Catalogue Search | MBRL
Are you sure you want to remove the book from the shelf?
{{itemTitle}}
86
result(s) for
"Vogel, Franziska"
Sort by:
The seasonal cycle of ice-nucleating particles linked to the abundance of biogenic aerosol in boreal forests
Ice-nucleating particles (INPs) trigger the formation of cloud ice crystals in the atmosphere. Therefore, they strongly influence cloud microphysical and optical properties and precipitation and the life cycle of clouds. Improving weather forecasting and climate projection requires an appropriate formulation of atmospheric INP concentrations. This remains challenging as the global INP distribution and variability depend on a variety of aerosol types and sources, and neither their short-term variability nor their long-term seasonal cycles are well covered by continuous measurements. Here, we provide the first year-long set of observations with a pronounced INP seasonal cycle in a boreal forest environment. Besides the observed seasonal cycle in INP concentrations with a minimum in wintertime and maxima in early and late summer, we also provide indications for a seasonal variation in the prevalent INP type. We show that the seasonal dependency of INP concentrations and prevalent INP types is most likely driven by the abundance of biogenic aerosol. As current parameterizations do not reproduce this variability, we suggest a new mechanistic description for boreal forest environments which considers the seasonal variation in INP concentrations. For this, we use the ambient air temperature measured close to the ground at 4.2 m height as a proxy for the season, which appears to affect the source strength of biogenic emissions and, thus, the INP abundance over the boreal forest. Furthermore, we provide new INP parameterizations based on the Ice Nucleation Active Surface Site (INAS) approach, which specifically describes the ice nucleation activity of boreal aerosols particles prevalent in different seasons. Our results characterize the boreal forest as an important but variable INP source and provide new perspectives to describe these new findings in atmospheric models.
Journal Article
On the drivers of ice nucleating particle diurnal variability in Eastern Mediterranean clouds
We report the drivers of spatiotemporal variability of ice nucleating particles (INPs) for mixed-phase orographic clouds (~−25 °C) in the Eastern Mediterranean. In the planetary boundary layer, pronounced INP diurnal periodicity is observed, which is mainly driven by biological (and to a lesser extent, dust) particles but not aerosols from biomass burning. The comparison of size-resolved and fluorescence-discriminated aerosol particle properties with INPs reveals the primary role of fluorescent bioaerosol. The presence of Saharan dust increases INPs during nighttime more than daytime, because of lower boundary layer height during nighttime which decreases the contribution of aerosols (including bioaerosols) from the boundary layer. INP diurnal periodicity is absent in the free troposphere, although levels are driven by the availability of bioaerosol and dust particles. Given the effective ice nucleation ability of bioaerosols and subsequent effects from ice multiplication at warm temperatures, the lack of such cycles in models points to important and overlooked drivers of cloud formation and precipitation in mountainous regions.
Journal Article
Empathy-based counterspeech can reduce racist hate speech in a social media field experiment
Despite heightened awareness of the detrimental impact of hate speech on social media platforms on affected communities and public discourse, there is little consensus on approaches to mitigate it. While content moderation—either by governments or social media companies—can curb online hostility, such policies may suppress valuable as well as illicit speech and might disperse rather than reduce hate speech. As an alternative strategy, an increasing number of international and nongovernmental organizations (I/NGOs) are employing counterspeech to confront and reduce online hate speech. Despite their growing popularity, there is scant experimental evidence on the effectiveness and design of counterspeech strategies (in the public domain). Modeling our interventions on current I/NGO practice, we randomly assign English-speaking Twitter users who have sent messages containing xenophobic (or racist) hate speech to one of three counterspeech strategies—empathy, warning of consequences, and humor—or a control group. Our intention-to-treat analysis of 1,350 Twitter users shows that empathy-based counterspeech messages can increase the retrospective deletion of xenophobic hate speech by 0.2 SD and reduce the prospective creation of xenophobic hate speech over a 4-wk follow-up period by 0.1 SD. We find, however, no consistent effects for strategies using humor or warning of consequences. Together, these results advance our understanding of the central role of empathy in reducing exclusionary behavior and inform the design of future counterspeech interventions.
