradient-based microchannels, achieving an ultra-wide linear range and high sensitivity simultaneously.
Journal Article
Flood sensitivity assessment of super cities
2023
In the context of global urbanization, more and more people are attracted to these cities with superior geographical conditions and strategic positions, resulting in the emergence of world super cities. However, with the increasing of urban development, the underlying surface of the city has changed, the soil originally covered with vegetation has been substituted by hardened pavement such as asphalt and cement roads. Therefore, the infiltration capacity of urban rainwater is greatly limited, and waterlogging is becoming more and more serious. In addition, the suburbs of the main urban areas of super cities are usually villages and mountains, and frequent flash floods seriously threaten the life and property safety of people in there. Flood sensitivity assessment is an effective method to predict and mitigate flood disasters. Accordingly, this study aimed at identifying the areas vulnerable to flood by using Geographic Information System (GIS) and Remote Sensing (RS) and apply Logistic Regression (LR) model to create a flood sensitivity map of Beijing. 260 flood points in history and 12 predictors [elevation, slope, aspect, distance to rivers, Topographic Wetness Index (TWI), Stream Power Index (SPI), Sediment Transport Index (STI), curvature, plan curvature, Land Use/Land Cover (LULC), soil, and rainfall] were used in this study. Even more noteworthy is that most of the previous studies discussed flash flood and waterlogging separately. However, flash flood points and waterlogging points were included together in this study. We evaluated the sensitivity of flash flood and waterlogging as a whole and obtained different results from previous studies. In addition, most of the previous studies focused on a certain river basin or small towns as the study area. Beijing is the world's ninth largest super cities, which was unusual in previous studies and has important reference significance for the flood sensitivity analysis of other super cities. The flood inventory data were randomly subdivided into training (70%) and test (30%) sets for model construction and testing using the Area Under Curve (AUC), respectively. The results turn out that: (1) elevation, slope, rainfall, LULC, soil and TWI were highly important among these elements, and were the most influential variables in the assessment of flood sensitivity. (2) The AUC of the test dataset revealed a prediction rate of 81.0%. The AUC was greater than 0.8, indicating that the model assessment accuracy was high. (3) The proportion of high risk and extremely high risk areas was 27.44%, including 69.26% of the flood events in this study, indicating that the flood distribution in these areas was relatively dense and the susceptibility was high. Super cities have a high population density, and once flood disasters occur, the losses brought by them are immeasurable. Thus, flood sensitivity map can provide meaningful information for policy makers to enact appropriate policies to reduce future damage.
Journal Article
Phototherapy in cancer treatment: strategies and challenges
2025
Phototherapy has emerged as a promising modality in cancer treatment, garnering considerable attention for its minimal side effects, exceptional spatial selectivity, and optimal preservation of normal tissue function. This innovative approach primarily encompasses three distinct paradigms: Photodynamic Therapy (PDT), Photothermal Therapy (PTT), and Photoimmunotherapy (PIT). Each of these modalities exerts its antitumor effects through unique mechanisms—specifically, the generation of reactive oxygen species (ROS), heat, and immune responses, respectively. However, significant challenges impede the advancement and clinical application of phototherapy. These include inadequate ROS production rates, subpar photothermal conversion efficiency, difficulties in tumor targeting, and unfavorable physicochemical properties inherent to traditional phototherapeutic agents (PTs). Additionally, the hypoxic microenvironment typical of tumors complicates therapeutic efficacy due to limited agent penetration in deep-seated lesions. To address these limitations, ongoing research is fervently exploring innovative solutions. The unique advantages offered by nano-PTs and nanocarrier systems aim to enhance traditional approaches’ effectiveness. Strategies such as generating oxygen in situ within tumors or inhibiting mitochondrial respiration while targeting the HIF-1α pathway may alleviate tumor hypoxia. Moreover, utilizing self-luminescent materials, near-infrared excitation sources, non-photoactivated sensitizers, and wireless light delivery systems can improve light penetration. Furthermore, integrating immunoadjuvants and modulating immunosuppressive cell populations while deploying immune checkpoint inhibitors holds promise for enhancing immunogenic cell death through PIT. This review seeks to elucidate the fundamental principles and biological implications of phototherapy while discussing dominant mechanisms and advanced strategies designed to overcome existing challenges—ultimately illuminating pathways for future research aimed at amplifying this intervention’s therapeutic efficacy.
Journal Article
Eye tracking and eye expression decoding based on transparent, flexible and ultra-persistent electrostatic interface
by
Chen, Xiangyu
,
Liu, Zhaoqi
,
Shi, Yuxiang
in
639/166/987
,
639/4077/4072/4062
,
Angular resolution
2023
Eye tracking provides valuable insight for analyzing visual attention and underlying thinking progress through the observation of eye movements. Here, a transparent, flexible and ultra-persistent electrostatic sensing interface is proposed for realizing active eye tracking (AET) system based on the electrostatic induction effect. Through a triple-layer structure combined with a dielectric bilayer and a rough-surface Ag nanowire (Ag NW) electrode layer, the inherent capacitance and interfacial trapping density of the electrostatic interface has been strongly enhanced, contributing to an unprecedented charge storage capability. The electrostatic charge density of the interface reached 1671.10 μC·m
−2
with a charge-keeping rate of 96.91% after 1000 non-contact operation cycles, which can finally realize oculogyric detection with an angular resolution of 5°. Thus, the AET system enables real-time decoding eye movements for customer preference recording and eye-controlled human-computer interaction, supporting its limitless potentiality in commercial purpose, virtual reality, human computer interactions and medical monitoring.
