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The NASA Cloud, Aerosol, and Monsoon Processes Philippines Experiment (CAMP²Ex) employed the NASA P-3, Stratton Park Engineering Company (SPEC) Learjet 35, and a host of satellites and surface sensors to characterize the coupling of aerosol processes, cloud physics, and atmospheric radiation within the Maritime Continent’s complex southwest monsoonal environment. Conducted in the late summer of 2019 from Luzon, Philippines, in conjunction with the Office of Naval Research Propagation of Intraseasonal Tropical Oscillations (PISTON) experiment with its R/V Sally Ride stationed in the northwestern tropical Pacific, CAMP²Ex documented diverse biomass burning, industrial and natural aerosol populations, and their interactions with small to congestus convection. The 2019 season exhibited El Niño conditions and associated drought, high biomass burning emissions, and an early monsoon transition allowing for observation of pristine to massively polluted environments as they advected through intricate diurnal mesoscale and radiative environments into the monsoonal trough. CAMP²Ex’s preliminary results indicate 1) increasing aerosol loadings tend to invigorate congestus convection in height and increase liquid water paths; 2) lidar, polarimetry, and geostationary Advanced Himawari Imager remote sensing sensors have skill in quantifying diverse aerosol and cloud properties and their interaction; and 3) high-resolution remote sensing technologies are able to greatly improve our ability to evaluate the radiation budget in complex cloud systems. Through the development of innovative informatics technologies, CAMP²Ex provides a benchmark dataset of an environment of extremes for the study of aerosol, cloud, and radiation processes as well as a crucible for the design of future observing systems.

The science of mountainous hydrology spans the atmosphere through the bedrock and inherently crosses physical and disciplinary boundaries: land–atmosphere interactions in complex terrain enhance clouds and precipitation, while watersheds retain and release water over a large range of spatial and temporal scales. Limited observations in complex terrain challenge efforts to improve predictive models of the hydrology in the face of rapid changes. The Upper Colorado River exemplifies these challenges, especially with ongoing mismatches between precipitation, snowpack, and discharge. Consequently, the U.S. Department of Energy’s (DOE) Atmospheric Radiation Measurement (ARM) user facility has deployed an observatory to the East River Watershed near Crested Butte, Colorado, between September 2021 and June 2023 to measure the main atmospheric drivers of water resources, including precipitation, clouds, winds, aerosols, radiation, temperature, and humidity. This effort, called the Surface Atmosphere Integrated Field Laboratory (SAIL), is also working in tandem with DOE-sponsored surface and subsurface hydrologists and other federal, state, and local partners. SAIL data can be benchmarks for model development by producing a wide range of observational information on precipitation and its associated processes, including those processes that impact snowpack sublimation and redistribution, aerosol direct radiative effects in the atmosphere and in the snowpack, aerosol impacts on clouds and precipitation, and processes controlling surface fluxes of energy and mass. Preliminary data from SAIL’s first year showcase the rich information content in SAIL’s many datastreams and support testing hypotheses that will ultimately improve scientific understanding and predictability of Upper Colorado River hydrology in 2023 and beyond.

