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This paper presents a comprehensive assessment of historical (1990–2010) global anthropogenic particulate matter (PM) emissions including the consistent and harmonized calculation of mass-based size distribution (PM1, PM2. 5, PM10), as well as primary carbonaceous aerosols including black carbon (BC) and organic carbon (OC). The estimates were developed with the integrated assessment model GAINS, where source- and region-specific technology characteristics are explicitly included. This assessment includes a number of previously unaccounted or often misallocated emission sources, i.e. kerosene lamps, gas flaring, diesel generators, refuse burning; some of them were reported in the past for selected regions or in the context of a particular pollutant or sector but not included as part of a total estimate. Spatially, emissions were calculated for 172 source regions (as well as international shipping), presented for 25 global regions, and allocated to 0.5°  ×  0.5° longitude–latitude grids. No independent estimates of emissions from forest fires and savannah burning are provided and neither windblown dust nor unpaved roads emissions are included. We estimate that global emissions of PM have not changed significantly between 1990 and 2010, showing a strong decoupling from the global increase in energy consumption and, consequently, CO2 emissions, but there are significantly different regional trends, with a particularly strong increase in East Asia and Africa and a strong decline in Europe, North America, and the Pacific region. This in turn resulted in important changes in the spatial pattern of PM burden, e.g. European, North American, and Pacific contributions to global emissions dropped from nearly 30 % in 1990 to well below 15 % in 2010, while Asia's contribution grew from just over 50 % to nearly two-thirds of the global total in 2010. For all PM species considered, Asian sources represented over 60 % of the global anthropogenic total, and residential combustion was the most important sector, contributing about 60 % for BC and OC, 45 % for PM2. 5, and less than 40 % for PM10, where large combustion sources and industrial processes are equally important. Global anthropogenic emissions of BC were estimated at about 6.6 and 7.2 Tg in 2000 and 2010, respectively, and represent about 15 % of PM2. 5 but for some sources reach nearly 50 %, i.e. for the transport sector. Our global BC numbers are higher than previously published owing primarily to the inclusion of new sources. This PM estimate fills the gap in emission data and emission source characterization required in air quality and climate modelling studies and health impact assessments at a regional and global level, as it includes both carbonaceous and non-carbonaceous constituents of primary particulate matter emissions. The developed emission dataset has been used in several regional and global atmospheric transport and climate model simulations within the ECLIPSE (Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants) project and beyond, serves better parameterization of the global integrated assessment models with respect to representation of black carbon and organic carbon emissions, and built a basis for recently published global particulate number estimates.

Methane is the second most important greenhouse gas after carbon dioxide contributing to human-made global warming. Keeping to the Paris Agreement of staying well below two degrees warming will require a concerted effort to curb methane emissions in addition to necessary decarbonization of the energy systems. The fastest way to achieve emission reductions in the 2050 timeframe is likely through implementation of various technical options. The focus of this study is to explore the technical abatement and cost pathways for reducing global methane emissions, breaking reductions down to regional and sector levels using the most recent version of IIASA's Greenhouse gas and Air pollution Interactions and Synergies (GAINS) model. The diverse human activities that contribute to methane emissions make detailed information on potential global impacts of actions at the regional and sectoral levels particularly valuable for policy-makers. With a global annual inventory for 1990-2015 as starting point for projections, we produce a baseline emission scenario to 2050 against which future technical abatement potentials and costs are assessed at a country and sector/technology level. We find it technically feasible in year 2050 to remove 54 percent of global methane emissions below baseline, however, due to locked in capital in the short run, the cumulative removal potential over the period 2020-2050 is estimated at 38 percent below baseline. This leaves 7.7 Pg methane released globally between today and 2050 that will likely be difficult to remove through technical solutions. There are extensive technical opportunities at low costs to control emissions from waste and wastewater handling and from fossil fuel production and use. A considerably more limited technical abatement potential is found for agricultural emissions, in particular from extensive livestock rearing in developing countries. This calls for widespread implementation in the 2050 timeframe of institutional and behavioural options in addition to technical solutions.

