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In a joint experimental and theoretical effort, we report on the formation of a macrodroplet state in an ultracold bosonic gas of erbium atoms with strong dipolar interactions. By precise tuning of the s -wave scattering length below the so-called dipolar length, we observe a smooth crossover of the ground state from a dilute Bose-Einstein condensate to a dense macrodroplet state of more than 2×104atoms . Based on the study of collective excitations and loss features, we prove that quantum fluctuations stabilize the ultracold gas far beyond the instability threshold imposed by mean-field interactions. Finally, we perform expansion measurements, showing that although self-bound solutions are prevented by losses, the interplay between quantum stabilization and losses results in a minimal time-of-flight expansion velocity at a finite scattering length.

The concept of a roton, a special kind of elementary excitation forming a minimum of energy at finite momentum, has been essential for the understanding of the properties of superfluid 4He (ref. 1). In quantum liquids, rotons arise from the strong interparticle interactions, whose microscopic description remains debated2. In the realm of highly controllable quantum gases, a roton mode has been predicted to emerge due to magnetic dipole–dipole interactions despite their weakly interacting character3. This prospect has raised considerable interest4–12; yet roton modes in dipolar quantum gases have remained elusive to observations. Here we report experimental and theoretical studies of the momentum distribution in Bose–Einstein condensates of highly magnetic erbium atoms, revealing the existence of the long-sought roton mode. Following an interaction quench, the roton mode manifests itself with the appearance of symmetric peaks at well-defined finite momentum. The roton momentum follows the predicted geometrical scaling with the inverse of the confinement length along the magnetization axis. From the growth of the roton population, we probe the roton softening of the excitation spectrum in time and extract the corresponding imaginary roton gap. Our results provide a further step in the quest towards supersolidity in dipolar quantum gases13.

The Hubbard model underlies our understanding of strongly correlated materials. Whereas its standard form only comprises interactions between particles at the same lattice site, extending it to encompass long-range interactions is predicted to profoundly alter the quantum behavior of the system. We realize the extended Bose-Hubbard model for an ultracold gas of strongly magnetic erbium atoms in a three-dimensional optical lattice. Controlling the orientation of the atomic dipoles, we reveal the anisotropic character of the onsite interaction and hopping dynamics and their influence on the superfluid-to-Mott insulator quantum phase transition. Moreover, we observe nearest-neighbor interactions, a genuine consequence of the long-range nature of dipolar interactions. Our results lay the groundwork for future studies of exotic many-body quantum phases.

A supersolid is a counterintuitive phase of matter that combines the global phase coherence of a superfluid with a crystal-like self-modulation in space. Recently, such states have been experimentally realized using dipolar quantum gases. Here we investigate the response of a dipolar supersolid to an interaction quench that shatters the global phase coherence. We identify a parameter regime in which this out-of-equilibrium state rephases, indicating superfluid flow across the sample as well as an efficient dissipation mechanism. We find a crossover to a regime where the tendency to rephase gradually decreases until the system relaxes into an incoherent droplet array. Although a dipolar supersolid is, by its nature, ‘soft’, we capture the essential behaviour of the de- and rephasing process within a rigid Josephson junction array model. Yet, both experiment and simulation indicate that the interaction quench causes substantial collective mode excitations that connect to phonons in solids and affect the phase dynamics.A supersolid is a phase of matter featuring both crystalline order as a solid and global phase coherence as a superfluid. Now an experiment shows how this global phase coherence can be established across the system in a non-equilibrium process.

By combining theory and experiments, we demonstrate that dipolar quantum gases of bothEr166andDy164support a state with supersolid properties, where a spontaneous density modulation and a global phase coherence coexist. This paradoxical state occurs in a well-defined parameter range, separating the phases of a regular Bose-Einstein condensate and of an insulating droplet array, and is rooted in the roton mode softening, on the one side, and in the stabilization driven by quantum fluctuations, on the other side. Here, we identify the parameter regime for each of the three phases. In the experiment, we rely on a detailed analysis of the interference patterns resulting from the free expansion of the gas, quantifying both its density modulation and its global phase coherence. Reaching the phases via a slow interaction tuning, starting from a stable condensate, we observe thatEr166andDy164exhibit a striking difference in the lifetime of the supersolid properties, due to the different atom loss rates in the two systems. Indeed, while inEr166the supersolid behavior survives only a few tens of milliseconds, we observe coherent density modulations for more than 150 ms inDy164. Building on this long lifetime, we demonstrate an alternative path to reach the supersolid regime, relying solely on evaporative cooling starting from a thermal gas.

