Explore the vast range of titles available.

Kerr soliton microcombs have recently emerged as a prominent topic in integrated photonics and have enabled new horizons for optical frequency metrology. Kerr soliton microcombs, as the name suggests, are based on high-order cubic optical nonlinearity. It is desirable to exploit quadratic photonic materials, namely Pockels materials, for soliton generation and on-chip implementation of 1f–2f comb self-referencing. Such quadratically driven solitons have been proposed theoretically, but have not yet been observed in a nanophotonic platform, despite recent progress in quadratic comb generation in free-space and crystalline resonators. Here, we report photonic-chip-based Pockels microcomb solitons driven by three-wave mixing in an aluminium nitride microring resonator. In contrast to typical Kerr solitons, the Pockels soliton features unity soliton generation fidelity, two-by-two evolution of multi-soliton states, favourable tuning dynamics and high pump-to-soliton conversion efficiency.Photonic-chip-based microcomb solitons driven by Pockels nonlinearity—the quadratic χ(2) effect—instead of the Kerr soliton are demonstrated in an aluminium nitride microring resonator with a conversion efficiency of 17%.

All-optical switches have attracted attention because they can potentially overcome the speed limitation of electric switches. However, ultrafast, energy-efficient all-optical switches have been challenging to realize owing to the intrinsically small optical nonlinearity in existing materials. As a solution, we propose the use of graphene-loaded deep-subwavelength plasmonic waveguides (30 × 20 nm2). Thanks to extreme light confinement, we have greatly enhanced optical nonlinear absorption in graphene, and achieved ultrafast all-optical switching with a switching energy of 35 fJ and a switching time of 260 fs. The switching energy is four orders of magnitude smaller than that in previous graphene-based devices and is the smallest value reported for any all-optical switch operating at a few picoseconds or less. This device can be efficiently connected to conventional silicon waveguides and used in silicon photonic integrated circuits. We believe that this graphene-based device will pave the way towards on-chip ultrafast and energy-efficient photonic processing.

Optical soliton dynamics can cause extreme alteration of the temporal and spectral shape of a propagating light pulse. This occurs at up to kilowatt peak powers in glass-core optical fibres and at the gigawatt level in gas-filled microstructured hollow-core fibres. Here, we demonstrate optical soliton dynamics in large-core hollow capillary fibres. This enables scaling of soliton effects by several orders of magnitude to the multi-millijoule energy and terawatt peak power level. We experimentally demonstrate two key soliton effects. First, we observe self-compression to sub-cycle pulses and infer the creation of sub-femtosecond field waveforms—a route to high-power optical attosecond pulse generation. Second, we efficiently generate continuously tunable high-energy (1–16 μJ) pulses in the vacuum and deep ultraviolet (110 nm to 400 nm) through resonant dispersive-wave emission. These results promise to be the foundation of a new generation of table-top light sources for ultrafast strong-field physics and advanced spectroscopy.Optical soliton dynamics in large-core hollow capillary fibres is demonstrated. The findings enable the scaling of soliton effects by several orders of magnitude to the multi-millijoule energy and terawatt peak power levels, and open up opportunities for new-generation table-top light sources for ultrafast strong-field physics and advanced spectroscopy.

Nonlinear optical devices and their implementation into modern nanophotonic architectures are constrained by their usually moderate nonlinear response. Recently, epsilon-near-zero (ENZ) materials have been found to have a strong optical nonlinearity, which can be enhanced through the use of cavities or nano-structuring. Here, we study the pump dependent properties of the plasmon resonance in the ENZ region in a thin layer of indium tin oxide (ITO). Exciting this mode using the Kretschmann-Raether configuration, we study reflection switching properties of a 60 nm layer close to the resonant plasmon frequency. We demonstrate a thermal switching mechanism, which results in a shift in the plasmon resonance frequency of 20 THz for a TM pump intensity of 70 GW cm −2 . For degenerate pump and probe frequencies, we highlight an additional two-beam coupling contribution, not previously isolated in ENZ nonlinear optics studies, which leads to an overall pump induced change in reflection from 1% to 45%. All-optical switching is important for integrated-photonics and communication devices. Here the authors demonstrate all-optical switching of an Epsilon-Near-Zero plasmon resonance using indium tin oxide thin film.

High-harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, thus far, the shortest isolated attosecond pulses have only been produced with linear polarization, which limits the range of physics that can be explored. Here, we demonstrate robust polarization control of isolated extreme-ultraviolet pulses by exploiting non-collinear high-harmonic generation driven by two counter-rotating few-cycle laser beams. The circularly polarized supercontinuum is produced at a central photon energy of 33 eV with a transform limit of 190 as and a predicted linear chirp of 330 as. By adjusting the ellipticity of the two counter-rotating driving pulses simultaneously, we control the polarization state of isolated extreme-ultraviolet pulses—from circular through elliptical to linear polarization—without sacrificing conversion efficiency. Access to the purely circularly polarized supercontinuum, combined with full helicity and ellipticity control, paves the way towards attosecond metrology of circular dichroism.

