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Atmospheric carbon monoxide (CO) distributions are controlled by anthropogenic emissions, biomass burning, transport and oxidation by reaction with the hydroxyl radical (OH). Quantifying trends in CO is therefore important for understanding changes related to all of these contributions. Here we present a comprehensive record of satellite observations from 2000 through 2011 of total column CO using the available measurements from nadir-viewing thermal infrared instruments: MOPITT, AIRS, TES and IASI. We examine trends for CO in the Northern and Southern Hemispheres along with regional trends for Eastern China, Eastern USA, Europe and India. We find that all the satellite observations are consistent with a modest decreasing trend ~ −1 % yr−1 in total column CO over the Northern Hemisphere for this time period and a less significant, but still decreasing trend in the Southern Hemisphere. Although decreasing trends in the United States and Europe have been observed from surface CO measurements, we also find a decrease in CO over E. China that, to our knowledge, has not been reported previously. Some of the interannual variability in the observations can be explained by global fire emissions, but the overall decrease needs further study to understand the implications for changes in anthropogenic emissions.

In this work absolute values of gravity wave (GW) momentum flux are derived from global temperature measurements by the satellite instruments High Resolution Dynamics Limb Sounder (HIRDLS) and Sounding of the Atmosphere using Broadband Emission Radiometry (SABER). Momentum fluxes in the stratosphere are derived for both instruments and for SABER in the whole mesosphere. The large‐scale atmospheric background state is removed by a two‐dimensional Fourier decomposition in longitude and time, covering even planetary‐scale waves with periods as short as 1–2 days. Therefore, it is possible to provide global distributions of GW momentum flux from observations for the first time in the mesosphere. Seasonal as well as longer‐term variations of the global momentum flux distribution are discussed. GWs likely contribute significantly to the equatorward tilt of the polar night jet and to the poleward tilt of the summertime mesospheric jet. Our results suggest that GWs can undergo large latitudinal shifts while propagating upward. In particular, GWs generated by deep convection in the subtropical monsoon regions probably contribute significantly to the mesospheric summertime wind reversal at mid‐ and high latitudes. Variations in the GW longitudinal distribution caused by those convectively generated GWs are still observed in the mesosphere and could be important for the generation of the quasi two‐day wave. Indications for quasi‐biennial oscillation (QBO) induced variations of GW momentum flux are found in the subtropics. Also variations at time scales of about one 11‐year solar cycle are observed and might indicate a negative correlation between solar flux and GW momentum flux. Key Points Gravity wave momentum flux global distributions in both strato‐ and mesosphere Interaction of gravity waves with zonal wind jets studied Discussion of variations on different timescales: seasonal, QBO, solar cycle

Using both thermal infrared (TIR) and near infrared (NIR) channels of MOPITT (Measurements of Pollution in the Troposphere) on EOS‐Terra, we demonstrate the first coincident multispectral retrievals of carbon monoxide (CO) from space. Exploiting both TIR and NIR channels has been possible due to recent progress in characterizing NIR channel radiance errors. This has allowed us to trade off sensitivity to near surface CO for larger random errors in the combined retrieval. By examining retrieval diagnostics such as DFS (degrees of freedom for signal) and averaging kernels for the multispectral retrieval (TIR + NIR) as compared to the TIR‐only retrieval, we find that adding the NIR channel to the retrieval significantly increases sensitivity to CO, especially near the surface, but with high spatial variability due to surface albedo variations. The cases with the largest increases in DFS are over regions with low thermal contrast between the surface and lower atmosphere. In the tropics (23.4°S–23.4°N), the fraction of daytime land cases with at least 0.4 DFS in the surface layer (surface to 800 hPa) is 20% for TIR‐only retrievals compared to 59% for multispectral retrievals. Vertical resolution for the surface layer is also improved, in some cases from around 6 km for TIR‐only to roughly 1 km for TIR + NIR. Since we apply a single a priori CO profile (unlike MOPITT V4) and error covariance in all the retrievals reported here, these increases are due solely to the addition of the NIR channel. Enhanced sensitivity to near surface CO is especially evident in a case study for central/east Asia where source regions for urban areas with high population density are clearly identifiable. Although these retrievals are still a research product and require further validation and scientific evaluation, they demonstrate the increased sensitivity to CO in the lowermost troposphere that can be obtained from multispectral MOPITT data.

The Measurements of Pollution in the Troposphere (MOPITT) Version 6 (V6) product for carbon monoxide (CO) incorporates several enhancements which will benefit many users of MOPITT data. V6 algorithm improvements are described in detail, and V6 validation results are presented. First, a geolocation bias related to the orientation of the MOPITT instrument relative to the TERRA platform was characterized and eliminated. Second, the variable a priori for CO concentrations for V6 is based on simulations performed with the chemical transport model Community Atmosphere Model with Chemistry (CAM-chem) for the years 2000–2009 instead of the model-derived climatology for 1997–2004 used for V5. Third, meteorological fields required for V6 retrieval processing are extracted from the MERRA (Modern-Era Retrospective Analysis For Research And Applications) reanalysis. Finally, a significant latitude-dependent retrieval bias in the upper troposphere in Version 5 products has been substantially reduced.

