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"Stohl, A."
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Collective action in organizations : interaction and engagement in an era of technological change
\"This book explores how people participate in public life through organizations. The authors examine The American Legion, AARP, and MoveOn, and show surprising similarities across these three organizations\"--Provided by publisher.
Atmospheric transport is a major pathway of microplastics to remote regions
by
Klimont, Zbigniew
,
Heyes, Chris
,
Lopez-Aparicio, Susana
in
704/106/35
,
704/172/4081
,
704/844/4081
2020
In recent years, marine, freshwater and terrestrial pollution with microplastics has been discussed extensively, whereas atmospheric microplastic transport has been largely overlooked. Here, we present global simulations of atmospheric transport of microplastic particles produced by road traffic (TWPs – tire wear particles and BWPs – brake wear particles), a major source that can be quantified relatively well. We find a high transport efficiencies of these particles to remote regions. About 34% of the emitted coarse TWPs and 30% of the emitted coarse BWPs (100 kt yr−1 and 40 kt yr−1 respectively) were deposited in the World Ocean. These amounts are of similar magnitude as the total estimated direct and riverine transport of TWPs and fibres to the ocean (64 kt yr−1). We suggest that the Arctic may be a particularly sensitive receptor region, where the light-absorbing properties of TWPs and BWPs may also cause accelerated warming and melting of the cryosphere.
Journal Article
Beautiful creatures : dark secrets will come to light
by
LaGravenese, Richard film director, screenwriter
,
Stoff, Erwin film producer
,
Kosove, Andrew A. film producer
in
Psychic ability Drama
,
Family secrets Drama
,
Unrequited love Drama
2000
\"Lena has just moved to the small, Southern town of Gatlin, where the only person who seems to understand her, or dream of bigger places or ideas, is a cute guy named Ethan Wate, who recognizes her instantly from the cryptic dreams he's been having every night. Lena is an orphan, and she's come to stay with her mysterious uncle, Macon Ravenwood, the patriarch of her powerful family. Powerful, because The Ravenwood clan are Casters, born with powers that ordinary mortals don't have, like the ability to move objects, control the elements, and even step out of normal space and time to communicate only with each other. But just as Lena feels ready to open up to Ethan, she discovers that their love is in imminent danger, because when female Casters turn 16, their destiny as either good or evil is revealed. Unwilling to let her nature be dictated by forces outside her control, Lena and Ethan set out together to uncover the strange, secret lore of their families' intertwined histories dating back to the Civil War, and figure out how to grant Lena the power to choose her own destiny\"--Allmovie.com, September 28, 2018.
The 3‐Week‐Long Transport History and Deep Tropical Origin of the 2021 Extreme Heat Wave in the Pacific Northwest
2023
The heat wave in late June of 2021 (PNW21) set new temperature records in the Pacific Northwest (PNW). In Lytton the highest temperature ever recorded in Canada was measured. Several studies have already explored this extreme event in detail, however, here we compare the atmospheric air mass transport and heating processes associated with this heat wave with the 34 other most extreme heat events in the same region during the period 1960–2021, using a long backtracking time of 25 days. We found significant differences in the heat waves. During PNW21 most of the air was coming from the Philippine Sea, with more than 40% of the air located south of 15°N, and anomalous advection of sensible and latent heat from the Tropics was the dominant cause of PNW21. The latent heat was efficiently converted into sensible heat by precipitation, which was unique, as most other extremes experienced net diabatic cooling. Plain Language Summary At the end of June in 2021 a heat wave occurred over the Pacific Northwest (PNW) and led to catastrophic damage in the region, notably the destruction of the town of Lytton by a wild fire 1 day after a new temperature record for Canada was set there. Here we look at where the air during this event was coming from and compare the atmospheric mass transport to 34 other extreme heat events in this region. We found that during the heat wave in June 2021 most of the air was coming from the Philippine Sea where it took up large amounts of heat and moisture. This source region is deeper in the Tropics than for all other extreme events. At the same time, the Philippine Sea was anomalously warm. Thus, the air was warmer and moister than for all the other extreme events already 3 weeks before reaching the PNW. The energy associated with the high tropical moisture content was efficiently converted into heat by precipitation along the Meiyu‐Baiu front—a unique process not found for any other extreme heat event. Key Points The air causing the heat wave in late June 2021 (PNW21) came from deep in the Tropics, more south and west compared to other events Three weeks prior to the event, the air was warmer and moister, indicating that advection of heat from the Tropics was an important driver Condensation in a warm conveyor belt caused heating for PNW21, while most other extreme events showed overall diabatic cooling
Journal Article
Frequency of extreme precipitation increases extensively with event rareness under global warming
2019
The intensity of the heaviest extreme precipitation events is known to increase with global warming. How often such events occur in a warmer world is however less well established, and the combined effect of changes in frequency and intensity on the total amount of rain falling as extreme precipitation is much less explored, in spite of potentially large societal impacts. Here, we employ observations and climate model simulations to document strong increases in the frequencies of extreme precipitation events occurring on decadal timescales. Based on observations we find that the total precipitation from these intense events almost doubles per degree of warming, mainly due to changes in frequency, while the intensity changes are relatively weak, in accordance to previous studies. This shift towards stronger total precipitation from extreme events is seen in observations and climate models, and increases with the strength – and hence the rareness – of the event. Based on these results, we project that if historical trends continue, the most intense precipitation events observed today are likely to almost double in occurrence for each degree of further global warming. Changes to extreme precipitation of this magnitude are dramatically stronger than the more widely communicated changes to global mean precipitation.
