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In recent years, airborne microplastics have been identified in a range of remote environments. However, data throughout the Southern Hemisphere, in particular Antarctica, are largely absent to date. We collected snow samples from 19 sites across the Ross Island region of Antarctica. Suspected microplastic particles were isolated and their composition confirmed using micro-Fourier transform infrared spectroscopy (µFTIR). We identified microplastics in all Antarctic snow samples at an average concentration of 29 particles L−1, with fibres the most common morphotype and polyethylene terephthalate (PET) the most common polymer. To investigate sources, backward air mass trajectories were run from the time of sampling. These indicate potential long-range transportation of up to 6000 km, assuming a residence time of 6.5 d. Local sources were also identified as potential inputs into the environment as the polymers identified were consistent with those used in clothing and equipment from nearby research stations. This study adds to the growing body of literature regarding microplastics as a ubiquitous airborne pollutant and establishes their presence in Antarctica.

ERA5 reanalysis is used to examine extreme precipitation using a spatially dependent precipitation threshold applied within a cyclone compositing framework. This is used to account for regional variation in precipitation generating processes within Southern Hemisphere mid‐latitude cyclones across the cyclone lifecycle. The spatial extent of extreme precipitation is limited to a smaller region around the cyclone center compared to non‐extreme precipitation, though extreme precipitation displays a good spatial correlation with non‐extreme precipitation. Extreme precipitation occurs more often during the deepening phase of the cyclone before it reaches peak intensity. Precipitation occurrence at the 90th and 98th percentiles reduces to 46% and 30% of the deepening value across the cyclone lifecycle, averaged over the composite. Precipitation fraction at the 90th and 98th percentile reduces to 80% and 60% of the deepening value. Our methodology provides a quantitative assessment of precipitation extremes both spatially and temporally, within a cyclone compositing framework. Plain Language Summary Extra‐tropical cyclones play a major role in the circulation within the atmosphere, acting to transfer heat toward the poles. Here we assess the representation of extreme precipitation within extra‐tropical cyclones. By applying a threshold for precipitation that changes with geographic location, we are able to determine how extreme precipitation varies within a cyclone‐centered coordinate system. When breaking cyclones into lifecycle stages representing deepening, peak intensity and decay, we find that extreme precipitation occurs most often as the cyclone is developing. The area of the cyclone relevant for extremes reduces toward the cyclone center as the threshold for determining extreme precipitation increases. Extreme precipitation weakens at a higher rate as cyclones becomes more intense, highlighting the importance of extremes in the growth phase of the cyclone. Key Points We detail a new methodology to assess precipitation extremes within cyclone composites using a spatially dependent precipitation threshold Extreme precipitation occurs preferentially and makes up a larger fraction of total accumulation before cyclones reach peak intensity Extreme precipitation is more constrained around the cyclone center and weakens more rapidly over time compared to moderate precipitation

Southern Ocean (SO) shortwave (SW) radiation biases are a common problem in contemporary general circulation models (GCMs), with most models exhibiting a tendency to absorb too much incoming SW radiation. These biases have been attributed to deficiencies in the representation of clouds during the austral summer months, either due to cloud cover or cloud albedo being too low. The problem has been the focus of many studies, most of which utilised satellite datasets for model evaluation. We use multi-year ship-based observations and the CERES spaceborne radiation budget measurements to contrast cloud representation and SW radiation in the atmospheric component Global Atmosphere (GA) version 7.1 of the HadGEM3 GCM and the MERRA-2 reanalysis. We find that the prevailing bias is negative in GA7.1 and positive in MERRA-2. GA7.1 performs better than MERRA-2 in terms of absolute SW bias. Significant errors of up to 21 W m−2 (GA7.1) and 39 W m−2 (MERRA-2) are present in both models in the austral summer. Using ship-based ceilometer observations, we find low cloud below 2 km to be predominant in the Ross Sea and the Indian Ocean sectors of the SO. Utilising a novel surface lidar simulator developed for this study, derived from an existing Cloud Feedback Model Intercomparison Project (CFMIP) Observation Simulator Package (COSP) – active remote sensing simulator (ACTSIM) spaceborne lidar simulator, we find that GA7.1 and MERRA-2 both underestimate low cloud and fog occurrence relative to the ship observations on average by 4 %–9 % (GA7.1) and 18 % (MERRA-2). Based on radiosonde observations, we also find the low cloud to be strongly linked to boundary layer atmospheric stability and the sea surface temperature. GA7.1 and MERRA-2 do not represent the observed relationship between boundary layer stability and clouds well. We find that MERRA-2 has a much greater proportion of cloud liquid water in the SO in austral summer than GA7.1, a likely key contributor to the difference in the SW radiation bias. Our results suggest that subgrid-scale processes (cloud and boundary layer parameterisations) are responsible for the bias and that in GA7.1 a major part of the SW radiation bias can be explained by cloud cover underestimation, relative to underestimation of cloud albedo.

