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The A-LIFE (Absorbing aerosol layers in a changing climate: aging, lifetime, and dynamics) field experiment, conducted in Cyprus in April 2017, employed a wide range of ground-based and airborne instruments, including passive/active remote sensing and in-situ techniques. This study presents the columnar records obtained by sun photometry. Two sun/sky/lunar photometers, belonging to AERONET network, were strategically placed at two sites: Pafos and Limassol, 40 km apart. Aerosol optical and microphysical properties derived from direct sun and sky radiance measurements are analysed to determine an inventory of aerosol event days during the experiment, with mineral dust being present in nearly 75 % of days. Ångström exponent values obtained from 1020 and 1640 nm channels (0.5 for Saharan dust and 0.34 for Arabian dust) can be served as a classification criterion. Dust sources are key point for a well understanding of the size distribution and absorption power. According to columnar records, Saharan dust exhibited less absorbing particles. The columnar volume efficiency factor (linear fit between aerosol optical depth and total volume concentration) was proved as a reliable proxy for the identification of dust origin since Arabian and Saharan dusts exhibit different slopes: 1.28 and 1.68 µm2 µm−3, respectively. Analysing all the inversion products mixtures of mineral dust were mainly dominated by Arabian dust, while mixtures of fine and coarse aerosols showed no clear prevalence of dust origin. No significant presence of black carbon-rich aerosols was detected in the atmospheric column, as absorption Ångström exponent values ranged from 1.6 to 3 across aerosol types identified.

Australian smoke from the extraordinary biomass burning in December 2019 was observed over Marambio, Antarctica from the 7th to the 10th January, 2020. The smoke plume was transported thousands of kilometers over the Pacific Ocean, and reached the Antarctic Peninsula at a hight of 13 km, as determined by satellite lidar observations. The proposed origin and trajectory of the aerosol are supported by back-trajectory model analyses. Ground-based Sun–Sky–Moon photometer belonging to the Aerosol Robotic Network (AERONET) measured aerosol optical depth (500 nm wavelength) above 0.3, which is unprecedented for the site. Inversion of sky radiances provide the optical and microphysical properties of the smoke over Marambio. The AERONET data near the fire origin in Tumbarumba, Australia, was used to investigate the changes in the measured aerosol properties after transport and ageing. The analysis shows an increase in the fine mode particle radius and a reduction in absorption (increase in the single scattering albedo). The available long-term AOD data series at Marambio suggests that smoke particles could have remained over Antarctica for several weeks after the analyzed event.

Sustained and coordinated efforts of lidar teams in Latin America at the beginning of the twenty-first century have built the Latin American Lidar Network (LALINET), the only observational network in Latin America created by the agreement and commitment of Latin American scientists. They worked with limited funding but an abundance of enthusiasm and commitment toward their joint goal. Before LALINET, there were a few pioneering lidar stations operating in Latin America, described briefly here. Biannual Latin American lidar workshops, held from 2001 to the present, supported both the development of the regional lidar community and LALINET. At those meetings, lidar researchers from Latin America met to conduct regular scientific and technical exchanges among themselves and with experts from the rest of the world. Regional and international scientific cooperation has played an important role in the development of both the individual teams and the network. The current LALINET status and activities are described, emphasizing the processes of standardization of the measurements, methodologies, calibration protocols, and retrieval algorithms. Failures and successes achieved in the buildup of LALINET are presented. In addition, the first LALINET joint measurement campaign and a set of aerosol extinction profile measurements obtained from the aerosol plume produced by the Calbuco volcano eruption on 22 April 2015 are described and discussed.

