Explore the vast range of titles available.

The FEBIAD ion source is routinely used to produce radioactive ions of halogens, molecules, and noble gases in several ISOL facilities worldwide. At TRIUMF, an extensive numerical and experimental campaign has been performed to fundamentally understand the source while improving its reliability and overall performance. Particularly, the cathode temperature has been studied by pyrometric measurements, Schottky analysis and numerical simulations to properly understand the electron emission driving the ionization. The temperature values found are consistent within the error bars and confirm the equivalence of the methodologies used. The findings can be used as part of a numerical ionization model for more realistic electron emission and the benchmarked thermal model can be used to propose novel and more robust geometries.

The ISAC-FEBIAD is an electron impact ion source typically used to ionize radioactive molecules or isotopes of elements beyond the reach of either surface or laser ion sources. The FEBIAD’s key tuning parameters are the cathode temperature defining the number of electrons created; the anode voltage establishing the electron energy; and the magnetic field controlling the electron density inside the anode volume. However, these parameters are typically scanned in a small and limited range when optimizing the source. Recent investigations have shown the need to explore the entire range of operational values accessible by the power supplies, not only due to the intrinsic variations from source to source but also to operate the source at optimal settings. To address this, a scanning algorithm has been implemented as a web interface thanks to the High-Level-Application (HLA) infrastructure available at TRIUMF. The ion beam intensity during both offline and online commissioning of the web app are presented here as contour plots. The optimal settings found for stable 20 Ne are confirmed as the optimal settings for radioactive 18 Ne. The main takeaway, however, is that the optimal ion source parameters differ between singly-charged, doubly-charged, and molecular species. This development demonstrate and facilitate the need for element and charge state-specific parameter optimization. Additionally, the results highlight the possibility of parameter optimization to enhance the ratio of the species of interest to co-ionized contamination.

At TRIUMF’s ISAC facility, 1+ Radioactive Ion Beams (RIBs) of noble gases, halogens, and molecules are created using a Forced Electron Beam Induced Arc Discharge (FEBIAD) ion source. Reported ionization efficiencies for FEBIADs range from 10% to 25% for 40 Ar + , while TRIUMF-FEBIAD ionization efficiency seems to be < 1% with a 90% emittance <15 μm. As RIB ion sources aim for a high ionization efficiency, an experimental and numerical campaign was conducted to investigate the comparably low efficiencies observed. The experimental results for 40 Ar + indicate that up to a 10% ionization efficiency is possible by operating the source at different parameters. The measurements agree with theoretical estimations; however, certain combinations of parameters produce an anomalously high electron current which enhances the ionization efficiency threefold. Present investigations aim to characterize and model the anomalous electron current because, if proven reliable, the argon ionization efficiency could reach 30% with no significant impact on beam emittance.

Any ISOL facility pushing the boundaries of nuclear physics must be able to provide cutting-edge ion beams to its users - beams of isotopes far from stability, with few contaminants, that may be difficult to extract from an ISOL target. The development of these pure, exotic beams must be supported by continuing research and development on targets and ion sources. In the ARIEL era, new target/ion source geometries and operational modes will provide new opportunities which can only be exploited with time for development. To prioritize this, TRIUMF proposes to build a dedicated test stand for target and ion source research which will model the critical features of the new ARIEL target stations. This stand will provide a testing ground for methods of increasing efficiency and selectivity, such as investigations of new surface ion source [1, 2] and Forced Electron Beam Induced Arc Discharge (FEBIAD) ion source [3, 2] designs. In addition, this will provide a development environment for new beams, either from new target materials, or through techniques such as extracting molecular beams. In order to maximize the gain from these investigations in on-line operation, the ion optical properties of the final beam will be investigated concurrently.

At ISAC-TRIUMF, a 500 MeV proton beam is impinged upon \"thick\" targets to induce nuclear reactions to produce reaction products that are delivered as a Radioactive Ion Beam (RIB) to experiments. Uranium carbide is among the most commonly used target materials which produces a vast radionuclide inventory coming from both spallation and fission-events. This can also represent a major limitation for the successful delivery of certain RIBs to experiments since, for a given mass, many isobaric isotopes are to be filtered by the dipole mass separator. These contaminants can exceed the yield of the isotope of interest by orders of magnitude, often causing a significant reduction in the sensitivity of experiments or even making them impossible. The design of a 50 kW proton-to-neutron (p2n) converter-target is ongoing to enhance the production of neutron-rich nuclei while significantly reducing the rate of neutron-deficient contaminants. The converter is made out of a bulk tungsten block which converts proton beams into neutrons through spallation. The neutrons, in turn, induce pure fission in an upstream UCx target. The present target design and the service infra-structure needed for its operation will be discussed in this paper.