Journal Article
Saharan dust transport event characterization in the Mediterranean atmosphere using 21 years of in-situ observations
The Mediterranean Basin is regularly affected by atmospheric dust transport from the Saharan desert. These recurring events have strong implications for the Earth’s energy budget, cloud formation processes, human health, and solar energy production. Monte Cimone, with 2165 m a.s.l., is an ideal platform to investigate dust outbreaks in Mediterranean Europe. In this study, we present 21 years (2003–2023) of dust transport event identification, derived from continuous measurements of the aerosol optical size distribution coupled with backward trajectories. Throughout all the years investigated, the fraction of dust transport days remained constant at values between 15 % and 20 % without any detectable trend. This absent trend was also observed in the particulate matter concentration. The annual cycle of dust transport days was characterized by two peaks from May to August and in October and November with values up to 20 %. A similar annual cycle was reflected in the particulate matter concentration with the highest concentrations in summer and the lowest in winter. Grouping consecutive dust transport days into dust transport events revealed that in the winter months a typical event had a duration of one or two days, whereas in the summer months dust transport events lasted longer (three or more days). The 21 years of measurements presented in this study will set a baseline to assess future dust transport scenarios. Furthermore, they can be used to validate dust forecast models to increase the accuracy of predicting atmospheric dust transport towards the Mediterranean Basin.
Journal Article
Synergistic HNO3–H2SO4–NH3 upper tropospheric particle formation
New particle formation in the upper free troposphere is a major global source of cloud condensation nuclei (CCN)
1
–
4
. However, the precursor vapours that drive the process are not well understood. With experiments performed under upper tropospheric conditions in the CERN CLOUD chamber, we show that nitric acid, sulfuric acid and ammonia form particles synergistically, at rates that are orders of magnitude faster than those from any two of the three components. The importance of this mechanism depends on the availability of ammonia, which was previously thought to be efficiently scavenged by cloud droplets during convection. However, surprisingly high concentrations of ammonia and ammonium nitrate have recently been observed in the upper troposphere over the Asian monsoon region
5
,
6
. Once particles have formed, co-condensation of ammonia and abundant nitric acid alone is sufficient to drive rapid growth to CCN sizes with only trace sulfate. Moreover, our measurements show that these CCN are also highly efficient ice nucleating particles—comparable to desert dust. Our model simulations confirm that ammonia is efficiently convected aloft during the Asian monsoon, driving rapid, multi-acid HNO
3
–H
2
SO
4
–NH
3
nucleation in the upper troposphere and producing ice nucleating particles that spread across the mid-latitude Northern Hemisphere.
By performing experiments under upper tropospheric conditions, nitric acid, sulfuric acid and ammonia can form particles synergistically, at rates orders of magnitude faster than any two of the three components.
Journal Article
Biological and dust aerosols as sources of ice-nucleating particles in the eastern Mediterranean: source apportionment, atmospheric processing and parameterization
Aerosol–cloud interactions in mixed-phase clouds (MPCs) are one of the most uncertain drivers of the hydrological cycle and climate change. A synergy of in situ, remote-sensing and modelling experiments were used to determine the source of ice-nucleating particles (INPs) for MPCs at Mount Helmos in the eastern Mediterranean. The influences of boundary layer turbulence, vertical aerosol distributions and meteorological conditions were also examined. When the observation site is in the free troposphere (FT), approximately 1 in ×106 aerosol particles serve as INPs around −25 °C. The INP abundance spans 3 orders of magnitude and increases in the following order: marine aerosols; continental aerosols; and, finally, dust plumes. Biological particles are important INPs observed in continental and marine aerosols, whereas they play a secondary, although important, role during Saharan dust events. Air masses in the planetary boundary layer (PBL) show both enriched INP concentrations and a higher proportion of INPs to total aerosol particles, compared with cases in the FT. The presence of precipitation/clouds enriches INPs in the FT but decreases INPs in the PBL. Additionally, new INP parameterizations are developed that incorporate the ratio of fluorescent-to-nonfluorescent or coarse-to-fine particles and predict >90 % of the observed INPs within an uncertainty range of a factor of 10; these new parameterizations exhibit better performance than current widely used parameterizations and allow ice formation in models to respond to variations in dust and biological particles. The improved parameterizations can help MPC formation simulations in regions with various INP sources or different regions with prevailing INP sources.
