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We present an improved algorithm based on the POlarization LIdar PHOtometer Networking (POLIPHON) method to retrieve cloud condensation nuclei (CCN) concentration profiles from spaceborne lidar observations. Our previous paper, which was the first study to demonstrate the feasibility of using measurements from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) to retrieve CCN is revisited. Our results focus on the Evaluation of CALIPSO’s Aerosol Classification scheme over Eastern Mediterranean (ACEMED) research campaign that took place over Thessaloniki, Greece, in September 2011. We compare our results with our earlier retrievals, discussing the critical changes that have been made and the importance of using the proper conversions factors. We also demonstrate the use of conversion factors acquired based on CALIPSO aerosol typing for CCN retrievals. The analysis highlights the strong influence of smoke on CCN concentrations and shows that the assumed aging state of the smoke can significantly alter the retrieval outcome.

Monitoring and describing the spatiotemporal variability in dust aerosols is crucial for understanding their multiple effects, related feedbacks, and impacts within the Earth system. This study describes the development of the ModIs Dust AeroSol (MIDAS) data set. MIDAS provides columnar daily dust optical depth (DOD) at 550 nm at a global scale and fine spatial resolution (0.1∘ × 0.1∘) over a 15-year period (2003–2017). This new data set combines quality filtered satellite aerosol optical depth (AOD) retrievals from MODIS-Aqua at swath level (Collection 6.1; Level 2), along with DOD-to-AOD ratios provided by the Modern-Era Retrospective analysis for Research and Applications version 2 (MERRA-2) reanalysis to derive DOD on the MODIS native grid. The uncertainties of the MODIS AOD and MERRA-2 dust fraction, with respect to the AEronet RObotic NETwork (AERONET) and LIdar climatology of vertical Aerosol Structure for space-based lidar simulation (LIVAS), respectively, are taken into account for the estimation of the total DOD uncertainty. MERRA-2 dust fractions are in very good agreement with those of LIVAS across the dust belt in the tropical Atlantic Ocean and the Arabian Sea; the agreement degrades in North America and the Southern Hemisphere, where dust sources are smaller. MIDAS, MERRA-2, and LIVAS DODs strongly agree when it comes to annual and seasonal spatial patterns, with colocated global DOD averages of 0.033, 0.031, and 0.029, respectively; however, deviations in dust loading are evident and regionally dependent. Overall, MIDAS is well correlated with AERONET-derived DODs (R=0.89) and only shows a small positive bias (0.004 or 2.7 %). Among the major dust areas of the planet, the highest R values (>0.9) are found at sites of North Africa, the Middle East, and Asia. MIDAS expands, complements, and upgrades the existing observational capabilities of dust aerosols, and it is suitable for dust climatological studies, model evaluation, and data assimilation.

We present a 3-D climatology of the desert dust distribution over South and East Asia derived using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) data. To distinguish desert dust from total aerosol load we apply a methodology developed in the framework of EARLINET (European Aerosol Research Lidar Network). The method involves the use of the particle linear depolarization ratio and updated lidar ratio values suitable for Asian dust, applied to multiyear CALIPSO observations (January 2007–December 2015). The resulting dust product provides information on the horizontal and vertical distribution of dust aerosols over South and East Asia along with the seasonal transition of dust transport pathways. Persistent high D_AOD (dust aerosol optical depth) values at 532 nm, of the order of 0.6, are present over the arid and semi-arid desert regions. Dust aerosol transport (range, height and intensity) is subject to high seasonality, with the highest values observed during spring for northern China (Taklimakan and Gobi deserts) and during summer over the Indian subcontinent (Thar Desert). Additionally, we decompose the CALIPSO AOD (aerosol optical depth) into dust and non-dust aerosol components to reveal the non-dust AOD over the highly industrialized and densely populated regions of South and East Asia, where the non-dust aerosols yield AOD values of the order of 0.5. Furthermore, the CALIPSO-based short-term AOD and D_AOD time series and trends between January 2007 and December 2015 are calculated over South and East Asia and over selected subregions. Positive trends are observed over northwest and east China and the Indian subcontinent, whereas over southeast China trends are mostly negative. The calculated AOD trends agree well with the trends derived from Aqua MODIS (Moderate Resolution Imaging Spectroradiometer), although significant differences are observed over specific regions.

