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Observation of the spin Nernst effect
2017
The observation of the spin Nernst effect in platinum thin film is reported. This and the spin Hall effects are found to be of similar magnitude.
The observation of the spin Hall effect
1
,
2
,
3
triggered intense research on pure spin current transport
4
. With the spin Hall effect
1
,
2
,
5
,
6
, the spin Seebeck effect
7
,
8
,
9
and the spin Peltier effect
10
,
11
already observed, our picture of pure spin current transport is almost complete. The only missing piece is the spin Nernst (–Ettingshausen) effect, which so far has been discussed only on theoretical grounds
12
,
13
,
14
,
15
. Here, we report the observation of the spin Nernst effect. By applying a longitudinal temperature gradient, we generate a pure transverse spin current in a Pt thin film. For readout, we exploit the magnetization-orientation-dependent spin transfer to an adjacent yttrium iron garnet layer, converting the spin Nernst current in Pt into a controlled change of the longitudinal and transverse thermopower voltage. Our experiments show that the spin Nernst and the spin Hall effect in Pt are of comparable magnitude, but differ in sign, as corroborated by first-principles calculations.
Journal Article
Fano resonances in photonics
by
Rybin, Mikhail V.
,
Limonov, Mikhail F.
,
Poddubny, Alexander N.
in
639/624/399
,
639/624/400/1021
,
Applied and Technical Physics
2017
The importance of the Fano resonance concept is recognized across multiple fields of physics. In this Review, Fano resonance is explored in the context of optics, with particular emphasis on dielectric nanostructures and metasurfaces.
Rapid progress in photonics and nanotechnology brings many examples of resonant optical phenomena associated with the physics of Fano resonances, with applications in optical switching and sensing. For successful design of photonic devices, it is important to gain deep insight into different resonant phenomena and understand their connection. Here, we review a broad range of resonant electromagnetic effects by using two effective coupled oscillators, including the Fano resonance, electromagnetically induced transparency, Kerker and Borrmann effects, and parity–time symmetry breaking. We discuss how to introduce the Fano parameter for describing a transition between two seemingly different spectroscopic signatures associated with asymmetric Fano and symmetric Lorentzian shapes. We also review the recent results on Fano resonances in dielectric nanostructures and metasurfaces.
Journal Article
Robust axion insulator and Chern insulator phases in a two-dimensional antiferromagnetic topological insulator
2020
The intricate interplay between non-trivial topology and magnetism in two-dimensional materials can lead to the emergence of interesting phenomena such as the quantum anomalous Hall effect. Here we investigate the quantum transport of both bulk crystal and exfoliated MnBi
2
Te
4
flakes in a field-effect transistor geometry. For the six septuple-layer device tuned into the insulating regime, we observe a large longitudinal resistance and zero Hall plateau, which are characteristics of an axion insulator state. The robust axion insulator state occurs in zero magnetic field, over a wide magnetic-field range and at relatively high temperatures. Moreover, a moderate magnetic field drives a quantum phase transition from the axion insulator phase to a Chern insulator phase with zero longitudinal resistance and quantized Hall resistance
h
/
e
2
, where
h
is Planck’s constant and
e
is electron charge. Our results pave the way for using even-number septuple-layer MnBi
2
Te
4
to realize the quantized topological magnetoelectric effect and axion electrodynamics in condensed matter systems.
A large longitudinal resistance and zero Hall plateau—hallmarks of an axion insulator—are found in MnBi
2
Te
4
. Moreover, a moderate magnetic field drives a quantum phase transition to a Chern insulator phase with zero longitudinal resistance and quantized Hall resistance
h
/
e
2
.
Journal Article
Colossal mid-infrared bulk photovoltaic effect in a type-I Weyl semimetal
2019
Broadband, efficient and fast conversion of light to electricity is crucial for sensing and clean energy. The bulk photovoltaic effect (BPVE) is a second-order nonlinear optical effect that intrinsically converts light into electrical current. Here, we demonstrate a large mid-infrared BPVE in microscopic devices of the Weyl semimetal TaAs. This discovery results from combining recent developments in Weyl semimetals, focused-ion beam fabrication and theoretical works suggesting a connection between BPVE and topology. We also present a detailed symmetry analysis that allows us to separate the shift current response from photothermal effects. The magnitude and wavelength range of the assigned shift current may impact optical detectors, clean energy and topology, and demonstrate the utility of Weyl semimetals for practical applications.A large bulk photovoltaic effect is observed in the type-I Weyl semimetal TaAs, and attributed to the diverging Berry curvature of the Weyl nodes.
