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18
result(s) for
"Märkisch, Bastian"
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SEI Growth Impacts of Lamination, Formation and Cycling in Lithium Ion Batteries
2020
The accumulation of solid electrolyte interphases (SEI) in graphite anodes related to elevated formation rates (0.1C, 1C and 2C), cycling rates (1C and 2C), and electrode-separator lamination is investigated. As shown previously, the lamination technique is beneficial for the capacity aging in graphite-LiNi1/3Mn1/3Co1/3O2 cells. Here, surface resistance growth phenomena are quantified using electrochemical impedance spectroscopy (EIS). The graphite anodes were extracted from the graphite NMC cells in their fully discharged state and irreversible accumulations of lithium in the SEI are revealed using neutron depth profiling (NDP). In this post-mortem study, NDP reveals uniform lithium accumulations as a function of depth with lithium situated at the surface of the graphite particles thus forming the SEI. The SEI was found to grow logarithmically with cycle number starting with the main formation in the initial cycles. Furthermore, the EIS measurements indicate that benefits from lamination arise from surface resistance growth phenomena aside from SEI growth in superior anode fractions.
Journal Article
Undetected electron backscattering in Perkeo III
2019
The beta asymmetry in neutron beta decay is used to determine the ratio of axial-vector coupling to vector coupling most precisely. In electron spectroscopy, backscattering of electrons from detectors can be a major source of systematic error. We present the determination of the correction for undetected backscattering for electron detection with the instrument Perkeo III . For the electron asymmetry, undetected backscattering leads to a fractional correction of 5 × 10 −4 , i.e. a change by 40% of the total systematic uncertainty.
Journal Article
Editorial: European Conference on Neutron Scattering 2023 in Garching
2023
This edition of the European Conference on Neutron Scattering, which is held every four years, took place in Garching, Germany and gathered over 500 people from all areas of neutron science. From new source or instrumental concepts to fundamental physics, and chemistry, all areas of this community were represented. Lively discussions in the lecture halls, poster areas,and social events around this conference contributed to a very fruitful exchange of new ideas.
Journal Article
Dark decay channel analysis ( n → χ + e + e − ) with the PERKEO II experiment
2019
Discrepancies from beam and bottle type experiments measuring the neutron lifetime are on the 4σ level. In recent publications Fornal and Grinstein proposed that the puzzle could be solved if the neutron would decay on the one percent level via a dark decay mode [1], one possible branch being n → χ + e + e − . With data from the Perkeo II experiment we set limits on the branching fraction and exclude a one percent contribution for 96% of the allowed mass range for the dark matter particle. With this publication, we give a detailed description of the experiment and some selected details of the analysis.
Journal Article
Towards a first measurement of the free neutron bound beta decay detecting hydrogen atoms at a throughgoing beamtube in a high flux reactor
2019
In addition to the common 3-body decay of the neutron n → pe - ν̅ e there should exist an effective 2-body subset with the electron and proton forming a Hydrogen bound state with well defined total momentum, total spin and magnetic quantum numbers. The atomic spectroscopic analysis of this bound system can reveal details about the underlying weak interaction as it mirrors the helicity distributions of all outgoing particles. Thus, it is unique in the information it carries, and an experiment unravelling this information is an analogue to the Goldhaber experiment performed more than 60 years ago. The proposed experiment will search for monoenergetic metastable BoB H atoms with 326 eV kinetic energy, which are generated at the center of a throughgoing beamtube of a high-flux reactor (e.g., at the PIK reactor, Gatchina). Although full spectroscopic information is needed to possibly reveal new physics our first aim is to prove the occurrence of this decay and learn about backgrounds. Key to the detection is the identification of a monoerergtic line of hydrogen atoms occurring at a rate of about 1 s −1 in the environment of many hydrogen atoms, however having a thermal distribution of about room temperature. Two scenarios for velocity (energy) filtering are discussed in this paper. The first builds on an purely electric chopper system, in which metastable hydrogen atoms are quenched to their ground state and thus remain mostly undetectable. This chopper system employs fast switchable Bradbury Nielsen gates. The second method exploits a strongly energy dependent charge exchange process of metastable hydrogen picking up an electron while traversing an argon filled gas cell, turning it into manipulable charged hydrogen. The final detection of hydrogen occurs through multichannel plate (MCP) detector. The paper describes the various methods and gives an outlook on rates and feasibility at the PIK reactor in Gatchina.
