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The impact of measurement imperfections on quantum metrology protocols has not been approached in a systematic manner so far. In this work, we tackle this issue by generalising firstly the notion of quantum Fisher information to account for noisy detection, and propose tractable methods allowing for its approximate evaluation. We then show that in canonical scenarios involving N probes with local measurements undergoing readout noise, the optimal sensitivity depends crucially on the control operations allowed to counterbalance the measurement imperfections—with global control operations, the ideal sensitivity (e.g., the Heisenberg scaling) can always be recovered in the asymptotic N limit, while with local control operations the quantum-enhancement of sensitivity is constrained to a constant factor. We illustrate our findings with an example of NV-centre magnetometry, as well as schemes involving spin-1/2 probes with bit-flip errors affecting their two-outcome measurements, for which we find the input states and control unitary operations sufficient to attain the ultimate asymptotic precision. The effects of detection noise on quantum metrology performances have not been rigorously investigated yet. Here, the authors fill this gap by generalising the quantum Fisher information to the case of noisy readout, and showing the consequences the imperfect measurements bring.

State-of-the-art methods for sensing weak AC fields are only efficient in the low frequency domain (<10 MHz). The inefficiency of sensing high-frequency signals is due to the lack of ability to use dynamical decoupling. In this paper we show that dynamical decoupling can be incorporated into high-frequency sensing schemes and by this we demonstrate that the high sensitivity achieved for low frequency can be extended to the whole spectrum. While our scheme is general and suitable to a variety of atomic and solid-state systems, we experimentally demonstrate it with the nitrogen-vacancy center in diamond. For a diamond with natural abundance of 13 C, we achieve coherence times up to 1.43 ms resulting in a smallest detectable magnetic field strength of 4 nT at 1.6 GHz. Attributed to the inherent nature of our scheme, we observe an additional increase in coherence time due to the signal itself. State-of-the-art methods for sensing weak AC fields are only efficient in the low frequency domain. Here, Stark et al. demonstrate a sensing scheme that is capable of probing high frequencies through continuous dynamical coupling by applying it to a nitrogen-vacancy centre in diamond.

Spin-based quantum information processing makes extensive use of spin-state manipulation. This ranges from dynamical decoupling of nuclear spins in quantum sensing experiments to applying logical gates on qubits in a quantum processor. Fast manipulation of spin states is highly desirable for accelerating experiments, enhancing sensitivity, and applying elaborate pulse sequences. Strong driving using intense radio-frequency (RF) fields can, therefore, facilitate fast manipulation and enable broadband excitation of spin species. In this work, we present an antenna for strong driving in quantum sensing experiments and theoretically address challenges of the strong driving regime. First, we designed and implemented a micron-scale planar spiral RF antenna capable of delivering intense fields to a sample. The planar antenna is tailored for quantum sensing experiments using the diamond’s nitrogen-vacancy (NV) center and should be applicable to other solid-state defects. The antenna has a broad bandwidth of 22 MHz, is compatible with scanning probes, and is suitable for cryogenic and ultrahigh vacuum conditions. We measure the magnetic field induced by the antenna and estimate a field-to-current ratio of 113 ± 16  G/A, representing a six-fold increase in efficiency compared to the state-of-the-art, crucial for cryogenic experiments. We demonstrate the antenna by driving Rabi oscillations in 1 H spins of an organic sample on the diamond surface and measure 1 H Rabi frequencies of over 500 kHz, i.e. π -pulses shorter than 1  μ s —an order of magnitude faster than previously reported in NV-based nuclear magnetic resonance (NMR). Finally, we discuss the implications of driving spins with a field tilted from the transverse plane in a regime where the driving amplitude is comparable to the spin-state splitting, such that the rotating wave approximation does not describe the dynamics well. We present a simple recipe to optimize pulse fidelity in this regime based on a phase and offset-shifted sine drive, which may be optimized in situ without numerical optimization procedures or precise modeling of the experiment. We consider this approach in a range of driving amplitudes and show that it is particularly efficient in the case of a tilted driving field. The results presented here constitute a foundation for implementing fast nuclear spin control in various systems.

Diffusion broadening of spectral lines is the main limitation to frequency resolution in non-polarized liquid state nano-NMR. This problem arises from the limited amount of information that can be extracted from the signal before losing coherence. For liquid state NMR as with most generic sensing experiments, the signal is thought to decay exponentially, severely limiting resolution. However, there is theoretical evidence that predicts a power law decay of the signal’s correlations due to diffusion noise in the non-polarized nano-NMR scenario. In this work we show that in the NV based nano-NMR setup such diffusion noise results in high spectral resolution.