Nuclear charge radii globally scale with atomic mass number A as A 1∕3 , and isotopes with an odd number of neutrons are usually slightly smaller in size than their even-neutron neighbours. This odd–even staggering, ubiquitous throughout the nuclear landscape 1 , varies with the number of protons and neutrons, and poses a substantial challenge for nuclear theory 2 – 4 . Here, we report measurements of the charge radii of short-lived copper isotopes up to the very exotic 78 Cu (with proton number Z = 29 and neutron number N = 49), produced at only 20 ions s –1 , using the collinear resonance ionization spectroscopy method at the Isotope Mass Separator On-Line Device facility (ISOLDE) at CERN. We observe an unexpected reduction in the odd–even staggering for isotopes approaching the N = 50 shell gap. To describe the data, we applied models based on nuclear density functional theory 5 , 6 and A -body valence-space in-medium similarity renormalization group theory 7 , 8 . Through these comparisons, we demonstrate a relation between the global behaviour of charge radii and the saturation density of nuclear matter, and show that the local charge radii variations, which reflect the many-body polarization effects, naturally emerge from A -body calculations fitted to properties of A ≤ 4 nuclei. Isotopes with an odd number of neutrons are usually slightly smaller in size than their even-neutron neighbours. In charge radii of short-lived copper isotopes, a reduction of this effect is observed when the neutron number approaches fifty.

In rare cases, the removal of a single proton (Z) or neutron (N) from an atomic nucleus leads to a dramatic shape change. These instances are crucial for understanding the components of the nuclear interactions that drive deformation. The mercury isotopes (Z = 80) are a striking example1,2: their close neighbours, the lead isotopes (Z = 82), are spherical and steadily shrink with decreasing N. The even-mass (A = N + Z) mercury isotopes follow this trend. The odd-mass mercury isotopes 181,183,185Hg, however, exhibit noticeably larger charge radii. Due to the experimental difficulties of probing extremely neutron-deficient systems, and the computational complexity of modelling such heavy nuclides, the microscopic origin of this unique shape staggering has remained unclear. Here, by applying resonance ionization spectroscopy, mass spectrometry and nuclear spectroscopy as far as 177Hg, we determine 181Hg as the shape-staggering endpoint. By combining our experimental measurements with Monte Carlo shell model calculations, we conclude that this phenomenon results from the interplay between monopole and quadrupole interactions driving a quantum phase transition, for which we identify the participating orbitals. Although shape staggering in the mercury isotopes is a unique and localized feature in the nuclear chart, it nicely illustrates the concurrence of single-particle and collective degrees of freedom at play in atomic nuclei.

The determination of the effective electron neutrino mass via kinematic analysis of beta and electron capture spectra is considered to be model-independent since it relies on energy and momentum conservation. At the same time the precise description of the expected spectrum goes beyond the simple phase space term. In particular for electron capture processes, many-body electron-electron interactions lead to additional structures besides the main resonances in calorimetrically measured spectra. A precise description of the 163Ho spectrum is fundamental for understanding the impact of low intensity structures at the endpoint region where a finite neutrino mass affects the shape most strongly. We present a low-background and high-energy resolution measurement of the 163Ho spectrum obtained in the framework of the ECHo experiment. We study the line shape of the main resonances and multiplets with intensities spanning three orders of magnitude. We discuss the need to introduce an asymmetric line shape contribution due to Auger–Meitner decay of states above the auto-ionisation threshold. With this we determine an enhancement of count rate at the endpoint region of about a factor of 2, which in turn leads to an equal reduction in the required exposure of the experiment to achieve a given sensitivity on the effective electron neutrino mass.

The Electron Capture in 163 Ho experiment, ECHo, is designed to investigate the electron neutrino mass in the sub-eV range by means of the analysis of the calorimetrically measured spectrum following the electron capture (EC) in 163 Ho. Arrays of low-temperature metallic magnetic calorimeters (MMCs), read-out by microwave SQUID multiplexing, will be used in this experiment. With a first MMC prototype having the 163 Ho source ion-implanted into the absorber, we performed the first high energy resolution measurement of the EC spectrum, which demonstrated the feasibility of such an experiment. In addition to the technological challenges for the development of MMC arrays, which preserve the single pixel performance in terms of energy resolution and bandwidth, the success of the experiment relies on the availability of large ultra-pure 163 Ho samples, on the precise description of the expected spectrum, and on the identification and reduction of background. We present preliminary results obtained with standard MMCs developed for soft X-ray spectroscopy, maXs-20, where the 163 Ho ion-implantation was performed using a high-purity 163 Ho source produced by advanced chemical and mass separation. With these measurements, we aim at determining an upper limit for the background level due to source contamination and provide a refined description of the calorimetrically measured spectrum. We discuss the plan for a medium scale experiment, ECHo-1k, in which about 1000 Bq of high-purity 163 Ho will be ion-implanted into detector arrays. With one year of measuring time, we will be able to achieve a sensitivity on the electron neutrino mass below 20 eV/c 2 (90  % C.L.), improving the present limit by more than one order of magnitude. This experiment will guide the necessary developments to reach the sub-eV sensitivity.