With low concentrations of tropospheric aerosol, the Southern Ocean offers a “natural laboratory” for studies of aerosol–cloud interactions. Aerosols over the Southern Ocean are produced from biogenic activity in the ocean, which generates sulfate aerosol via dimethylsulfide (DMS) oxidation, and from strong winds and waves that lead to bubble bursting and sea spray emission. Here, we evaluate the representation of Southern Ocean aerosols in the Hadley Centre Global Environmental Model version 3, Global Atmosphere 7.1 (HadGEM3-GA7.1) chemistry–climate model. Compared with aerosol optical depth (AOD) observations from two satellite instruments (the Moderate Resolution Imaging Spectroradiometer, MODIS-Aqua c6.1, and the Multi-angle Imaging Spectroradiometer, MISR), the model simulates too-high AOD during winter and too-low AOD during summer. By switching off DMS emission in the model, we show that sea spray aerosol is the dominant contributor to AOD during winter. In turn, the simulated sea spray aerosol flux depends on near-surface wind speed. By examining MODIS AOD as a function of wind speed from the ERA-Interim reanalysis and comparing it with the model, we show that the sea spray aerosol source function in HadGEM3-GA7.1 overestimates the wind speed dependency. We test a recently developed sea spray aerosol source function derived from measurements made on a Southern Ocean research voyage in 2018. In this source function, the wind speed dependency of the sea spray aerosol flux is less than in the formulation currently implemented in HadGEM3-GA7.1. The new source function leads to good agreement between simulated and observed wintertime AODs over the Southern Ocean; however, it reveals partially compensating errors in DMS-derived AOD. While previous work has tested assumptions regarding the seawater climatology or sea–air flux of DMS, we test the sensitivity of simulated AOD, cloud condensation nuclei and cloud droplet number concentration to three atmospheric sulfate chemistry schemes. The first scheme adds DMS oxidation by halogens and the other two test a recently developed sulfate chemistry scheme for the marine troposphere; one tests gas-phase chemistry only, while the second adds extra aqueous-phase sulfate reactions. We show how simulated sulfur dioxide and sulfuric acid profiles over the Southern Ocean change as a result and how the number concentration and particle size of the soluble Aitken, accumulation and coarse aerosol modes are affected. The new DMS chemistry scheme leads to a 20 % increase in the number concentration of cloud condensation nuclei and cloud droplets, which improves agreement with observations. Our results highlight the importance of atmospheric chemistry for simulating aerosols and clouds accurately over the Southern Ocean.

Automatic lidars and ceilometers (ALCs) provide valuable information on cloud and aerosols but have not been systematically used in the evaluation of general circulation models (GCMs) and numerical weather prediction (NWP) models. Obstacles associated with the diversity of instruments, a lack of standardisation of data products and open processing tools mean that the value of large ALC networks worldwide is not being realised. We discuss a tool, called the Automatic Lidar and Ceilometer Framework (ALCF), that overcomes these problems and also includes a ground-based lidar simulator, which calculates the radiative transfer of laser radiation and allows one-to-one comparison with models. Our ground-based lidar simulator is based on the Cloud Feedback Model Intercomparison Project (CFMIP) Observation Simulator Package (COSP), which has been extensively used for spaceborne lidar intercomparisons. The ALCF implements all steps needed to transform and calibrate raw ALC data and create simulated attenuated volume backscattering coefficient profiles for one-to-one comparison and complete statistical analysis of clouds. The framework supports multiple common commercial ALCs (Vaisala CL31, CL51, Lufft CHM 15k and Droplet Measurement Technologies MiniMPL), reanalyses (JRA-55, ERA5 and MERRA-2) and models (the Unified Model and AMPS – the Antarctic Mesoscale Prediction System). To demonstrate its capabilities, we present case studies evaluating cloud in the supported reanalyses and models using CL31, CL51, CHM 15k and MiniMPL observations at three sites in New Zealand. We show that the reanalyses and models generally underestimate cloud fraction. If sufficiently high-temporal-resolution model output is available (better than 6-hourly), a direct comparison of individual clouds is also possible. We demonstrate that the ALCF can be used as a generic evaluation tool to examine cloud occurrence and cloud properties in reanalyses, NWP models, and GCMs, potentially utilising the large amounts of ALC data already available. This tool is likely to be particularly useful for the analysis and improvement of low-level cloud simulations which are not well monitored from space. This has previously been identified as a critical deficiency in contemporary models, limiting the accuracy of weather forecasts and future climate projections. While the current focus of the framework is on clouds, support for aerosol in the lidar simulator is planned in the future.

