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Simulations are performed for the period 2000–2015 by two different regional climate models, ALADIN and RegCM, to quantify the direct and semi-direct radiative effects of biomass-burning aerosols (BBAs) in the southeast Atlantic (SEA) region. Different simulations have been performed using strongly absorbing BBAs in accordance with recent in situ observations over the SEA. For the July–August–September (JAS) season, the single scattering albedo (SSA) and total aerosol optical depth (AOD) simulated by the ALADIN and RegCM models are consistent with the MACv2 climatology and MERRA-2 and CAMS-RA reanalyses near the biomass-burning emission sources. However, the above-cloud AOD is slightly underestimated compared to satellite (MODIS and POLDER) data during the transport over the SEA. The direct radiative effect exerted at the continental and oceanic surfaces by BBAs is significant in both models and the radiative effects at the top of the atmosphere indicate a remarkable regional contrast over SEA (in all-sky conditions), with a cooling (warming) north (south) of 10 ∘S, which is in agreement with the recent MACv2 climatology. In addition, the two models indicate that BBAs are responsible for an important shortwave radiative heating of ∼0.5–1 K per day over SEA during JAS with maxima between 2 and 4 km a.m.s.l. (above mean sea level). At these altitudes, BBAs increase air temperature by ∼0.2–0.5 K, with the highest values being co-located with low stratocumulus clouds. Vertical changes in air temperature limit the subsidence of air mass over SEA, creating a cyclonic anomaly. The opposite effect is simulated over the continent due to the increase in lower troposphere stability. The BBA semi-direct effect on the lower troposphere circulation is found to be consistent between the two models. Changes in the cloud fraction are moderate in response to the presence of smoke, and the models differ over the Gulf of Guinea. Finally, the results indicate an important sensitivity of the direct and semi-direct effects to the absorbing properties of BBAs. Over the stratocumulus (Sc) region, DRE varies from +0.94 W m−2 (scattering BBAs) to +3.93 W m−2 (most absorbing BBAs).

In the present work, we report daytime latent heat flux profile measurements in the convective boundary layer (CBL) obtained from the combined use of a wind lidar and a thermodynamic Raman lidar. Water vapour flux profiles and, consequently, latent heat flux profiles were obtained as the covariance between the vertical profiles of the water vapour mixing ratio and vertical wind fluctuations. Profile measurements of the water vapour mixing ratio were carried out by the thermodynamic Raman lidar CONCERNING, while simultaneous profile measurements of the vertical wind speed were carried out by a co-located Doppler wind lidar. The considered dataset was collected in the frame of the international field campaign “Water Vapor Lidar Network Assimilation” (WaLiNeAs). Three cloud-free time intervals on 31 October, 28 November, and 8 December 2022 were selected as case studies. Measurements of turbulent kinetic energy (TKE) were also carried out over the same time intervals based on the use of wind lidar data. The three selected case studies were characterised by different atmospheric stability conditions and, consequently, by a different potential for the occurrence of convective activity. More specifically, the atmospheric conditions on 31 October 2022 were very unstable, with intensive convective activity taking place in the area and ultimately leading to relatively intense thunderstorms and rainfall events. The atmospheric conditions on 28 November 2022 were moderately unstable, ultimately leading to light convective activity, with scattered rain episodes observed throughout the day but with no severe thunderstorms taking place. Stratiform precipitations were present on 8 December 2022, with weak embedded convective processes taking place within stratiform clouds and leading to moderate additional precipitation. In all three selected case studies, representative of pre-convective conditions, both latent heat flux and TKE profiles are characterised by values increasing with altitude up to approx. 500 m, while both latent heat flux and TKE are found to decrease, with a steeper negative gradient up to approx. 600 m and more gradually above this altitude, returning to zero just above the top of the CBL. In all three cases, peak values of TKE appear to be strongly correlated with corresponding peak values of the latent heat flux; the higher the maximum values of TKE and latent heat flux, the more intense the following precipitation events.

