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The neutrino mass experiment KATRIN uses conversion electrons from the 32.2-keV transition of the nuclear isomer 83mKr for calibration. Comparing the measured energies to the appropriate literature values allows for an independent evaluation of the energy scale, but the uncertainties in some of the literature values obtained by gamma spectroscopy are a limiting factor. Building upon the already excellent linearity of KATRIN’s energy scale, this paper proposes a novel method for determining the 83mKr transition energies via high-precision electron spectroscopy. Notably, the method makes use of conversion electrons from the 41.6-keV direct transition of 83mKr to its ground state in addition to conversion electrons from the much more frequent cascade of a 32.2-keV and a 9.4-keV transition. By implementing this method, KATRIN may be able to deliver order-of-magnitude improvements in precision over current 83mKr transition energy literature values. Although concretely described here in the context of the KATRIN experiment and with 83mKr, the method’s underlying principles are general enough for it to likely be a useful tool in various other nuclear spectroscopy settings.

Since the discovery of neutrino oscillations, we know that neutrinos have non-zero mass. However, the absolute neutrino-mass scale remains unknown. Here we report the upper limits on effective electron anti-neutrino mass, m ν , from the second physics run of the Karlsruhe Tritium Neutrino experiment. In this experiment, m ν is probed via a high-precision measurement of the tritium β -decay spectrum close to its endpoint. This method is independent of any cosmological model and does not rely on assumptions whether the neutrino is a Dirac or Majorana particle. By increasing the source activity and reducing the background with respect to the first physics campaign, we reached a sensitivity on m ν of 0.7 eV  c –2  at a 90% confidence level (CL). The best fit to the spectral data yields m ν 2  = (0.26 ± 0.34) eV 2   c –4 , resulting in an upper limit of m ν  < 0.9 eV  c –2  at 90% CL. By combining this result with the first neutrino-mass campaign, we find an upper limit of m ν  < 0.8 eV  c –2 at 90% CL. In its second measurement campaign, the Karlsruhe Tritium Neutrino experiment achieved a sub-electronvolt sensitivity on the effective electron anti-neutrino mass.

In this work we present a keV-scale sterile-neutrino search with a low-tritium-activity data set of the KATRIN experiment, acquired in a commissioning run in 2018. KATRIN performs a spectroscopic measurement of the tritium β -decay spectrum with the main goal of directly determining the effective electron anti-neutrino mass. During this commissioning phase a lower tritium activity facilitated the measurement of a wider part of the tritium spectrum and thus the search for sterile neutrinos with a mass of up to 1.6 keV . We do not find a signal and set an exclusion limit on the sterile-to-active mixing amplitude of sin 2 θ < 5 × 10 - 4 ( 95 % C.L.) at a mass of 0.3 keV. This result improves current laboratory-based bounds in the sterile-neutrino mass range between 0.1 and 1.0 keV.

The projected sensitivity of the effective electron neutrino-mass measurement with the KATRIN experiment is below 0.3 eV (90 % CL) after 5 years of data acquisition. The sensitivity is affected by the increased rate of the background electrons from KATRIN’s main spectrometer. A special shifted-analysing-plane (SAP) configuration was developed to reduce this background by a factor of two. The complex layout of electromagnetic fields in the SAP configuration requires a robust method of estimating these fields. We present in this paper a dedicated calibration measurement of the fields using conversion electrons of gaseous 83m Kr, which enables the neutrino-mass measurements in the SAP configuration.

Precision spectroscopy of the electron spectrum of the tritium β -decay near the kinematic endpoint is a direct method to determine the effective electron antineutrino mass. The KArlsruhe TRItium Neutrino (KATRIN) experiment aims to determine this quantity with a sensitivity of better than 0.3 eV ( 90 %  C.L.). An inhomogeneous electric potential in the tritium source of KATRIN can lead to distortions of the β -spectrum, which directly impact the neutrino-mass observable. This effect can be quantified through precision spectroscopy of the conversion-electrons of co-circulated metastable 83 m Kr . Therefore, dedicated, several-weeks long measurement campaigns have been performed within the KATRIN data taking schedule. In this work, we infer the tritium source potential observables from these measurements, and present their implications for the neutrino-mass determination.

The KATRIN experiment is designed for a direct and model-independent determination of the effective electron anti-neutrino mass via a high-precision measurement of the tritium β-decay endpoint region with a sensitivity on mν of 0.2 eV/c2 (90% CL). For this purpose, the β-electrons from a high-luminosity windowless gaseous tritium source traversing an electrostatic retarding spectrometer are counted to obtain an integral spectrum around the endpoint energy of 18.6 keV. A dominant systematic effect of the response of the experimental setup is the energy loss of β-electrons from elastic and inelastic scattering off tritium molecules within the source. We determined the energy-loss function in-situ with a pulsed angular-selective and monoenergetic photoelectron source at various tritium-source densities. The data was recorded in integral and differential modes; the latter was achieved by using a novel time-of-flight technique. We developed a semi-empirical parametrization for the energy-loss function for the scattering of 18.6-keV electrons from hydrogen isotopologs. This model was fit to measurement data with a 95% T2 gas mixture at 30 K, as used in the first KATRIN neutrino-mass analyses, as well as a D2 gas mixture of 96% purity used in KATRIN commissioning runs. The achieved precision on the energy-loss function has abated the corresponding uncertainty of σ(mν2)<10-2eV2 [1] in the KATRIN neutrino-mass measurement to a subdominant level.

