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For the first time, a closure study of the relationship between the ice-nucleating particle concentration (INP; INPC) and ice crystal number concentration (ICNC) in altocumulus and cirrus layers, solely based on ground-based active remote sensing, is presented. Such aerosol–cloud closure experiments are required (a) to better understand aerosol–cloud interaction in the case of mixed-phase clouds, (b) to explore to what extent heterogeneous ice nucleation can contribute to cirrus formation, which is usually controlled by homogeneous freezing, and (c) to check the usefulness of available INPC parameterization schemes, applied to lidar profiles of aerosol optical and microphysical properties up to the tropopause level. The INPC–ICNC closure studies were conducted in Cyprus (Limassol and Nicosia) during a 6-week field campaign in March–April 2015 and during the 17-month CyCARE (Cyprus Clouds Aerosol and Rain Experiment) campaign. The focus was on altocumulus and cirrus layers which developed in pronounced Saharan dust layers at heights from 5 to 11 km. As a highlight, a long-lasting cirrus event was studied which was linked to the development of a very strong dust-infused baroclinic storm (DIBS) over Algeria. The DIBS was associated with strong convective cloud development and lifted large amounts of Saharan dust into the upper troposphere, where the dust influenced the evolution of an unusually large anvil cirrus shield and the subsequent transformation into an cirrus uncinus cloud system extending from the eastern Mediterranean to central Asia, and thus over more than 3500 km. Cloud top temperatures of the three discussed closure study cases ranged from −20 to −57 ∘C. The INPC was estimated from polarization/Raman lidar observations in combination with published INPC parameterization schemes, whereas the ICNC was retrieved from combined Doppler lidar, aerosol lidar, and cloud radar observations of the terminal velocity of falling ice crystals, radar reflectivity, and lidar backscatter in combination with the modeling of backscattering at the 532 and 8.5 mm wavelengths. A good-to-acceptable agreement between INPC (observed before and after the occurrence of the cloud layer under investigation) and ICNC values was found in the discussed three proof-of-concept closure experiments. In these case studies, INPC and ICNC values matched within an order of magnitude (i.e., within the uncertainty ranges of the INPC and ICNC estimates), and they ranged from 0.1 to 10 L−1 in the altocumulus layers and 1 to 50 L−1 in the cirrus layers observed between 8 and 11 km height. The successful closure experiments corroborate the important role of heterogeneous ice nucleation in atmospheric ice formation processes when mineral dust is present. The observed long-lasting cirrus event could be fully explained by the presence of dust, i.e., without the need for homogeneous ice nucleation processes.

ISCCP continues to quantify the global distribution and diurnal-to-interannual variations of cloud properties in a revised version. This paper summarizes assessments of the previous version, describes refinements of the analysis and enhanced features of the product design, discusses the few notable changes in the results, and illustrates the long-term variations of global mean cloud properties and differing high cloud changes associated with ENSO. The new product design includes a global, pixel-level product on a 0.1° grid, all other gridded products at 1.0°-equivalent equal area, separate satellite products with ancillary data for regional studies, more detailed, embedded quality information, and all gridded products in netCDF format. All the data products including all input data, expanded documentation, the processing code, and an operations guide are available online. Notable changes are 1) a lowered ice–liquid temperature threshold, 2) a treatment of the radiative effects of aerosols and surface temperature inversions, 3) refined specification of the assumed cloud microphysics, and 4) interpolation of the main daytime cloud information overnight. The changes very slightly increase the global monthly mean cloud amount with a little more high cloud and a little less middle and low cloud. Over the whole period, total cloud amount slowly decreases caused by decreases in cumulus/altocumulus; consequently, average cloud-top temperature and optical thickness have increased. The diurnal and seasonal cloud variations are very similar to earlier versions. Analysis of the whole record shows that high cloud variations, but not low clouds, exhibit different patterns in different ENSO events.

