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"Clerbaux, Cathy"
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Surface-to-Space Atmospheric Waves From Hunga Tonga–Hunga Ha’apai Eruption
2022
The January 2022 Hunga Tonga–Hunga Ha’apai eruption was one of the most explosive volcanic events of the modern era, producing a vertical plume that peaked more than 50 km above the Earth. The initial explosion and subsequent plume triggered atmospheric waves that propagated around the world multiple times. A global-scale wave response of this magnitude from a single source has not previously been observed. Here we show the details of this response, using a comprehensive set of satellite and ground-based observations to quantify it from surface to ionosphere. A broad spectrum of waves was triggered by the initial explosion, including Lamb waves propagating at phase speeds of 318.2 ± 6 m s^(−1) at surface level and between 308 ± 5 to 319 ± 4 m s^(−1) in the stratosphere, and gravity waves propagating at 238 ± 3 to 269 ± 3 m s^(−1) in the stratosphere. Gravity waves at sub-ionospheric heights have not previously been observed propagating at this speed or over the whole Earth from a single source. Latent heat release from the plume remained the most significant individual gravity wave source worldwide for more than 12 h, producing circular wavefronts visible across the Pacific basin in satellite observations. A single source dominating such a large region is also unique in the observational record. The Hunga Tonga eruption represents a key natural experiment in how the atmosphere responds to a sudden point-source-driven state change, which will be of use for improving weather and climate models.
Journal Article
Remote sensing and model analysis of biomass burning smoke transported across the Atlantic during the 2020 Western US wildfire season
by
Parrington, Mark
,
Clerbaux, Cathy
,
Coopman, Quentin
in
704/106/35/823
,
704/106/694/2739
,
704/172/169/824
2023
Biomass burning is the main source of air pollution in several regions worldwide nowadays. This predominance is expected to increase in the upcoming years as a result of the rising number of devastating wildfires due to climate change. Harmful pollutants contained in the smoke emitted by fires can alter downwind air quality both locally and remotely as a consequence of the recurrent transport of biomass burning plumes across thousands of kilometers. Here, we demonstrate how observations of carbon monoxide and aerosol optical depth retrieved from polar orbiting and geostationary meteorological satellites can be used to study the long-range transport and evolution of smoke plumes. This is illustrated through the megafire events that occurred during summer 2020 in the Western United States and the transport of the emitted smoke across the Atlantic Ocean to Europe. Analyses from the Copernicus Atmosphere Monitoring Service, which combine satellite observations with an atmospheric model, are used for comparison across the region of study and along simulated air parcel trajectories. Lidar observation from spaceborne and ground-based instruments are used to verify consistency of passive observations. Results show the potential of joint satellite-model analysis to understand the emission, transport, and processing of smoke across the world.
Journal Article
Global, regional and national trends of atmospheric ammonia derived from a decadal (2008–2018) satellite record
by
van Zanten, Margreet
,
Clerbaux, Cathy
,
Erisman, Jan Willem
in
agriculture
,
Air quality
,
Ammonia
2021
Excess atmospheric ammonia (NH 3 ) leads to deleterious effects on biodiversity, ecosystems, air quality and health, and it is therefore essential to monitor its budget and temporal evolution. Hyperspectral infrared satellite sounders provide daily NH 3 observations at global scale for over a decade. Here we use the version 3 of the Infrared Atmospheric Sounding Interferometer (IASI) NH 3 dataset to derive global, regional and national trends from 2008 to 2018. We find a worldwide increase of 12.8 ± 1.3 % over this 11-year period, driven by large increases in east Asia (5.80 ± 0.61% increase per year), western and central Africa (2.58 ± 0.23 % yr −1 ), North America (2.40 ± 0.45 % yr −1 ) and western and southern Europe (1.90 ± 0.43 % yr −1 ). These are also seen in the Indo-Gangetic Plain, while the southwestern part of India exhibits decreasing trends. Reported national trends are analyzed in the light of changing anthropogenic and pyrogenic NH 3 emissions, meteorological conditions and the impact of sulfur and nitrogen oxides emissions, which alter the atmospheric lifetime of NH 3 . We end with a short case study dedicated to the Netherlands and the ‘Dutch Nitrogen crisis’ of 2019.
Journal Article
Ethylene industrial emitters seen from space
by
Clarisse, Lieven
,
Coheur, Pierre-François
,
Clerbaux, Cathy
in
639/638/169/824
,
704/172/169/824
,
704/445/824
2022
Volatile organic compounds are emitted abundantly from a variety of natural and anthropogenic sources. However, in excess, they can severely degrade air quality. Their fluxes are currently poorly represented in inventories due to a lack of constraints from global measurements. Here, we track from space over 300 worldwide hotspots of ethylene, the most abundant industrially produced organic compound. We identify specific emitters associated with petrochemical clusters, steel plants, coal-related industries, and megacities. Satellite-derived fluxes reveal that the ethylene emissions of the industrial sources are underestimated or missing in the state-of-the-art Emission Database for Global Atmospheric Research (EDGAR) inventory. This work exposes global emission point-sources of a short-lived carbonated gas, complementing the ongoing large-scale efforts on the monitoring of inorganic pollutants.