Journal Article
Ultrafast generation of pseudo-magnetic field for valley excitons in WSe₂ monolayers
2014
The valley pseudospin is a degree of freedom that emerges in atomically thin two-dimensional transition metal dichalcogenides (MX2). The capability to manipulate it, in analogy to the control of spin in spintronics, can open up exciting opportunities. Here, we demonstrate that an ultrafast and ultrahigh valley pseudo-magnetic field can be generated by using circularly polarized femtosecond pulses to selectively control the valley degree of freedom in monolayer MX2. Using ultrafast pump-probe spectroscopy, we observed a pure and valley-selective optical Stark effect in WSe2 monolayers from the nonresonant pump, resulting in an energy splitting of more than 10 milli-electron volts between the K and K' valley exciton transitions. Our study opens up the possibility to coherently manipulate the valley polarization for quantum information applications.
Journal Article
Spin current from sub-terahertz-generated antiferromagnetic magnons
by
Li, Junxue
,
Aldosary, Mohammed
,
Shi, Jing
in
639/766/119/1001
,
639/766/119/997
,
Antiferromagnetism
2020
Spin dynamics in antiferromagnets has much shorter timescales than in ferromagnets, offering attractive properties for potential applications in ultrafast devices
1
–
3
. However, spin-current generation via antiferromagnetic resonance and simultaneous electrical detection by the inverse spin Hall effect in heavy metals have not yet been explicitly demonstrated
4
–
6
. Here we report sub-terahertz spin pumping in heterostructures of a uniaxial antiferromagnetic Cr
2
O
3
crystal and a heavy metal (Pt or Ta in its β phase). At 0.240 terahertz, the antiferromagnetic resonance in Cr
2
O
3
occurs at about 2.7 tesla, which excites only right-handed magnons. In the spin-canting state, another resonance occurs at 10.5 tesla from the precession of induced magnetic moments. Both resonances generate pure spin currents in the heterostructures, which are detected by the heavy metal as peaks or dips in the open-circuit voltage. The pure-spin-current nature of the electrically detected signals is unambiguously confirmed by the reversal of the voltage polarity observed under two conditions: when switching the detector metal from Pt to Ta, reversing the sign of the spin Hall angle
7
–
9
, and when flipping the magnetic-field direction, reversing the magnon chirality
4
,
5
. The temperature dependence of the electrical signals at both resonances suggests that the spin current contains both coherent and incoherent magnon contributions, which is further confirmed by measurements of the spin Seebeck effect and is well described by a phenomenological theory. These findings reveal the unique characteristics of magnon excitations in antiferromagnets and their distinctive roles in spin–charge conversion in the high-frequency regime.
Pure spin currents are simultaneously generated and detected electrically through sub-terahertz magnons in the antiferromagnetic insulator Cr
2
O
3
, demonstrating the potential of magnon excitations in antiferromagnets for high-frequency spintronic devices.
Journal Article
Exciton-polariton topological insulator
2018
Topological insulators—materials that are insulating in the bulk but allow electrons to flow on their surface—are striking examples of materials in which topological invariants are manifested in robustness against perturbations such as defects and disorder
1
. Their most prominent feature is the emergence of edge states at the boundary between areas with different topological properties. The observable physical effect is unidirectional robust transport of these edge states. Topological insulators were originally observed in the integer quantum Hall effect
2
(in which conductance is quantized in a strong magnetic field) and subsequently suggested
3
–
5
and observed
6
to exist without a magnetic field, by virtue of other effects such as strong spin–orbit interaction. These were systems of correlated electrons. During the past decade, the concepts of topological physics have been introduced into other fields, including microwaves
7
,
8
, photonic systems
9
,
10
, cold atoms
11
,
12
, acoustics
13
,
14
and even mechanics
15
. Recently, topological insulators were suggested to be possible in exciton-polariton systems
16
–
18
organized as honeycomb (graphene-like) lattices, under the influence of a magnetic field. Exciton-polaritons are part-light, part-matter quasiparticles that emerge from strong coupling of quantum-well excitons and cavity photons
19
. Accordingly, the predicted topological effects differ from all those demonstrated thus far. Here we demonstrate experimentally an exciton-polariton topological insulator. Our lattice of coupled semiconductor microcavities is excited non-resonantly by a laser, and an applied magnetic field leads to the unidirectional flow of a polariton wavepacket around the edge of the array. This chiral edge mode is populated by a polariton condensation mechanism. We use scanning imaging techniques in real space and Fourier space to measure photoluminescence and thus visualize the mode as it propagates. We demonstrate that the topological edge mode goes around defects, and that its propagation direction can be reversed by inverting the applied magnetic field. Our exciton-polariton topological insulator paves the way for topological phenomena that involve light–matter interaction, amplification and the interaction of exciton-polaritons as a nonlinear many-body system.