An energy budget combining atmospheric moist static energy (MSE) and upper ocean heat content (OHC) is used to examine the processes impacting day-to-day convective variability in the tropical Indian and western Pacific Oceans. Feedbacks arising from atmospheric and oceanic transport processes, surface fluxes, and radiation drive the cyclical amplification and decay of convection around suppressed and enhanced convective equilibrium states, referred to as shallow and deep convective discharge–recharge (D–R) cycles, respectively. The shallow convective D–R cycle is characterized by alternating enhancements of shallow cumulus and stratocumulus, often in the presence of extensive cirrus clouds. The deep convective D–R cycle is characterized by sequential increases in shallow cumulus, congestus, narrow deep precipitation, wide deep precipitation, a mix of detached anvil and altostratus and altocumulus, and once again shallow cumulus cloud types. Transitions from the shallow to deep D–R cycle are favored by a positive “column process” feedback, while discharge of convective instability and OHC by mesoscale convective systems (MCSs) contributes to transitions from the deep to shallow D–R cycle. Variability in the processes impacting MSE is comparable in magnitude to, but considerably more balanced than, variability in the processes impacting OHC. Variations in the quantity of atmosphere–ocean coupled static energy (MSE + OHC) result primarily from atmospheric and oceanic transport processes, but are mainly realized as changes in OHC. MCSs are unique in their ability to rapidly discharge both lower-tropospheric convective instability and OHC.

Surface solar irradiance variability is present under all broken clouds, but the patterns, magnitude of variability, and driving mechanisms vary greatly with cloud type. In this study, we performed numerical experiments to understand which main mechanisms drive surface solar irradiance (SSI) variations across a diverse set of observation-based cloud conditions. The results show that four mechanisms capture the essence. We find that for optically thin (τ<6) clouds, scattering in the forward direction (forward escape) dominates. In cloud fields with enough optically thin area, such as altocumulus, forward escape alone can drive areas of irradiance enhancement of over 50 % of clear-sky irradiance. For flat, optically thick clouds (τ>6), irradiance is instead scattered diffusely downward (downward escape), and (extreme) enhancements are thus found directly below the cloud. For vertically structured clouds, side escape dominates the domain-averaged diffuse irradiance enhancement until the sides become shaded by anvil clouds. Lastly, under optically thick cloud cover, surface albedo enhances radiative fluxes due to multiple scatterings between surface and cloud. This brightens shadows and contributes 10 % to 60 % of the total irradiance enhancement for low (0.2) to high (0.8) albedo. With these four mechanisms, we provide a framework for understanding the vast diversity and complexity found in surface solar irradiance and cloudiness. A next step is to apply this analysis to multi-layered cloud fields and non-isolated deep convective clouds.

