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result(s) for
"Conduction electrons"
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Casimir Effect Invalidates the Drude Model for Transverse Electric Evanescent Waves
by
Klimchitskaya, Galina L.
,
Mostepanenko, Vladimir M.
in
Casimir force
,
Conduction electrons
,
Dissipation
2023
We consider the Casimir pressure between two metallic plates and calculate the four contributions to it determined by the propagating and evanescent waves and by the transverse magnetic and transverse electric polarizations of the electromagnetic field. The range of interplate separations is considered where nearly the whole pressure has its origin in the electromagnetic response of conduction electrons. In the Casimir physics, this response is described either by the dissipative Drude model resulting in contradictions with the measurement data or by the experimentally consistent but dissipationless plasma model. It is shown that the total transverse magnetic contribution to the Casimir pressure due to both the propagating and evanescent waves and the transverse electric contribution due to only the propagating waves, computed by means of the Drude model, correlate well with the corresponding results obtained using the plasma model. We conclude that the disagreement between the theoretical predictions obtained using the Drude model and precision measurements of the Casimir force is not caused by the account of dissipation in itself, but arises from an incorrect description of the response of metals to the low-frequency transverse electric evanescent waves by this model. It is demonstrated that the Drude model has no supporting experimental evidence in the range of transverse electric evanescent waves, so that the above conclusion is consistent with all available information. The alternative test of the Drude model for the transverse electric evanescent waves suggested in the framework of classical electrodynamics is discussed.
Journal Article
Correct determination of electron concentration in n-GaSb by electrical measurements
by
Belov, Aleksandr G.
,
Molodtsova, Elena V.
,
Parkhomenko, Yuri N.
in
concentrates
,
concentrating
,
Conduction bands
2022
The concentrations of conduction electrons in n -GaSb at 295 and 77 K have been calculated taking into account the non-parabolic deviation of the conduction band shape. We show that at T = 295 K the concentration of heavy electrons in the L -valley of the conduction band is higher than the concentration of light electrons in the Г-valley. On the contrary, at T = 77 K the conduction electrons are mostly concentrated in the Г-valley. Hall data for tellurium doped CZ n -GaSb specimens have been reported. Analysis of experimental data for T = 295 K requires the existence of two types of electrons be taken into account (the light and the heavy ones), the concentrations of which cannot be determined. The apparent increase in the electron concentration with a decrease in the temperature from 295 to 77 K is not true. The concentration of conduction electrons at T = 77 K can be measured correctly with the Hall method.
Journal Article
Gate-tunable heavy fermions in a moiré Kondo lattice
by
Shen, Bowen
,
Han, Zhongdong
,
Kang, Kaifei
in
639/766/119/1000/1018
,
639/766/119/997
,
639/766/483/3926
2023
The Kondo lattice—a matrix of local magnetic moments coupled through spin-exchange interactions to itinerant conduction electrons—is a prototype of strongly correlated quantum matter
1
–
4
. Usually, Kondo lattices are realized in intermetallic compounds containing lanthanide or actinide
1
,
2
. The complex electronic structure and limited tunability of both the electron density and exchange interactions in these bulk materials pose considerable challenges to studying Kondo lattice physics. Here we report the realization of a synthetic Kondo lattice in AB-stacked MoTe
2
/WSe
2
moiré bilayers, in which the MoTe
2
layer is tuned to a Mott insulating state, supporting a triangular moiré lattice of local moments, and the WSe
2
layer is doped with itinerant conduction carriers. We observe heavy fermions with a large Fermi surface below the Kondo temperature. We also observe the destruction of the heavy fermions by an external magnetic field with an abrupt decrease in the Fermi surface size and quasi-particle mass. We further demonstrate widely and continuously gate-tunable Kondo temperatures through either the itinerant carrier density or the Kondo interaction. Our study opens the possibility of in situ access to the phase diagram of the Kondo lattice with exotic quantum criticalities in a single device based on semiconductor moiré materials
2
–
9
.
A Kondo lattice was realized in AB-stacked MoTe
2
/WSe
2
moiré bilayers and widely and continuously gate-tunable Kondo temperatures were demonstrated.
Journal Article
Femtosecond formation dynamics of the spin Seebeck effect revealed by terahertz spectroscopy
by
Brouwer, Piet W.