Arid regions are a major source of mineral dust aerosol. Transport from these sources can have a great impact on aerosol climatology in distant regions. In order to assess the impact of dust on climate we must understand how dust properties change after long distance transport from sources. This study addresses the changes in columnar aerosol properties when mineral dust outbreaks from western Africa arrive over the eastern Caribbean after transport across the Atlantic Ocean, a transit of 5–7 days. We use data from the NASA Aerosol Robotic Network (AERONET) located at five Caribbean and two western Africa sites to characterize changes in columnar aerosol properties: aerosol optical depth (AOD), size distribution, single scattering albedo, and refractive indexes. We first characterized the local aerosol climatology at each site and then using air mass back trajectories we identified those days when trajectories over Caribbean sites back-tracked to western Africa. Over the period 1996–2014 we identify 3174 days, an average of 167 days per year, when the air mass over the Caribbean sites could be linked to at least one of the two western Africa sites. For 1162 of these days, AOD data are available for the Caribbean sites as well as for the corresponding western Africa sites about 5–7 days earlier, when the air mass passed over these sites. We identified dust outbreaks as those air masses yielding AOD  ≥  0.2 and an Ångström exponent below 0.6. On this basis of the total 1162 days, 484 meet the criteria for mineral dust outbreaks. We observe that the AOD at 440 nm decreases by about 0.16 or 30 % during transport. The volume particle size distribution shows a similar decrease in the volume concentration, mainly in the coarse mode. The single scattering albedo, refractive indexes, and asymmetry factor remain unchanged. The difference in the effective radius over western Africa sites with respect to Caribbean sites ranges between 0 and −0.3 µm. Finally we conclude that in about half of the cases only non-spherical dust particles are present in the atmosphere over the western Africa and Caribbean sites, while in the other cases dust particles were mixed with other types of aerosol particles.

The transition to renewable energies is an unavoidable step to guarantee a peaceful and sustainable future for humankind. Although solar radiation is one of the main sources of renewable energy, there are broad regions of the planet where it has not been characterized appropriately to provide the necessary information for regional and local planning and design of the different solar powered systems. The Caribbean, and Cuba in particular, lacked until very recently at least one long-term series of surface solar radiation measurements. Here we present the first long-term records of solar radiation for this region. Solar radiation measurements manually conducted and recorded on paper were rescued, reprocessed and quality controlled to develop the solar radiation climatology at the Actinometrical Station of Camagüey, in Cuba (21.422°N; 77.850°W; 122 m a.s.l.) for the period 1981–2016. The diurnal cycle based on the average hourly values of the global, direct and diffuse horizontal variables for the entire period have been determined and analyzed showing the dependence on solar zenith angle (SZA) and clouds. The annual cycle of global solar component given by the mean monthly daily values presents two maxima, one in April and another one in July with values of 5.06 and 4.91 kWh m−2, respectively (18.23 and 17.67 MJ m−2 per day for insolation), and the minimum in December (3.15 kWh m−2 or 11.33 MJ m−2). The maxima are governed by the direct solar components and are modulated by cloudiness. Both, diurnal and annual cycles of the diffuse solar component show a smoothed bell shaped behavior. In general solar radiation at this station presents a strong influence of clouds, with little seasonal variation but with higher values during the rainy season. Daily global radiation annual averages showed its maximum value in the year 1983, with 17.45 MJ m−2 explained by very low cloudiness this year, and the minimum value was reported in 2009 with a value of 12.43 MJ m−2 that could not explained by the cloud coverage or the aerosols optical depths registered that year. The effects of the 1982 El Chichón and 1991 Mount Pinatubo volcanic eruptions on the solar radiation variables at Camagüey are also shown and discussed. The results achieved in this study shown the characteristics of solar radiation in this area and their potential for solar power applications.

This work introduces CAECENET, a new system capable of automatically retrieving columnar and vertically-resolved aerosol properties running the GRASP (Generalized Retrieval of Atmosphere and Surface Properties) algorithm using sun-sky photometer (aerosol optical depth, AOD; and sky radiance measurements) and ceilometer (range corrected signal; RCS) data as input. This method, so called GRASP pac , is implemented in CAECENET, which assimilates sun-sky photometers data from CÆLIS database and ceilometer data from ICENET database (Iberian Ceilometer Network). CAECENET allows for continuous and near-real-time monitoring of both vertical and columnar aerosol properties. The main characteristics and workflow of CAECENET are explained in detail. This work also explores the potential of CAECENET to monitor and analyze the evolution of transported aerosol events on a regional scale by means of the distribution of CAECENET stations across the Iberian Peninsula. As an example, this paper analyzes, using the CAECENET products, the case of a Saharan dust outbreak that occurred between the 3rd and 5th of October 2022. This was an intense event, with AOD at 440 nm values around 0.5 in Madrid and Valladolid, and reaching 1.55 in Granada. Transport from the Canadian wildfires at the end of June 2023 is also studied. Despite the long-range transport of the smoke particles in this event, measured volume concentrations reached and surpassed 80 μm 3 /cm 3 in some stations. The results obtained point to the utility of this CAECENET tool for analyzing changes in the height and speed of the event propagation, in the aerosol concentration, and how this affects the optical properties.

