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Because gadolinium (Gd) has the highest thermal neutron capture cross section, resulting in an 8 MeV gamma cascade upon capture, it has been proposed for dissolution in water Cherenkov detectors to achieve efficient neutron tagging capabilities. Whereas metallic Gd is insoluble in water, several compounds are very easy to dissolve. Gadolinium sulfate, Gd2(SO4)3, has been thoroughly tested and proposed as the best candidate. Accurate measurement of its concentration, free of doubt from impurities in water, is crucial. An atomic absorption spectrophotometer (AAS) is a device that suits this purpose and is widely used to measure the concentration of many elements. In this study, we describe three different approaches to measure Gd sulfate concentrations in water using an AAS: doping samples with potassium and lanthanum, and employing tantalum and tungsten platforms.

This paper reports the development and detailed properties of about 13 metric tons of gadolinium sulfate octahydrate, $\\rm Gd_2(\\rm SO_4)_3\\cdot \\rm 8H_2O$, which has been dissolved into Super-Kamiokande (SK) in the summer of 2020. We evaluate the impact of radioactive impurities in $\\rm Gd_2(\\rm SO_4)_3\\cdot \\rm 8H_2O$ on diffuse supernova neutrino background searches and solar neutrino observation and confirm the need to reduce radioactive and fluorescent impurities by about three orders of magnitude from commercially available high-purity $\\rm Gd_2(\\rm SO_4)_3\\cdot \\rm 8H_2O$. In order to produce ultra-high-purity $\\rm Gd_2(\\rm SO_4)_3\\cdot \\rm 8H_2O$, we have developed a method to remove impurities from gadolinium oxide, Gd2O3, consisting of acid dissolution, solvent extraction, and pH control processes, followed by a high-purity sulfation process. All of the produced ultra-high-purity $\\rm Gd_2(\\rm SO_4)_3\\cdot \\rm 8H_2O$ is assayed by inductively coupled plasma mass spectrometry and high-purity germanium detectors to evaluate its quality. Because of the long measurement time of high-purity germanium detectors, we have employed several underground laboratories for making parallel measurements including the Laboratorio Subterráneo de Canfranc in Spain, Boulby in the UK, and Kamioka in Japan. In the first half of production, the measured batch purities were found to be consistent with the specifications. However, in the latter half, the $\\rm Gd_2(\\rm SO_4)_3\\cdot \\rm 8H_2O$ contained one order of magnitude more 228Ra than the budgeted mean contamination. This was correlated with the corresponding characteristics of the raw material Gd2O3, in which an intrinsically large contamination was present. Based on their modest impact on SK physics, they were nevertheless introduced into the detector. To reduce 228Ra for the next stage of gadolinium loading to SK, a new process has been successfully established.

The charge-conjugation and parity-reversal (CP) symmetry of fundamental particles is a symmetry between matter and antimatter. Violation of this CP symmetry was first observed in 1964 1 , and CP violation in the weak interactions of quarks was soon established 2 . Sakharov proposed 3 that CP violation is necessary to explain the observed imbalance of matter and antimatter abundance in the Universe. However, CP violation in quarks is too small to support this explanation. So far, CP violation has not been observed in non-quark elementary particle systems. It has been shown that CP violation in leptons could generate the matter–antimatter disparity through a process called leptogenesis 4 . Leptonic mixing, which appears in the standard model’s charged current interactions 5 , 6 , provides a potential source of CP violation through a complex phase δ CP , which is required by some theoretical models of leptogenesis 7 – 9 . This CP violation can be measured in muon neutrino to electron neutrino oscillations and the corresponding antineutrino oscillations, which are experimentally accessible using accelerator-produced beams as established by the Tokai-to-Kamioka (T2K) and NOvA experiments 10 , 11 . Until now, the value of δ CP has not been substantially constrained by neutrino oscillation experiments. Here we report a measurement using long-baseline neutrino and antineutrino oscillations observed by the T2K experiment that shows a large increase in the neutrino oscillation probability, excluding values of δ CP that result in a large increase in the observed antineutrino oscillation probability at three standard deviations (3 σ ). The 3 σ confidence interval for δ CP , which is cyclic and repeats every 2π, is [−3.41, −0.03] for the so-called normal mass ordering and [−2.54, −0.32] for the inverted mass ordering. Our results indicate CP violation in leptons and our method enables sensitive searches for matter–antimatter asymmetry in neutrino oscillations using accelerator-produced neutrino beams. Future measurements with larger datasets will test whether leptonic CP violation is larger than the CP violation in quarks. The T2K experiment constrains CP symmetry in neutrino oscillations, excluding 46% of possible values of the CP violating parameter at a significance of three standard deviations; this is an important milestone to test CP symmetry conservation in leptons and whether the Universe’s matter–antimatter imbalance originates from leptons.

