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Scintillators, materials that produce light pulses upon interaction with ionizing radiation, are widely employed in radiation detectors. In advanced medical-imaging technologies, fast scintillators enabling a time resolution of tens of picoseconds are required to achieve high-resolution imaging at the millimetre length scale. Here we demonstrate that composite materials based on fluorescent metal–organic framework (MOF) nanocrystals can work as fast scintillators. We present a prototype scintillator fabricated by embedding MOF nanocrystals in a polymer. The MOF comprises zirconium oxo-hydroxy clusters, high-Z linking nodes interacting with the ionizing radiation, arranged in an orderly fashion at a nanometric distance from 9,10-diphenylanthracene ligand emitters. Their incorporation in the framework enables fast sensitization of the ligand fluorescence, thus avoiding issues typically arising from the intimate mixing of complementary elements. This proof-of-concept prototype device shows an ultrafast scintillation rise time of ~50 ps, thus supporting the development of new scintillators based on engineered fluorescent MOF nanocrystals.Composites of fluorescent metal–organic framework nanocrystals in a polymer are exploited to create fast scintillators with a rise time of about 50 ps.

The R&D project COSINUS (Cryogenic Observatory for SIgnatures seen in Next-generation Underground Searches) aims to develop a cryogenic scintillating calorimeter using an undoped NaI-crystal as target for direct dark matter search. Dark matter particles interacting with the detector material generate both a phonon signal and scintillation light. While the phonon signal provides a precise determination of the deposited energy, the simultaneously measured scintillation light allows for particle identification on an event-by-event basis, a powerful tool to study material-dependent interactions, and to suppress backgrounds. Using the same target material as the DAMA/LIBRA collaboration, the COSINUS technique may offer a unique possibility to investigate and contribute information to the presently controversial situation in the dark matter sector. We report on the dedicated design planned for the NaI proof-of-principle detector and the objectives of using this detection technique in the light of direct dark matter detection.

As quantum coherence times of superconducting circuits have increased from nanoseconds to hundreds of microseconds, they are currently one of the leading platforms for quantum information processing. However, coherence needs to further improve by orders of magnitude to reduce the prohibitive hardware overhead of current error correction schemes. Reaching this goal hinges on reducing the density of broken Cooper pairs, so-called quasiparticles. Here, we show that environmental radioactivity is a significant source of nonequilibrium quasiparticles. Moreover, ionizing radiation introduces time-correlated quasiparticle bursts in resonators on the same chip, further complicating quantum error correction. Operating in a deep-underground lead-shielded cryostat decreases the quasiparticle burst rate by a factor thirty and reduces dissipation up to a factor four, showcasing the importance of radiation abatement in future solid-state quantum hardware. Background radiation has been identified as a key factor limiting the coherence times of superconducting circuits. Here, the authors measure the impact of environmental and cosmic radiation on a superconducting resonator with varying degrees of shielding, including an underground facility.

Radioactivity was recently discovered as a source of decoherence and correlated errors for the real-world implementation of superconducting quantum processors. In this work, we measure levels of radioactivity present in a typical laboratory environment (from muons, neutrons, and γ -rays emitted by naturally occurring radioactive isotopes) and in the most commonly used materials for the assembly and operation of state-of-the-art superconducting qubits. We present a GEANT-4 based simulation to predict the rate of impacts and the amount of energy released in a qubit chip from each of the mentioned sources. We finally propose mitigation strategies for the operation of next-generation qubits in a radio-pure environment.

Among the detectors used for rare event searches, such as neutrinoless Double Beta Decay (0 ν DBD) and Dark Matter experiments, bolometers are very promising because of their favorable properties (excellent energy resolution, high detector efficiency, a wide choice of different materials used as absorber, …). However, up to now, the actual interesting possibility to identify the interacting particle, and thus to greatly reduce the background, can be fulfilled only with a double read-out (i.e. the simultaneous and independent read out of heat and scintillation light or heat and ionization). This double read-out could greatly complicate the assembly of a huge, multi-detector array, such as CUORE and EURECA. The possibility to recognize the interacting particle through the shape of the thermal pulse is then clearly a very interesting opportunity. While detailed analyses of the signal time development in purely thermal detectors have not produced so far interesting results, similar analyses on macro-bolometers (∼10–500 g) built with scintillating crystals showed that it is possible to distinguish between an electron or γ -ray and an α particle interaction (i.e. the main source of background for 0 ν DBD experiments based on the bolometric technique). Results on pulse shape analysis of a CaMoO 4 crystal operated as bolometer are reported as an example. An explanation of this behavior, based on the energy partition in the heat and scintillation channels, is also presented.

