Explore the vast range of titles available.

Superfluidity, first discovered in liquid 4 He, is closely related to Bose–Einstein condensation (BEC) phenomenon. However, even at zero temperature, a fraction of the quantum liquid is excited out of the condensate into higher momentum states via interaction-induced fluctuations—the phenomenon of quantum depletion. Quantum depletion of atomic BECs in thermal equilibrium is well understood theoretically but is difficult to measure. This measurement is even more challenging in driven-dissipative exciton–polariton condensates, since their non-equilibrium nature is predicted to suppress quantum depletion. Here, we observe quantum depletion of a high-density exciton–polariton condensate by detecting the spectral branch of elementary excitations populated by this process. Analysis of this excitation branch shows that quantum depletion of exciton–polariton condensates can closely follow or strongly deviate from the equilibrium Bogoliubov theory, depending on the exciton fraction in an exciton polariton. Our results reveal beyond mean-field effects of exciton–polariton interactions and call for a deeper understanding of the relationship between equilibrium and non-equilibrium BECs. Many aspects of polariton condensate behaviour can be captured by mean-field theories but interactions introduce additional quantum effects. Here the authors observe quantum depletion in a driven-dissipative condensate and find that deviations from equilibrium predictions depend on the excitonic fraction.

We present an experimental study on optical properties and dynamics of direct and spatially and momentum indirect excitons in AlGaAs/AlAs quantum wells near the crossover between Γ - and X -valley confined electron states. The time-integrated photoluminescence experiment at T=4.8 K revealed three simultaneously observed optical transitions resulting from (a) a direct exciton recombination, involving an electron and a hole states both located in the Γ -valley in the quantum well layer, and (b) two spatially and momentum indirect excitons, comprising of the confined electron states in the X -valley in the AlAs barrier with different effective masses and quantum well holes in the Γ -valley. This interpretation has been based on the optical pumping density-dependent, temperature-dependent and spatially-resolved photoluminescence measurements, which provided the characterization of the structure, crucial in potential system’s applications. Additionally, the time-resolved photoluminescence experiments unveiled complex carrier relaxation dynamics in the investigated quantum well system, which is strongly governed by a non-radiative carrier recombination - the characteristics further critical in potential system’s use. This solid state platform hosting both direct and indirect excitons in a highly tunable monolithic system can benefit and underline the operation principles of novel electronic and photonic devices.

Semiconductor microcavities are often influenced by structural imperfections, which can disturb the flow and dynamics of exciton-polariton condensates. Additionally, in exciton-polariton condensates there is a variety of dynamical scenarios and instabilities, owing to the properties of the incoherent excitonic reservoir. We investigate the dynamics of an exciton-polariton condensate which emerges in semiconductor microcavity subject to disorder, which determines its spatial and temporal behaviour. Our experimental data revealed complex burst-like time evolution under non-resonant optical pulsed excitation. The temporal patterns of the condensate emission result from the intrinsic disorder and are driven by properties of the excitonic reservoir, which decay in time much slower with respect to the polariton condensate lifetime. This feature entails a relaxation oscillation in polariton condensate formation, resulting in ultrafast emission pulses of coherent polariton field. The experimental data can be well reproduced by numerical simulations, where the condensate is coupled to the excitonic reservoir described by a set of rate equations. Theory suggests the existence of slow reservoir temporarily emptied by stimulated scattering to the condensate, generating ultrashort pulses of the condensate emission.

Many bosons can occupy a single quantum state without a limit. It is described by the quantum-mechanical Bose–Einstein statistic, which allows Bose–Einstein condensation at low temperatures and high particle densities. Photons, historically the first considered bosonic gas, were late to show this phenomenon, observed in rhodamine-filled microcavities and doped fibre cavities. These findings have raised the question of whether condensation is also common in other laser systems with potential technological applications. Here we show the Bose–Einstein condensation of photons in a broad-area vertical-cavity surface-emitting laser with a slight cavity-gain spectral detuning. We observed a Bose–Einstein condensate in the fundamental transversal optical mode at a critical phase-space density. The experimental results follow the equation of state for a two-dimensional gas of bosons in thermal equilibrium, although the extracted spectral temperatures were lower than the device’s. This is interpreted as originating from the driven-dissipative nature of the photon gas. In contrast, non-equilibrium lasing action is observed in the higher-order modes in more negatively detuned device. Our work opens the way for the potential exploration of superfluid physics of interacting photons mediated by semiconductor optical nonlinearities. It also shows great promise for enabling single-mode high-power emission from a large-aperture device. Bose–Einstein condensation of photons is demonstrated in a large-aperture electrically driven InGaAs vertical-cavity surface-emitting laser diode at room temperature. The observed photon Bose–Einstein condensate exhibits the fundamental transversal optical mode at a critical phase-space density.