Clouds play an important role in Arctic amplification. This term represents the recently observed enhanced warming of the Arctic relative to the global increase of near-surface air temperature. However, there are still important knowledge gaps regarding the interplay between Arctic clouds and aerosol particles, and surface properties, as well as turbulent and radiative fluxes that inhibit accurate model simulations of clouds in the Arctic climate system. In an attempt to resolve this so-called Arctic cloud puzzle, two comprehensive and closely coordinated field studies were conducted: the Arctic Cloud Observations Using Airborne Measurements during Polar Day (ACLOUD) aircraft campaign and the Physical Feedbacks of Arctic Boundary Layer, Sea Ice, Cloud and Aerosol (PASCAL) ice breaker expedition. Both observational studies were performed in the framework of the German Arctic Amplification: Climate Relevant Atmospheric and Surface Processes, and Feedback Mechanisms (AC) project. They took place in the vicinity of Svalbard, Norway, in May and June 2017. ACLOUD and PASCAL explored four pieces of the Arctic cloud puzzle: cloud properties, aerosol impact on clouds, atmospheric radiation, and turbulent dynamical processes. The two instrumented Polar 5 and Polar 6 aircraft; the icebreaker Research Vessel (R/V) Polarstern; an ice floe camp including an instrumented tethered balloon; and the permanent ground-based measurement station at Ny-Ålesund, Svalbard, were employed to observe Arctic low- and mid-level mixed-phase clouds and to investigate related atmospheric and surface processes. The Polar 5 aircraft served as a remote sensing observatory examining the clouds from above by downward-looking sensors; the Polar 6 aircraft operated as a flying in situ measurement laboratory sampling inside and below the clouds. Most of the collocated Polar 5/6 flights were conducted either above the R/V Polarstern or over the Ny-Ålesund station, both of which monitored the clouds from below using similar but upward-looking remote sensing techniques as the Polar 5 aircraft. Several of the flights were carried out underneath collocated satellite tracks. The paper motivates the scientific objectives of the ACLOUD/PASCAL observations and describes the measured quantities, retrieved parameters, and the applied complementary instrumentation. Furthermore, it discusses selected measurement results and poses critical research questions to be answered in future papers analyzing the data from the two field campaigns.

The light-absorbing organic aerosol (OA) commonly referred to as “brown carbon” (BrC) has attracted considerable attention in recent years because of its potential to affect atmospheric radiation balance, especially in the ultraviolet region and thus impact photochemical processes. A growing amount of data has indicated that BrC is prevalent in the atmosphere, which has motivated numerous laboratory and field studies; however, our understanding of the relationship between the chemical composition and optical properties of BrC remains limited. We conducted chamber experiments to investigate the effect of various volatile organic carbon (VOC) precursors, NOx concentrations, photolysis time, and relative humidity (RH) on the light absorption of selected secondary organic aerosols (SOA). Light absorption of chamber-generated SOA samples, especially aromatic SOA, was found to increase with NOx concentration, at moderate RH, and for the shortest photolysis aging times. The highest mass absorption coefficient (MAC) value is observed from toluene SOA products formed under high-NOx conditions at moderate RH, in which nitro-aromatics were previously identified as the major light-absorbing compounds. BrC light absorption is observed to decrease with photolysis time, correlated with a decline of the organic nitrate fraction of SOA. SOA formed from mixtures of aromatics and isoprene absorb less visible (Vis) and ultraviolet (UV) light than SOA formed from aromatic precursors alone on a mass basis. However, the mixed SOA absorption was underestimated when optical properties were predicted using a two-product SOA formation model, as done in many current climate models. Further investigation, including analysis on detailed mechanisms, are required to explain the discrepancy.

The U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) user facility recently initiated the Large-Eddy Simulation (LES) ARM Symbiotic Simulation and Observation (LASSO) activity focused on shallow convection at ARM’s Southern Great Plains (SGP) atmospheric observatory in Oklahoma. LASSO is designed to overcome an oft-shared difficulty of bridging the gap from point-based measurements to scales relevant for model parameterization development, and it provides an approach to add value to observations through modeling. LASSO is envisioned to be useful to modelers, theoreticians, and observationalists needing information relevant to cloud processes. LASSO does so by combining a suite of observations, LES inputs and outputs, diagnostics, and skill scores into data bundles that are freely available, and by simplifying user access to the data to speed scientific inquiry. The combination of relevant observations with observationally constrained LES output provides detail that gives context to the observations by showing physically consistent connections between processes based on the simulated state. A unique approach for LASSO is the generation of a library of cases for days with shallow convection combined with an ensemble of LES for each case. The library enables researchers to move beyond the single-case-study approach typical of LES research. The ensemble members are produced using a selection of different large-scale forcing sources and spatial scales. Since large-scale forcing is one of the most uncertain aspects of generating the LES, the ensemble informs users about potential uncertainty for each date and increases the probability of having an accurate forcing for each case.

