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398 result(s) for "BGO (crystal)"
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Controlling the propagation asymmetry of hyperbolic shear polaritons in beta-gallium oxide
Structural anisotropy in crystals is crucial for controlling light propagation, particularly in the infrared spectral regime where optical frequencies overlap with crystalline lattice resonances, enabling light-matter coupled quasiparticles called phonon polaritons (PhPs). Exploring PhPs in anisotropic materials like hBN and MoO 3 has led to advancements in light confinement and manipulation. In a recent study, PhPs in the monoclinic crystal β-Ga 2 O 3 (bGO) were shown to exhibit strongly asymmetric propagation with a frequency dispersive optical axis. Here, using scanning near-field optical microscopy (s-SNOM), we directly image the symmetry-broken propagation of hyperbolic shear polaritons in bGO. Further, we demonstrate the control and enhancement of shear-induced propagation asymmetry by varying the incident laser orientation and polariton momentum using different sizes of nano-antennas. Finally, we observe significant rotation of the hyperbola axis by changing the frequency of incident light. Our findings lay the groundwork for the widespread utilization and implementation of polaritons in low-symmetry crystals. Hyperbolic phonon polaritons occurring in anisotropic materials exhibit strong light confinement and propagation directionality. Matson et al. report real-space imaging and control of recently discovered hyperbolic shear phonon-polaritons in beta-Ga2O3, arising from symmetry breaking in the dielectric response.
Hard X-ray transient grating spectroscopy on bismuth germanate
Optical-domain transient grating (TG) spectroscopy is a versatile background-free four-wave-mixing technique that is used to probe vibrational, magnetic and electronic degrees of freedom in the time domain1. The newly developed coherent X-ray free-electron laser sources allow its extension to the X-ray regime. X-rays offer multiple advantages for TG: their large penetration depth allows probing the bulk properties of materials, their element specificity can address core excited states, and their short wavelengths create excitation gratings with unprecedented momentum transfer and spatial resolution. Here, we demonstrate TG excitation in the hard X-ray range at 7.1 keV. In bismuth germanate (BGO), the non-resonant TG excitation generates coherent optical phonons detected as a function of time by diffraction of an optical probe pulse. This experiment demonstrates the ability to probe bulk properties of materials and paves the way for ultrafast coherent four-wave-mixing techniques using X-ray probes and involving nanoscale TG spatial periods.A four-wave mixing technique is developed in the hard X-ray range. A diamond phase grating in an X-ray beam path creates a periodic excitation pattern on a sample via the Talbot effect. The response of the periodic excitation is probed by an optical pulse.
First direct limit on the 395 keV resonance of the 22Ne(α, γ)26Mg reaction
The 22Ne(α, γ)26Mg reaction (Q = 10614.74 keV) competes with the 22Ne(α, n)25Mg reaction (Q = −478.34 keV) which is the main source of neutrons for the s-process in low-mass Asymptotic Giant Branch and massive stars. The cross sections of these reactions are crucial to fix the cross over temperature at which (α, n) rate exceeds the (α, γ) one. Moreover, the uncertainty on the 22Ne(α, γ)26Mg reaction rate affects also the nucleosynthesis of isotopes between 26Mg and 31P in intermediate-mass stars. At lower temperatures (T < 300 MK) where the (α, γ) channel is dominant, the rate of the 22Ne(α, γ)26Mg reaction is influenced by several resonances. The present study focuses on the Eα = 395 keV resonance which so far have been studied only indirectly leading to a wide range of possible values for its resonance strength (10−15 −10−9 eV). The experiment has been completed at LUNA using the intense alpha beam of the LUNA 400 kV accelerator and a windowless differential-pumped gas target combined with a high efficiency BGO detector. Experimental details and preliminary results will be shown.