We report the first search result for the flux of astrophysical electron antineutrinos for energies (10)MeV in the gadolinium-loaded Super-Kamiokande (SK) detector. In 2020 June, gadolinium was introduced to the ultrapure water of the SK detector in order to detect neutrons more efficiently. In this new experimental phase, SK-Gd, we can search for electron antineutrinos via inverse beta decay with efficient background rejection thanks to the high efficiency of the neutron tagging technique. In this paper, we report the result for the initial stage of SK-Gd, during 2020 August 26, and 2022 June 1 with a 22.5 × 552 kton · day exposure at 0.01% Gd mass concentration. No significant excess over the expected background in the observed events is found for the neutrino energies below 31.3 MeV. Thus, the flux upper limits are placed at the 90% confidence level. The limits and sensitivities are already comparable with the previous SK result with pure water (22.5 × 2970 kton · day) owing to the enhanced neutron tagging. Operation with Gd increased to 0.03% started in 2022 June.

A bstract The NEXT experiment aims at the sensitive search of the neutrinoless double beta decay in 136 Xe, using high-pressure gas electroluminescent time projection chambers. The NEXT-White detector is the first radiopure demonstrator of this technology, operated in the Laboratorio Subterráneo de Canfranc. Achieving an energy resolution of 1% FWHM at 2.6 MeV and further background rejection by means of the topology of the reconstructed tracks, NEXT-White has been exploited beyond its original goals in order to perform a neu- trinoless double beta decay search. The analysis considers the combination of 271.6 days of 136 Xe-enriched data and 208.9 days of 136 Xe-depleted data. A detailed background modeling and measurement has been developed, ensuring the time stability of the radiogenic and cosmogenic contributions across both data samples. Limits to the neutrinoless mode are obtained in two alternative analyses: a background-model-dependent approach and a novel direct background-subtraction technique, offering results with small dependence on the background model assumptions. With a fiducial mass of only 3.50 ± 0.01 kg of 136 Xe-enriched xenon, 90% C.L. lower limits to the neutrinoless double beta decay are found in the T 1 / 2 0 ν > 5 . 5 × 10 23 − 1 . 3 × 10 24 yr range, depending on the method. The presented techniques stand as a proof-of-concept for the searches to be implemented with larger NEXT detectors.

A bstract NEXT-100 is an electroluminescent high-pressure xenon gas time projection chamber that will search for the neutrinoless double beta (0 νββ ) decay of 136 Xe. The detector possesses two features of great value for 0 νββ searches: energy resolution better than 1% FWHM at the Q value of 136 Xe and track reconstruction for the discrimination of signal and background events. This combination results in excellent sensitivity, as discussed in this paper. Material-screening measurements and a detailed Monte Carlo detector simulation predict a background rate for NEXT-100 of at most 4 × 10 −4 counts keV −1 kg −1 yr −1 . Accordingly, the detector will reach a sensitivity to the 0 νββ -decay half-life of 2.8 × 10 25 years (90% CL) for an exposure of 100 kg·year, or 6.0 × 10 25 years after a run of 3 effective years.