We experimentally quantified the impact of cloud fraction and cloud type on the heating rate (HR) of black and brown carbon (HRBC and HRBrC). In particular, we examined in more detail the cloud effect on the HR detected in a previous study (Ferrero et al., 2018). High-time-resolution measurements of the aerosol absorption coefficient at multiple wavelengths were coupled with spectral measurements of the direct, diffuse and surface reflected irradiance and with lidar–ceilometer data during a field campaign in Milan, Po Valley (Italy). The experimental set-up allowed for a direct determination of the total HR (and its speciation: HRBC and HRBrC) in all-sky conditions (from clear-sky conditions to cloudy). The highest total HR values were found in the middle of winter (1.43 ± 0.05 K d−1), and the lowest were in spring (0.54 ± 0.02 K d−1). Overall, the HRBrC accounted for 13.7 ± 0.2 % of the total HR, with the BrC being characterized by an absorption Ångström exponent (AAE) of 3.49 ± 0.01. To investigate the role of clouds, sky conditions were classified in terms of cloudiness (fraction of the sky covered by clouds: oktas) and cloud type (stratus, St; cumulus, Cu; stratocumulus, Sc; altostratus, As; altocumulus, Ac; cirrus, Ci; and cirrocumulus–cirrostratus, Cc–Cs). During the campaign, clear-sky conditions were present 23 % of the time, with the remaining time (77 %) being characterized by cloudy conditions. The average cloudiness was 3.58 ± 0.04 oktas (highest in February at 4.56 ± 0.07 oktas and lowest in November at 2.91 ± 0.06 oktas). St clouds were mostly responsible for overcast conditions (7–8 oktas, frequency of 87 % and 96 %); Sc clouds dominated the intermediate cloudiness conditions (5–6 oktas, frequency of 47 % and 66 %); and the transition from Cc–Cs to Sc determined moderate cloudiness (3–4 oktas); finally, low cloudiness (1–2 oktas) was mostly dominated by Ci and Cu (frequency of 59 % and 40 %, respectively). HR measurements showed a constant decrease with increasing cloudiness of the atmosphere, enabling us to quantify for the first time the bias (in %) of the aerosol HR introduced by the simplified assumption of clear-sky conditions in radiative-transfer model calculations. Our results showed that the HR of light-absorbing aerosol was ∼ 20 %–30 % lower in low cloudiness (1–2 oktas) and up to 80 % lower in completely overcast conditions (i.e. 7–8 oktas) compared to clear-sky ones. This means that, in the simplified assumption of clear-sky conditions, the HR of light-absorbing aerosol can be largely overestimated (by 50 % in low cloudiness, 1–2 oktas, and up to 500 % in completely overcast conditions, 7–8 oktas). The impact of different cloud types on the HR was also investigated. Cirrus clouds were found to have a modest impact, decreasing the HRBC and HRBrC by −5 % at most. Cumulus clouds decreased the HRBC and HRBrC by −31 ± 12 % and −26 ± 7 %, respectively; cirrocumulus–cirrostratus clouds decreased the HRBC and HRBrC by −60 ± 8 % and −54 ± 4 %, which was comparable to the impact of altocumulus (−60 ± 6 % and −46 ± 4 %). A higher impact on the HRBC and HRBrC suppression was found for stratocumulus (−63 ± 6 % and −58 ± 4 %, respectively) and altostratus (−78 ± 5 % and −73 ± 4 %, respectively). The highest impact was associated with stratus, suppressing the HRBC and HRBrC by −85 ± 5 % and −83 ± 3 %, respectively. The presence of clouds caused a decrease of both the HRBC and HRBrC (normalized to the absorption coefficient of the respective species) of −11.8 ± 1.2 % and −12.6 ± 1.4 % per okta. This study highlights the need to take into account the role of both cloudiness and different cloud types when estimating the HR caused by both BC and BrC and in turn decrease the uncertainties associated with the quantification of their impact on the climate.

Influences of cloud liquid water, cloud ice, rain, snow, and graupel on all-sky simulations of the Cross-track Infrared Sounder (CrIS) brightness temperature (TB) are assessed for the 399 data assimilation (DA) channels. The analyses generated by the Gridpoint Statistical Interpolation (GSI) 3D-Var system assimilating conventional and clear-sky satellite radiance observations are used as initial conditions for the Weather Research and Forecasting Model to generate 6-h forecasts with three different microphysics schemes (WSM6, Thompson, and Morrison), which are then used as input to the Community Radiative Transfer Model for all-sky TB simulations. Under all-sky conditions, biases with the WSM6 scheme are negative for all channels and greater in magnitude than −3.5 K. The biases with the Thompson and Morrison schemes vary between −1 and 1 K for all channels. Bias differences among three MP schemes are small in stratus, altocumulus, and cumulus clouds, but large in cirrus and cirrocumulus clouds. The TB simulations in stratus, altocumulus, and cumulus clouds are mostly influenced by the cloud top pressure, while that in cirrus and cirrocumulus clouds depends strongly on cloud optical depth. All-sky TB simulations in cirrus conditions are more positively biased than those under cirrocumulus conditions, probably due to the microphysics schemes producing too thick cirrus clouds. Sensitivity experiments suggest that the TB discrepancies among DA experiments with three MP schemes are mostly caused by the ice or snow type rather than the effective radius of hydrometeor in the upper troposphere. Finally, we propose to combine a cloud-effect parameter with cloud types for modeling observation error characteristics in all-sky DA.