Scenarios that limit global warming to 1.5 °C describe major transformations in energy supply and ever-rising energy demand. Here, we provide a contrasting perspective by developing a narrative of future change based on observable trends that results in low energy demand. We describe and quantify changes in activity levels and energy intensity in the global North and global South for all major energy services. We project that global final energy demand by 2050 reduces to 245 EJ, around 40% lower than today, despite rises in population, income and activity. Using an integrated assessment modelling framework, we show how changes in the quantity and type of energy services drive structural change in intermediate and upstream supply sectors (energy and land use). Down-sizing the global energy system dramatically improves the feasibility of a low-carbon supply-side transformation. Our scenario meets the 1.5 °C climate target as well as many sustainable development goals, without relying on negative emission technologies. Achieving sustainable development goals while meeting the 1.5 °C climate target requires radical changes to how we use energy. A scenario of low energy demand shows how this can be done by down-sizing the global energy system to enable feasible deployment rates of renewable energy resources.

High levels of air pollution pose an urgent social and public health challenge in many Asian regions. This study evaluates the role of key factors that determined the changes in emission levels in China, India and Japan over the past 25 years. While emissions of air pollutants have been declining in Japan since the 1990s, China and India have experienced a rapid growth in pollution levels in recent years. Around 2005, control measures for sulfur emissions started to deliver expected reductions in China, followed by cuts in nitrogen oxides ten years later. Despite recent policy interventions, growing emission trends in India persist. A decomposition analysis of emission-driving factors indicates that emission levels would have been at least two-times higher without the improvements in energy intensity and efficiency, combined with end-of-pipe measures. Due to the continuous reliance on fossil fuels, the abatement effect of a cleaner fuel mix was in most cases significantly smaller than other factors. A reassessment of emission projections developed in the past suggests a decisive impact of energy and environmental policies. It is expected that targeted legislative instruments will play a dominant role in achieving future air-quality goals in Asia.

Low-carbon investments are necessary for driving the energy system transformation that is called for by both the Paris Agreement and Sustainable Development Goals. Improving understanding of the scale and nature of these investments under diverging technology and policy futures is therefore of great importance to decision makers. Here, using six global modelling frameworks, we show that the pronounced reallocation of the investment portfolio required to transform the energy system will not be initiated by the current suite of countries’ Nationally Determined Contributions. Charting a course toward ‘well below 2 °C’ instead sees low-carbon investments overtaking fossil investments globally by around 2025 or before and growing thereafter. Pursuing the 1.5 °C target demands a marked upscaling in low-carbon capital beyond that of a 2 °C-consistent future. Actions consistent with an energy transformation would increase the costs of achieving the goals of energy access and food security, but reduce the costs of achieving air-quality goals. The scale and nature of energy investments under diverging technology and policy futures is of great importance to decision makers. Here, a multi-model study projects investment needs under countries’ nationally determined contributions and in pathways consistent with achieving the 2 °C and 1.5 °C targets as well as certain SDGs.

Low-carbon pathways consistent with the 2 °C and 1.5 °C long-term climate goals defined in the Paris Agreement are likely to induce substantial co-benefits for air pollution and associated health impacts. In this analysis, using five global integrated assessment models, we quantify the emission reductions in key air pollutants resulting from the decarbonization of energy systems and the resulting changes in premature mortality attributed to the exposure to ambient concentrations of fine particulate matter. The emission reductions differ by sectors. Sulfur emissions are mainly reduced from power plants and industry, cuts in nitrogen oxides are dominated by the transport sector, and the largest abatement of primary fine particles is achieved in the residential sector. The analysis also shows that health benefits are the largest when policies addressing climate change mitigation and stringent air pollution controls are coordinated. We decompose the key factors that determine the extent of health co-benefits, focusing on Asia: changes in emissions, urbanization rates, population growth and ageing. Demographic processes, particularly due to ageing population, counteract in many regions the mortality reductions realized through lower emissions.