Journal Article
A review of sea-spray aerosol source functions using a large global set of sea salt aerosol concentration measurements
2014
Sea-spray aerosols (SSA) are an important part of the climate system because of their effects on the global radiative budget – both directly as scatterers and absorbers of solar and terrestrial radiation, and indirectly as cloud condensation nuclei (CCN) influencing cloud formation, lifetime, and precipitation. In terms of their global mass, SSA have the largest uncertainty of all aerosols. In this study we review 21 SSA source functions from the literature, several of which are used in current climate models. In addition, we propose a~new function. Even excluding outliers, the global annual SSA mass produced spans roughly 3–70 Pg yr−1 for the different source functions, for particles with dry diameter Dp < 10 μm, with relatively little interannual variability for a given function. The FLEXPART Lagrangian particle dispersion model was run in backward mode for a large global set of observed SSA concentrations, comprised of several station networks and ship cruise measurement campaigns. FLEXPART backward calculations produce gridded emission sensitivity fields, which can subsequently be multiplied with gridded SSA production fluxes in order to obtain modeled SSA concentrations. This allowed us to efficiently and simultaneously evaluate all 21 source functions against the measurements. Another advantage of this method is that source-region information on wind speed and sea surface temperatures (SSTs) could be stored and used for improving the SSA source function parameterizations. The best source functions reproduced as much as 70% of the observed SSA concentration variability at several stations, which is comparable with \"state of the art\" aerosol models. The main driver of SSA production is wind, and we found that the best fit to the observation data could be obtained when the SSA production is proportional to U103.5, where U10 is the source region averaged 10 m wind speed. A strong influence of SST on SSA production, with higher temperatures leading to higher production, could be detected as well, although the underlying physical mechanisms of the SST influence remains unclear. Our new source function with wind speed and temperature dependence gives a global SSA production for particles smaller than Dp < 10 μm of 9 Pg yr−1, and is the best fit to the observed concentrations.
Journal Article
Xenon-133 and caesium-137 releases into the atmosphere from the Fukushima Dai-ichi nuclear power plant: determination of the source term, atmospheric dispersion, and deposition
2012
On 11 March 2011, an earthquake occurred about 130 km off the Pacific coast of Japan's main island Honshu, followed by a large tsunami. The resulting loss of electric power at the Fukushima Dai-ichi nuclear power plant developed into a disaster causing massive release of radioactivity into the atmosphere. In this study, we determine the emissions into the atmosphere of two isotopes, the noble gas xenon-133 (133Xe) and the aerosol-bound caesium-137 (137Cs), which have very different release characteristics as well as behavior in the atmosphere. To determine radionuclide emissions as a function of height and time until 20 April, we made a first guess of release rates based on fuel inventories and documented accident events at the site. This first guess was subsequently improved by inverse modeling, which combined it with the results of an atmospheric transport model, FLEXPART, and measurement data from several dozen stations in Japan, North America and other regions. We used both atmospheric activity concentration measurements as well as, for 137Cs, measurements of bulk deposition. Regarding 133Xe, we find a total release of 15.3 (uncertainty range 12.2–18.3) EBq, which is more than twice as high as the total release from Chernobyl and likely the largest radioactive noble gas release in history. The entire noble gas inventory of reactor units 1–3 was set free into the atmosphere between 11 and 15 March 2011. In fact, our release estimate is higher than the entire estimated 133Xe inventory of the Fukushima Dai-ichi nuclear power plant, which we explain with the decay of iodine-133 (half-life of 20.8 h) into 133Xe. There is strong evidence that the 133Xe release started before the first active venting was made, possibly indicating structural damage to reactor components and/or leaks due to overpressure which would have allowed early release of noble gases. For 137Cs, the inversion results give a total emission of 36.6 (20.1–53.1) PBq, or about 43% of the estimated Chernobyl emission. Our results indicate that 137Cs emissions peaked on 14–15 March but were generally high from 12 until 19 March, when they suddenly dropped by orders of magnitude at the time when spraying of water on the spent-fuel pool of unit 4 started. This indicates that emissions may not have originated only from the damaged reactor cores, but also from the spent-fuel pool of unit 4. This would also confirm that the spraying was an effective countermeasure. We explore the main dispersion and deposition patterns of the radioactive cloud, both regionally for Japan as well as for the