Optical trapping has been proven to be an effective method of separating exciton-polariton condensates from the incoherent high-energy excitonic reservoir located at the pumping laser position. This technique has significantly improved the coherent properties of exciton-polariton condensates, when compared to a quasi-homogeneous spot excitation scheme. Here, we compare two experimental methods on a sample, where a single spot excitation experiment allowed only to observe photonic lasing in the weak coupling regime. In contrast, the ring-shaped excitation resulted in the two-threshold behavior, where an exciton-polariton condensate manifests itself at the first and photon lasing at the second threshold. Both lasing regimes are trapped in an optical potential created by the pump. We interpret the origin of this confining potential in terms of repulsive interactions of polaritons with the reservoir at the first threshold and as a result of the excessive free-carrier induced refractive index change of the microcavity at the second threshold. This observation offers a way to achieve multiple phases of photonic condensates in samples, e.g., containing novel materials as an active layer, where two-threshold behavior is impossible to achieve with a single excitation spot.

Exciton-polariton laser is a promising source of coherent light for low-energy applications due to its low-threshold operation. However, a detailed experimental study of its spectral purity, which directly affects its coherence properties is still missing. Here}, we present a high-resolution spectroscopic investigation of the energy and linewidth of an exciton-polariton laser in the single-mode regime, which derives its coherent emission from an optically pumped and confined exciton-polariton condensate. We report an ultra-narrow linewidth of 56~MHz or 0.24~\\(\\mu\\)eV, corresponding to a coherence time of 5.7~ns. The narrow linewidth is consistently achieved by using an exciton-polariton condensate with a high photonic content confined in an optically induced trap. Contrary to previous studies, we show that the excitonic reservoir created by the pump and responsible for creating the trap does not strongly affect the emission linewidth as long as the condensate is trapped and the pump power is well above the condensation (lasing) threshold. \\red{The long coherence time of the exciton-polariton system uncovered here opens up opportunities for manipulating its macroscopic quantum state, which is essential for applications in classical and quantum computing.

We provide an analytical and numerical description of relaxation oscillations in the nonresonantly pumped polariton condensate. The presented considerations are based on the open dissipative Gross-Pitaevskii equation coupled to a pair of rate equations. The evolution of the condensate density can be explained qualitatively by studying the topology of the trajectory in phase space. We use a fixed points analysis for the classification of the different regimes of condensate dynamics, including fast stabilization, slow oscillations and ultrashort pulse emission. We obtain an analytical condition for the occurrence of relaxation oscillations. Continuous and pulsed condensate excitation considered and we demonstrate that in the latter case the existence of the second reservoir is necessary for the emergence of oscillations. We show that relaxation oscillations should be expected to occur in systems with relatively short polariton lifetime.

We present an experimental study on optical properties and dynamics of direct and spatially and momentum indirect excitons in AlGaAs/AlAs quantum wells near the crossover between \\(\\varGamma-\\) and \\(X\\)-valley confined electron states. The time-integrated photoluminescence experiment at \\(T=\\)4.8 K revealed three simultaneously observed optical transitions resulting from (a) a direct exciton recombination, involving an electron and a hole states both located in the \\(\\varGamma\\)-valley in the quantum well layer, and (b) two spatially and momentum indirect excitons, comprising of the confined electron states in the \\(X\\)-valley in the AlAs barrier with different effective masses and quantum well holes in the \\(\\varGamma\\)-valley. This interpretation has been based on the optical pumping density-dependent, temperature-dependent and spatially-resolved photoluminescence measurements, which provided the characterization of the structure, crucial in potential system's applications. Additionally, the time-resolved photoluminescence experiments unveiled complex carrier relaxation dynamics in the investigated quantum well system, which is strongly governed by a non-radiative carrier recombination - the characteristics further critical in potential system's use. This solid state platform hosting both direct and indirect excitons in a highly tunable monolithic system can benefit and underline the operation principles of novel electronic and photonic devices.

Although energy level repulsion is typically observed in interacting quantum systems, non-Hermitian physics predicts the effect of level attraction, which occurs when significant energy dissipation is present. Here, we show a manifestation of dissipative coupling in a high-quality AlGaAs-based polariton microcavity, where two polariton branches attract, resulting in an anomalous, inverted dispersion of the lower branch in momentum dispersion. Using angle-resolved photoluminescence measurements we observe the evolution of the level attraction with exciton-photon detuning, leading to changes in anomalous dispersion shape within a single sample. The dissipative coupling is explained by the interaction with an indirect exciton, acting as a highly dissipative channel in our system, and the observed dispersions are well captured within a phenomenological model. Our results present a new mechanism of dissipative coupling in light-matter systems and offer a tunable and well-controlled AlGaAs-based platform for engineering the non-Hermitian and negative mass effects in polariton systems.

We demonstrate an experimental approach to create dissipative solitons in a microcavity laser. In particular, we shape the spatial gain profile of a quasi-one-dimensional microcavity laser with a nonresonant, pulsed optical pump to create spatially localised structures, called gain-pinned dissipative solitons that exist due to the balance of gain and nonlinear losses and are confined to a diffraction-limited volume. The ultrafast formation dynamics and decay of the gain-pinned solitons are probed directly, showing that they are created on a picosecond timescale, orders of magnitude faster than laser cavity solitons. All of the experimentally observed features and dynamics are reconstructed by using a standard complex Ginzburg-Landau model.