Eye tracking systems are crucial for eye health-monitoring and human-machine engineering. Here, Shi et. al. report a transparent and flexible active eye tracking system based on an electrostatic induction effect, enabling visual preference analysis and eye-controlled human-computer interaction.
Journal Article
Power generation from the interaction of a liquid droplet and a liquid membrane
2019
Triboelectric nanogenerators are an energy harvesting technology that relies on the coupling effects of contact electrification and electrostatic induction between two solids or a liquid and a solid. Here, we present a triboelectric nanogenerator that can work based on the interaction between two pure liquids. A liquid–liquid triboelectric nanogenerator is achieved by passing a liquid droplet through a freely suspended liquid membrane. We investigate two kinds of liquid membranes: a grounded membrane and a pre-charged membrane. The falling of a droplet (about 40 μL) can generate a peak power of 137.4 nW by passing through a pre-charged membrane. Moreover, this membrane electrode can also remove and collect electrostatic charges from solid objects, indicating a permeable sensor or charge filter for electronic applications. The liquid–liquid triboelectric nanogenerator can harvest mechanical energy without changing the object motion and it can work for many targets, including raindrops, irrigation currents, microfluidics, and tiny particles.
Triboelectric nanogenerators harvest energy by contacting two solids or a liquid and a solid. Here the authors use a conductive liquid membrane as a permeable electrode to demonstrate triboelectrification via liquid–liquid contact by passing liquid droplets through a liquid membrane to generate power.
Journal Article
Fabrication of triboelectric polymer films via repeated rheological forging for ultrahigh surface charge density
2022
Triboelectric polymer with high charge density is the foundation to promote the wide range of applications of triboelectric nanogenerators. This work develops a method to produce triboelectric polymer based on repeated rheological forging. The fluorinated ethylene propylene film fabricated by repeated forging method not only has excellent mechanical properties and good transmittance, but also can maintain an ultrahigh tribo-charge density. Based on the film with a thickness of 30 μm, the output charge density from contact-separation nanogenerator reaches 352 μC·m
−2
. Then, the same film is applied for the nanogenerator with air-breakdown mode and a charge density of 510 μC·m
−2
is further achieved. The repeated forging method can effectively regulate the composition of surface functional groups, the crystallinity, and the dielectric constants of the fluorinated ethylene propylene, leading to the superior capability of triboelectrification. Finally, we summarize the key parameters for elevating the electrification performance on the basis of molecular structure and related fabrication crafts, which can guide the further development of triboelectric polymers.
High charge density is the foundation to promote a wide range of applications of triboelectric nanogenerators. Here, authors propose a processing method based on the repeated rheological forging of triboelectric polymers achieving an enhanced triboelectricity and further study its mechanism.
Journal Article
Health status monitoring of cutting arm of anchor excavator based on digital twin
2026
Considering that the traditional finite element method takes a long time to calculate and can not meet the real-time stress analysis of complex equipment such as anchor-digging machine, this paper takes the cutting mechanism of anchor-digging machine as the research object. in this paper, a fast analysis method of mechanical characteristics based on digital twinning is proposed, and this method is combined with digital twinning technology. In this paper, a digital twin model is established, which can be used to analyze the real-time mechanical characteristics of the cutting arm of the excavating and anchoring machine. Firstly, based on dimensional analysis and similarity principle, the simulation model of cutting mechanism test-bed of anchor-digging machine is established, and the model is used in finite element simulation and digital twin model. Secondly, the finite element analysis of the cutting arm of the integrated digging and anchoring machine is carried out, and the finite element calculation results are evaluated. Then, a fast analysis method of mechanical characteristics of cutting mechanism of anchor-digging integrated machine based on agent model is put forward, and an agent model for mechanical characteristic analysis of anchor-digging integrated machine is established. After verifying the fitting accuracy of the surrogate model, the established surrogate model is applied to analyze the mechanical characteristics of the cutting arm of the integrated digging and anchoring machine, and the necessary evaluation of the analysis results is made. Finally, the agent model of rapid analysis of mechanical characteristics is applied to the digital twin model, and the digital twin monitoring platform of cutting mechanism of anchor-digging machine is built in Unity, which realizes the real-time mechanical characteristic analysis, real-time residual life analysis and health monitoring of the cutting mechanism of anchor-digging machine.
Journal Article
Simulation study on the vibration compaction process of concrete paving
2026
Vibration compaction is the core process for automatic pavers to achieve efficient compaction of materials, and its mechanism involves the complex coupling of particle dynamics and energy transfer. In this paper, a combined simulation of the discrete element method (EDEM) and reaction dynamics (RecurDyn) is adopted, combined with theoretical analysis, numerical simulation and laboratory experiments, to conduct an in-depth study on this process. Based on EDEM, a three-dimensional model of material particles is established to accurately simulate the particle motion trajectory, contact force distribution and stress transfer characteristics under vibration. The influence laws of vibration frequency, vibration area, vibration duration and paving thickness on the compaction effect are systematically analyzed. The results show that within a certain frequency range, the concrete compaction effect is continuously enhanced with the increase of vibration frequency; within a certain period of time, the extension of vibration duration can promote the improvement of compactness, the discharge of air bubbles and the structural stability; under a smaller paving area, the vibration energy transfer is more uniform and the compaction efficiency is higher; the increase of paving thickness will prolong the energy transfer path, intensify energy loss, and easily lead to uneven compactness between the upper and lower layers.
Journal Article