CUPID-0 is the first large mass array of enriched Zn\\[^{82}\\]Se scintillating low temperature calorimeters, operated at LNGS since 2017. During its first scientific runs, CUPID-0 collected an exposure of 9.95 kg year. Thanks to the excellent rejection of \\[\\alpha \\] particles, we attained the lowest background ever measured with thermal detectors in the energy region where we search for the signature of \\[^{82}\\hbox {Se}\\] neutrinoless double beta decay. In this work we develop a model to reconstruct the CUPID-0 background over the whole energy range of experimental data. We identify the background sources exploiting their distinctive signatures and we assess their extremely low contribution [down to \\[\\sim 10^{-4}\\] counts/(keV kg year)] in the region of interest for \\[^{82}\\hbox {Se}\\] neutrinoless double beta decay search. This result represents a crucial step towards the comprehension of the background in experiments based on scintillating calorimeters and in next generation projects such as CUPID.

The suppression of spurious events in the region of interest for neutrinoless double beta decay will play a major role in next generation experiments. The background of detectors based on the technology of cryogenic calorimeters is expected to be dominated by \\[\\alpha \\] particles, that could be disentangled from double beta decay signals by exploiting the difference in the emission of the scintillation light. CUPID-0, an array of enriched Zn\\[^{82}\\]Se scintillating calorimeters, is the first large mass demonstrator of this technology. The detector started data-taking in 2017 at the Laboratori Nazionali del Gran Sasso with the aim of proving that dual read-out of light and heat allows for an efficient suppression of the \\[\\alpha \\] background. In this paper we describe the software tools we developed for the analysis of scintillating calorimeters and we demonstrate that this technology allows to reach an unprecedented background for cryogenic calorimeters.

We present the performances of a 330 g zinc molybdate (ZnMoO 4 ) crystal working as scintillating bolometer as a possible candidate for a next generation experiment to search for neutrinoless double beta decay of 100 Mo. The energy resolution, evaluated at the 2615 keV γ -line of 208 Tl, is 6.3 keV FWHM. The internal radioactive contaminations of the ZnMoO 4 were evaluated as <6 μBq/kg ( 228 Th) and 27±6 μBq/kg ( 226 Ra). We also present the results of the α vs β / γ discrimination, obtained through the scintillation light as well as through the study of the shape of the thermal signal alone.

The CUPID-0 experiment searches for double beta decay using cryogenic calorimeters with double (heat and light) read-out. The detector, consisting of 24 ZnSe crystals 95\\[\\%\\] enriched in \\[^{82}\\]Se and two natural ZnSe crystals, started data-taking in 2017 at Laboratori Nazionali del Gran Sasso. We present the search for the neutrino-less double beta decay of \\[^{82}\\]Se into the 0\\[_1^+\\], 2\\[_1^+\\] and 2\\[_2^+\\] excited states of \\[^{82}\\]Kr with an exposure of 5.74 kg\\[\\cdot \\]yr (2.24\\[\\times \\]10\\[^{25}\\] emitters\\[\\cdot \\]yr). We found no evidence of the decays and set the most stringent limits on the widths of these processes: \\[\\varGamma \\](\\[^{82}\\]Se \\[\\rightarrow ^{82}\\]Kr\\[_{0_1^+}\\])8.55\\[\\times \\]10\\[^{-24}\\] yr\\[^{-1}\\], \\[\\varGamma \\] (\\[^{82}\\] Se \\[\\rightarrow ^{82}\\] Kr \\[_{2_1^+}\\])\\[\\,{<}\\,6.25 \\,{\\times }\\,10^{-24}\\] yr\\[^{-1}\\], \\[\\varGamma \\](\\[^{82}\\]Se \\[\\rightarrow ^{82}\\]Kr\\[_{2_2^+}\\])8.25\\[\\times \\]10\\[^{-24}\\] yr\\[^{-1}\\] (90\\[\\%\\] credible interval).

CUORE, an array of 988 TeO 2 bolometers, is about to be one of the most sensitive experiments searching for neutrinoless double-beta decay. Its sensitivity could be further improved by removing the background from α radioactivity. A few years ago it was pointed out that the signal from β s can be tagged by detecting the emitted Cherenkov light, which is not produced by α s. In this paper we confirm this possibility. For the first time we measured the Cherenkov light emitted by a CUORE crystal, and found it to be 100 eV at the Q -value of the decay. To completely reject the α background, we compute that one needs light detectors with baseline noise below 20 eV RMS, a value which is 3–4 times smaller than the average noise of the bolometric light detectors we are using. We point out that an improved light detector technology must be developed to obtain TeO 2 bolometric experiments able to probe the inverted hierarchy of neutrino masses.