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"Empl, A."
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8.4% efficient fullerene-free organic solar cells exploiting long-range exciton energy transfer
2014
In order to increase the power conversion efficiency of organic solar cells, their absorption spectrum should be broadened while maintaining efficient exciton harvesting. This requires the use of multiple complementary absorbers, usually incorporated in tandem cells or in cascaded exciton-dissociating heterojunctions. Here we present a simple three-layer architecture comprising two non-fullerene acceptors and a donor, in which an energy-relay cascade enables an efficient two-step exciton dissociation process. Excitons generated in the remote wide-bandgap acceptor are transferred by long-range Förster energy transfer to the smaller-bandgap acceptor, and subsequently dissociate at the donor interface. The photocurrent originates from all three complementary absorbing materials, resulting in a quantum efficiency above 75% between 400 and 720 nm. With an open-circuit voltage close to 1 V, this leads to a remarkable power conversion efficiency of 8.4%. These results confirm that multilayer cascade structures are a promising alternative to conventional donor-fullerene organic solar cells.
Organic solar cells usually require the incorporation of costly fullerene acceptor layers. Cnops
et al.
report a multilayer organic solar cell that extracts photogenerated excitons by a two-step mechanism and achieves unprecedented conversion efficiencies of up to 8.4% without the use of fullerenes.
Journal Article
The DarkSide Multiton Detector for the Direct Dark Matter Search
2015
Although the existence of dark matter is supported by many evidences, based on astrophysical measurements, its nature is still completely unknown. One major candidate is represented by weakly interacting massive particles (WIMPs), which could in principle be detected through their collisions with ordinary nuclei in a sensitive target, producing observable low-energy (<100 keV) nuclear recoils. The DarkSide program aims at the WIPMs detection using a liquid argon time projection chamber (LAr-TPC). In this paper we quickly review the DarkSide program focusing in particular on the next generation experiment DarkSide-G2, a 3.6-ton LAr-TPC. The different detector components are described as well as the improvements needed to scale the detector from DarkSide-50 (50 kg LAr-TPC) up to DarkSide-G2. Finally, the preliminary results on background suppression and expected sensitivity are presented.
Journal Article
DarkSide-20k: A 20 tonne two-phase LAr TPC for direct dark matter detection at LNGS
2018
.
Building on the successful experience in operating the DarkSide-50 detector, the DarkSide Collaboration is going to construct DarkSide-20k, a direct WIMP search detector using a two-phase Liquid Argon Time Projection Chamber (LAr TPC) with an active (fiducial) mass of 23 t (20 t). This paper describes a preliminary design for the experiment, in which the DarkSide-20k LAr TPC is deployed within a shield/veto with a spherical Liquid Scintillator Veto (LSV) inside a cylindrical Water Cherenkov Veto (WCV). This preliminary design provides a baseline for the experiment to achieve its physics goals, while further development work will lead to the final optimization of the detector parameters and an eventual technical design. Operation of DarkSide-50 demonstrated a major reduction in the dominant
39
Ar background when using argon extracted from an underground source, before applying pulse shape analysis. Data from DarkSide-50, in combination with MC simulation and analytical modeling, shows that a rejection factor for discrimination between electron and nuclear recoils of
>
3
×
10
9
is achievable. This, along with the use of the veto system and utilizing silicon photomultipliers in the LAr TPC, are the keys to unlocking the path to large LAr TPC detector masses, while maintaining an experiment in which less than
<
0
.
1
events (other than
ν
-induced nuclear recoils) is expected to occur within the WIMP search region during the planned exposure. DarkSide-20k will have ultra-low backgrounds than can be measured
in situ
, giving sensitivity to WIMP-nucleon cross sections of
1
.
2
×
10
-
47
cm
2
(
1
.
1
×
10
-
46
cm
2
) for WIMPs of 1 TeV/c
2
(10 TeV/c
2
) mass, to be achieved during a 5 yr run producing an exposure of 100 t yr free from any instrumental background.
Journal Article
Neutrinos from the primary proton–proton fusion process in the Sun
by
Ranucci, G
,
Montuschi, M
,
Fomenko, K
in
639/766/33/34/866
,
639/766/387/1126
,
639/766/419/1131
2014
In the core of the Sun, energy is released through sequences of nuclear reactions that convert hydrogen into helium. The primary reaction is thought to be the fusion of two protons with the emission of a low-energy neutrino. These so-called
pp
neutrinos constitute nearly the entirety of the solar neutrino flux, vastly outnumbering those emitted in the reactions that follow. Although solar neutrinos from secondary processes have been observed, proving the nuclear origin of the Sun’s energy and contributing to the discovery of neutrino oscillations, those from proton–proton fusion have hitherto eluded direct detection. Here we report spectral observations of
pp
neutrinos, demonstrating that about 99 per cent of the power of the Sun, 3.84 × 10
33
ergs per second, is generated by the proton–proton fusion process.