Understanding the West African monsoon (WAM) dynamics in the mid-Holocene (MH) is a crucial issue in climate modeling, because numerical models typically fail to reproduce the extensive precipitation suggested by proxy evidence. This discrepancy may be largely due to the assumption of both unrealistic land surface cover and atmospheric aerosol concentration. In this study, the MH environment is simulated in numerical experiments by imposing extensive vegetation over the Sahara and the consequent reduction in airborne dust concentration. A dramatic increase in precipitation is simulated across the whole of West Africa, up to the Mediterranean coast. This precipitation response is in better agreement with proxy data, in comparison with the case in which only changes in orbital forcing are considered. Results show a substantial modification of the monsoonal circulation, characterized by an intensification of large-scale deep convection through the entire Sahara, and a weakening and northward shift (∼6.5°) of the African easterly jet. The greening of the Sahara also leads to a substantial reduction in the African easterly wave activity and associated precipitation. The reorganization of the regional atmospheric circulation is driven by the vegetation effect on radiative forcing and associated heat fluxes, with the reduction in dust concentration to enhance this response. The results for the WAM in the MH present important implications for understanding future climate scenarios in the region and in teleconnected areas, in the context of projected wetter conditions in West Africa.

Climate variability associated with the West African monsoon (WAM) has important environmental and socio-economic impacts in the region. However, state-of-the-art climate models still struggle in producing reliable climate predictions. An important cause of this low predictive skill is the sensitivity of climate models to different forcings. In this study, the mechanisms linking the WAM dynamics to the CO 2 forcing are investigated, by comparing the effect of the CO 2 direct radiative effect with its indirect effect mediated by the global sea surface warming. The July-to-September WAM variability is studied in climate simulations extracted from the Coupled Model Intercomparison Project Phase 5 archive, driven by prescribed sea surface temperature (SST). The individual roles of global SST warming and CO 2 atmospheric concentration increase are investigated through idealized experiments simulating a 4 K warmer SST and a quadrupled CO 2 concentration, respectively. Results show opposite and competing responses in the WAM dynamics and precipitation. A dry response (−0.6 mm/day) to the SST warming is simulated in the Sahel, with dryer conditions over western Sahel (−0.8 mm/day). Conversely, the CO 2 increase produces wet conditions (+0.5 mm/day) in the Sahel, with the strongest response over central-eastern Sahel (+0.7 mm/day). The associated responses in the atmospheric dynamics are also analysed, showing that the SST warming affects the Sahelian precipitation through modifications in the global tropical atmospheric dynamics, reducing the importance of the regional drivers, while the CO 2 increase reinforces the coupling between precipitation and regional dynamics. A general agreement in model responses demonstrates the robustness of the identified mechanisms linking the WAM dynamics to the CO 2 direct and indirect forcing, and indicates that these primary mechanisms are captured by climate models. Results also suggest that the spread in future projections may be caused by unbalanced model responses to the CO 2 direct and indirect forcing.