Combining 13 years of satellite measurements led to the discovery of 300 global hotspots of atmospheric ethylene (C
2
H
4
). They are found to be linked to heavy industries and megacities, and are currently misrepresented in emission inventories.
Journal Article
Version 2 of the IASI NH3 neural network retrieval algorithm: near-real-time and reanalysed datasets
by
Whitburn, Simon
,
Clerbaux, Cathy
,
Pierre-François Coheur
in
Algorithms
,
Ammonia
,
Artificial neural networks
2017
Recently, presented a neural-network-based algorithm for retrieving atmospheric ammonia (NH3) columns from Infrared Atmospheric Sounding Interferometer (IASI) satellite observations. In the past year, several improvements have been introduced, and the resulting new baseline version, Artificial Neural Network for IASI (ANNI)-NH3-v2.1, is documented here. One of the main changes to the algorithm is that separate neural networks were trained for land and sea observations, resulting in a better training performance for both groups. By reducing and transforming the input parameter space, performance is now also better for observations associated with favourable sounding conditions (i.e. enhanced thermal contrasts). Other changes relate to the introduction of a bias correction over land and sea and the treatment of the satellite zenith angle. In addition to these algorithmic changes, new recommendations for post-filtering the data and for averaging data in time or space are formulated. We also introduce a second dataset (ANNI-NH3-v2.1R-I) which relies on ERA-Interim ECMWF meteorological input data, along with surface temperature retrieved from a dedicated network, rather than the operationally provided Eumetsat IASI Level 2 (L2) data used for the standard near-real-time version. The need for such a dataset emerged after a series of sharp discontinuities were identified in the NH3 time series, which could be traced back to incremental changes in the IASI L2 algorithms for temperature and clouds. The reanalysed dataset is coherent in time and can therefore be used to study trends. Furthermore, both datasets agree reasonably well in the mean on recent data, after the date when the IASI meteorological L2 version 6 became operational (30 September 2014).
Journal Article
The unintended consequence of SO2 and NO2 regulations over China: increase of ammonia levels and impact on PM2.5 concentrations
by
Siour, Guillaume
,
Clerbaux, Cathy
,
tems-Cheiney, Audrey
in
Air pollution
,
Ammonia
,
Ammonia content
2019
Air pollution reaching hazardous levels in many Chinese cities has been a major concern in China over the past decades. New policies have been applied to regulate anthropogenic pollutant emissions, leading to changes in atmospheric composition and in particulate matter (PM) production. Increasing levels of atmospheric ammonia columns have been observed by satellite during recent years. In particular, observations from the Infrared Atmospheric Sounding Interferometer (IASI) reveal an increase of these columns by 15 % and 65 % from 2011 to 2013 and 2015, respectively, over eastern China. In this paper we performed model simulations for 2011, 2013 and 2015 in order to understand the origin of this increase and to quantify the link between ammonia and the inorganic components of particles: NH4(p)+/SO4(p)2-/NO3(p)-. Interannual change of meteorology can be excluded as a reason: year 2015 meteorology leads to enhanced sulfate production over eastern China, which increases the ammonium and decreases the ammonia content, which is contrary to satellite observations. Reductions in SO2 and NOx emissions from 2011 to 2015 of 37.5 % and 21 % respectively, as constrained from satellite data, lead to decreased inorganic matter (by 14 % for NH4(p)++SO4(p)2-+NO3(p)-). This in turn leads to increased gaseous NH3(g) tropospheric columns by as much as 24 % and 49 % (sampled corresponding to IASI data availability) from 2011 to 2013 and 2015 respectively and thus can explain most of the observed increase.
Journal Article
Local hourly trends in near-surface and land surface temperatures
2025
Essential Climate Variables, such as near-surface (T2m) and land surface temperatures (LST), are typically reported in Coordinated Universal Time (UTC) for global consistency. However, their diurnal variability leads to temperature trends that differ by the local hour, a factor not analyzed on the global nor regional scale. Using ECMWF ERA5-Land reanalysis data (1981–2022), we assess temperature trends by local hour and month. Our results show that the trends can change significantly during the day. LST and T2m warming or cooling trends peak in the afternoon, while showing large spatial variability across both hemispheres. Using MODIS observations, we show how the nominal Equator crossing times of TERRA and AQUA influence LST trends. These findings highlight the necessity of accounting for local time in climate assessments to improve adaptation strategies.
