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41
result(s) for
"Tschirhart, C. L."
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Intrinsic quantized anomalous Hall effect in a moiré heterostructure
2020
Quantum anomalous Hall effect—the appearance of quantized Hall conductance at zero magnetic field—has been observed in thin films of the topological insulator Bi 2 Se 3 doped with magnetic atoms. The doping, however, introduces inhomogeneity, reducing the temperature at which the effect occurs. Two groups have now observed quantum anomalous Hall effect in intrinsically magnetic materials (see the Perspective by Wakefield and Checkelsky). Serlin et al. did so in twisted bilayer graphene aligned to hexagonal boron nitride, where the effect enabled the switching of magnetization with tiny currents. In a complementary work, Deng et al. observed quantum anomalous Hall effect in the antiferromagnetic layered topological insulator MnBi 2 Te 4 . Science , this issue p. 900 , p. 895 ; see also p. 848 Transport measurements indicate quantized Hall conductance without a magnetic field. The quantum anomalous Hall (QAH) effect combines topology and magnetism to produce precisely quantized Hall resistance at zero magnetic field. We report the observation of a QAH effect in twisted bilayer graphene aligned to hexagonal boron nitride. The effect is driven by intrinsic strong interactions, which polarize the electrons into a single spin- and valley-resolved moiré miniband with Chern number C = 1. In contrast to magnetically doped systems, the measured transport energy gap is larger than the Curie temperature for magnetic ordering, and quantization to within 0.1% of the von Klitzing constant persists to temperatures of several kelvin at zero magnetic field. Electrical currents as small as 1 nanoampere controllably switch the magnetic order between states of opposite polarization, forming an electrically rewritable magnetic memory.
Journal Article
Electrical switching of magnetic order in an orbital Chern insulator
2020
Magnetism typically arises from the joint effect of Fermi statistics and repulsive Coulomb interactions, which favours ground states with non-zero electron spin. As a result, controlling spin magnetism with electric fields—a longstanding technological goal in spintronics and multiferroics
1
,
2
—can be achieved only indirectly. Here we experimentally demonstrate direct electric-field control of magnetic states in an orbital Chern insulator
3
–
6
, a magnetic system in which non-trivial band topology favours long-range order of orbital angular momentum but the spins are thought to remain disordered
7
–
14
. We use van der Waals heterostructures consisting of a graphene monolayer rotationally faulted with respect to a Bernal-stacked bilayer to realize narrow and topologically non-trivial valley-projected moiré minibands
15
–
17
. At fillings of one and three electrons per moiré unit cell within these bands, we observe quantized anomalous Hall effects
18
with transverse resistance approximately equal to
h
/2
e
2
(where
h
is Planck’s constant and
e
is the charge on the electron), which is indicative of spontaneous polarization of the system into a single-valley-projected band with a Chern number equal to two. At a filling of three electrons per moiré unit cell, we find that the sign of the quantum anomalous Hall effect can be reversed via field-effect control of the chemical potential; moreover, this transition is hysteretic, which we use to demonstrate non-volatile electric-field-induced reversal of the magnetic state. A theoretical analysis
19
indicates that the effect arises from the topological edge states, which drive a change in sign of the magnetization and thus a reversal in the favoured magnetic state. Voltage control of magnetic states can be used to electrically pattern non-volatile magnetic-domain structures hosting chiral edge states, with applications ranging from reconfigurable microwave circuit elements to ultralow-power magnetic memories.
Non-volatile electrical switching of magnetic order in an orbital Chern insulator is experimentally demonstrated using a moiré heterostructure and analysis shows that the effect is driven by topological edge states.
Journal Article
Intrinsic spin Hall torque in a moiré Chern magnet
2023
In spin torque magnetic memories, electrically actuated spin currents are used to switch a magnetic bit. Typically, these require a multilayer geometry including both a free ferromagnetic layer and a second layer providing spin injection. For example, spin may be injected by a non-magnetic layer exhibiting a large spin Hall effect, a phenomenon known as spin–orbit torque. Here we demonstrate a spin–orbit torque magnetic bit in a single two-dimensional system with intrinsic magnetism and strong Berry curvature. We study AB-stacked MoTe2/WSe2, which hosts a magnetic Chern insulator at a carrier density of one hole per moiré superlattice site. We observe hysteretic switching of the resistivity as a function of applied current. Magnetic imaging reveals that current switches correspond to reversals of individual magnetic domains. The real space pattern of domain reversals aligns with spin accumulation measured near the Hubbard band edges with high Berry curvature. This suggests that intrinsic spin or valley Hall torques drive the observed current-driven magnetic switching in both MoTe2/WSe2 and other moiré materials. The switching current density is substantially less than those reported in other platforms, suggesting that moiré heterostructures are a suitable platform for efficient control of magnetic order.Switching of magnetic behaviour is one of the main ideas that drives spintronics. Now, magnetic switching via spin-orbit torque is shown in a moiré bilayer, introducing a platform for spintronic applications.
Journal Article
Intervalley coherence and intrinsic spin–orbit coupling in rhombohedral trilayer graphene
by
Huber, Martin E.