Shallow convective clouds are common, occurring over many areas of the world, and are an important component in the atmospheric radiation budget. In addition to synoptic and mesoscale meteorological conditions, land–atmosphere interactions and aerosol–radiation–cloud interactions can influence the formation of shallow clouds and their properties. These processes exhibit large spatial and temporal variability and occur at the subgrid scale for all current climate, operational forecast, and cloud-system-resolving models; therefore, they must be represented by parameterizations. Uncertainties in shallow cloud parameterization predictions arise from many sources, including insufficient coincident data needed to adequately represent the coupling of cloud macrophysical and microphysical properties with inhomogeneity in the surface-layer, boundary layer, and aerosol properties. Predictions of the transition of shallow to deep convection and the onset of precipitation are also affected by errors in simulated shallow clouds. Coincident data are a key factor needed to achieve a more complete understanding of the life cycle of shallow convective clouds and to develop improved model parameterizations. To address these issues, the Holistic Interactions of Shallow Clouds, Aerosols and Land Ecosystems (HI-SCALE) campaign was conducted near the Atmospheric Radiation Measurement (ARM) Southern Great Plains site in north-central Oklahoma during the spring and summer of 2016. We describe the scientific objectives of HI-SCALE as well as the experimental approach, overall weather conditions during the campaign, and preliminary findings from the measurements. Finally, we discuss scientific gaps in our understanding of shallow clouds that can be addressed by analysis and modeling studies that use HI-SCALE data.

Accurate estimation of the wind profile, especially in the lowest few hundred meters of the atmosphere, is of great significance for the weather, climate, and renewable energy sector. Nevertheless, the Monin–Obukhov similarity theory fails above the surface layer over a heterogeneous underlying surface, causing an unreliable wind profile to be obtained from conventional extrapolation methods. To solve this problem, we propose a novel method called the PLM-RF method that combines the power-law method (PLM) with the random forest (RF) algorithm to extend wind profiles beyond the surface layer. The underlying principle is to treat the wind profile as a power-law distribution in the vertical direction, with the power-law exponent (α) determined by the PLM-RF model. First, the PLM-RF model is constructed based on the atmospheric sounding data from 119 radiosonde (RS) stations across China and in conjunction with other data such as surface wind speed, land cover type, surface roughness, friction velocity, geographical location, and meteorological parameters from June 2020 to May 2021. Afterwards, the performance of the PLM-RF, PLM, and RF methods over China is evaluated by comparing them with RS observations. Overall, the wind speed at 100 m from the PLM-RF model exhibits high consistency with RS measurements, with a determination coefficient (R2) of 0.87 and a root mean squared error (RMSE) of 0.92 m s−1. By contrast, the R2 and RMSE of wind speed results from the PLM (RF) method are 0.75 (0.83) and 1.37 (1.04) m s−1, respectively. This indicates that the estimates from the PLM-RF method are much closer to observations than those from the PLM and RF methods. Moreover, the RMSE of the wind profiles estimated by the PLM-RF model is relatively large for highlands, while it is small for plains. This result indicates that the performance of the PLM-RF model is affected by the terrain factor. Finally, the PLM-RF model is applied to three atmospheric radiation measurement sites for independent validation, and the wind profiles estimated by the PLM-RF model are found to be consistent with Doppler wind lidar observations. This confirms that the PLM-RF model has good applicability. These findings have great implications for the weather, climate, and renewable energy sector.

Ice clouds play an important role in the atmospheric radiation budget, both by reflecting shortwave radiation and by absorbing or emitting longwave radiation. These effects can modulate the cloud radiative heating (CRH) rate, which in turn influences circulation and precipitation. Ice cloud radiative properties depend on the size, shape (or habit), and complexity, including surface roughness or hollowness, of in-cloud ice crystals. To better predict ice cloud radiative effects, there has been a continuous effort to account for more ice crystal habits and complexity in current radiative transfer calculations. Here, we conduct a series of idealized single-column radiative transfer calculations to study how ice CRH responds to including ice crystal complexity. We evaluate four ice optical schemes for a range of ice cloud formation temperatures or altitudes, geometrical depths, ice water paths (IWPs), and ice crystal effective radii. In addition, we present a heating rate sensitivity matrix as a condensed visualization of the CRH response across a broad parameter space. We find that including ice complexity in cold thin clouds with high IWPs can diminish the net in-cloud heating and cloud-top cooling by 2.5 and 15 K d−1, respectively. Furthermore, while temperature-based schemes behave similarly to other schemes at warmer temperatures, they predict net CRH at the cloud bottom more than 10 K d−1 higher than size-dependent schemes at the coldest temperatures. Either weakening of CRH by ice complexity or strengthening by temperature-dependent schemes can alter anvil cloud lifetime and evolution, as well as large-scale atmospheric circulation.