Journal Article
Global ammonia distribution derived from infrared satellite observations
by
Clarisse, Lieven
,
Coheur, Pierre-François
,
Clerbaux, Cathy
in
Air quality
,
Algal blooms
,
Ammonia
2009
Ammonia is a significant atmospheric pollutant, accelerating the formation of particulate matter and damaging aquatic and terrestrial ecosystems. Infrared measurements of ammonia concentrations, obtained by the IASI/MetOp satellite, suggest that ammonia emissions in the Northern Hemisphere have been markedly underestimated.
Global ammonia emissions have more than doubled since pre-industrial times, largely owing to agricultural intensification and widespread fertilizer use
1
. In the atmosphere, ammonia accelerates particulate matter formation, thereby reducing air quality. When deposited in nitrogen-limited ecosystems, ammonia can act as a fertilizer. This can lead to biodiversity reductions in terrestrial ecosystems, and algal blooms in aqueous environments
2
,
3
,
4
,
5
,
6
,
7
,
8
. Despite its ecological significance, there are large uncertainties in the magnitude of ammonia emissions, mainly owing to a paucity of ground-based observations and a virtual absence of atmospheric measurements
3
,
8
,
9
,
10
,
11
. Here we use infrared spectra, obtained by the IASI/MetOp satellite, to map global ammonia concentrations from space over the course of 2008. We identify several ammonia hotspots in middle–low latitudes across the globe. In general, we find a good qualitative agreement between our satellite measurements and simulations made using a global atmospheric chemistry transport model. However, the satellite data reveal substantially higher concentrations of ammonia north of 30
∘
N, compared with model projections. We conclude that ammonia emissions could have been significantly underestimated in the Northern Hemisphere, and suggest that satellite monitoring of ammonia from space will improve our understanding of the global nitrogen cycle.
Journal Article
Tropical Cyclone Detection from the Thermal Infrared Sensor IASI Data Using the Deep Learning Model YOLOv3
2023
Tropical cyclone (TC) detection is essential to mitigate natural disasters, as TCs can cause significant damage to life, infrastructure and economy. In this study, we applied the deep learning object detection model YOLOv3 to detect TCs in the North Atlantic Basin, using data from the Thermal InfraRed (TIR) Atmospheric Sounding Interferometer (IASI) onboard the Metop satellites. IASI measures the outgoing TIR radiation of the Earth-Atmosphere. For the first time, we provide a proof of concept of the possibility of constructing images required by YOLOv3 from a TIR remote sensor that is not an imager. We constructed a dataset by selecting 50 IASI radiance channels and using them to create images, which we labeled by constructing bounding boxes around TCs using the hurricane database HURDAT2. We trained the YOLOv3 on two settings, first with three “best” selected channels, then using an autoencoder to exploit all 50 channels. We assessed its performance with the Average Precision (AP) metric at two different intersection over union (IoU) thresholds (0.1 and 0.5). The model achieved promising results with AP at IoU threshold 0.1 of 78.31%. Lower performance was achieved with IoU threshold 0.5 (31.05%), showing the model lacks precision regarding the size and position of the predicted boxes. Despite that, we show YOLOv3 demonstrates great potential for TC detection using TIR instruments data.
Journal Article
Monitoring emissions from the 2015 Indonesian fires using CO satellite data
by
Nechita-Banda, Narcisa
,
van der Werf, Guido R.
,
Kaiser, Johannes W.
in
Air Pollutants - analysis
,
Atmosphere
,
Atmospheric and Oceanic Physics
2018
Southeast Asia, in particular Indonesia, has periodically struggled with intense fire events. These events convert substantial amounts of carbon stored as peat to atmospheric carbon dioxide (CO2) and significantly affect atmospheric composition on a regional to global scale. During the recent 2015 El Niño event, peat fires led to strong enhancements of carbon monoxide (CO), an air pollutant and well-known tracer for biomass burning. These enhancements were clearly observed from space by the Infrared Atmospheric Sounding Interferometer (IASI) and the Measurements of Pollution in the Troposphere (MOPITT) instruments. We use these satellite observations to estimate CO fire emissions within an inverse modelling framework. We find that the derived CO emissions for each sub-region of Indonesia and Papua are substantially different from emission inventories, highlighting uncertainties in bottom-up estimates. CO fire emissions based on either MOPITT or IASI have a similar spatial pattern and evolution in time, and a 10% uncertainty based on a set of sensitivity tests we performed. Thus, CO satellite data have a high potential to complement existing operational fire emission estimates based on satellite observations of fire counts, fire radiative power and burned area, in better constraining fire occurrence and the associated conversion of peat carbon to atmospheric CO2. A total carbon release to the atmosphere of 0.35–0.60 Pg C can be estimated based on our results.
This article is part of a discussion meeting issue ‘The impact of the 2015/2016 El Niño on the terrestrial tropical carbon cycle: patterns, mechanisms and implications'.
Journal Article