This paper explores the potential of all-sky cameras to retrieve aerosol properties with the GRASP code (Generalized Retrieval of Atmosphere and Surface Properties). To this end, normalized sky radiances (NSRs) extracted from an all-sky camera at three effective wavelengths (467, 536 and 605 nm) are used in this study. NSR observations are a set of relative (uncalibrated) sky radiances in arbitrary units. NSR observations have been simulated for different aerosol loads and types with the forward radiative transfer module of GRASP, indicating that NSR observations contain information about the aerosol type, as well as about the aerosol optical depth (AOD), at least for low and moderate aerosol loads. An additional sensitivity study with synthetic data has been carried out to quantify the theoretical accuracy and precision of the aerosol properties (AOD, size distribution parameters, etc.) retrieved by GRASP using NSR observations as input. As a result, the theoretical accuracy of AOD is within ±0.02 for AOD values lower than or equal to 0.4, while the theoretical precision goes from 0.01 to 0.05 when AOD at 467 nm varies from 0.1 to 0.5. NSR measurements recorded at Valladolid (Spain) with an all-sky camera for more than 2 years have been inverted with GRASP. The retrieved aerosol properties are compared with independent values provided by co-located AERONET (AErosol RObotic NETwork) measurements. AODs from both data sets correlate with determination coefficient (r2) values of about 0.87. Finally, the novel multi-pixel approach of GRASP is applied to daily camera radiances together by constraining the temporal variation in certain aerosol properties. This temporal linkage (multi-pixel approach) provides promising results, reducing the highly temporal variation in some aerosol properties retrieved with the standard (one by one or single-pixel) approach. This work implies an advance in the use of all-sky cameras for the retrieval of aerosol properties.

A reliable identification of desert dust (DD) episodes over north-central Spain is carried out based on the AErosol RObotic NETwork (AERONET) columnar aerosol sun photometer (aerosol optical depth, AOD, and Ångström exponent, α) and European Monitoring and Evaluation Programme (EMEP) surface particulate-mass concentration (PMx, x = 10, 2.5, and 2.5–10 µm) as the main core data. The impact of DD on background aerosol conditions is detectable by means of aerosol load thresholds and complementary information provided by HYSPLIT (Hybrid Single Particle Lagrangian Integrated Trajectory Model) air mass back trajectories, MODIS (Moderate Resolution Imaging Spectroradiometer) images, forecast aerosol models, and synoptic maps, which have been carefully reviewed by a human observer for each day included in the DD inventory. This identification method allows the detection of low and moderate DD intrusions and also of mixtures of mineral dust with other aerosol types by means of the analysis of α. During the period studied (2003–2014), a total of 152 DD episodes composed of 418 days are identified. Overall, this means ∼ 13 episodes and ∼ 35 days per year with DD intrusion, representing 9.5 % days year−1. During the identified DD intrusions, 19 daily exceedances over 50 µg m−3 are reported at the surface. The occurrence of DD event days during the year peaks in March and June, with a marked minimum in April and lowest occurrence in winter. A large interannual variability is observed showing a statistically significant temporal decreasing trend of ∼ 3 days year−1. The DD impact on the aerosol climatology is addressed by evaluating the DD contribution in magnitude and percent (in brackets) for AOD, PM10, PM2.5, and PM2.5 − 10, obtaining mean values of 0.015 (11.5 %), 1.3 µg m−3 (11.8 %), 0.55 µg m−3 (8.5 %) and 0.79 µg m−3 (16.1 %), respectively. Annual cycles of the DD contribution for AOD and PM10 present two maxima – one in summer (0.03 and 2.4 µg m−3 for AOD in June and PM10 in August) and another in March (0.02 for AOD and 2.2 µg m−3 for PM10) – both displaying a similar evolution with exceptions in July and September. The seasonal cycle of the DD contribution to AOD does not follow the pattern of the total AOD (close to a bell shape), whereas both PM10 cycles (total and DD contribution) are more similar to each other in shape, with an exception in September. The interannual evolution of the DD contribution to AOD and PM10 has evidenced a progressive decrease. This decline in the levels of mineral dust aerosols can explain up to 30 % of the total aerosol load decrease observed in the study area during the period 2003–2014. The relationship between columnar and surface DD contribution shows a correlation coefficient of 0.81 for the interannual averages. Finally, synoptic conditions during DD events are also analysed, observing that the north African thermal low causes most of the events ( ∼  53 %). The results presented in this study highlight the relevance of the area studied since it can be considered representative of the clean background in the western Mediterranean Basin where DD events have a high impact on aerosol load levels.