The biogeochemical formation of dimethyl sulfide (DMS) from the Southern Ocean is complex, dynamic, and driven by physical, chemical, and biological processes. Such processes, produced by marine biogenic activity, are the dominant source of sulfate aerosol over the Southern Ocean. Using an atmosphere-only configuration of the United Kingdom Earth System Model (UKESM1-AMIP), we performed eight 10-year simulations for the recent past (2009–2018) during austral summer. We tested the sensitivity of atmospheric DMS to four oceanic DMS datasets and three DMS transfer velocity parameterizations. One oceanic DMS dataset was developed here from satellite chlorophyll a. We find that the choice of oceanic DMS dataset has a larger influence on atmospheric DMS than the choice of DMS transfer velocity. Simulations with linear transfer velocity parameterizations show a more accurate representation of atmospheric DMS concentration than those using quadratic relationships. This work highlights that the oceanic DMS and DMS transfer velocity parameterizations currently used in climate models are poorly constrained for the Southern Ocean region. Simulations using oceanic DMS derived from satellite chlorophyll a data, and when combined with a recently developed linear transfer velocity parameterization for DMS, show better spatial variability than the UKESM1 configuration. We also demonstrate that capturing large-scale spatial variability can be more important than large-scale interannual variability. We recommend that models use a DMS transfer velocity parameterization that was developed specifically for DMS and improvements to oceanic DMS spatial variability. Such improvements may provide a more accurate process-based representation of oceanic and atmospheric DMS, and therefore sulfate aerosol, in the Southern Ocean region.

Uncertainty in cloud feedbacks in climate models is a major limitation in projections of future climate. Therefore, evaluation and improvement of cloud simulation are essential to ensure the accuracy of climate models. We analyse cloud biases and cloud change with respect to global mean near-surface temperature (GMST) in climate models relative to satellite observations and relate them to equilibrium climate sensitivity, transient climate response and cloud feedback. For this purpose, we develop a supervised deep convolutional artificial neural network for determination of cloud types from low-resolution (2.5∘×2.5∘) daily mean top-of-atmosphere shortwave and longwave radiation fields, corresponding to the World Meteorological Organization (WMO) cloud genera recorded by human observers in the Global Telecommunication System (GTS). We train this network on top-of-atmosphere radiation retrieved by the Clouds and the Earth’s Radiant Energy System (CERES) and GTS and apply it to the Coupled Model Intercomparison Project Phase 5 and 6 (CMIP5 and CMIP6) model output and the European Centre for Medium-Range Weather Forecasts (ECMWF) Reanalysis version 5 (ERA5) and the Modern-Era Retrospective Analysis for Research and Applications version 2 (MERRA-2) reanalyses. We compare the cloud types between models and satellite observations. We link biases to climate sensitivity and identify a negative linear relationship between the root mean square error of cloud type occurrence derived from the neural network and model equilibrium climate sensitivity (ECS), transient climate response (TCR) and cloud feedback. This statistical relationship in the model ensemble favours models with higher ECS, TCR and cloud feedback. However, this relationship could be due to the relatively small size of the ensemble used or decoupling between present-day biases and future projected cloud change. Using the abrupt-4×CO2 CMIP5 and CMIP6 experiments, we show that models simulating decreasing stratiform and increasing cumuliform clouds tend to have higher ECS than models simulating increasing stratiform and decreasing cumuliform clouds, and this could also partially explain the association between the model cloud type occurrence error and model ECS.