Spectral observations of the low-energy neutrinos produced by proton–proton fusion in the Sun demonstrate that about 99 per cent of the Sun’s power is generated by this process.
Sun's elusive
pp
neutrinos tracked down
The Sun's energy output derives from a sequence of nuclear reactions that converts hydrogen into helium, most of it from the fusion of two protons (the proton–proton or
pp
reaction) accompanied by the release of a low-energy neutrino. These neutrinos have proved elusive: only solar neutrinos from secondary reactions had been directly observed. But here the Borexino collaboration reports observations of the
pp
neutrinos themselves, so providing a direct view of the principal fusion process that powers the Sun.
Journal Article
The FLUKA code: an overview
2006
FLUKA is a multipurpose MonteCarlo code which can transport a variety of particles over a wide energy range in complex geometries. The code is a joint project of INFN and CERN: part of its development is also supported by the University of Houston and NASA. FLUKA is successfully applied in several fields, including but not only, particle physics, cosmic ray physics, dosimetry, radioprotection, hadron therapy, space radiation, accelerator design and neutronics. The code is the standard tool used at CERN for dosimetry, radioprotection and beam-machine interaction studies. Here we give a glimpse into the code physics models with a particular emphasis to the hadronic and nuclear sector.
Journal Article
The DarkSide Experiment: Present Status and Future
2017
DarkSide is a multi-stage program devoted to direct searches of Dark Matter particles with detectors based on double phase liquid Argon Time Projection Chamber. The DarkSide-50 setup is running underground at the Laboratori Nazionali del Gran Sasso. First it was operated with Atmospheric Argon and during that run (1422 ± 67) kg×d of truly background-free exposure has been accumulated. Obtained data made it possible to set a 90% C.L. upper limit on the WIMP-nucleon cross section of 6.1 × 10−44 cm2 (for a WIMP mass of 100 GeV/c2). Presently the detector is filled with Underground Argon, which is depleted in 39Ar by a factor of (1.4 ± 0.2)×103 with respect to Atmospheric Argon. Acquired so far (2616 ± 43) kg×d (71 live days) in combination with the data from the Atmospheric Argon run give us the 90% C.L. upper limit on the WIMP-nucleon spin-independent cross section of 2.0×10−44 cm2 for a WIMP mass of 100 GeV/c2. Up to date this is the best limit obtained with an argon target.
Journal Article
The DarkSide awakens
The DarkSide program at LNGS aims to perform background-free WIMP searches using two phase liquid argon time projection chambers, with the ultimate goal of covering all parameters down to the so-called neutrino floor. One of the distinct features of the program is the use of underground argon with has a reduced content of the radioactive 39Ar compared to atmospheric argon. The DarkSide Collaboration is currently operating the DarkSide-50 experiment, the first such WIMP detector using underground argon. Operations with underground argon indicate a suppression of 39Ar by a factor (1.4 ± 0.2) × 103 relative to atmospheric argon. The new results obtained with DarkSide-50 and the plans for the next steps of the DarkSide program, the 20t fiducial mass DarkSide-20k detector and the 200 t fiducial Argo, are reviewed in this proceedings.
Journal Article
Direct Search for Dark Matter with DarkSide
2015
The DarkSide experiment is designed for the direct detection of Dark Matter with a double phase liquid Argon TPC operating underground at Laboratori Nazionali del Gran Sasso. The TPC is placed inside a 30 tons liquid organic scintillator sphere, acting as a neutron veto, which is in turn installed inside a 1 kt water Cherenkov detector. The current detector is running since November 2013 with a 50 kg atmospheric Argon fill and we report here the first null results of a Dark Matter search for a (1422 ± 67) kg.d exposure. This result correspond to a 90% CL upper limit on the WIMP-nucleon cross section of 6.1 × 10-44 cm2 (for a WIMP mass of 100 GeV c2) and it's currently the most sensitive limit obtained with an Argon target.
Journal Article
The DarkSide-50 outer detectors
2016
DarkSide-50 is a dark matter detection experiment searching for Weakly Interacting Massive Particles (WIMPs), in Gran Sasso National Laboratory. For experiments like DarkSide-50, neutrons are one of the primary backgrounds that can mimic WIMP signals. The experiment consists of three nested detectors: a liquid argon time projection chamber surrounded by two outer detectors. The outermost detector is a 10 m by 11 m cylindrical water Cherenkov detector with 80 PMTs, designed to provide shielding and muon vetoing. Inside the water Cherenkov detector is the 4 m diameter spherical boron-loaded liquid scintillator veto, with a cocktail of pseudocumene, trimethyl borate, and PPO wavelength shifter, designed to provide shielding, neutron vetoing, and in situ measurements of the TPC backgrounds. We present design and performance details of the DarkSide-50 outer detectors.
Journal Article