Hyper-Kamiokande consists of two identical water-Cherenkov detectors of total 520 kt, with the first one in Japan at 295 km from the J-PARC neutrino beam with 2.5 $^\\circ$off-axis angles (OAAs), and the second one possibly in Korea at a later stage. Having the second detector in Korea would benefit almost all areas of neutrino oscillation physics, mainly due to longer baselines. There are several candidate sites in Korea with baselines of 1000–1300 km and OAAs of 1 $^\\circ$ –3 $^\\circ$ . We conducted sensitivity studies on neutrino oscillation physics for a second detector, either in Japan (JD$\\times$2) or Korea (JD + KD), and compared the results with a single detector in Japan. Leptonic charge–parity (CP) symmetry violation sensitivity is improved, especially when the CP is non-maximally violated. The larger matter effect at Korean candidate sites significantly enhances sensitivities to non-standard interactions of neutrinos and mass ordering determination. Current studies indicate the best sensitivity is obtained at Mt. Bisul (1088 km baseline,$1.3^\\circ$OAA). Thanks to a larger (1000 m) overburden than the first detector site, clear improvements to sensitivities for solar and supernova relic neutrino searches are expected.

Among multimessenger observations of the next Galactic core-collapse supernova, Super-Kamiokande (SK) plays a critical role in detecting the emitted supernova neutrinos, determining the direction to the supernova (SN), and notifying the astronomical community of these observations in advance of the optical signal. In 2022, SK has increased the gadolinium dissolved in its water target (SK-Gd) and has achieved a Gd concentration of 0.033%, resulting in enhanced neutron detection capability, which in turn enables more accurate determination of the supernova direction. Accordingly, SK-Gd’s real-time supernova monitoring system has been upgraded. SK_SN Notice, a warning system that works together with this monitoring system, was released on 2021 December 13, and is available through GCN Notices. When the monitoring system detects an SN-like burst of events, SK_SN Notice will automatically distribute an alarm with the reconstructed direction to the supernova candidate within a few minutes. In this paper, we present a systematic study of SK-Gd’s response to a simulated Galactic SN. Assuming a supernova situated at 10 kpc, neutrino fluxes from six supernova models are used to characterize SK-Gd’s pointing accuracy using the same tools as the online monitoring system. The pointing accuracy is found to vary from 3° to 7° depending on the models. However, if the supernova is closer than 10 kpc, SK_SN Notice can issue an alarm with three-degree accuracy, which will benefit follow-up observations by optical telescopes with large fields of view.

Hyper-Kamiokande will be a next-generation underground water Cherenkov detector with a total (fiducial) mass of 0.99 (0.56) million metric tons, approximately 20 (25) times larger than that of Super-Kamiokande. One of the main goals of Hyper-Kamiokande is the study of $CP$ asymmetry in the lepton sector using accelerator neutrino and anti-neutrino beams. In this paper, the physics potential of a long-baseline neutrino experiment using the Hyper-Kamiokande detector and a neutrino beam from the J-PARC proton synchrotron is presented. The analysis uses the framework and systematic uncertainties derived from the ongoing T2K experiment. With a total exposure of 7.5 MW $\\times 10^7$s integrated proton beam power (corresponding to $1.56 \\times 10^{22}$ protons on target with a 30 GeV proton beam) to a $2.5^\\circ$ off-axis neutrino beam, it is expected that the leptonic $CP$ phase $\\delta _{CP}$ can be determined to better than 19 degrees for all possible values of $\\delta _{CP}$, and $CP$ violation can be established with a statistical significance of more than $3\\,\\sigma$ ($5\\,\\sigma$) for $76{\\%}$ ($58{\\%}$) of the ${\\delta _{CP}}$ parameter space. Using both $\\nu _e$ appearance and $\\nu _\\mu$ disappearance data, the expected 1$\\sigma$ uncertainty of $\\sin ^2\\theta _{23}$ is 0.015(0.006) for $\\sin ^2\\theta _{23}=0.5(0.45)$.