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49
result(s) for
"Zeitler, Uli"
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Full superconducting dome of strong Ising protection in gated monolayer WS2
2018
SignificanceCompared with 3D superconductors, atomically thin superconductors are expected to be easier to engineer for electronic applications. Here, we use field effect gating to induce superconductivity in a monolayer semiconducting transition metal dichalcogenide, WS2, grown by chemical vapor deposition. The remarkable doping range allows access to a cascade of electronic phases from a band insulator, a superconductor, to a reentrant insulator at high doping. The large spin-orbit coupling of ∼30 meV makes the Ising paring in WS2 arguably the most strongly protected superconducting state against external magnetic field. The wide tunability revealed by spanning over a complete superconducting dome paves the way for the integration of monolayer superconductors to functional electronic devices exploiting the field effect control of quantum phases.
Many recent studies show that superconductivity not only exists in atomically thin monolayers but can exhibit enhanced properties such as a higher transition temperature and a stronger critical field. Nevertheless, besides being unstable in air, the weak tunability in these intrinsically metallic monolayers has limited the exploration of monolayer superconductivity, hindering their potential in electronic applications (e.g., superconductor–semiconductor hybrid devices). Here we show that using field effect gating, we can induce superconductivity in monolayer WS2 grown by chemical vapor deposition, a typical ambient-stable semiconducting transition metal dichalcogenide (TMD), and we are able to access a complete set of competing electronic phases over an unprecedented doping range from band insulator, superconductor, to a reentrant insulator at high doping. Throughout the superconducting dome, the Cooper pair spin is pinned by a strong internal spin–orbit interaction, making this material arguably the most resilient superconductor in the external magnetic field. The reentrant insulating state at positive high gating voltages is attributed to localization induced by the characteristically weak screening of the monolayer, providing insight into many dome-like superconducting phases observed in field-induced quasi-2D superconductors.
Journal Article
Extremely large magnetoresistance and ultrahigh mobility in the topological Weyl semimetal candidate NbP
2015
Weyl semimetals are predicted to exhibit a host of unusual transport properties. NbP, a system predicted to share characteristics of both normal and Weyl semimetals, is now shown to have a very large, non-saturating magnetoresistance.
Recent experiments have revealed spectacular transport properties in semimetals, such as the large, non-saturating magnetoresistance exhibited by WTe
2
(ref.
1
). Topological semimetals with massless relativistic electrons have also been predicted
2
as three-dimensional analogues of graphene
3
. These systems are known as Weyl semimetals, and are predicted to have a range of exotic transport properties and surface states
4
,
5
,
6
,
7
, distinct from those of topological insulators
8
,
9
. Here we examine the magneto-transport properties of NbP, a material the band structure of which has been predicted to combine the hallmarks of a Weyl semimetal
10
,
11
with those of a normal semimetal. We observe an extremely large magnetoresistance of 850,000% at 1.85 K (250% at room temperature) in a magnetic field of up to 9 T, without any signs of saturation, and an ultrahigh carrier mobility of 5 × 10
6
cm
2
V
−1
s
−1
that accompanied by strong Shubnikov–de Haas (SdH) oscillations. NbP therefore presents a unique example of a material combining topological and conventional electronic phases, with intriguing physical properties resulting from their interplay.
Journal Article
Extremely high magnetoresistance and conductivity in the type-II Weyl semimetals WP2 and MoP2
2017
The peculiar band structure of semimetals exhibiting Dirac and Weyl crossings can lead to spectacular electronic properties such as large mobilities accompanied by extremely high magnetoresistance. In particular, two closely neighboring Weyl points of the same chirality are protected from annihilation by structural distortions or defects, thereby significantly reducing the scattering probability between them. Here we present the electronic properties of the transition metal diphosphides, WP
2
and MoP
2
, which are type-II Weyl semimetals with robust Weyl points by transport, angle resolved photoemission spectroscopy and first principles calculations. Our single crystals of WP
2
display an extremely low residual low-temperature resistivity of 3 nΩ cm accompanied by an enormous and highly anisotropic magnetoresistance above 200 million % at 63 T and 2.5 K. We observe a large suppression of charge carrier backscattering in WP
2
from transport measurements. These properties are likely a consequence of the novel Weyl fermions expressed in this compound.
