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Light is confined transversely and delivered axially in a waveguide. However, waveguides are lossy static structures whose modal characteristics are fundamentally determined by their boundary conditions. Here we show that unpatterned planar waveguides can provide low-loss two-dimensional waveguiding by using space-time wave packets, which are unique one-dimensional propagation-invariant pulsed optical beams. We observe hybrid guided space-time modes that are index-guided in one transverse dimension and localized along the unbounded dimension. We confirm that these fields enable overriding the boundary conditions by varying post-fabrication the group index of the fundamental mode in a 2-μm-thick, 25-mm-long silica film, achieved by modifying the field’s spatio-temporal structure. Tunability of the group index over an unprecedented range from 1.26 to 1.77 is verified while maintaining a spectrally flat zero-dispersion profile. Our work paves the way to utilizing space-time wave packets in on-chip platforms, and enable phase-matching strategies that circumvent restrictions due to intrinsic material properties. Waveguides typically function by using boundary conditions to contain light. Here, the authors show that by using space-time wavepackets, light can be guided in an unpatterned planar waveguide as the field remains localized along the unbounded dimension.

Surface plasmon polaritons (SPPs) at metal-dielectric interfaces provide strong out-of-plane confinement enabling nano-scale sensing and imaging, yet diffraction causes spatial delocalization. Conventional strategies to combat diffraction through spatial structuring are inapplicable to dimensionally restricted SPPs, except for nonlocalized cosine plasmons and Airy plasmons that follow curved trajectories. Here we demonstrate space-time SPPs (ST-SPPs), ultrashort (16-fs) diffraction-free SPPs that propagate rectilinearly via precise sculpting of their spatiotemporal spectra. By synthesizing a spatiotemporally structured field in free space and coupling the field to an axially invariant ST-SPP at a metal-dielectric surface, we control the ST-SPP group velocity and propagation characteristics. Time-resolved two-photon fluorescence microscopy reconstructs the surface-bound field in space and time, verifying the predicted spatiotemporal wavefront and diffraction-free propagation. Our work opens new avenues for combining spatiotemporally structured light with the field-localization associated with nanophotonics, and may thus enable novel applications in surface-enhanced sensing and nonlinear optical interactions. The authors report the observation of diffraction-free space-time surface plasmon polaritons propagating along straight paths at metal-dielectric interfaces. This enhances the control of wavepacket propagation for nanophotonics applications.

Relatively new materials for mid-infrared tunable lasing using chromium-doped Cd sub(1-x)Mn sub(x)Te and cobalt-doped Cd sub(1-x)Mn sub(x)Te have been developed. Previously, ZnS and ZnSe were used as host materials for chromium to produce mid-infrared (MIR) lasing. Compared to these materials, large diameter CdMnTe is easier to grow (using the Bridgman technique) and can be made more homogeneous. Moreover, the ternary nature of Cd sub(1-x)Mn sub(x)Te offers the unique opportunity to optimize the optical properties of the material through variation of chemical composition and lattice parameter. Using Cd sub(0.55)Mn sub(0.45)Te:Cr, we have demonstrated room temperature lasing from 2.1 to 3.1 mu m, and we have demonstrated quasi-continuous wave (cw) lasing. To our knowledge, the observed tuning range ([similar to]840 nm) of Cr super(2+):Cd sub(0.55)Mn sub(0.45)Te is the largest ever reported from a transition metal ion laser. Furthermore, this is the first time that a room temperature quasi-cw laser operating at 3 mu m has been demonstrated using this type of material. Also, preliminary work on Cd sub(0.55)Mn sub(0.45)Te:Co indicates its potential for tunable mid-infrared lasing around 3600 nm at cryogenic temperatures. Results from inductively coupled plasma mass spectrometry (ICP-MS), which determine the concentration of dopant that has been incorporated into the host lattice, will be reported, as will the materials characterization and lasing results. The processing issues for optimizing the laser performance in these material systems will also be discussed.