Southern West Africa (SWA) is an African pollution hotspot but a relatively poorly sampled region of the world. We present an overview of in situ aerosol optical measurements collected over SWA in June and July 2016 as part as of the DACCIWA (Dynamics-Aerosol-Chemistry-Clouds Interactions in West Africa) airborne campaign. The aircraft sampled a wide range of air masses, including anthropogenic pollution plumes emitted from the coastal cities, long-range transported biomass burning plumes from central and southern Africa and dust plumes from the Sahara and Sahel region, as well as mixtures of these plumes. The specific objective of this work is to characterize the regional variability of the vertical distribution of aerosol particles and their spectral optical properties (single scattering albedo: SSA, asymmetry parameter, extinction mass efficiency, scattering Ångström exponent and absorption Ångström exponent: AAE). The first findings indicate that aerosol optical properties in the planetary boundary layer were dominated by a widespread and persistent biomass burning loading from the Southern Hemisphere. Despite a strong increase in aerosol number concentration in air masses downwind of urban conglomerations, spectral SSA were comparable to the background and showed signatures of the absorption characteristics of biomass burning aerosols. In the free troposphere, moderately to strongly absorbing aerosol layers, dominated by either dust or biomass burning particles, occurred occasionally. In aerosol layers dominated by mineral dust particles, SSA varied from 0.81 to 0.92 at 550 nm depending on the variable proportion of anthropogenic pollution particles externally mixed with the dust. For the layers dominated by biomass burning particles, aerosol particles were significantly more light absorbing than those previously measured in other areas (e.g. Amazonia, North America), with SSA ranging from 0.71 to 0.77 at 550 nm. The variability of SSA was mainly controlled by variations in aerosol composition rather than in aerosol size distribution. Correspondingly, values of AAE ranged from 0.9 to 1.1, suggesting that lens-coated black carbon particles were the dominant absorber in the visible range for these biomass burning aerosols. Comparison with the literature shows a consistent picture of increasing absorption enhancement of biomass burning aerosol from emission to remote location and underscores that the evolution of SSA occurred a long time after emission. The results presented here build a fundamental basis of knowledge about the aerosol optical properties observed over SWA during the monsoon season and can be used in climate modelling studies and satellite retrievals. In particular and regarding the very high absorbing properties of biomass burning aerosols over SWA, our findings suggest that considering the effect of internal mixing on absorption properties of black carbon particles in climate models should help better assess the direct and semi-direct radiative effects of biomass burning particles.

Trade-wind cumuli constitute the cloud type with the highest frequency of occurrence on Earth, and it has been shown that their sensitivity to changing environmental conditions will critically influence the magnitude and pace of future global warming. Research over the last decade has pointed out the importance of the interplay between clouds, convection and circulation in controling this sensitivity. Numerical models represent this interplay in diverse ways, which translates into different responses of trade-cumuli to climate perturbations. Climate models predict that the area covered by shallow cumuli at cloud base is very sensitive to changes in environmental conditions, while process models suggest the opposite. To understand and resolve this contradiction, we propose to organize a field campaign aimed at quantifying the physical properties of trade-cumuli (e.g., cloud fraction and water content) as a function of the large-scale environment. Beyond a better understanding of clouds-circulation coupling processes, the campaign will provide a reference data set that may be used as a benchmark for advancing the modelling and the satellite remote sensing of clouds and circulation. It will also be an opportunity for complementary investigations such as evaluating model convective parameterizations or studying the role of ocean mesoscale eddies in air–sea interactions and convective organization.

The present study examines the impact of the environmental moisture structure in the lower troposphere (below 2 km above sea level, a.s.l.) on the precipitation development, observed in southern France during Intensive Observation Period (IOP) 13 of the first Special Observation Period of the Hydrological cycle in the Mediterranean Experiment (HyMeX SOP-1), through a series of sensitivity experiments using the non-hydrostatic mesoscale atmospheric numerical model (Meso-NH). The control simulation (CNTL) and all the other 12 sensitivity experiments examined in this study succeed in reproducing a heavy precipitation event (HPE) in the coastal mountainous region of Var in south-eastern France as observed. The sensitivity experiments are designed to investigate the response of the HPE to the variability of the water vapour content upstream in the moist marine atmospheric boundary layer (MABL) and the drier air above. The comparisons between CNTL and the 12 sensitivity experiments show how the life cycle of precipitation associated with the HPE, but also the upstream flow (over the sea), is modified, even for moisture content changes of only 1 g kg−1 below 2 km a.s.l. Within the low-level wind convergence between southerlies and south-westerlies, a small increase of moisture content in the MABL prolongs moderate precipitation (≥5 mm in 15 min) and enlarges the area of weak precipitation (≥1 mm in 15 min). The moistening in the 1–2 km a.s.l. layer, just above the MABL, prolongs the duration of moderate precipitation, for a similar total precipitation amount as in CNTL. The drier MABL and 1–2 km a.s.l. layer shorten the lifetime of precipitation and reduce the total precipitation amount with respect to CNTL. We also found that the moisture in the MABL has a stronger impact on producing enhanced precipitation (both in terms of amount and intensity) than the moisture just above (1–2 km a.s.l.). Also, it is worth noting that adding moisture in the MABL does not necessarily lead to enhanced precipitation amount. In moistening the MABL, the duration of moderate precipitation increases with increasing moisture as does the area covered by weak precipitation, while the area covered by the intense precipitation (≥30 mm) decreases. Despite a simplified moisture-profile modification approach, this study suggests that moisture structure in the lower troposphere is key for accurate prediction at short-term range of the timing and location of precipitation in the coastal mountainous region in southern France.