Nitrogen-Vacancy (NV) centers in diamonds have been shown in recent years to be excellent magnetometers on the nanoscale. One of the recent applications of the quantum sensor is retrieving the Nuclear Magnetic Resonance (NMR) spectrum of a minute sample, whose net polarization is well below the Signal-to-Noise Ratio (SNR) of classic devices. The information in the magnetic noise of diffusing particles has also been shown in decoherence spectroscopy approaches to provide a method for measuring different physical parameters. Similar noise is induced on the NV center by a flowing liquid. However, when the noise created by diffusion effects is more dominant than the noise of the drift, it is unclear whether the velocity can be efficiently estimated. Here we propose a non-intrusive setup for measuring the drift velocity near the surface of a flow channel based on magnetic field quantum sensing using NV centers. We provide a detailed analysis of the sensitivity for different measurement protocols, and we show that our nanoscale velocimetry scheme outperforms current fluorescence based approaches even when diffusion noise is dominant. Our scheme can be applied for the investigation of microfluidic channels, where the drift velocity is usually low and the flow properties are currently unclear. A better understanding of these properties is essential for the future development of microfluidic and nanofluidic infrastructures.

We present a novel method for engineering an optical clock transition that is robust against external field fluctuations and is able to overcome limits resulting from field inhomogeneities. The technique is based on the application of continuous driving fields to form a pair of dressed states essentially free of all relevant shifts. Specifically, the clock transition is robust to magnetic field shifts, quadrupole and other tensor shifts, and amplitude fluctuations of the driving fields. The scheme is applicable to either a single ion or an ensemble of ions, and is relevant for several types of ions, such as 40 Ca + , 88 Sr + , 138 Ba + and 176 Lu + . Taking a spherically symmetric Coulomb crystal formed by 400 40 Ca + ions as an example, we show through numerical simulations that the inhomogeneous linewidth of tens of Hertz in such a crystal together with linear Zeeman shifts of order 10 MHz are reduced to form a linewidth of around 1 Hz. We estimate a two-order-of-magnitude reduction in averaging time compared to state-of-the art single ion frequency references, assuming a probe laser fractional instability of 10 − 15 . Furthermore, a statistical uncertainty reaching 2.9 × 10−16 in 1 s is estimated for a cascaded clock scheme in which the dynamically decoupled Coulomb crystal clock stabilizes the interrogation laser for an 27 Al + clock.

A novel two-qubit entangling gate for trapped-ion quantum processors is proposed theoretically and demonstrated experimentally. During the gate, double-dressed quantum states are created by applying a phase-modulated continuous driving field. The speed of this quantum gate is an order of magnitude higher than that of previously demonstrated rf controlled two-qubit entangling gates in static magnetic field gradients. At the same time, the field driving the gate dynamically decouples the qubits from amplitude and frequency noise, increasing the qubits’ coherence time by 3 orders of magnitude. The gate requires only a single continuous rf field per qubit, making it well suited for scaling a quantum processor to large numbers of qubits. Implementing this entangling gate, we generate the Bell states | Φ + ⟩ and | Ψ + ⟩ in less than or equal to 313 μ s with fidelities up to 98 − 3 + 2 % in a static magnetic gradient of only 19.09 T / m . At higher magnetic field gradients, the entangling gate speed can be further improved to match that of laser-based counterparts.

Precise frequency measurements are important in applications ranging from navigation and imaging to computation and communication. Here we outline the optimal quantum strategies for frequency discrimination and estimation in the context of quantum spectroscopy, and we compare the effectiveness of different readout strategies. Using a single NV center in diamond, we implement the optimal frequency discrimination protocol to discriminate two frequencies separated by 2 kHz with a single 44 μs measurement, a factor of ten below the Fourier limit. For frequency estimation, we achieve a frequency sensitivity of 1.6 µHz/Hz2 for a 1.7 µT amplitude signal, which is within a factor of 2 from the quantum limit. Our results are foundational for discrimination and estimation problems in nanoscale nuclear magnetic resonance spectroscopy.

We present a novel continuous dynamical decoupling scheme for the construction of a robust qubit in a three-level system. By means of a clock transition adjustment, we first show how robustness to environmental noise is achieved, while eliminating drive-noise, to first-order. We demonstrate this scheme with the spin sub-levels of the NV-centre’s electronic ground state. By applying drive fields with moderate Rabi frequencies, the drive noise is eliminated and an improvement of 2 orders of magnitude in the coherence time is obtained compared to the pure dephasing time. We then show how the clock transition adjustment can be tuned to eliminate also the second-order effect of the environmental noise with moderate drive fields. A further detailed theoretical investigation suggests an additional improvement of more than 1 order of magnitude in the coherence time which is supported by simulations. Hence, our scheme predicts that the coherence time may be prolonged towards the lifetime-limit using a relatively simple experimental setup.