,
Ciccarelli, Chiara
,
Jaiswal, Samridh
in
140/125
,
639/624/400/561
,
639/766/119/1001
2018
Understanding the transfer of spin angular momentum is essential in modern magnetism research. A model case is the generation of magnons in magnetic insulators by heating an adjacent metal film. Here, we reveal the initial steps of this spin Seebeck effect with <27 fs time resolution using terahertz spectroscopy on bilayers of ferrimagnetic yttrium iron garnet and platinum. Upon exciting the metal with an infrared laser pulse, a spin Seebeck current
j
s
arises on the same ~100 fs time scale on which the metal electrons thermalize. This observation highlights that efficient spin transfer critically relies on carrier multiplication and is driven by conduction electrons scattering off the metal–insulator interface. Analytical modeling shows that the electrons’ dynamics are almost instantaneously imprinted onto
j
s
because their spins have a correlation time of only ~4 fs and deflect the ferrimagnetic moments without inertia. Applications in material characterization, interface probing, spin-noise spectroscopy and terahertz spin pumping emerge.
Probing spin pumping in the terahertz regime allows one to reveal its initial elementary steps. Here, the authors show that the formation of the spin Seebeck current in YIG/Pt critically relies on hot thermalized metal electrons because they impinge on the metal-insulator interface with maximum noise.
Journal Article
Artificial heavy fermions in a van der Waals heterostructure
by
Lado, Jose L.
,
Vaňo, Viliam
,
Kezilebieke, Shawulienu
in
639/766/119/544
,
639/766/119/995
,
639/766/119/997
2021
Heavy-fermion systems represent one of the paradigmatic strongly correlated states of matter
1
–
5
. They have been used as a platform for investigating exotic behaviour ranging from quantum criticality and non-Fermi liquid behaviour to unconventional topological superconductivity
4
–
12
. The heavy-fermion phenomenon arises from the exchange interaction between localized magnetic moments and conduction electrons leading to Kondo lattice physics, and represents one of the long-standing open problems in quantum materials
3
. In a Kondo lattice, the exchange interaction gives rise to a band with heavy effective mass. This intriguing phenomenology has so far been realized only in compounds containing rare-earth elements with 4
f
or 5
f
electrons
1
,
4
,
13
,
14
. Here we realize a designer van der Waals heterostructure where artificial heavy fermions emerge from the Kondo coupling between a lattice of localized magnetic moments and itinerant electrons in a 1T/1H-TaS
2
heterostructure. We study the heterostructure using scanning tunnelling microscopy and spectroscopy and show that depending on the stacking order of the monolayers, we can reveal either the localized magnetic moments and the associated Kondo effect, or the conduction electrons with a heavy-fermion hybridization gap. Our experiments realize an ultimately tunable platform for future experiments probing enhanced many-body correlations, dimensional tuning of quantum criticality and unconventional superconductivity in two-dimensional artificial heavy-fermion systems
15
–
17
.
A study demonstrates the synthesis and characterization of a two-dimensional van der Waals heterostructure hosting artificial heavy fermions, providing a tunable platform for investigations of heavy-fermion physics.
Journal Article
Distinguishing between plasmon-induced and photoexcited carriers in a device geometry
by
Nordlander, Peter
,
Manjavacas, Alejandro
,
Halas, Naomi J.
in
639/624/1075/524
,
639/766/400/1021
,
639/925/927
2015
The use of surface plasmons, charge density oscillations of conduction electrons of metallic nanostructures, to boost the efficiency of light-harvesting devices through increased light-matter interactions could drastically alter how sunlight is converted into electricity or fuels. These excitations can decay directly into energetic electron–hole pairs, useful for photocurrent generation or photocatalysis. However, the mechanisms behind plasmonic carrier generation remain poorly understood. Here we use nanowire-based hot-carrier devices on a wide-bandgap semiconductor to show that plasmonic carrier generation is proportional to internal field-intensity enhancement and occurs independently of bulk absorption. We also show that plasmon-induced hot electrons have higher energies than carriers generated by direct excitation and that reducing the barrier height allows for the collection of carriers from plasmons and direct photoexcitation. Our results provide a route to increasing the efficiency of plasmonic hot-carrier devices, which could lead to more efficient devices for converting sunlight into usable energy.
Plasmonic excitations of electrons in metallic nanostructures are promising for the enhanced conversion of light in semiconductor solar cells. Here, the authors are able to experimentally distinguish the absorption phenomena of plasmonic carrier generation and excitation of carriers by light absorption.
Journal Article
Anisotropic spin-orbit torque generation in epitaxial SrIrO₃ by symmetry design
by
Eom, C. B.
,
Anderson, T. J.