Journal Article
ANNI – A pulsed cold neutron beam facility for particle physics at the ESS
by
Abele, Hartmut
,
Märkisch, Bastian
,
Theroine, Camille
in
Cold
,
Cold neutrons
,
Design optimization
2019
Pulsed beams have tremendous advantages for precision experiments with cold neutrons. In order to minimise and measure systematic effects, they are used at continuous sources in spite of the related substantial decrease in intensity. At the European Spallation Source ESS these experiments will profit from the pulse structure of the source and its 50 times higher peak brightness compared to the most intense reactor facilities, making novel concepts feasible. Therefore, the cold neutron beam facility for particle physics ANNI was proposed as part of the ESS instrument suite. The proposed design has been re-optimised to take into account the present ESS cold moderator layout. We present design considerations, the optimised instrument parameters and performance, and expected gain factors for several reference experiments.
Journal Article
Design of the magnet system of the neutron decay facility PERC
2019
The PERC (Proton and Electron Radiation Channel) facility is currently under construction at the research reactor FRM II, Garching. It will serve as an intense and clean source of electrons and protons from neutron beta decay for precision studies. It aims to contribute to the determination of the Cabibbo-Kobayashi-Maskawa quark-mixing element V ud from neutron decay data and to search for new physics via new effective couplings. PERC's central component is a 12 m long superconducting magnet system. It hosts an 8 m long decay region in a uniform field. An additional high-field region selects the phase space of electrons and protons which can reach the detectors and largely improves systematic uncertainties. We discuss the design of the magnet system and the resulting properties of the magnetic field.
Journal Article
Precise Measurements of the Decay of Free Neutrons
2021
The impact of new and highly precise neutron eta decay data is reviewed. We focus on recent results from neutron lifetime, eta asymmetry, and electron-neutrino correlation experiments. From these results, weak interaction parameters are extracted with unprecedented precision, possible also due to progress in effective field theory and lattice QCD. Limits on New Physics beyond the Standard Model derived from neutron decay data are sharper than those derived from high-energy experiments, except for processes involving right-handed neutrinos.
Gaussian Processes and Bayesian Optimization for High Precision Experiments
by
Mattis Bestehorn
,
Lamparth, Max
,
Märkisch, Bastian
in
Bayesian analysis
,
Electron energy
,
Gaussian process
2022
High-precision measurements require optimal setups and analysis tools to achieve continuous improvements. Systematic corrections need to be modeled with high accuracy and known uncertainty to reconstruct underlying physical phenomena. To this end, we present Gaussian processes for modeling experiments and usage with Bayesian optimization, on the example of an electron energy detector, achieving optimal performance. We demonstrate the method's strengths and outline stochastic variational Gaussian processes for physics applications with large data sets, enabling new solutions for current problems.
Depolarization studies on low-depolarizing Cu/Ti and Ni(Mo)/Ti neutron supermirrors
by
Gómez-Guzmán, Jose Manuel
,
Märkisch, Bastian
,
Klauser, Christine
in
Confidence intervals
,
Copper
,
Decay
2025
Neutron supermirrors (SMs) are a crucial part of many scattering and particle physics experiments. So far, Ni(Mo)/Ti SMs have been used in experiments that require to transport a polarized neutron beam due to their lower saturation magnetization compared to Ni/Ti SMs. However, next generation \\(\\) decay experiments require SMs that depolarize below \\(10^-4\\) per reflection to reach their targeted precision. The depolarization of a polarized neutron beam due to reflection from Ni(Mo)/Ti SMs has not yet been measured to that precision. Recently developed Cu/Ti SMs with a very low saturation magnetization compared to Ni(Mo)/Ti may serve as an alternative. In this paper, we test the performance of both mirrors. At a first stage, we present four-states polarized neutron reflectivity (PNR) curves of Ni(Mo) and Cu monolayers measured at the neutron reflectometer SuperADAM and perform a full polarization analysis, showing a difference between the magnetic scattering length density (mSLD) of both materials, with Cu having a lower mSLD than Ni(Mo). These results are corroborated with the full polarization analysis of four-states PNR curves of \\(m=2\\) Ni(Mo)/Ti and Cu/Ti SMs. In a second stage, we measured the depolarization (\\(D\\)) that a polarized neutron beam suffers after reflection from the same Ni(Mo)/Ti and Cu/Ti SMs by using the Opaque Test Bench setup. We find upper limits for the depolarization of \\(D_Cu/Ti(4N5)<7.6 10^-5\\), \\(D_Ni(Mo)/Ti<8.5 10^-5\\), and \\(D_Cu/Ti(2N6)<6.0 10^-5\\) at the \\(1\\) confidence level, where (4N5) corresponds to a Ti purity of \\(99.995\\%\\) and (2N6) to \\(99.6\\%\\). The uncertainties are statistical. These results show that all three SMs are suitable for being used in next generation \\(\\) decay experiments. We found no noticeable dependence of \\(D\\) on the \\(q\\) value or the magnetizing field, in which the samples were placed.