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Advanced quantum technologies require scalable and controllable quantum resources 1 , 2 . Gaussian states of multimode light, such as squeezed states and cluster states, are scalable quantum systems 3 – 5 , which can be generated on demand. However, non-Gaussian features are indispensable in many quantum protocols, especially to reach a quantum computational advantage 6 . Embodying non-Gaussianity in a multimode quantum state remains a challenge as non-Gaussian operations generally cannot maintain coherence among multiple modes. Here, we generate non-Gaussian quantum states of a multimode light field by removing a single photon in a mode-selective manner from a Gaussian state 7 . To highlight the potential for continuous-variable quantum technologies, we first demonstrated the capability to generate negativity of the Wigner function in a controlled mode. Subsequently, we explored the interplay between non-Gaussianity and quantum entanglement and verify a theoretical prediction 8 about the propagation of non-Gaussianity along the nodes of photon-subtracted cluster states. Our results demonstrate large-scale non-Gaussianity with great flexibility along with an ensured compatibility with quantum information protocols. This range of features makes our approach ideal to explore the physics of non-Gaussian entanglement 9 , 10 and to develop quantum protocols, which range across quantum computing 11 , 12 , entanglement distillation 13 and quantum simulations 14 . Continuous-variables quantum information processing requires non-Gaussian states and operations. The generation of non-Gaussian quantum states of a multimode field is now reported through a mode-selective photon-subtraction scheme

Quantum optical metrology aims to identify ultimate sensitivity bounds for the estimation of parameters encoded into quantum states of the electromagnetic field. In many practical applications, including imaging, microscopy, and remote sensing, the parameter of interest is not only encoded in the quantum state of the field, but also in its spatio-temporal distribution, i.e. in its mode structure. In this mode-encoded parameter estimation setting, we derive an analytical expression for the quantum Fisher information valid for arbitrary multimode Gaussian fields. To illustrate the power of our approach, we apply our results to the estimation of the transverse displacement of a beam and to the temporal separation between two pulses. For these examples, we show how the estimation sensitivity can be enhanced by adding squeezing into specific modes.

Super resolution is one of the key issues at the crossroads of contemporary quantum optics and metrology. Recently, it was shown that for an idealized case of two balanced sources, spatial mode demultiplexing (SPADE) achieves resolution better than direct imaging even in the presence of measurement crosstalk (Gessner et al 2020 Phys. Rev. Lett. 125 100501). In this work, we consider arbitrarily unbalanced sources and provide a systematic analysis of the impact of crosstalk on the resolution obtained from SPADE. As we dissect, in this generalized scenario, SPADE’s effectiveness depends non-trivially on the strength of crosstalk, relative brightness and the separation between the sources. In particular, for any source imbalance, SPADE performs worse than ideal direct imaging in the asymptotic limit of vanishing source separations. Nonetheless, for realistic values of crosstalk strength, SPADE is still the superior method for several orders of magnitude of source separations.

Entanglement and non-Gaussianity are physical resources that are essential for a large number of quantum-optics protocols. Non-Gaussian entanglement is indispensable for quantum-computing advantage and outperforms its Gaussian counterparts in a number of quantum-information protocols. The characterization of non-Gaussian entanglement is a critical matter as it is in general highly demanding in terms of resources. We propose a simple protocol based on the Fisher information for witnessing entanglement in an important class of non-Gaussian entangled states: photon-subtracted states. We demonstrate that our protocol is relevant for the detection of non-Gaussian entanglement generated by multiple photon-subtraction and that it is experimentally feasible through homodyne detection.

One of the most pertinent problems in the debate on non-trivial quantum effects in biology concerns natural photosynthesis. Since sunlight is composed of thermal photons, it was argued to be unable to induce quantum coherence in matter, and that quantum mechanics is therefore irrelevant for the dynamical processes following photoabsorption. Our present analysis of a toy 'molecular aggregate'-composed of two dipole-dipole interacting two-level atoms treated as an open quantum system-however shows that incoherent excitations indeed can trigger persistent, coherent dynamics in both the site and the exciton bases: we demonstrate that collective decay processes induced by the dipole-dipole interactions create coherent intermolecular transport-regardless of the coherence properties of the incoming radiation. Our analysis shows that the steady state coherence is mediated by the population imbalance between the molecules and, therefore, increases with the energy difference between the two-level atoms. Our results establish the importance of collective decay processes in the study of ultrafast photophysics, and especially their potential role to generate stationary coherence in incoherently driven quantum transport.