Semimetals with the band structure exhibiting Dirac and Weyl crossings can show special electronic and magnetic properties. Here the authors explore the electronic properties of the type-II Weyl semimetals, MoP
2
and WP
2
with robust Weyl points which display very high magnetoresistance and conductivity.
Journal Article
High electron mobility, quantum Hall effect and anomalous optical response in atomically thin InSe
by
Gorbachev, Roman V.
,
Grigorieva, Irina V.
,
Zólyomi, Viktor
in
639/301/357/1018
,
639/925/918/1052
,
639/925/927/1007
2017
Encapsulated few-layer InSe exhibits a remarkably high electronic quality, which is promising for the development of ultrathin-body high-mobility nanoelectronics.
A decade of intense research on two-dimensional (2D) atomic crystals has revealed that their properties can differ greatly from those of the parent compound
1
,
2
. These differences are governed by changes in the band structure due to quantum confinement and are most profound if the underlying lattice symmetry changes
3
,
4
. Here we report a high-quality 2D electron gas in few-layer InSe encapsulated in hexagonal boron nitride under an inert atmosphere. Carrier mobilities are found to exceed 10
3
cm
2
V
−1
s
−1
and 10
4
cm
2
V
−1
s
−1
at room and liquid-helium temperatures, respectively, allowing the observation of the fully developed quantum Hall effect. The conduction electrons occupy a single 2D subband and have a small effective mass. Photoluminescence spectroscopy reveals that the bandgap increases by more than 0.5 eV with decreasing the thickness from bulk to bilayer InSe. The band-edge optical response vanishes in monolayer InSe, which is attributed to the monolayer's mirror-plane symmetry. Encapsulated 2D InSe expands the family of graphene-like semiconductors and, in terms of quality, is competitive with atomically thin dichalcogenides
5
,
6
,
7
and black phosphorus
8
,
9
,
10
,
11
.
Journal Article
Extremely high conductivity observed in the triple point topological metal MoP
by
Guin, Satya N.
,
Watzman, Sarah J.
,
Young, Olga
in
639/766/119/2792/4128
,
639/766/119/995
,
Coherent scattering
2019
Weyl and Dirac fermions have created much attention in condensed matter physics and materials science. Recently, several additional distinct types of fermions have been predicted. Here, we report ultra-high electrical conductivity in MoP at low temperature, which has recently been established as a triple point fermion material. We show that the electrical resistivity is 6 nΩ cm at 2 K with a large mean free path of 11 microns. de Haas-van Alphen oscillations reveal spin splitting of the Fermi surfaces. In contrast to noble metals with similar conductivity and number of carriers, the magnetoresistance in MoP does not saturate up to 9 T at 2 K. Interestingly, the momentum relaxing time of the electrons is found to be more than 15 times larger than the quantum coherence time. This difference between the scattering scales shows that momentum conserving scattering dominates in MoP at low temperatures.
Although novel topological quasiparticles have recently been evidenced, their electrical transport properties remain elusive. Here, the authors report ultra-low resistivity down to 6 nΩcm at 2 K in MoP with a large mean free path, which hints on the exotic properties of triple point fermions.
Journal Article
Anomalous Hall effect in Weyl semimetal half-Heusler compounds RPtBi (R = Gd and Nd)
by
Wu, Shu-Chun
,
Felser, C.
,
Grinenko, V.
in
Antiferromagnetism
,
Condensed matter physics
,
Conductivity
2018
Topological materials ranging from topological insulators to Weyl and Dirac semimetals form one of the most exciting current fields in condensed-matter research. Many half-Heusler compounds, RPtBi (R = rare earth), have been theoretically predicted to be topological semimetals. Among various topological attributes envisaged in RPtBi, topological surface states, chiral anomaly, and planar Hall effect have been observed experimentally. Here, we report an unusual intrinsic anomalous Hall effect (AHE) in the antiferromagnetic Heusler Weyl semimetal compounds GdPtBi and NdPtBi that is observed over a wide temperature range. In particular, GdPtBi exhibits an anomalous Hall conductivity of up to 60 Ω−1·cm−1 and an anomalous Hall angle as large as 23%. Muon spin-resonance (μSR) studies of GdPtBi indicate a sharp antiferromagnetic transition (T
N) at 9 K without any noticeable magnetic correlations above T
N. Our studies indicate that Weyl points in these half-Heuslers are induced by a magnetic field via exchange splitting of the electronic bands at or near the Fermi energy, which is the source of the chiral anomaly and the AHE.