Dynamical processes leading to dust emission over Iran and surrounding countries in the summer as well as the subsequent transport of dust toward northwest Iran are analyzed on the basis of two case studies using a suite of ground‐based and spaceborne remote sensing platforms together with modeling tools. Ground‐based lidar measurements acquired in Zanjan provide new insight into the vertical distribution of dust linked to transport over northwest Iran and highlight the importance of low‐level transport of dust from both Iraq and Iran for air quality issues in Tehran. During the 3–5 August 2007 case, dust emission regions are located in Syria/Iraq and close to Qom, Iran, in a large intermittent salt lake in the western part of the Dasht‐e Kavir desert. The visibility in Tehran associated with this event decreases significantly (reaching 7 km) on 5 August 2007 only. During the 11–13 September 2008 case, the dust transported to northwest Iran originates from Syria/Iraq only. The visibility in Tehran during this case is low throughout the period, sometimes less than 5 km due to the transport of dust at low levels. In both cases, emissions in Syria and Iraq occur in response to strong Shamal winds. However, transport of dust toward Iran takes place at different levels: above 700 hPa in August and below 700 hPa in September. This is found to be related to the presence of strong northeasterly winds over the Zagros Mountains as well as in its lee (south of the range) in the August case only. In August also, dust emissions in the Qom region results from strong winds blowing over the Dasht‐e Kavir desert.

Differential Absorption Lidar (DiAL) method is widely used for a number of ground-based and airborne greenhouse gas measurement applications. However, for a direct detection in the 2µm range, other sources of random noise can be neglected in front of the detection noise which increases with ranging. We therefore propose to evaluate the effect of non-constant Scheimpflug-like averaging to reduce the signal-to-noise ratio along the line of sight, during a 5-hour measurement campaign in the Paris region.

The international field campaign called the Convective and Orographically-induced Precipitation Study (COPS) took place from June to August 2007 in southwestern Germany/eastern France. The overarching goal of COPS is to advance the quality of forecasts of orographically-induced convective precipitation by four-dimensional observations and modeling of its life cycle. COPS was endorsed as one of the Research and Development Projects of the World Weather Research Program (WWRP), and combines the efforts of institutions and scientists from eight countries. A strong collaboration between instrument principal investigators and experts on mesoscale modeling has been established within COPS. In order to study the relative importance of large-scale and small-scale forcing leading to convection initiation in low mountains, COPS is coordinated with a one-year General Observations Period in central Europe, the WWRP Forecast Demonstration Project MAP D-PHASE, and the first summertime European THORPEX Regional Campaign. Furthermore, the Atmospheric Radiation Measurement program Mobile Facility operated in the central COPS observing region for nine months in 2007. The article describes the scientific preparation of this project and the design of the observation systems. COPS will rest on three pillars: A unique synergy of observing systems, the next-generation high-resolution mesoscale models with improved model physics, and advanced data assimilation and ensemble prediction systems. These tools will be used to separate and to quantify errors in quantitative precipitation forecasting as well as to study the predictability of convective precipitation.