Walk-through flat panel total-body PET: a patient-centered design for high throughput imaging at lower cost using DOI-capable high-resolution monolithic detectors
PurposeLong axial field-of-view (LAFOV) systems have a much higher sensitivity than standard axial field-of-view (SAFOV) PET systems for imaging the torso or full body, which allows faster and/or lower dose imaging. Despite its very high sensitivity, current total-body PET (TB-PET) throughput is limited by patient handling (positioning on the bed) and often a shortage of available personnel. This factor, combined with high system costs, makes it hard to justify the implementation of these systems for many academic and nearly all routine nuclear medicine departments. We, therefore, propose a novel, cost-effective, dual flat panel TB-PET system for patients in upright standing positions to avoid the time-consuming positioning on a PET-CT table; the walk-through (WT) TB-PET. We describe a patient-centered, flat panel PET design that offers very efficient patient throughput and uses monolithic detectors (with BGO or LYSO) with depth-of-interaction (DOI) capabilities and high intrinsic spatial resolution. We compare system sensitivity, component costs, and patient throughput of the proposed WT-TB-PET to a SAFOV (= 26 cm) and a LAFOV (= 106 cm) LSO PET systems.MethodsPatient width, height (= top head to start of thighs) and depth (= distance from the bed to front of patient) were derived from 40 randomly selected PET-CT scans to define the design dimensions of the WT-TB-PET. We compare this new PET system to the commercially available Siemens Biograph Vision 600 (SAFOV) and Siemens Quadra (LAFOV) PET-CT in terms of component costs, system sensitivity, and patient throughput. System cost comparison was based on estimating the cost of the two main components in the PET system (Silicon Photomultipliers (SiPMs) and scintillators). Sensitivity values were determined using Gate Monte Carlo simulations. Patient throughput times (including CT and scout scan, patient positioning on bed and transfer) were recorded for 1 day on a Siemens Vision 600 PET. These timing values were then used to estimate the expected patient throughput (assuming an equal patient radiotracer injected activity to patients and considering differences in system sensitivity and time-of-flight information) for WT-TB-PET, SAFOV and LAFOV PET.ResultsThe WT-TB-PET is composed of two flat panels; each is 70 cm wide and 106 cm high, with a 50-cm gap between both panels. These design dimensions were justified by the patient sizes measured from the 40 random PET-CT scans. Each panel consists of 14 × 20 monolithic BGO detector blocks that are 50 × 50 × 16 mm in size and are coupled to a readout with 6 × 6 mm SiPMs arrays. For the WT-TB-PET, the detector surface is reduced by a factor of 1.9 and the scintillator volume by a factor of 2.2 compared to LAFOV PET systems, while demonstrating comparable sensitivity and much better uniform spatial resolution (< 2 mm in all directions over the FOV). The estimated component cost for the WT-TB-PET is 3.3 × lower than that of a 106 cm LAFOV system and only 20% higher than the PET component costs of a SAFOV. The estimated maximum number of patients scanned on a standard 8-h working day increases from 28 (for SAFOV) to 53–60 (for LAFOV in limited/full acceptance) to 87 (for the WT-TB-PET). By scanning faster (more patients), the amount of ordered activity per patient can be reduced drastically: the WT-TB-PET requires 66% less ordered activity per patient than a SAFOV.ConclusionsWe propose a monolithic BGO or LYSO-based WT-TB-PET system with DOI measurements that departs from the classical patient positioning on a table and allows patients to stand upright between two flat panels. The WT-TB-PET system provides a solution to achieve a much lower cost TB-PET approaching the cost of a SAFOV system. High patient throughput is increased by fast patient positioning between two vertical flat panel detectors of high sensitivity. High spatial resolution (< 2 mm) uniform over the FOV is obtained by using DOI-capable monolithic scintillators.