This work focuses on total organic carbon (TOC) and contributing species in cloud water over Southeast Asia using a rare airborne dataset collected during NASA's Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex), in which a wide variety of maritime clouds were studied, including cumulus congestus, altocumulus, altostratus, and cumulus. Knowledge of TOC masses and their contributing species is needed for improved modeling of cloud processing of organics and to understand how aerosols and gases impact and are impacted by clouds. This work relies on 159 samples collected with an axial cyclone cloud-water collector at altitudes of 0.2–6.8 km that had sufficient volume for both TOC and speciated organic composition analysis. Species included monocarboxylic acids (glycolate, acetate, formate, and pyruvate), dicarboxylic acids (glutarate, adipate, succinate, maleate, and oxalate), methanesulfonic acid (MSA), and dimethylamine (DMA). TOC values range between 0.018 and 13.66 ppm C with a mean of 0.902 ppm C. The highest TOC values are observed below 2 km with a general reduction aloft. An exception is samples impacted by biomass burning for which TOC remains enhanced at altitudes as high as 6.5 km (7.048 ppm C). Estimated total organic matter derived from TOC contributes a mean of 30.7 % to total measured mass (inorganics + organics). Speciated organics contribute (on a carbon mass basis) an average of 30.0 % to TOC in the study region and account for an average of 10.3 % to total measured mass.The order of the average contribution of species to TOC, in decreasing contribution of carbon mass, is as follows (±1 standard deviation): acetate (14.7 ± 20.5 %), formate (5.4 ± 9.3 %), oxalate (2.8 ± 4.3 %), DMA (1.7 ± 6.3 %), succinate (1.6 ± 2.4 %), pyruvate (1.3 ± 4.5 %), glycolate (1.3 ± 3.7 %), adipate (1.0 ± 3.6 %), MSA (0.1 ± 0.1 %), glutarate (0.1 ± 0.2 %), and maleate (< 0.1 ± 0.1 %). Approximately 70 % of TOC remains unaccounted for, highlighting the complex nature of organics in the study region; in samples collected in biomass burning plumes, up to 95.6 % of TOC mass is unaccounted for based on the species detected. Consistent with other regions, monocarboxylic acids dominate the speciated organic mass (∼ 75 %) and are about 4 times more abundant than dicarboxylic acids.Samples are categorized into four cases based on back-trajectory history, revealing source-independent similarity between the bulk contributions of monocarboxylic and dicarboxylic acids to TOC (16.03 %–23.66 % and 3.70 %–8.75 %, respectively). Furthermore, acetate, formate, succinate, glutarate, pyruvate, oxalate, and MSA are especially enhanced during biomass burning periods, which is attributed to peat emissions transported from Sumatra and Borneo. Lastly, dust (Ca2+) and sea salt (Na+/Cl-) tracers exhibit strong correlations with speciated organics, supporting how coarse aerosol surfaces interact with these water-soluble organics.