,
Babikyan, Grigory
,
Taniguchi, Takashi
in
639/766/119/995
,
639/766/119/997
,
Atomic
2024
Rhombohedral graphene multilayers provide a clean and highly reproducible platform to explore the emergence of superconductivity and magnetism in a strongly interacting electron system. Here we reveal a subtle competition between valley-imbalanced orbital ferromagnets and intervalley-coherent states in which electron wavefunctions in the two momentum-space valleys develop a macroscopically coherent relative phase. We focus on a rhombohedral trilayer in the quarter-metal regime—where there is a single Fermi surface that spontaneously breaks spin and valley-isospin symmetry—and employ local magnetometry and global charge sensing techniques. Comparing the in-plane spin susceptibility of the intervalley-coherent and valley-imbalanced phases reveals the influence of graphene’s intrinsic spin–orbit coupling, which drives the emergence of a distinct correlated phase that is their hybrid. Spin–orbit coupling also suppresses the in-plane magnetic susceptibility of the valley-imbalanced phase, allowing us to extract the spin–orbit-coupling strength of approximately 50 μeV for our hexagonal-boron-nitride-encapsulated graphene system. We discuss the implications of a finite spin–orbit coupling on the spin-triplet superconductors observed in both rhombohedral and twisted graphene multilayers.
The role of electron–electron interactions in generating superconductivity in few-layer graphene remains controversial. Now, the observation of interaction-driven intervalley coherence may help to explain the Cooper pairing mechanism.
Journal Article
TOPOLOGICAL MATTER
2020
The quantum anomalous Hall (QAH) effect combines topology and magnetism to produce precisely quantized Hall resistance at zero magnetic field. We report the observation of a QAH effect in twisted bilayer graphene aligned to hexagonal boron nitride. The effect is driven by intrinsic strong interactions, which polarize the electrons into a single spin- and valley-resolved moiré miniband with Chern number C = 1. In contrast to magnetically doped systems, the measured transport energy gap is larger than the Curie temperature for magnetic ordering, and quantization to within 0.1% of the von Klitzing constant persists to temperatures of several kelvin at zero magnetic field. Electrical currents as small as 1 nanoampere controllably switch the magnetic order between states of opposite polarization, forming an electrically rewritable magnetic memory.
Journal Article
Intrinsic quantized anomalous Hall effect in a moiré heterostructure
2019
The quantum anomalous Hall (QAH) effect combines topology and magnetism to produce precisely quantized Hall resistance at zero magnetic field. We report the observation of a QAH effect in twisted bilayer graphene aligned to hexagonal boron nitride. The effect is driven by intrinsic strong interactions, which polarize the electrons into a single spin- and valley-resolved moiré miniband with Chern numberC= 1. In contrast to magnetically doped systems, the measured transport energy gap is larger than the Curie temperature for magnetic ordering, and quantization to within 0.1% of the von Klitzing constant persists to temperatures of several kelvin at zero magnetic field. Electrical currents as small as 1 nanoampere controllably switch the magnetic order between states of opposite polarization, forming an electrically rewritable magnetic memory.
Journal Article
Intervalley coherence and intrinsic spin-orbit coupling in rhombohedral trilayer graphene
by
Yaar Vituri
,
Babikyan, Grigory
,
Taniguchi, Takashi
in
Boron nitride
,
Coherence
,
Compressibility
2023
Rhombohedral graphene multilayers provide a clean and highly reproducible platform to explore the emergence of superconductivity and magnetism in a strongly interacting electron system. Here, we use electronic compressibility and local magnetometry to explore the phase diagram of this material class in unprecedented detail. We focus on rhombohedral trilayer in the quarter metal regime, where the electronic ground state is characterized by the occupation of a single spin and valley isospin flavor. Our measurements reveal a subtle competition between valley imbalanced (VI) orbital ferromagnets and intervalley coherent (IVC) states in which electron wave functions in the two momentum space valleys develop a macroscopically coherent relative phase. Contrasting the in-plane spin susceptibility of the IVC and VI phases reveals the influence of graphene's intrinsic spin-orbit coupling, which drives the emergence of a distinct correlated phase with hybrid VI and IVC character. Spin-orbit also suppresses the in-plane magnetic susceptibility of the VI phase, which allows us to extract the spin-orbit coupling strength of \\(\\lambda \\approx 50\\mu\\)eV for our hexagonal boron nitride-encapsulated graphene system. We discuss the implications of finite spin-orbit coupling on the spin-triplet superconductors observed in both rhombohedral and twisted graphene multilayers.
Intrinsic spin Hall torque in a moire Chern magnet
2022
In spin torque magnetic memories, electrically actuated spin currents are used to switch a magnetic bit. Typically, these require a multilayer geometry including both a free ferromagnetic layer and a second layer providing spin injection. For example, spin may be injected by a nonmagnetic layer exhibiting a large spin Hall effect, a phenomenon known as spin-orbit torque. Here, we demonstrate a spin-orbit torque magnetic bit in a single two-dimensional system with intrinsic magnetism and strong Berry curvature. We study AB-stacked MoTe2/WSe2, which hosts a magnetic Chern insulator at a carrier density of one hole per moire superlattice site. We observe hysteretic switching of the resistivity as a function of applied current. Magnetic imaging using a superconducting quantum interference device reveals that current switches correspond to reversals of individual magnetic domains. The real space pattern of domain reversals aligns precisely with spin accumulation measured near the high-Berry curvature Hubbard band edges. This suggests that intrinsic spin- or valley-Hall torques drive the observed current-driven magnetic switching in both MoTe2/WSe2 and other moire materials. The switching current density of 10^3 Amps per square centimeter is significantly less than reported in other platforms paving the way for efficient control of magnetic order.