Journal Article
Interaction phenomena in graphene seen through quantum capacitance
by
Wiedmann, S.
,
Belle, Branson
,
Novoselov, Kostya S.
in
Capacitance
,
Capacitors
,
Compressibility
2013
Capacitance measurements provide a powerful means of probing the density of states. The technique has proved particularly successful in studying 2D electron systems, revealing a number of interesting many-body effects. Here, we use large-area high-quality graphene capacitors to study behavior of the density of states in this material in zero and high magnetic fields. Clear renormalization of the linear spectrum due to electron–electron interactions is observed in zero field. Quantizing fields lead to splitting of the spin- and valley-degenerate Landau levels into quartets separated by interaction-enhanced energy gaps. These many-body states exhibit negative compressibility but the compressibility returns to positive in ultrahigh B. The reentrant behavior is attributed to a competition between field-enhanced interactions and nascent fractional states.
Journal Article
Quantum Hall effect in a CVD-grown oxide
2024
Two-dimensional (2D) electron systems are promising for investigating correlated quantum phenomena. In particular, 2D oxides provide a platform that can host various quantum phases such as quantized Hall effect, superconductivity, or magnetism. The realization of such quantum phases in 2D oxides heavily relies on dedicated heterostructure growths. Here we show the integer quantum Hall effect achieved in chemical vapor deposition grown Bi
2
O
2
Se - a representative member of a more accessible oxide family. A single or few subband 2D electron system can be prepared in thin films of Bi
2
O
2
Se, where the film thickness acts as the key subband design parameter and the occupation is determined by the electric field effect. This oxide platform exhibits characteristic advantages in structural flexibility due to its layered nature, making it suitable for scalable growth. The unique small mass distinguishes Bi
2
O
2
Se from other high-mobility oxides, providing a new platform for exploring quantum Hall physics in 2D oxides.
The authors demonstrate quantum Hall effect in semiconducting layered oxide Bi
2
O
2
Se. Its unique low mass among the oxides of 0.14
m
e
and pronounced layered structure makes Bi
2
O
2
Se highly susceptible to the quantum confinement effects.
Journal Article
Phonon-mediated room-temperature quantum Hall transport in graphene
by
Taniguchi, Takashi
,
Salvador-Sánchez, Juan
,
Müller, Claudius S. A.
in
639/766/119/2794
,
639/925/918/1052
,
Boron
2023
The quantum Hall (QH) effect in two-dimensional electron systems (2DESs) is conventionally observed at liquid-helium temperatures, where lattice vibrations are strongly suppressed and bulk carrier scattering is dominated by disorder. However, due to large Landau level (LL) separation (~2000 K at
B
= 30 T), graphene can support the QH effect up to room temperature (RT), concomitant with a non-negligible population of acoustic phonons with a wave-vector commensurate to the inverse electronic magnetic length. Here, we demonstrate that graphene encapsulated in hexagonal boron nitride (hBN) realizes a novel transport regime, where dissipation in the QH phase is governed predominantly by electron-phonon scattering. Investigating thermally-activated transport at filling factor 2 up to RT in an ensemble of back-gated devices, we show that the high
B
-field behaviour correlates with their zero
B
-field transport mobility. By this means, we extend the well-accepted notion of phonon-limited resistivity in ultra-clean graphene to a hitherto unexplored high-field realm.
Monolayer graphene can support the quantum Hall effect up to room temperature. Here, the authors provide evidence that graphene encapsulated in hexagonal boron nitride realizes a novel transport regime where dissipation in the quantum Hall phase is mediated predominantly by electron-phonon scattering rather than disorder scattering.
Journal Article