Journal Article
The Portable Ice Nucleation Experiment (PINE): a new online instrument for laboratory studies and automated long-term field observations of ice-nucleating particles
Atmospheric ice-nucleating particles (INPs) play an important role in determining the phase of clouds, which affects their albedo and lifetime. A lack of data on the spatial and temporal variation of INPs around the globe limits our predictive capacity and understanding of clouds containing ice. Automated instrumentation that can robustly measure INP concentrations across the full range of tropospheric temperatures is needed in order to address this knowledge gap. In this study, we demonstrate the functionality and capacity of the new Portable Ice Nucleation Experiment (PINE) to study ice nucleation processes and to measure INP concentrations under conditions pertinent for mixed-phase clouds, with temperatures from about −10 to about −40 ∘C. PINE is a cloud expansion chamber which avoids frost formation on the cold walls and thereby omits frost fragmentation and related background ice signals during the operation. The development, working principle and treatment of data for the PINE instrument is discussed in detail. We present laboratory-based tests where PINE measurements were compared with those from the established AIDA (Aerosol Interaction and Dynamics in the Atmosphere) cloud chamber. Within experimental uncertainties, PINE agreed with AIDA for homogeneous freezing of pure water droplets and the immersion freezing activity of mineral aerosols. Results from a first field campaign conducted at the Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) observatory in Oklahoma, USA, from 1 October to 14 November 2019 with the latest PINE design (a commercially available PINE chamber) are also shown, demonstrating PINE's ability to make automated field measurements of INP concentrations at a time resolution of about 8 min with continuous temperature scans for INP measurements between −10 and −30 ∘C. During this field campaign, PINE was continuously operated for 45 d in a fully automated and semi-autonomous way, demonstrating the capability of this new instrument to also be used for longer-term field measurements and INP monitoring activities in observatories.
Journal Article
Ice-nucleating particles active below −24 °C in a Finnish boreal forest and their relationship to bioaerosols
Cloud properties are strongly influenced by ice formation; hence, we need to understand the sources of ice-nucleating particles (INPs) around the globe. Boreal forests are known as sources of bioaerosol, and recent work indicates that these dominate the INP spectra above −24 °C. To quantify the INP population at temperatures below −24 °C, we deployed a portable cloud expansion chamber (PINE) in a Finnish boreal forest from 13 March 2018 to 11 May 2018. Using the 6 min time resolution PINE data, we present several lines of evidence that INPs below −24 °C in this location are also from biological sources: (i) an INP parameterization developed for a pine forest site in Colorado, where many INPs were shown to be biological, produced a good fit to our measurements; a moderate correlation of INPs with aerosol concentration larger than 0.5 µm and the fluorescent bioaerosol concentration; (ii) a negative correlation with relative humidity that may relate to enhanced release of bioaerosol at low humidity from local sources such as the prolific lichen population in boreal forests; and (iii) the absence of correlation with ultra-fine particles (3.5 to 50 nm), indicating that new particle formation events are not sources of INPs. This study should motivate further work to establish whether the commonality in bioaerosol ice-nucleating properties between spring in Finland and summer in Colorado is more generally applicable to different coniferous forest locations and times and also to determine to what extent these bioaerosols are transported to locations where they may affect clouds.
Journal Article
From fine to giant: multi-instrument assessment of the dust particle size distribution at an emission source during the J-WADI field campaign
Mineral dust particles emitted from dry, uncovered soil can be transported over vast distances, thereby influencing climate and environment. Its impacts are highly size-dependent, yet large particles with diameters dp>10 µm remain understudied due to their low number concentrations and instrumental limitations. Accurately characterizing the particle size distribution (PSD) at emission is crucial for understanding dust transport and climate interactions. Here we characterize the dust PSD at an emission source during the Jordan Wind Erosion and Dust Investigation (J-WADI) campaign, conducted in Wadi Rum, Jordan, in September 2022, focusing on super-coarse (1062.5 µm) particles. This study is the first to continuously cover the full range of diameters from dp=0.4 to 200 µm at an emission source by using a suite of aerosol spectrometers with overlapping size ranges. This overlap enabled a systematic intercomparison and validation across instruments, improving PSD reliability. Results show significant PSD variability over the course of the campaign. During periods with friction velocities (u*) above 0.22 m s−1 (or ∼ 3.3 m s−1 threshold 4 m wind speed), the approximate threshold for local dust emission by saltation, both dust concentrations and the contributions of super-coarse and giant particles typically increased with increasing u*, especially under neutral to unstable atmospheric stability conditions. These large particles accounted for about 90 % of the total mass concentration during the campaign. A prominent mass concentration peak was observed near dp=60 µm in geometric diameter. While particle concentrations for dp<10 µm showed good agreement among most instruments, discrepancies appeared for larger dp due to reduced instrument sensitivity at the size range boundaries and sampling inefficiencies. Despite these challenges, physical samples collected using a flat-plate sampler largely confirmed the PSDs derived from the aerosol spectrometers. These findings help to advance our understanding of the dust PSD and the abundance of super-coarse and giant particle at emission sources.
Journal Article