A polynya is an area of open water or reduced concentration of sea ice surrounded by either concentrated sea ice or land ice. They are often seen as sites of intense ocean–atmosphere heat exchange and as ice production factories. Given their importance, it is crucial to quantify the accuracy of satellite-derived polynya information. Polynyas in their early evolution phase are generally narrow and occur at scales likely too fine to be detected by widely used passive microwave (PMW) radiometric sensors. We derived 40 m scale polynya information over the western Ross Sea from high-resolution Synthetic Aperture Radar (SAR) Sentinel-1 C-band data and examined discrepancies with larger-scale estimates. We utilized two automated algorithms, supervised (a rule-based approach) and unsupervised (a combination of texture analysis with k-means clustering), to accurately identify the polynya areas. We generated data for validation using Sentinel-1 data at instances where polynyas can be visually delineated. Results from PMW sensors (NSIDC and AMSR2) and SAR-based algorithms (rule-based and texture-based) are compared with manually delineated polynya areas obtained through Sentinel-1. Analysis using PMW sensors revealed that NSIDC overestimates larger polynyas and underestimates smaller polynyas compared to AMSR2. We were more accurately able to identify polynya presence and area using Sentinel-1 SAR observations, especially in clear cases and cases when PMW data miscalculates the polynya’s presence. Of our SAR-based algorithms, the rule-based approach was more accurate than the texture-based approach at identifying clear polynyas when validated against manually delineated regions. Altogether, we emphasize the need for finer spatio-temporal resolution data for polynya studies.

Location information from long-duration super-pressure balloons flying in the Southern Hemisphere lower stratosphere during 2014 as part of X Project Loon are used to assess the quality of a number of different reanalyses including National Centers for Environmental Prediction Climate Forecast System version 2 (NCEP-CFSv2), European Centre for Medium-Range Weather Forecasts (ERA-Interim), NASA Modern Era Retrospective-Analysis for Research and Applications (MERRA), and the recently released MERRA version 2. Balloon GPS location information is used to derive wind speeds which are then compared with values from the reanalyses interpolated to the balloon times and locations. All reanalysis data sets accurately describe the winds, with biases in zonal winds of less than 0.37 m s−1 and meridional biases of less than 0.08 m s−1. The standard deviation on the differences between Loon and reanalyses zonal winds is latitude-dependent, ranging between 2.5 and 3.5 m s−1, increasing equatorward. Comparisons between Loon trajectories and those calculated by applying a trajectory model to reanalysis wind fields show that MERRA-2 wind fields result in the most accurate simulated trajectories with a mean 5-day balloon–reanalysis trajectory separation of 621 km and median separation of 324 km showing significant improvements over MERRA version 1 and slightly outperforming ERA-Interim. The latitudinal structure of the trajectory statistics for all reanalyses displays marginally lower mean separations between 15 and 35° S than between 35 and 55° S, despite standard deviations in the wind differences increasing toward the equator. This is shown to be related to the distance travelled by the balloon playing a role in the separation statistics.

The Ross Sea region, including three main polynya areas in McMurdo Sound, Terra Nova Bay, and in front of the Ross Ice Shelf, has experienced a significant increase in sea ice extent in the first four decades of satellite observations. Here, we use Co-Registration of Optically Sensed Images and Correlation (COSI-Corr) to estimate 894 high-resolution sea ice motion fields of the Western Ross Sea in order to explore ice-atmosphere interactions based on sequential high-resolution Advanced Synthetic Aperture Radar (ASAR) images from the Envisat satellite acquired between 2002–2012. Validation of output motion vectors with manually drawn vectors for 24 image pairs show Pearson correlation coefficients of 0.92 ± 0.09 with a mean deviation in direction of −3.17 ± 6.48 degrees. The high-resolution vectors were also validated against the Environment and Climate Change Canada sea ice motion tracking algorithm, resulting in correlation coefficients of 0.84 ± 0.20 and the mean deviation in the direction of −0.04 ± 17.39 degrees. A total of 480 one-day separated velocity vector fields have been compared to an available NSIDC low-resolution sea ice motion vector product, showing much lower correlations and high directional differences. The high-resolution product is able to better identify short-term and spatial variations, whereas the low-resolution product underestimates the actual sea ice velocities by 47% in this important near-coastal region. The large-scale pattern of sea ice drift over the full time period is similar in both products. Improved image coverage is still desired to capture drift variations shorter than 24 h.