Non-Gaussian states of an optical field are important as a proposed resource in quantum information applications. While conditional preparation is a highly successful approach to preparing such states, their quality is limited by detector non-idealities such as dead time, narrow dynamic range, limited quantum efficiency and dark noise. Mesoscopic photon counters, with peak performance at higher photon number, offer many practical advantages over single-photon level conditioning detectors. Here we propose a novel approach involving displacement of the ancilla field into the regime where mesoscopic detectors can be used. We explore this strategy theoretically and present simulations accounting for experimental non-idealities such as loss and amplification noise, showing that precise photon-number resolution is not necessary to herald highly nonclassical states. We conclude that states with strong Wigner negativity can be prepared at high rates by this technique under experimentally attainable conditions.

Wigner negativity, as a well-known indicator of nonclassicality, plays an essential role in quantum computing and simulation using continuous-variable systems. The conditional preparation of Wigner-negative states through appropriate non-Gaussian operations on an auxiliary mode is common procedure in quantum optics experiments. Motivated by the demand of real-world quantum network, here we investigate the remote creation and distribution of Wigner negativity in the multipartite scenario from a quantitative perspective. By establishing a monogamy relation akin to the generalized Coffman-Kundu-Wootters inequality, we show that the amount of Wigner negativity cannot be freely distributed among different modes. Moreover, for photon subtraction—one of the main experimentally realized non-Gaussian operations—we provide an intuitive method to quantify remotely generated Wigner negativity. Our results pave the way for exploiting Wigner negativity as a valuable resource for numerous quantum information protocols based on non-Gaussian scenario.

We establish a mathematically rigorous, general and quantitative framework to describe currents of non- (or weakly) interacting, indistinguishable particles driven far from equilibrium. We derive tight upper and lower bounds for the achievable fermionic and bosonic steady state current, respectively, which can serve as benchmarks for special cases of interacting many-particle dynamics. For fermionic currents, we identify a symmetry-induced enhancement mechanism in parameter regimes where the coupling between system and reservoirs is weak. This mechanism is broadly applicable provided the inter-particle interaction strength is small as compared to typical exchange interactions.

Quantum optical metrology aims to identify ultimate sensitivity bounds for the estimation of parameters econded into quantum states of the electromagnetic field. In many practical applications, including imaging, microscopy, and remote sensing, the parameter of interest is not only encoded in the quantum state of the field, but also in its spatio-temporal distribution, i.e. in its mode structure. In this mode-encoded parameter estimation setting, we derive an analytical expression for the quantum Fisher information valid for arbitrary multimode Gaussian fields. To illustrate the power of our approach, we apply our results to the estimation of the transverse separation between two point sources observed with a diffraction-limited imaging system. In this context, we determine the ultimate resolution provided by mutual coherence and squeezing of the sources.

Multi-particle interference is an essential ingredient for fundamental quantum mechanics phenomena and for quantum information processing to provide a computational advantage, as recently emphasized by boson sampling experiments. Hence, developing a reliable and efficient technique to witness its presence is pivotal in achieving the practical implementation of quantum technologies. Here, we experimentally identify genuine many-body quantum interference via a recent efficient protocol, which exploits statistical signatures at the output of a multimode quantum device. We successfully apply the test to validate three-photon experiments in an integrated photonic circuit, providing an extensive analysis on the resources required to perform it. Moreover, drawing upon established techniques of machine learning, we show how such tools help to identify the—a priori unknown—optimal features to witness these signatures. Our results provide evidence on the efficacy and feasibility of the method, paving the way for its adoption in large-scale implementations.