,
Nan, T.
in
Angular momentum
,
Anisotropy
,
Applied Physical Sciences
2019
Spin-orbit coupling (SOC), the interaction between the electron spin and the orbital angular momentum, can unlock rich phenomena at interfaces, in particular interconverting spin and charge currents. Conventional heavy metals have been extensively explored due to their strong SOC of conduction electrons. However, spin-orbit effects in classes of materials such as epitaxial 5d-electron transition-metal complex oxides, which also host strong SOC, remain largely unreported. In addition to strong SOC, these complex oxides can also provide the additional tuning knob of epitaxy to control the electronic structure and the engineering of spin-to-charge conversion by crystalline symmetry. Here, we demonstrate room-temperature generation of spin-orbit torque on a ferromagnet with extremely high efficiency via the spin-Hall effect in epitaxial metastable perovskite SrIrO₃. We first predict a large intrinsic spin-Hall conductivity in orthorhombic bulk SrIrO₃ arising from the Berry curvature in the electronic band structure. By manipulating the intricate interplay between SOC and crystalline symmetry, we control the spin-Hall torque ratio by engineering the tilt of the corner-sharing oxygen octahedra in perovskite SrIrO₃ through epitaxial strain. This allows the presence of an anisotropic spin-Hall effect due to a characteristic structural anisotropy in SrIrO₃ with orthorhombic symmetry. Our experimental findings demonstrate the heteroepitaxial symmetry design approach to engineer spin-orbit effects. We therefore anticipate that these epitaxial 5d transition-metal oxide thin films can be an ideal building block for low-power spintronics.
Journal Article
Observation of topological states residing at step edges of WTe2
2017
Topological states emerge at the boundary of solids as a consequence of the nontrivial topology of the bulk. Recently, theory predicts a topological edge state on single layer transition metal dichalcogenides with 1
T
’ structure. However, its existence still lacks experimental proof. Here, we report the direct observations of the topological states at the step edge of WTe
2
by spectroscopic-imaging scanning tunneling microscopy. A one-dimensional electronic state residing at the step edge of WTe
2
is observed, which exhibits remarkable robustness against edge imperfections. First principles calculations rigorously verify the edge state has a topological origin, and its topological nature is unaffected by the presence of the substrate. Our study supports the existence of topological edge states in 1
T
’-WTe
2
, which may envision in-depth study of its topological physics and device applications.
Two-dimensional topological insulators support edge conduction electrons but its realization in real materials is rare. Here, Peng et al. report the direct observation of topological states at the step edge of WTe
2
.
Journal Article
Kondo effect and spin–orbit coupling in graphene quantum dots
by
Taniguchi, Takashi
,
Knothe, Angelika
,
Garreis, Rebekka
in
639/766/119/995
,
639/766/119/997
,
639/925/927/1007
2021
The Kondo effect is a cornerstone in the study of strongly correlated fermions. The coherent exchange coupling of conduction electrons to local magnetic moments gives rise to a Kondo cloud that screens the impurity spin. Here we report on the interplay between spin–orbit interaction and the Kondo effect, that can lead to a underscreened Kondo effects in quantum dots in bilayer graphene. More generally, we introduce a different experimental platform for studying Kondo physics. In contrast to carbon nanotubes, where nanotube chirality determines spin–orbit coupling breaking the SU(4) symmetry of the electronic states relevant for the Kondo effect, we study a planar carbon material where a small spin–orbit coupling of nominally flat graphene is enhanced by zero-point out-of-plane phonons. The resulting two-electron triplet ground state in bilayer graphene dots provides a route to exploring the Kondo effect with a small spin–orbit interaction.
The Kondo effect has been observed in a variety of systems, including carbon nanotube quantum dots and graphene in the presence of impurities. Here, the authors report the observation of the Kondo effect in bilayer graphene quantum dots and study its interplay with weak spin-orbit coupling.
Journal Article
Observation of interlayer plasmon polaron in graphene/WS2 heterostructures
by
Ulstrup, Søren
,
Rotenberg, Eli
,
Koch, Roland J.
in
639/301/357/1018
,
639/766/119/544
,
639/766/119/995
2024
Harnessing electronic excitations involving coherent coupling to bosonic modes is essential for the design and control of emergent phenomena in quantum materials. In situations where charge carriers induce a lattice distortion due to the electron-phonon interaction, the conducting states get “dressed\", which leads to the formation of polaronic quasiparticles. The exploration of polaronic effects on low-energy excitations is in its infancy in two-dimensional materials. Here, we present the discovery of an interlayer plasmon polaron in heterostructures composed of graphene on top of single-layer WS
2
. By using micro-focused angle-resolved photoemission spectroscopy during in situ doping of the top graphene layer, we observe a strong quasiparticle peak accompanied by several carrier density-dependent shake-off replicas around the single-layer WS
2
conduction band minimum. Our results are explained by an effective many-body model in terms of a coupling between single-layer WS
2
conduction electrons and an interlayer plasmon mode. It is important to take into account the presence of such interlayer collective modes, as they have profound consequences for the electronic and optical properties of heterostructures that are routinely explored in many device architectures involving 2D transition metal dichalcogenides.
Here, the authors report the observation of an interlayer plasmon polaron in heterostructures composed of graphene and monolayer WS
2
. This is manifested in the ARPES spectra as a strong quasiparticle peak accompanied by several carrier density-dependent shake-off replicas around the WS
2
conduction band minimum.
Journal Article