An efficient simulator for quantum systems is one of the original goals for the efforts to develop a quantum computer. In recent years, synthetic dimensions in photonics have emerged as a potentially powerful approach for simulation that is free from the constraint of geometric dimensionality. Here we demonstrate a quantum-correlated synthetic crystal that is based on a coherently controlled broadband quantum frequency comb produced in a chip-scale, dynamically modulated lithium niobate microresonator. The time–frequency entanglement inherent with the comb modes greatly extends the dimensionality of the synthetic space, creating a massive, nearly 400 × 400 synthetic lattice with electrically controlled tunability. With such a system, we are able to utilize the evolution of quantum correlations between entangled photons to perform a series of simulations, demonstrating quantum random walks, Bloch oscillations and multilevel Rabi oscillations in the time and frequency correlation space (demonstrated in a 5 × 5 mode subspace). The device combines the simplicity of monolithic nanophotonic architecture, high dimensionality of a quantum-correlated synthetic space and on-chip coherent control, which opens up an avenue towards chip-scale implementation of large-scale analogue quantum simulation and computation in the time–frequency domain.A special-purpose quantum simulator, based on a coherently controlled broadband quantum frequency comb produced in a chip-scale dynamically modulated monolithic lithium niobate microresonator, is demonstrated, opening paths for chip-scale implementation of large-scale analogue quantum simulation and computation in the time–frequency domain.

Soliton microcombs—phase-locked microcavity frequency combs—have become the foundation of several classical technologies in integrated photonics, including spectroscopy, LiDAR and optical computing. Despite the predicted multimode entanglement across the comb, experimental study of the quantum optics of the soliton microcomb has been elusive. In this work we use second-order photon correlations to study the underlying quantum processes of soliton microcombs in an integrated silicon carbide microresonator. We show that a stable temporal lattice of solitons can isolate a multimode below-threshold Gaussian state from any admixture of coherent light, and predict that all-to-all entanglement can be realized for the state. Our work opens a pathway toward a soliton-based multimode quantum resource.The quantum aspect of soliton microcomb from an integrated silicon carbide microresonator is studied in several regimes — below threshold, above threshold and in the soliton regime — using a single-photon optical spectrum analyser for second-order photon correlation measurement.

Multidimensional solitary states (MDSS)—self-sustained wavepackets—have attracted renewed interest in many different fields of physics. They are of particular importance in nonlinear optics, especially for the nonlinear propagation of ultrashort pulses in multimode fibres, which contain rich spatiotemporal intermodal interactions and dynamics, albeit often in an unstable manner. Here, we report the observation of the formation of highly stable multidimensional solitary states in a molecular gas-filled large-core hollow-core fibre. We experimentally and numerically demonstrate the creation of MDSS by multimillijoule, subpicosecond near-infrared pulses and the underlying physics. We find that the MDSS have a broadband redshifted spectra with an uncommon negative quadratic spectral phase at the output of the hollow-core fibre, originating from Raman enhancement due to the strong intermodal nonlinear interactions. The spatial and temporal localization of MDSS enables the compression of the broadened pulses at the output to 10.8 fs by simple linear propagation in a piece of fused silica. The high spatiotemporal quality of MDSS is further verified by high-harmonic generation. Our results present new opportunities for studying multimodal spatiotemporal dynamics in the high-energy regime. This work also presents a route toward a new class of compact, tunable and high-energy spatiotemporally engineered coherent light sources based on picosecond ytterbium technology.The formation of multidimensional solitary states through the nonlinear propagation of high-energy pulses in a molecular gas-filled large-core hollow-core fibre is demonstrated, offering new opportunities for studying multimodal spatiotemporal dynamics in the high-energy regime.

Optical nonlinear functions are crucial for various applications in integrated photonics, including all-optical information processing1, photonic neural networks2,3 and on-chip ultrafast light sources4,5. However, the weak native nonlinearity of most nanophotonic platforms has imposed barriers for such functions by necessitating large driving energies, high-Q cavities or integration with other materials with stronger nonlinearity. Here we effectively utilize the strong and instantaneous quadratic nonlinearity of lithium niobate nanowaveguides for the realization of cavity-free all-optical switching. By simultaneous engineering of the dispersion and quasi-phase matching, we design and demonstrate a nonlinear splitter that can achieve ultralow switching energies down to 80 fJ, featuring a fastest switching time of ~46 fs and a lowest energy–time product of 3.7 × 10−27 J s in integrated photonics. Our results can enable on-chip ultrafast and energy-efficient all-optical information processing, computing systems and light sources.Researchers exploit the quadratic nonlinearity of lithium niobate nanowaveguides and demonstrate cavity-free all-optical switching. Switching energies down to 80 fJ, switching times down to ~46 fs and energy–time products of 3.7 × 10−27 J s are shown.

Microcavity-based frequency combs, or ‘microcombs’1,2, have enabled many fundamental breakthroughs3–21 through the discovery of temporal cavity-solitons. These self-localized waves, described by the Lugiato–Lefever equation22, are sustained by a background of radiation usually containing 95% of the total power23. Simple methods for their efficient generation and control are currently being investigated to finally establish microcombs as out-of-the-lab tools24. Here, we demonstrate microcomb laser cavity-solitons. Laser cavity-solitons are intrinsically background-free and have underpinned key breakthroughs in semiconductor lasers22,25–28. By merging their properties with the physics of multimode systems29, we provide a new paradigm for soliton generation and control in microcavities. We demonstrate 50-nm-wide bright soliton combs induced at average powers more than one order of magnitude lower than the Lugiato–Lefever soliton power threshold22, measuring a mode efficiency of 75% versus the theoretical limit of 5% for bright Lugiato–Lefever solitons23. Finally, we can tune the repetition rate by well over a megahertz without any active feedback.By nesting a Kerr microresonator in a fibre loop with gain, 50-nm-wide bright microcavity-based soliton combs with a mode efficiency of 75% can be induced at average powers more than one order of magnitude lower than the Lugiato–Lefever soliton power threshold, facilitating real-world applications.