This paper analyses factors that contributed to the evolution of SO₂, NOₓ and CO₂ emissions in Europe from 1960 to 2010. Historical energy balances, along with population and economic growth data, are used to quantify the impacts of major determinants of changing emission levels, including energy intensity, conversion efficiency, fuel mix, and pollution control. Time series of emission levels are compared for countries in Western and Eastern Europe, throwing light on differences in the importance of particular emission-driving forces. Three quarters of the decline in SO₂ emissions in Western Europe resulted from a combination of reduced energy intensity and improved fuel mix, while dedicated end-of-pipe abatement measures played a dominant role in the reduction of NOₓ emissions. The increase in atmospheric emissions in Eastern Europe through the mid-1990s was associated with the growth of energy-intensive industries, which off-setted the positive impact of better fuel quality and changes in fuel mix. A continuous decrease in energy intensity and higher conversion efficiencies have been the main factors responsible for the moderate rate of growth of European CO₂ emissions.

Despite low per capita emissions, with over a billion population, India is pivotal for climate change mitigation globally, ranking as the third largest emitter of greenhouse gases. We linked a previously published multidimensional population projection with emission projections from an integrated assessment model to quantify the localised (i.e. state-level) health benefits from reduced ambient fine particulate matter in India under global climate change mitigation scenarios in line with the Paris Agreement targets and national scenarios for maximum feasible air quality control. We incorporated assumptions about future demographic, urbanisation and epidemiological trends and accounted for model feedbacks. Our results indicate that compared to a business-as-usual scenario, pursuit of aspirational climate change mitigation targets can avert up to 8.0 million premature deaths and add up to 0.7 years to life expectancy (LE) at birth due to cleaner air by 2050. Combining aggressive climate change mitigation efforts with maximum feasible air quality control can add 1.6 years to LE. Holding demographic change constant, we find that climate change mitigation and air quality control will contribute slightly more to increases in LE in urban areas than in rural areas and in states with lower socio-economic development.

Many children in India face the double burden of high exposure to ambient (AAP) and household air pollution, both of which can affect their linear growth. Although climate change mitigation is expected to decrease AAP, climate policies could increase the cost of clean cooking fuels. Here, we develop a static microsimulation model to project the air pollution-related burden of child stunting in India up to 2050 under four scenarios combining climate change mitigation (2 °C target) with national policies for AAP control and subsidised access to clean cooking. We link data from a nationally representative household survey, satellite-based estimates of fine particulate matter (PM 2.5 ), a multi-dimensional demographic projection and PM 2.5 and clean cooking access projections from an integrated assessment model. We find that the positive effects on child linear growth from reductions in AAP under the 2 °C Paris Agreement target could be fully offset by the negative effects of climate change mitigation through reduced clean cooking access. Targeted AAP control or subsidised access to clean cooking could shift this trade-off to result in net benefits of 2.8 (95% uncertainty interval [UI]: 1.4, 4.2) or 6.5 (UI: 6.3, 6.9) million cumulative prevented cases of child stunting between 2020–50 compared to business-as-usual. Implementation of integrated climate, air quality, and energy access interventions has a synergistic impact, reducing cumulative number of stunted children by 12.1 (UI: 10.7, 13.7) million compared to business-as-usual, with the largest health benefits experienced by the most disadvantaged children and geographic regions. Findings underscore the importance of complementing climate change mitigation efforts with targeted air quality and energy access policies to concurrently deliver on carbon mitigation, health and air pollution and energy poverty reduction goals in India.

A shift from fossil fuel to renewable energy is crucial in limiting global temperature increase to 2 °C above preindustrial levels. However, renewable energy technologies, solar photovoltaics, wind turbines, and electric vehicles are metal-intensive, and the mining and smelting processes to obtain the needed metals are emission-intensive. We estimate the future PM2.5 emissions from mining and smelting to meet the metal demand of renewable energy technologies in two climate pathways to be 0.3–0.6 Tg yr−1 in the 2020–2050 period, which are projected to contribute 10%–30% of total anthropogenic primary PM2.5 combustion emissions in many countries. The concentration of mineral reserves in a few regions means the impacts are also regionally concentrated. Rapid decarbonization could lead to a faster reduction of overall anthropogenic PM2.5 emissions but also could create more unevenness in the distributions of emissions relative to where demand occurs. Options to reduce metal-related PM2.5 emissions by over 90% exist and are well understood; introducing policy requiring their installation could avoid emission hotspots.