The KArlsruhe TRItium Neutrino experiment (KATRIN) aims to determine the effective electron (anti)-neutrino mass with a sensitivity of 0.2eV/c 2 by precisely measuring the endpoint region of the tritium β -decay spectrum. It uses a tandem of electrostatic spectrometers working as magnetic adiabatic collimation combined with an electrostatic (MAC-E) filters. In the space between the pre-spectrometer and the main spectrometer, creating a Penning trap is unavoidable when the superconducting magnet between the two spectrometers, biased at their respective nominal potentials, is energized. The electrons accumulated in this trap can lead to discharges, which create additional background electrons and endanger the spectrometer and detector section downstream. To counteract this problem, “electron catchers” were installed in the beamline inside the magnet bore between the two spectrometers. These catchers can be moved across the magnetic-flux tube and intercept on a sub-ms time scale the stored electrons along their magnetron motion paths. In this paper, we report on the design and the successful commissioning of the electron catchers and present results on their efficiency in reducing the experimental background.

Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere is important to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe data sets and a methodology to quantify all major components of the global carbon budget, including their uncertainties, based on the combination of a range of data, algorithms, statistics and model estimates and their interpretation by a broad scientific community. We discuss changes compared to previous estimates, consistency within and among components, alongside methodology and data limitations. CO2 emissions from fossil-fuel combustion and cement production (EFF) are based on energy statistics, while emissions from land-use change (ELUC), mainly deforestation, are based on combined evidence from land-cover change data, fire activity associated with deforestation, and models. The global atmospheric CO2 concentration is measured directly and its rate of growth (GATM) is computed from the annual changes in concentration. The mean ocean CO2 sink (SOCEAN) is based on observations from the 1990s, while the annual anomalies and trends are estimated with ocean models. The variability in SOCEAN is evaluated for the first time in this budget with data products based on surveys of ocean CO2 measurements. The global residual terrestrial CO2 sink (SLAND) is estimated by the difference of the other terms of the global carbon budget and compared to results of independent dynamic global vegetation models forced by observed climate, CO2 and land cover change (some including nitrogen–carbon interactions). All uncertainties are reported as ±1σ, reflecting the current capacity to characterise the annual estimates of each component of the global carbon budget. For the last decade available (2003–2012), EFF was 8.6 ± 0.4 GtC yr−1, ELUC 0.9 ± 0.5 GtC yr−1, GATM 4.3 ± 0.1 GtC yr−1, SOCEAN 2.5 ± 0.5 GtC yr−1, and SLAND 2.8 ± 0.8 GtC yr−1. For year 2012 alone, EFF grew to 9.7 ± 0.5 GtC yr−1, 2.2% above 2011, reflecting a continued growing trend in these emissions, GATM was 5.1 ± 0.2 GtC yr−1, SOCEAN was 2.9 ± 0.5 GtC yr−1, and assuming an ELUC of 1.0 ± 0.5 GtC yr−1 (based on the 2001–2010 average), SLAND was 2.7 ± 0.9 GtC yr−1. GATM was high in 2012 compared to the 2003–2012 average, almost entirely reflecting the high EFF. The global atmospheric CO2 concentration reached 392.52 ± 0.10 ppm averaged over 2012. We estimate that EFF will increase by 2.1% (1.1–3.1%) to 9.9 ± 0.5 GtC in 2013, 61% above emissions in 1990, based on projections of world gross domestic product and recent changes in the carbon intensity of the economy. With this projection, cumulative emissions of CO2 will reach about 535 ± 55 GtC for 1870–2013, about 70% from EFF (390 ± 20 GtC) and 30% from ELUC (145 ± 50 GtC). This paper also documents any changes in the methods and data sets used in this new carbon budget from previous budgets (Le Quéré et al., 2013). All observations presented here can be downloaded from the Carbon Dioxide Information Analysis Center (doi:10.3334/CDIAC/GCP_2013_V2.3).

The KATRIN experiment aims to measure the effective electron antineutrino mass \\[m_{\\overline{\\nu }_e}\\] with a sensitivity of \\[{0.2}\\,{\\hbox {eV}/\\hbox {c}^2}\\] using a gaseous tritium source combined with the MAC-E filter technique. A low background rate is crucial to achieving the proposed sensitivity, and dedicated measurements have been performed to study possible sources of background electrons. In this work, we test the hypothesis that gamma radiation from external radioactive sources significantly increases the rate of background events created in the main spectrometer (MS) and observed in the focal-plane detector. Using detailed simulations of the gamma flux in the experimental hall, combined with a series of experimental tests that artificially increased or decreased the local gamma flux to the MS, we set an upper limit of \\[{0.006}\\,{\\hbox {count}/\\hbox {s}}\\] (90% C.L.) from this mechanism. Our results indicate the effectiveness of the electrostatic and magnetic shielding used to block secondary electrons emitted from the inner surface of the MS.

Interannual anomalies in the sea-air carbon dioxide (CO2 ) exchange have been estimated from surface-ocean CO2 partial pressure measurements. Available data are sufficient to constrain these anomalies in large parts of the tropical and North Pacific and in the North Atlantic, in some areas covering the period from the mid 1980s to 2011. Global interannual variability is estimated as about 0.31 Pg C yr-1 (temporal standard deviation 1993-2008). The tropical Pacific accounts for a large fraction of this global variability, closely tied to El Niño-Southern Oscillation (ENSO). Anomalies occur more than 6 months later in the east than in the west. The estimated amplitude and ENSO response are roughly consistent with independent information from atmospheric oxygen data. This both supports the variability estimated from surface-ocean carbon data and demonstrates the potential of the atmospheric oxygen signal to constrain ocean biogeochemical processes. The ocean variability estimated from surface-ocean carbon data can be used to improve land CO2 flux estimates from atmospheric inversions.