The lack of aerosol optical depth (AOD) data at night can be partially addressed through Moon photometer measurements or fully covered with star photometer observations. However, the limited availability and complexity of star photometers have motivated this study to use all-sky cameras to extract starlight signals and derive AOD at night using star photometry. For this purpose, eight all-sky cameras were configured and deployed in nine different locations to capture raw images with varying exposure times every 2 min during the night. This work proposes a novel methodology to extract the starlight signal from the raw data from all-sky cameras and convert it into AOD values. This process consists of the following steps: removing the background image, selecting the pixels, and extracting the signal for each star from a predefined list of 56 stars; performing in situ Langley calibration of the instruments and retrieving the total optical depth (TOD); calculating the effective wavelength for each camera channel; deriving the AOD by subtracting the gas contribution to TOD; and averaging, cloud-screening, and quality-assuring the AOD time series. The AOD time series obtained through this methodology are compared with independent AOD measurements from collocated Moon photometers in the nine locations. The obtained results show that the AOD values derived with the proposed method generally correlate with reference values, often achieving correlation coefficients (r) above 0.90. The AOD values retrieved using the cameras tend to overestimate the reference values by approximately 0.02 and exhibit a precision of around 0.03–0.04. The agreement between the two datasets varies with wavelength and decreases at high-latitude locations, likely due to the poorer performance of Langley calibration in these regions. AOD values align well with day-to-night transitions obtained by solar photometers, demonstrating their reliability. Despite the slight overestimation, the AOD values derived by this new method approximate the real values and provide coverage throughout the entire night, without requiring the presence of the Moon. Therefore, they serve to study and monitor the nocturnal evolution of AOD.

All-sky cameras are frequently used to detect cloud cover; however, this work explores the use of these instruments for the more complex purpose of extracting relative sky radiances. An all-sky camera (SONA202-NF model) with three colour filters narrower than usual for this kind of cameras is configured to capture raw images at seven exposure times. A detailed camera characterization of the black level, readout noise, hot pixels and linear response is carried out. A methodology is proposed to obtain a linear high dynamic range (HDR) image and its uncertainty, which represents the relative sky radiance (in arbitrary units) maps at three effective wavelengths. The relative sky radiances are extracted from these maps and normalized by dividing every radiance of one channel by the sum of all radiances at this channel. Then, the normalized radiances are compared with the sky radiance measured at different sky points by a sun and sky photometer belonging to the Aerosol Robotic Network (AERONET). The camera radiances correlate with photometer ones except for scattering angles below 10∘, which is probably due to some light reflections on the fisheye lens and camera dome. Camera and photometer wavelengths are not coincident; hence, camera radiances are also compared with sky radiances simulated by a radiative transfer model at the same camera effective wavelengths. This comparison reveals an uncertainty on the normalized camera radiances of about 3.3 %, 4.3 % and 5.3 % for 467, 536 and 605 nm, respectively, if specific quality criteria are applied.