We show that for ultracold magnetic lanthanide atoms chaotic scattering emerges due to a combination of anisotropic interaction potentials and Zeeman coupling under an external magnetic field. This scattering is studied in a collaborative experimental and theoretical effort for both dysprosium and erbium. We present extensive atom-loss measurements of their dense magnetic Feshbach-resonance spectra, analyze their statistical properties, and compare to predictions from a random-matrix-theory-inspired model. Furthermore, theoretical coupled-channels simulations of the anisotropic molecular Hamiltonian at zero magnetic field show that weakly bound, near threshold diatomic levels form overlapping, uncoupled chaotic series that when combined are randomly distributed. The Zeeman interaction shifts and couples these levels, leading to a Feshbach spectrum of zero-energy bound states with nearest-neighbor spacings that changes from randomly to chaotically distributed for increasing magnetic field. Finally, we show that the extreme temperature sensitivity of a small, but sizable fraction of the resonances in the Dy and Er atom-loss spectra is due to resonant nonzero partial-wave collisions. Our threshold analysis for these resonances indicates a large collision-energy dependence of the three-body recombination rate.

Activating transitions between a set of atomic internal states has emerged as an elegant scheme by which lattice models can be designed in ultracold atomic gases. In this approach, the internal states can be viewed as fictitious lattice sites defined along a synthetic dimension, hence offering a powerful method by which the spatial dimensionality of the system can be extended. Inter-particle collisions generically lead to infinite-range interactions along the synthetic dimensions, which a priori precludes the design of Bose-Hubbard-type models featuring on-site interactions. In this article, we solve this obstacle by introducing a protocol that realizes strong and tunable \"on-site\" interactions along an atomic synthetic dimension. Our scheme is based on pulsing strong intra-spin interactions in a fast and periodic manner, hence realizing the desired \"on-site\" interactions in a digital (Trotterized) manner. We explore the viability of this protocol by means of numerical calculations, which we perform on various examples that are relevant to ultracold-atom experiments. This general method, which could be applied to various atomic species by means of fast-response protocols based on Fano-Feshbach resonances, opens the route for the exploration of strongly-correlated matter in synthetic dimensions.

We investigate the excitation spectrum and compressibility of a dipolar Bose-Einstein condensate in an infinite tube potential in the parameter regime where the transition between superfluid and supersolid phases occurs. Our study focuses on the density range in which crystalline order develops continuously across the transition. Above the transition the superfluid shows a single gapless excitation band, phononic at small momenta and with a roton at a finite momentum. Below the transition, two gapless excitations branches (three at the transition point) emerge in the supersolid. We examine the two gapless excitation bands and their associated speeds of sound in the supersolid phase. Our results show that the speeds of sound and the compressibility are discontinuous at the transition, indicating a second-order phase transition. These results provide valuable insights into the identification of supersolid phenomena in dipolar quantum gases and the relationship to supersolidity in spin-orbit coupled gases.

We present a theory for the emergence of a supersolid state in a cigar-shaped dipolar quantum Bose gas. Our approach is based on a reduced three-dimensional (3D) theory, where the condensate wavefunction is decomposed into an axial field and a transverse part described variationally. This provides an accurate fully 3D description that is specific to the regime of current experiments and efficient to compute. We apply this theory to understand the phase diagram for a gas in an infinite tube potential. We find that the supersolid transition has continuous and discontinuous regions as the averaged density varies. We develop two simplified analytic models to characterize the phase diagram and elucidate the roles of quantum droplets and of the roton excitation.

An accurate knowledge of the scattering length is fundamental in ultracold quantum gas experiments and essential for the characterisation of the system as well as for a meaningful comparison to theoretical models. Here, we perform a careful characterisation of the s-wave scattering length \\(a_s\\) for the four highest-abundance isotopes of erbium, in the magnetic field range from 0G to 5G. We report on cross-dimensional thermalization measurements and apply the Enskog equations of change to numerically simulate the thermalization process and to analytically extract an expression for the so-called number of collisions per re-thermalization (NCPR) to obtain \\(a_s\\) from our experimental data. We benchmark the applied cross-dimensional thermalization technique with the experimentally more demanding lattice modulation spectroscopy and find good agreement for our parameter regime. Our experiments are compatible with a dependence of the NCPR with \\(a_s\\), as theoretically expected in the case of strongly dipolar gases. Surprisingly, we experimentally observe a dependency of the NCPR on the density, which might arise due to deviations from an ideal harmonic trapping configuration. Finally, we apply a model for the dependency of the background scattering length with the isotope mass, allowing to estimate the number of bound states of erbium.