entire Northern Hemisphere. While at first sight it seemed fortunate that westerly winds prevailed most of the time during the accident, a different picture emerges from our detailed analysis. Exactly during and following the period of the strongest 137Cs emissions on 14 and 15 March as well as after another period with strong emissions on 19 March, the radioactive plume was advected over Eastern Honshu Island, where precipitation deposited a large fraction of 137Cs on land surfaces. Radioactive clouds reached North America on 15 March and Europe on 22 March. By middle of April, 133Xe was fairly uniformly distributed in the middle latitudes of the entire Northern Hemisphere and was for the first time also measured in the Southern Hemisphere (Darwin station, Australia). In general, simulated and observed concentrations of 133Xe and 137Cs both at Japanese as well as at remote sites were in good quantitative agreement. Altogether, we estimate that 6.4 PBq of 137Cs, or 18% of the total fallout until 20 April, were deposited over Japanese land areas, while most of the rest fell over the North Pacific Ocean. Only 0.7 PBq, or 1.9% of the total fallout were deposited on land areas other than Japan.
Journal Article
Black carbon in the Arctic: the underestimated role of gas flaring and residential combustion emissions
by
Novigatsky, A. N.
,
Klimont, Z.
,
Shevchenko, V. P.
in
Aerosols
,
Air pollution control
,
Air temperature
2013
Arctic haze is a seasonal phenomenon with high concentrations of accumulation-mode aerosols occurring in the Arctic in winter and early spring. Chemistry transport models and climate chemistry models struggle to reproduce this phenomenon, and this has recently prompted changes in aerosol removal schemes to remedy the modeling problems. In this paper, we show that shortcomings in current emission data sets are at least as important. We perform a 3 yr model simulation of black carbon (BC) with the Lagrangian particle dispersion model FLEXPART. The model is driven with a new emission data set (\"ECLIPSE emissions\") which includes emissions from gas flaring. While gas flaring is estimated to contribute less than 3% of global BC emissions in this data set, flaring dominates the estimated BC emissions in the Arctic (north of 66° N). Putting these emissions into our model, we find that flaring contributes 42% to the annual mean BC surface concentrations in the Arctic. In March, flaring even accounts for 52% of all Arctic BC near the surface. Most of the flaring BC remains close to the surface in the Arctic, so that the flaring contribution to BC in the middle and upper troposphere is small. Another important factor determining simulated BC concentrations is the seasonal variation of BC emissions from residential combustion (often also called domestic combustion, which is used synonymously in this paper). We have calculated daily residential combustion emissions using the heating degree day (HDD) concept based on ambient air temperature and compare results from model simulations using emissions with daily, monthly and annual time resolution. In January, the Arctic-mean surface concentrations of BC due to residential combustion emissions are 150% higher when using daily emissions than when using annually constant emissions. While there are concentration reductions in summer, they are smaller than the winter increases, leading to a systematic increase of annual mean Arctic BC surface concentrations due to residential combustion by 68% when using daily emissions. A large part (93%) of this systematic increase can be captured also when using monthly emissions; the increase is compensated by a decreased BC burden at lower latitudes. In a comparison with BC measurements at six Arctic stations, we find that using daily-varying residential combustion emissions and introducing gas flaring emissions leads to large improvements of the simulated Arctic BC, both in terms of mean concentration levels and simulated seasonality. Case studies based on BC and carbon monoxide (CO) measurements from the Zeppelin observatory appear to confirm flaring as an important BC source that can produce pollution plumes in the Arctic with a high BC / CO enhancement ratio, as expected for this source type. BC measurements taken during a research ship cruise in the White, Barents and Kara seas north of the region with strong flaring emissions reveal very high concentrations of the order of 200–400 ng m−3. The model underestimates these concentrations substantially, which indicates that the flaring emissions (and probably also other emissions in northern Siberia) are rather under- than overestimated in our emission data set. Our results suggest that it may not be \"vertical transport that is too strong or scavenging rates that are too low\" and \"opposite biases in these processes\" in the Arctic and elsewhere in current aerosol models, as suggested in a recent review article (Bond et al., Bounding the role of black carbon in the climate system: a scientific assessment, J. Geophys. Res., 2013), but missing emission sources and lacking time resolution of the emission data that are causing opposite model biases in simulated BC concentrations in the Arctic and in the mid-latitudes.