Default aerosol extinction coefficient profiles are commonly used instead of measured profiles in radiative transfer modeling, increasing the uncertainties in the simulations. The present study aimed to determine the magnitude of these uncertainties and contribute towards the understanding of the complex interactions between aerosols and solar radiation. Default, artificial and measured profiles of the aerosol extinction coefficient were used to simulate the profiles of different radiometric quantities in the atmosphere for different surface, atmospheric, and aerosol properties and for four spectral bands: ultraviolet-B, ultraviolet-A, visible, and near-infrared. Case studies were performed over different areas in Europe and North Africa. Analysis of the results showed that under cloudless skies, changing the altitude of an artificial aerosol layer has minor impact on the levels of shortwave radiation at the top and bottom of the atmosphere, even for high aerosol loads. Differences of up to 30% were, however, detected for individual spectral bands. Using measured instead of default profiles for the simulations led to more significant differences in the atmosphere, which became very large during dust episodes (10–60% for actinic flux at altitudes between 1 and 2 km, and up to 15 K/day for heating rates depending on the site and solar elevation).

This study estimates the impact of dust aerosols on surface solar radiation and solar energy in Egypt based on Earth Observation (EO) related techniques. For this purpose, we exploited the synergy of monthly mean and daily post processed satellite remote sensing observations from the MODerate resolution Imaging Spectroradiometer (MODIS), radiative transfer model (RTM) simulations utilizing machine learning, in conjunction with 1-day forecasts from the Copernicus Atmosphere Monitoring Service (CAMS). As cloudy conditions in this region are rare, aerosols in particular dust, are the most common sources of solar irradiance attenuation, causing performance issues in the photovoltaic (PV) and concentrated solar power (CSP) plant installations. The proposed EO-based methodology is based on the solar energy nowcasting system (SENSE) that quantifies the impact of aerosol and dust on solar energy potential by using the aerosol optical depth (AOD) in terms of climatological values and day-to-day monitoring and forecasting variability from MODIS and CAMS, respectively. The forecast accuracy was evaluated at various locations in Egypt with substantial PV and CSP capacity installed and found to be within 5–12% of that obtained from the satellite observations, highlighting the ability to use such modelling approaches for solar energy management and planning (M&P). Particulate matter resulted in attenuation by up to 64–107 kWh/m2 for global horizontal irradiance (GHI) and 192–329 kWh/m2 for direct normal irradiance (DNI) annually. This energy reduction is climatologically distributed between 0.7% and 12.9% in GHI and 2.9% to 41% in DNI with the maximum values observed in spring following the frequent dust activity of Khamaseen. Under extreme dust conditions the AOD is able to exceed 3.5 resulting in daily energy losses of more than 4 kWh/m2 for a 10 MW system. Such reductions are able to cause financial losses that exceed the daily revenue values. This work aims to show EO capabilities and techniques to be incorporated and utilized in solar energy studies and applications in sun-privileged locations with permanent aerosol sources such as Egypt.

North Africa, the Middle East, and Europe (NAMEE domain) host a variety of suspended particles characterized by different optical and microphysical properties. In the current study, we investigate the importance of the lidar ratio (LR) on Cloud-Aerosol Lidar with Orthogonal Polarization–Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIOP-CALIPSO) aerosol retrievals towards assessing aerosols’ impact on the Earth-atmosphere radiation budget. A holistic approach has been adopted involving collocated Aerosol Robotic Network (AERONET) observations, Radiative Transfer Model (RTM) simulations, as well as reference radiation measurements acquired using spaceborne (Clouds and the Earth’s Radiant Energy System-CERES) and ground-based (Baseline Surface Radiation Network-BSRN) instruments. We are assessing the clear-sky shortwave (SW) direct radiative effects (DREs) on 550 atmospheric scenes, identified within the 2007–2020 period, in which the primary tropospheric aerosol species (dust, marine, polluted continental/smoke, elevated smoke, and clean continental) are probed using CALIPSO. RTM runs have been performed relying on CALIOP retrievals in which the default and the DeLiAn (Depolarization ratio, Lidar ratio, and Ångström exponent)-based aerosol-speciated LRs are considered. The simulated fields from both configurations are compared against those produced when AERONET AODs are applied. Overall, the DeLiAn LRs leads to better results mainly when mineral particles are either solely recorded or coexist with other aerosol species (e.g., sea-salt). In quantitative terms, the errors in DREs are reduced by ~26–27% at the surface (from 5.3 to 3.9 W/m2) and within the atmosphere (from −3.3 to −2.4 W/m2). The improvements become more significant (reaching up to ~35%) for moderate-to-high aerosol loads (AOD ≥ 0.2).