Li2MnCl4 for neutron detection: tailoring red emission via doping
In this work, we report on the growth of red-emitting lithium manganese(II) chloride (Li2MnCl4, LMC), a potential candidate for thermal neutron detection. The doping of Li2MnCl4 was proposed to optimize scintillation efficiency and three single crystals of Li2MnCl4:Sm2+, Li2MnCl4:Ti3+, and Li2MnCl4:In+ were grown by miniaturized vertical Bridgman method (mVB). While crystal growth was successful, the results from optical measurements indicated limited achievement in the optimization of luminescence properties. Ti3+ incorporation into the Li2MnCl4 lattice was highly uncertain, as neither the absorbance data nor the radioluminescence (RL) spectrum exhibited bands corresponding to the Ti3+ 2E → 2T2 radiative transition. In the case of Sm2+- and In+_doping, the RL efficiencies achieved only 3.39 and 2.14% of the bismuth germanate (Bi4Ge3O12, BGO) reference sample, respectively. Since the Li2MnCl4:Sm2+ photoluminescence (PL) spectra revealed line emissions corresponding to the Sm2+ forbidden 4f6 → 4f6 transitions, the temperature-dependent PL was measured. At higher temperatures (specifically, from 437 K), the broad emission of the 4f55d → 4f6 transition dominated, which indicated the thermal population of the 5d state.
Light speed variation from gamma ray bursts: criteria for low energy photons
We examine a method to detect the light speed variation from gamma ray burst data observed by the Fermi Gamma-ray Space Telescope (FGST). We suggest new criteria to determine the characteristic time for low energy photons by the energy curve and the average energy curve respectively, and obtain similar results compared with those from the light curve. We offer a new criterion with both the light curve and the average energy curve to determine the characteristic time for low energy photons. We then apply the new criteria to the GBM NaI data, the GBM BGO data, and the LAT LLE data, and obtain consistent results for three different sets of low energy photons from different FERMI detectors.
The challenging direct measurement of the 65 keV resonance strength of the 17O(p, γ)18F reaction at LUNA
The 17O(p, γ)18F reaction plays a crucial role in AGB nucleosynthesis as well as in explosive hydrogen burning occurring in type Ia novae. At the temperatures of interest for the former scenario ( 20MK < T < 80MK) the main contribution to the astrophysical reaction rate comes from the poorly constrained ER = 65 keV resonance. The strength of this resonance is presently determined only through indirect measurements, with an adopted value ωγ =(16 ± 3) peV.A new high sensitivity setup was installed at LUNA, located at LNGS. The underground location of the LUNA 400kV accelerator guarantees a reduction of the cosmic ray background by several orders of magnitude. The residual background was further reduced installing a devoted shielding. On the other hand, to increase the efficiency, the 4π BGO detector was coupled with Al target chamber and holder. With more than 400C accumulated on Ta2O5 targets, nominal 17O enrichment of 90%, the LUNA collaboration has performed the first direct measurement of the 65 keV resonance strength.
An extended bore length solid-state digital-BGO PET/CT system: design, preliminary experience, and performance characteristics
Purpose A solid-state PET/CT system uses bismuth germanium oxide (BGO) scintillating crystals coupled to silicon photomultipliers over an extended 32 cm axial field-of-view (FOV) to provide high spatial resolution and very high sensitivity. Performance characteristics were determined for this digital-BGO system, including NEMA and EARL standards. Methods Spatial resolution, scatter fraction (SF), noise equivalent count rate (NECR), sensitivity, count rate accuracy, and image quality (IQ) were evaluated for the digital-BGO system as per NEMA NU 2-2018, at 2 sites of first clinical install. System energy resolution was measured. Bayesian penalized-likelihood reconstruction (BPL) was used for IQ. EARL Standards 2 studies were reconstructed by BPL combined with a contrast-enhancing deep learning algorithm. An Esser PET phantom was evaluated. Three patient examples were obtained with low-dose radiotracer activity: 2 MBq/kg of [ 18 F]FDG ([ 18 F]-2-fluoro-2-deoxy- d -glucose), 2.3 MBq/kg [ 68 Ga]Ga-DOTA-TATE ([dodecane tetra-acetic acid,Tyr 3 ]-octreotate), and 14.5 MBq/kg [ 82 Rb]RbCl ([ 82 Rb]-rubidium-chloride). Total scan times were ≤ 8 min. Results NEMA sensitivity was 47.6 cps/kBq at the axial center. Spatial resolution at 1 cm from the center axis was ≤4.5 mm (filtered back projection) and ≤3.8 mm (ordered subset expectation maximization). SF was 35.6%, count rate accuracy was 2.16%, and peak NECR was 485.2 kcps at 16.9 kBq/mL. Contrast for IQ was 61.1 to 90.7% (smallest to largest sphere) with background variations from 7.6 to 2.1%, and a “lung” error of 4.7%. The average detector energy resolution was 9.67%. Image quality for patient scans was good. EARL Standards 2 criteria were robustly met and Esser phantom features ≥4.8 mm were resolved at 2 min per bed position. Conclusion A solid-state 32 cm axial FOV digital-BGO PET/CT system provides good spatial and energy resolution, high count rates, and superior NEMA sensitivity in its class, enabling fast clinical acquisitions with low-dose radiotracer activity.