When an optical pulse is focused into a multimode waveguide or fiber, the energy is divided among the available guided modes. Consequently, the initially localized intensity spreads transversely, the spatial profile undergoes rapid variations with axial propagation, and the pulse disperses temporally. Space-time (ST) supermodes are pulsed guided field configurations that propagate invariantly in multimode waveguides by assigning each mode to a prescribed wavelength. ST supermodes can be thus viewed as spectrally discrete, guided-wave counterpart of the recently demonstrated propagation-invariant ST wave packets in free space. The group velocity of an ST supermode is tunable independently -- in principle -- of the waveguide structure, group-velocity dispersion is eliminated or dramatically curtailed, and the time-averaged intensity profile is axially invariant along the waveguide in absence of mode-coupling. We establish here a theoretical framework for studying ST supermodes in planar waveguides. Modal engineering allows sculpting this axially invariant transverse intensity profile from an on-axis peak or dip (dark beam), to a multi-peak or flat distribution. Moreover, ST supermodes can be synthesized using spectrally incoherent light, thus paving the way to potential applications in optical beam delivery for lighting applications.

High-finesse planar Fabry-Pérot (FP) cavities spectrally filter the incident field at discrete resonances, and thus cannot be utilized to resonantly enhance the field of ultrashort pulses. Introducing judicious angular dispersion into a pulse can give rise to `omni-resonance', whereby the entire bandwidth of a spatiotemporally structured ultrafast pulse couples to a single longitudinal cavity resonance, even when the pulse bandwidth far exceeds the resonant linewidth. Here we show that omni-resonance increases the intra-cavity peak intensity above that of a pulse having equal energy and bandwidth when tightly focused in free space -- maintained across its entire bandwidth and along a cavity longer than the Rayleigh length of the focused pulse. This paves the way towards broadband resonant enhancement of nonlinear optical effects, thereby bridging the gap between ultrafast optics and resonant photonics.

In addition to longitudinal spin angular momentum (SAM) along the axis of propagation of light, spatially structured electromagnetic fields such as evanescent waves and focused beams have recently been found to possess transverse SAM in the direction perpendicular to the axis of propagation. In particular, the SAM of SPPs with spatial structure has been extensively studied in the last decade after it became clear that evanescent fields with spatially structured energy flow generate threedimensional spin texture. Here we present numerical calculations of the space-time surface plasmon polariton (ST-SPP) wave packet, a plasmonic bullet that propagates at an arbitrary group velocity while maintaining its spatial distribution. ST-SPP wave packets with complex spatial structure and energy flow density distribution determined by the group velocity are found to propagate with accompanying three-dimensional spin texture and finite topological charge density. Furthermore, the spatial distribution of the spin texture and topological charge density determined by the spatial structure of the SPP is controllable, and the deformation associated with propagation is negligible. ST-SPP wave packets, which can stably transport customizable three-dimensional spin textures and topological charge densities, can be excellent subjects of observation in studies of spinphotonics and optical topological materials.

Because surface plasmon polaritons (SPPs) are surface waves characterized by one free transverse dimension, the only monochromatic diffraction-free spatial profiles for SPPs are cosine and Airy waves. Pulsed SPP wave packets have been recently formulated that are propagation-invariant and localized in the in-plane dimensions by virtue of a tight spectral association between their spatial and temporal frequencies, which have thus been dubbed `space-time' (ST) SPPs. Because of the spatio-temporal spectral structure unique to ST-SPPs, the optimal launching strategy of such novel plasmonic field configurations remains an open question. We present here a critical step towards realizing ST-SPPs by reporting observations of ultrabroadband striped ST-SPPs. These are SPPs in which each wavelength travels at a prescribed angle with respect to the propagation axis to produce a periodic (striped) transverse spatial profile that is diffraction-free. We start with a free-space ST wave packet that is coupled to a ST-SPP at a gold-dielectric interface, and unambiguously identify the ST-SPP via an axial beating detected in two-photon fluorescence produced by the superposition of incident ST wave packet and the excited surface-bound ST-SPP. These results highlight a viable approach for efficient and reliable coupling to ST-SPPs, and thus represent the first crucial step towards realization of the full potential of ST-SPPs for plasmonic sensing and imaging.