Journal Article
The sources of atmospheric black carbon at a European gateway to the Arctic
by
Eckhardt, Sabine
,
Winiger, Patrik
,
Gustafsson, Örjan
in
704/106/35/824
,
704/106/694/682
,
704/172/4081
2016
Black carbon (BC) aerosols from incomplete combustion of biomass and fossil fuel contribute to Arctic climate warming. Models—seeking to advise mitigation policy—are challenged in reproducing observations of seasonally varying BC concentrations in the Arctic air. Here we compare year-round observations of BC and its δ
13
C/Δ
14
C-diagnosed sources in Arctic Scandinavia, with tailored simulations from an atmospheric transport model. The model predictions for this European gateway to the Arctic are greatly improved when the emission inventory of anthropogenic sources is amended by satellite-derived estimates of BC emissions from fires. Both BC concentrations (R
2
=0.89,
P
<0.05) and source contributions (R
2
=0.77,
P
<0.05) are accurately mimicked and linked to predominantly European emissions. This improved model skill allows for more accurate assessment of sources and effects of BC in the Arctic, and a more credible scientific underpinning of policy efforts aimed at efficiently reducing BC emissions reaching the European Arctic.
Black carbon (BC) contributes positively to the radiation budget, yet models are unable to correctly capture its seasonal variability in the Arctic. Here, the authors demonstrate improved model skill in simulating BC concentration and sources when including estimates of BC emissions from fires.
Journal Article
The Neisseria gonorrhoeae type IV pilus promotes resistance to hydrogen peroxide- and LL-37-mediated killing by modulating the availability of intracellular, labile iron
by
Stohl, Elizabeth A.
,
Hu, Linda I.
,
Seifert, H Steven
in
Antibiotics
,
Antiinfectives and antibacterials
,
Antimicrobial agents
2022
The Neisseria gonorrhoeae Type IV pilus is a multifunctional, dynamic fiber involved in host cell attachment, DNA transformation, and twitching motility. We previously reported that the N . gonorrhoeae pilus is also required for resistance against hydrogen peroxide-, antimicrobial peptide LL-37-, and non-oxidative, neutrophil-mediated killing. We tested whether the hydrogen peroxide, LL-37, and neutrophil hypersensitivity phenotypes in non-piliated N . gonorrhoeae could be due to elevated iron levels. Iron chelation in the growth medium rescued a nonpiliated pilE mutant from both hydrogen peroxide- and antimicrobial peptide LL-37-mediated killing, suggesting these phenotypes are related to iron availability. We used the antibiotic streptonigrin, which depends on free cytoplasmic iron and oxidation to kill bacteria, to determine whether piliation affected intracellular iron levels. Several non-piliated, loss-of-function mutants were more sensitive to streptonigrin killing than the piliated parental strain. Consistent with the idea that higher available iron levels in the under- and non-piliated strains were responsible for the higher streptonigrin sensitivity, iron limitation by desferal chelation restored resistance to streptonigrin in these strains and the addition of iron restored the sensitivity to streptonigrin killing. The antioxidants tiron and dimethylthiourea rescued the pilE mutant from streptonigrin-mediated killing, suggesting that the elevated labile iron pool in non-piliated bacteria leads to streptonigrin-dependent reactive oxygen species production. These antioxidants did not affect LL-37-mediated killing. We confirmed that the pilE mutant is not more sensitive to other antibiotics showing that the streptonigrin phenotypes are not due to general bacterial envelope disruption. The total iron content of the cell was unaltered by piliation when measured using ICP-MS suggesting that only the labile iron pool is affected by piliation. These results support the hypothesis that piliation state affects N . gonorrhoeae iron homeostasis and influences sensitivity to various host-derived antimicrobial agents.
Journal Article