A part-light, part-matter exciton-polariton topological insulator is created in an array of semiconductor microcavities.
Journal Article
Sound Isolation and Giant Linear Nonreciprocity in a Compact Acoustic Circulator
by
Alù, Andrea
,
Fleury, Romain
,
Sieck, Caleb F.
in
Acoustic modes
,
Acoustic resonance
,
Acoustics
2014
Acoustic isolation and nonreciprocal sound transmission are highly desirable in many practical scenarios. They may be realized with nonlinear or magneto-acoustic effects, but only at the price of high power levels and impractically large volumes. In contrast, nonreciprocal electromagnetic propagation is commonly achieved based on the Zeeman effect, or modal splitting in ferromagnetic atoms induced by a magnetic bias. Here, we introduce the acoustic analog of this phenomenon in a subwavelength meta-atom consisting of a resonant ring cavity biased by a circulating fluid. The resulting angular momentum bias splits the ring's azimuthal resonant modes, producing giant acoustic nonreciprocity in a compact device. We applied this concept to build a linear, magnetic-free circulator for airborne sound waves, observing up to 40-decibel nonreciprocal isolation at audible frequencies.
Journal Article
Piezoelectric and pyroelectric effects induced by interface polar symmetry
2020
Interfaces in heterostructures have been a key point of interest in condensed-matter physics for decades owing to a plethora of distinctive phenomena—such as rectification
1
, the photovoltaic effect
2
, the quantum Hall effect
3
and high-temperature superconductivity
4
—and their critical roles in present-day technical devices. However, the symmetry modulation at interfaces and the resultant effects have been largely overlooked. Here we show that a built-in electric field that originates from band bending at heterostructure interfaces induces polar symmetry therein that results in emergent functionalities, including piezoelectricity and pyroelectricity, even though the component materials are centrosymmetric. We study classic interfaces—namely, Schottky junctions—formed by noble metal and centrosymmetric semiconductors, including niobium-doped strontium titanium oxide crystals, niobium-doped titanium dioxide crystals, niobium-doped barium strontium titanium oxide ceramics, and silicon. The built-in electric field in the depletion region induces polar structures in the semiconductors and generates substantial piezoelectric and pyroelectric effects. In particular, the pyroelectric coefficient and figure of merit of the interface are over one order of magnitude larger than those of conventional bulk polar materials. Our study enriches the functionalities of heterostructure interfaces, offering a distinctive approach to realizing energy transduction beyond the conventional limitation imposed by intrinsic symmetry.
A built-in electric field at the interface of metals and centrosymmetric semiconductors is shown to induce polar structures in the semiconductors and generate substantial piezoelectric and pyroelectric effects.
Journal Article
Large tunable photoeffect on ion conduction in halide perovskites and implications for photodecomposition
by
Gee Yeong Kim
,
Maier, Joachim
,
Yang, Tae-Youl
in
Conduction
,
Conductivity
,
Decomposition reactions
2018
In the same way as electron transport is crucial for information technology, ion transport is a key phenomenon in the context of energy research. To be able to tune ion conduction by light would open up opportunities for a wide realm of new applications, but it has been challenging to provide clear evidence for such an effect. Here we show through various techniques, such as transference-number measurements, permeation studies, stoichiometric variations, Hall effect experiments and the use of blocking electrodes, that light excitation enhances by several orders of magnitude the ionic conductivity of methylammonium lead iodide, the archetypal metal halide photovoltaic material. We provide a rationale for this unexpected phenomenon and show that it straightforwardly leads to a hitherto unconsidered photodecomposition path of the perovskite.
Journal Article