Turkey is located in the heart of complex transition geography between Eurasia and the Middle East. In the grand scheme, the so-called eastern Mediterranean Basin is located almost in the middle of the dusty belt, and is a hot spot of climate change. The downstream location of dust-carrying winds from close desert sources reveals Turkey as an open plane to particulate matter exposure throughout the year. In order to clarify this phenomenon, this paper aims to determine the desert dust climatology of Turkey via CALIPSO onboard Lidar. This prominent instrument enables us to understand clouds, aerosols and their types, and related climatic systems, with its valuable products. In this study, a 9-year CALIPSO-derived pure dust product dataset was formed to explain horizontal and vertical distributions, transport heights and case incidences. The results indicated that the pure dust extinction coefficient increased as the location shifted from west to east. Moreover, in the same direction of west to east, the dominant spring months changed to summer and autumn. Mountain range systems surrounding Anatolia were the main obstacles against lofted and buoyant dust particles travelling to northern latitudes. Even if high ridges accumulated mass load on the southern slopes, they also enabled elevated particles to reach the ground level of the inner cities.

A record-breaking dust episode took place in Crete on 22 March 2018. The event was characterized by surface concentrations exceeding 1 mg m−3 for a period of 4–7 h, reaching record values higher than 6 mg m−3 at the background station of Finokalia. We present here a detailed analysis of the atmospheric dynamical processes during this period, to identify the main reasons for such extreme dust advection over Crete. At the synoptic scale, the weakening of the polar vortex and the meridional transport of polar air masses at upper tropospheric layers resulted in a strong jet streak over north Africa and Central Mediterranean and corresponding tropospheric folding that brought cold stratospheric air in mid and upper troposphere. Cyclogenesis occurred at the Gulf of Sirte in Libya, resulting in strong winds over the north-east parts of Libya, enhancing particle emissions. The dust plume traveled at low altitude (0.5–3 km) along the warm conveyor belt preceding the depression cold front. This type of dusty southerly wind is commonly known as “Khamsin”. As the flow approached Crete, Foehn winds at the lee side of the island favored the downward mixing of dust towards the surface, resulting in local maxima of PM10 in Heraklion and Finokalia. The analysis is based on the combination of high-resolution WRF-Chem simulations reaching up to 1 × 1 km grid space over Crete, ground-based and satellite remote sensing of the dust plumes (PollyXT LiDAR, MSG-SEVIRI, MODIS) and detailed surface aerosol in situ measurements at urban (Heraklion, Chania, Greece) and background (Finokalia) stations in Crete.

We present here the first cloud condensation nuclei (CCN) concentration profiles derived from measurements with the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) aboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO), for different aerosol types at a supersaturation of 0.15%. CCN concentrations, along with the corresponding uncertainties, were inferred for a nighttime CALIPSO overpass on 9 September 2011, with coincident observations with the Facility for Airborne Atmospheric Measurements (FAAM) BAe-146 research aircraft, within the framework of the Evaluation of CALIPSO’s Aerosol Classification scheme over Eastern Mediterranean (ACEMED) research campaign over Thessaloniki, Greece. The CALIPSO aerosol typing is evaluated, based on data from the Copernicus Atmosphere Monitoring Service (CAMS) reanalysis. Backward trajectories and satellite-based fire counts are used to examine the origin of air masses on that day. Our CCN retrievals are evaluated against particle number concentration retrievals at different height levels, based on the ACEMED airborne measurements and compared against CCN-related retrievals from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensors aboard Terra and Aqua product over Thessaloniki showing that it is feasible to obtain CCN concentrations from CALIPSO, with an uncertainty of a factor of two to three.

During August 2016, a quasi-stationary high-pressure system spreading over Central and North-Eastern Europe, caused weather conditions that allowed for 24/7 observations of aerosol optical properties by using a complex multi-wavelength PollyXT lidar system with Raman, polarization and water vapour capabilities, based at the European Aerosol Research Lidar Network (EARLINET network) urban site in Warsaw, Poland. During 24–30 August 2016, the lidar-derived products (boundary layer height, aerosol optical depth, Ångström exponent, lidar ratio, depolarization ratio) were analysed in terms of air mass transport (HYSPLIT model), aerosol load (CAMS data) and type (NAAPS model) and confronted with active and passive remote sensing at the ground level (PolandAOD, AERONET, WIOS-AQ networks) and aboard satellites (SEVIRI, MODIS, CATS sensors). Optical properties for less than a day-old fresh biomass burning aerosol, advected into Warsaw’s boundary layer from over Ukraine, were compared with the properties of long-range transported 3–5 day-old aged biomass burning aerosol detected in the free troposphere over Warsaw. Analyses of temporal changes of aerosol properties within the boundary layer, revealed an increase of aerosol optical depth and Ångström exponent accompanied by an increase of surface PM10 and PM2.5. Intrusions of advected biomass burning particles into the urban boundary layer seem to affect not only the optical properties observed but also the top height of the boundary layer, by moderating its increase.