Angular dispersion (AD) is a ubiquitous phenomenon in optics after light traverses a diffractive or dispersive device, whereby each wavelength propagates at a different angle. AD is useful in a variety of applications; for example, modifying the group velocity or group-velocity dispersion of pulsed lasers in free space or optical materials, which are essential ingredients in group-velocity matching and dispersion compensation. Conventional optical components introduce `differentiable' AD, so that the propagation angle can be expanded perturbatively around a fixed frequency, in which only a few low AD-orders are typically relevant. However, this model does not encompass newly emerging classes of propagation-invariant pulsed optical fields, such as `space-time wave packets', which incorporate a new form of AD that we call `non-differentiable AD'. This is a surprising feature: there exists a frequency at which the derivative of the propagation angle with respect to frequency is not defined. Consequently, the propagation angle cannot be expanded perturbatively at this frequency, and a large number of independently controllable AD orders are needed to approximate this condition. Synthesizing these new AD-induced field configurations requires constructing a `universal AD synthesizer' capable of accessing the magnitude and sign of any AD order, a capability missing from any single optical component to date. This Perspective article provides a unified schema for studying differentiable and non-differentiable AD, shows that non-differentiable AD enables circumventing many well-established constraints in optics -- thereby giving rise to new applications, and outlines the requirements for a universal AD synthesizer capable of producing both forms of AD.

Surface plasmon polaritons (SPPs) are surface-bound waves at metal-dielectric interfaces that exhibit strong out-of-plane field confinement, a key feature for applications is nano-scale sensing and imaging. However, this advantage is offset by diffractive spreading during in-plane propagation, leading to transverse spatial delocalization. Conventional strategies to combat diffraction through spatial structuring are not applicable for dimensionally restricted SPPs -- except for cosine plasmons that are not localized or Airy plasmons that propagate along a curved trajectory. Here, we report the first realization of space-time SPPs (ST-SPPs), ultrashort (16 fs) diffraction-free SPPs that propagate in a straight line, whose unique propagation characteristics stem from precise sculpting of their spatiotemporal spectra. By first synthesizing a spatiotemporally structured field in free space, we couple the field to an axially invariant ST-SPP at a metal-dielectric surface via an ultra-broadband nanoslit coupling mechanism, further enabling control over the ST-SPP group velocity and propagation characteristics. Time-resolved two-photon fluorescence interference microscopy enables reconstructing the surface-bound field in space and time, thereby verifying their predicted phase-tilted spatiotemporal wave-front and diffraction-free propagation. Our work opens new avenues for combining spatiotemporally structured light with the field-localization associated with nanophotonics, and may thus enable novel applications in surface-enhanced sensing and nonlinear optical interactions.

When an optical pulse is spatially localized in a highly multimoded waveguide, its energy is typically distributed among a multiplicity of modes, thus giving rise to a speckled transverse spatial profile that undergoes erratic changes with propagation. It has been suggested theoretically that pulsed multimode fields in which each wavelength is locked to an individual mode at a prescribed axial wave number will propagate invariantly along the waveguide at a tunable group velocity. In this conception, an initially localized field remains localized along the waveguide. Here, we provide proof-of-principle experimental confirmation for the existence of this new class of pulsed guided fields, which we denote space-time supermodes, and verify their propagation invariance in a planar waveguide. By superposing up to 21 modes, each assigned to a prescribed wavelength, we construct space-time supermodes in a 170-micron-thick planar glass waveguide with group indices extending from 1 to 2. The initial transverse width of the field is 6 microns, and the waveguide length is 9.1 mm, which is 257x the associated Rayleigh range. A variety of axially invariant transverse spatial profiles are produced by judicious selection of the modes contributing to the ST supermode, including single-peak and multi-peak fields, dark fields (containing a spatial dip), and even flat uniform intensity profiles.