This paper describes a new radiation scheme ecRad for use both in the model of the European Centre for Medium‐Range Weather Forecasts (ECMWF), and off‐line for noncommercial research. Its modular structure allows the spectral resolution, the description of cloud and aerosol optical properties, and the solver, to be changed independently. The available solvers include the Monte Carlo Independent Column Approximation (McICA), Tripleclouds, and the Speedy Algorithm for Radiative Transfer through Cloud Sides (SPARTACUS), the latter which makes ECMWF the first global model capable of representing the 3‐D radiative effects of clouds. The new implementation of the operational McICA solver produces less noise in atmospheric heating rates, and is 41% faster, which can yield indirect forecast skill improvements via calling the radiation scheme more frequently. We demonstrate how longwave scattering may be implemented for clouds but not aerosols, which is only 4% more computationally costly overall than neglecting longwave scattering and yields further modest forecast improvements. It is also shown how a sequence of radiation changes in the last few years has led to a substantial reduction in stratospheric temperature biases. Plain Language Summary Solar and thermal infrared radiation provide the energy that drives weather systems and ultimately controls the Earth's climate. Accurately simulating these energy flows is therefore a crucial part of the computer models used for weather and climate prediction. This paper describes a flexible and efficient new software package, ecRad, for computing radiation exchange. It became operational in the forecast model of the European Centre for Medium‐Range Weather Forecasts (ECMWF) in July 2017, and is 41% computationally faster than the previous package. This offers the possibility to update the radiation fields in the model simulations more frequently for the same overall computational cost, which we show in turn can improve the skill of weather forecasts. A unique feature for a radiation package of this kind is the ability to simulate radiation flows through the sides of clouds, not just through the base and top, making it well suited as a tool for research into atmospheric radiation exchange. Key Points A new radiation scheme for the ECMWF model is described that is 41% faster than the original scheme We describe how longwave scattering by clouds can be represented with only a 4% increase in computational cost, improving forecast skill A sequence of changes have reduced the long‐standing warm bias in the middle to upper stratosphere of the ECMWF model

One of the most intense air mass transformations on Earth happens when cold air flows from frozen surfaces to much warmer open water in cold-air outbreaks (CAOs), a process captured beautifully in satellite imagery. Despite the ubiquity of the CAO cloud regime over highlatitude oceans, we have a rather poor understanding of its properties, its role in energy and water cycles, and its treatment in weather and climate models. The Cold-Air Outbreaks in the Marine Boundary Layer Experiment (COMBLE) was conducted to better understand this regime and its representation in models. COMBLE aimed to examine the relations between surface fluxes, boundary layer structure, aerosol, cloud, and precipitation properties, and mesoscale circulations in marine CAOs. Processes affecting these properties largely fall in a range of scales where boundary layer processes, convection, and precipitation are tightly coupled, which makes accurate representation of the CAO cloud regime in numerical weather prediction and global climate models most challenging. COMBLE deployed an Atmospheric Radiation Measurement Mobile Facility at a coastal site in northern Scandinavia (69°N), with additional instruments on Bear Island (75°N), from December 2019 to May 2020. CAO conditions were experienced 19% (21%) of the time at the main site (on Bear Island). A comprehensive suite of continuous in situ and remote sensing observations of atmospheric conditions, clouds, precipitation, and aerosol were collected. Because of the clouds’ well-defined origin, their shallow depth, and the broad range of observed temperature and aerosol concentrations, the COMBLE dataset provides a powerful modeling testbed for improving the representation of mixed-phase cloud processes in large-eddy simulations and large-scale models.