The cloud type product 2B-CLDCLASS-LIDAR based on CloudSat and CALIPSO from June 2006 to May 2017 is used to examine the temporal and spatial distribution characteristics and interannual variability of eight cloud types (high cloud, altostratus, altocumulus, stratus, stratocumulus, cumulus, nimbostratus, and deep convection) and three phases (ice, mixed, and water) in the Arctic. Possible reasons for the observed interannual variability are also discussed. The main conclusions are as follows: (1) More water clouds occur on the Atlantic side, and more ice clouds occur over continents. (2) The average spatial and seasonal distributions of cloud types show three patterns: high clouds and most cumuliform clouds are concentrated in low-latitude locations and peak in summer; altostratus and nimbostratus are concentrated over and around continents and are less abundant in summer; stratocumulus and stratus are concentrated near the inner Arctic and peak during spring and autumn. (3) Regional averaged interannual frequencies of ice clouds and altostratus clouds significantly decrease, while those of water clouds, altocumulus, and cumulus clouds increase significantly. (4) Significant features of the linear trends of cloud frequencies are mainly located over ocean areas. (5) The monthly water cloud frequency anomalies are positively correlated with air temperature in most of the troposphere, while those for ice clouds are negatively correlated. (6) The decrease in altostratus clouds is associated with the weakening of the Arctic front due to Arctic warming, while increased water vapor transport into the Arctic and higher atmospheric instability lead to more cumulus and altocumulus clouds.

The environment of elevated nocturnal deep convection initiation (CI) on 24 June 2015 is investigated using radiosonde data from the Plains Elevated Convection at Night (PECAN) field experiment and a convection-allowing simulation. Elevated CI occurs around midnight in ascending westerly flow above the northeastern terminus of the nocturnal low-level jet (LLJ) several hundred kilometers poleward of the leading edge of a surface warm front. This CI originates from within preexisting banded altocumulus clouds that are supported by persistent large-scale ascent within the entrance region of a midtropospheric jet streak. Model trajectories calculated backward from convective updraft cores during CI indicate abrupt lifting at the leading edge of the surface front during the late afternoon to altitudes above that of the subsequent southerly LLJ. This air remains significantly subsaturated during northward movement until after several hours of weaker but persistent ascent within the highly elevated westerly airstream during the evening. Unlike in many previous studies of frontal overrunning by the LLJ, strong local drying occurs within the LLJ core. Nevertheless, vertical displacements from persistent mesoscale ascent were sufficient for trajectory air parcels to reach their LFC and sustain deep convection. The mesoscale upward displacement along trajectories is well explained by isentropic upglide associated with frontal overrunning at horizontal distances greater than 100 km from the CI and subsequent mature convection. However, the significant additional mesoscale vertical displacements needed for deep CI to occur in the westerlies above the horizontally convergent ~100-km-wide LLJ terminus region, were associated with local cooling and are not accounted for by steady isentropic upglide.

We developed a simple algorithm to classify clouds based on global radiation and cloud base height measured by pyranometer and ceilometer, respectively. We separated clouds into seven different classes (stratus, stratocumulus, cumulus, nimbostratus, altocumulus + altostratus, cirrus + cirrocumulus + cirrostratus and clear sky + cirrus). We also included classes for cumulus and cirrus clouds causing global radiation enhancement, and we classified multilayered clouds, when captured by the ceilometer, based on their height and characteristics (transmittance, patchiness and uniformity). The overall performance of the algorithm was nearly 70 % when compared with classification by an observer using total-sky images. The performance was best for clouds having well-distinguishable effects on solar radiation: nimbostratus clouds were classified correctly in 100 % of the cases. The worst performance corresponds to cirriform clouds (50 %). Although the overall performance of the algorithm was good, it is likely to miss the occurrences of high and multilayered clouds. This is due to the technical limits of the instrumentation: the vertical detection range of the ceilometer and occultation of the laser pulse by the lowest cloud layer. We examined the use of clearness index, which is defined as a ratio between measured global radiation and modeled radiation at the top of the atmosphere, as an indicator of clear-sky conditions. Our results show that cumulus, altocumulus, altostratus and cirriform clouds can be present when the index indicates clear-sky conditions. Those conditions have previously been associated with enhanced aerosol formation under clear skies. This is an important finding especially in the case of low clouds coupled to the surface, which can influence aerosol population via aerosol–cloud interactions. Overall, caution is required when the clearness index is used in the analysis of processes affected by partitioning of radiation by clouds.