Deep learning–based time-of-flight (ToF) image enhancement of non-ToF PET scans
Abstract PurposeTo improve the quantitative accuracy and diagnostic confidence of PET images reconstructed without time-of-flight (ToF) using deep learning models trained for ToF image enhancement (DL-ToF).MethodsA total of 273 [18F]-FDG PET scans were used, including data from 6 centres equipped with GE Discovery MI ToF scanners. PET data were reconstructed using the block-sequential-regularised-expectation–maximisation (BSREM) algorithm with and without ToF. The images were then split into training (n = 208), validation (n = 15), and testing (n = 50) sets. Three DL-ToF models were trained to transform non-ToF BSREM images to their target ToF images with different levels of DL-ToF strength (low, medium, high). The models were objectively evaluated using the testing set based on standardised uptake value (SUV) in 139 identified lesions, and in normal regions of liver and lungs. Three radiologists subjectively rated the models using testing sets based on lesion detectability, diagnostic confidence, and image noise/quality.ResultsThe non-ToF, DL-ToF low, medium, and high methods resulted in − 28 ± 18, − 28 ± 19, − 8 ± 22, and 1.7 ± 24% differences (mean; SD) in the SUVmax for the lesions in testing set, compared to ToF-BSREM image. In background lung VOIs, the SUVmean differences were 7 ± 15, 0.6 ± 12, 1 ± 13, and 1 ± 11% respectively. In normal liver, SUVmean differences were 4 ± 5, 0.7 ± 4, 0.8 ± 4, and 0.1 ± 4%. Visual inspection showed that our DL-ToF improved feature sharpness and convergence towards ToF reconstruction. Blinded clinical readings of testing sets for diagnostic confidence (scale 0–5) showed that non-ToF, DL-ToF low, medium, and high, and ToF images scored 3.0, 3.0, 4.1, 3.8, and 3.5 respectively. For this set of images, DL-ToF medium therefore scored highest for diagnostic confidence.ConclusionDeep learning–based image enhancement models may provide converged ToF-equivalent image quality without ToF reconstruction. In clinical scoring DL-ToF-enhanced non-ToF images (medium and high) on average scored as high as, or higher than, ToF images. The model is generalisable and hence, could be applied to non-ToF images from BGO-based PET/CT scanners.
Improvement on mechanical and flame retardancy behaviour of bio-exfoliated graphene-filled epoxy/glass fibre composites using compression moulding approach
Bio-reduction of composite materials is the modern approach to facilitate the researchers to avoid toxic chemical exposure during reduction process. In this study, the green reduction of graphene oxide using Abutilon indicum (Tamil name: Thuthi) plant leaves extracted from various solvents were used as green filler material (0.3, 0.6 and 1 wt.%) in glass fibre epoxy composite. Compression moulding process was adopted to fabricate bio-reduced graphene oxide (BGO) filler incorporated polymer matrix composite. Tensile, flexural, toughness, impact test and fracture surface morphology analysis have been conducted over developed composite. Flame retardancy behaviour was studied based on UL94 standard. Outcome of the study revealed that Abutilon indicum act as the better reducing agent to reduce graphene oxide. XRD, FTIR results depicts the proper distortion of graphite flask. Addition of BGO in polymer matrix improvises the tensile, flexural and impact strength of matrix material up to 28%, 55% and 80%. Herein addition of 0.6 wt.% of BGO showcase better fracture toughness and flexural strength, further increment in BGO show negative effect in strength. Occurrence of delamination failure was notified in fracture surface morphology.