Data from the High Resolution Dynamics Limb Sounder (HIRDLS) instrument on NASA's Aura satellite are used to investigate the relative numerical variability of observed gravity wave packets as a function of both horizontal and vertical wavenumber, with support from the Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) instrument on TIMED. We see that these distributions are dominated by large vertical and small horizontal wavenumbers, and have a similar spectral form at all heights and latitudes, albeit with important differences. By dividing our observed wavenumber distribution into particular subspecies of waves, we demonstrate that these distributions exhibit significant temporal and spatial variability, and that small-scale variability associated with particular geophysical phenomena such as the monsoon arises due to variations in specific parts of the observed spectrum. We further show that the well-known Andes/Antarctic Peninsula gravity wave hotspot during southern winter, home to some of the largest wave fluxes on the planet, is made up of relatively few waves, but with a significantly increased flux per wave due to their spectral characteristics. These results have implications for the modelling of gravity wave phenomena.

For the August‐September 2008 Olympic and the Paralympic Games held in Beijing, China, strict controls on pollutant emissions and motor vehicle traffic were imposed on Beijing and neighboring provinces to the South to improve the air quality in and around the city. Satellite measurements over Beijing between July and September showed 43% reductions of tropospheric column nitrogen dioxide, compared to the past three years. When neighboring provinces to the south are included in our analyses, satellite measurements show boundary layer sulfur dioxide reductions of 13% and carbon monoxide reductions of 12% at 700 hPa. Thus, based on satellites observations alone, noticeable reductions in these pollutant tracers were measured during both games.

Carbon monoxide (CO) is a key atmospheric compound that can be remotely sensed by satellite on the global scale. Fifteen years of continuous observations are now available from the MOPITT/Terra mission (2000 to present). Another 15 and more years of observations will be provided by the IASI/MetOp instrument series (2007–2023 >). In order to study long-term variability and trends, a homogeneous record is required, which is not straightforward as the retrieved quantities are instrument and processing dependent. The present study aims at evaluating the consistency between the CO products derived from the MOPITT and IASI missions, both for total columns and vertical profiles, during a 6-year overlap period (2008–2013). The analysis is performed by first comparing the available 2013 versions of the retrieval algorithms (v5T for MOPITT and v20100815 for IASI), and second using a dedicated reprocessing of MOPITT CO profiles and columns using the same a priori information as the IASI product. MOPITT total columns are generally slightly higher over land (bias ranging from 0 to 13 %) than IASI data. When IASI and MOPITT data are retrieved with the same a priori constraints, correlation coefficients are slightly improved. Large discrepancies (total column bias over 15 %) observed in the Northern Hemisphere during the winter months are reduced by a factor of 2 to 2.5. The detailed analysis of retrieved vertical profiles compared with collocated aircraft data from the MOZAIC-IAGOS network, illustrates the advantages and disadvantages of a constant vs. a variable a priori. On one hand, MOPITT agrees better with the aircraft profiles for observations with persisting high levels of CO throughout the year due to pollution or seasonal fire activity (because the climatology-based a priori is supposed to be closer to the real atmospheric state). On the other hand, IASI performs better when unexpected events leading to high levels of CO occur, due to a larger variability associated with the a priori.

Vertical profiles of carbon monoxide (CO) concentration and corresponding total column values derived from measurements made by the Measurements of Pollution in the Troposphere (MOPITT) satellite instrument are now being processed operationally with the “version 4” (V4) retrieval algorithm. This algorithm exploits the results of analyses of in situ data, chemical transport modeling, and radiative transfer modeling in the MOPITT postlaunch era. Improvements in the V4 product are evident in both clean and polluted conditions. The new products are validated using CO in situ measurements acquired from aircraft from 2000 to 2007. As determined by both retrieval simulations and observations, retrieval bias drift is typically about 1 ppbv/yr for levels in the middle troposphere and about 2 ppbv/yr in the upper troposphere. Retrieval simulations indicate that observed bias drift may be the result of gradual on‐orbit changes in the instrument's modulation cell parameters.

Measurements from the High Resolution Dynamics Limb Sounder (HIRDLS) on NASA's Aura satellite are used to quantify gravity wave momentum fluxes generated from monsoon regions across the globe over the 3 years 2005–2007. Momentum fluxes in the altitude range 16–60 km over eight individual monsoon regions in both hemispheres are examined and compared to convective data from National Oceanic and Atmospheric Administration's Outgoing Longwave Radiation time series and precipitation data from the Tropical Rainfall Monitoring Mission. Good correlations are observed over seven of these eight regions, the exception being the North American monsoon region. An increase in measured momentum flux of approximately 50% is observed over the 10°N–30°N latitude band during the boreal monsoon period, with around half of the annual momentum flux for this latitude range measured during this period; however, the limited correspondence in the North American region suggests that at least some of this increase may be due to other processes. Key Points There is a good correlation between monsoons and stratospheric gravity waves A significant increase in gravity wave MF is observed during the monsoon This applies to monsoons in both hemispheres

Observations from the High Resolution Dynamics Limb Sounder (HIRDLS) instrument on NASA's Aura satellite are used to quantify gravity wave momentum fluxes in the middle atmosphere. The period around the 2006 Arctic sudden stratospheric warming (SSW) is investigated, during which a substantial elevation of the stratopause occurred. Analysis of the HIRDLS results, together with analysis of European Centre for Medium‐Range Weather Forecasting zonal winds, provide direct evidence of wind filtering of the gravity wave spectrum during this period. This confirms previous hypotheses from model studies and further contributes to our understanding of the effects of gravity wave driving on the winter polar stratopause.