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Water ice, abundant in the outer solar system, is volatile in the inner solar system. On the largest airless bodies of the inner solar system (Mercury, the Moon, Ceres), water can be an exospheric species but also occurs in its condensed form. Mercury hosts water ice deposits in permanently shadowed regions near its poles that act as cold traps. Water ice is also present on the Moon, where these polar deposits are of great interest in the context of future lunar exploration. The lunar surface releases either OH or H 2 O during meteoroid showers, and both of these species are generated by reaction of implanted solar wind protons with metal oxides in the regolith. A consequence of the ongoing interaction between the solar wind and the surface is a surficial hydroxyl population that has been observed on the Moon. Dwarf planet Ceres has enough gravity to have a gravitationally-bound water exosphere, and also has permanently shadowed regions near its poles, with bright ice deposits found in the most long-lived of its cold traps. Tantalizing evidence for cold trapped water ice and exospheres of molecular water has emerged, but even basic questions remain open. The relative and absolute magnitudes of sources of water on Mercury and the Moon remain largely unknown. Exospheres can transport water to cold traps, but the efficiency of this process remains uncertain. Here, the status of observations, theory, and laboratory measurements is reviewed.

In this review we discuss all the relevant solar/stellar radiation and plasma parameters and processes that act together in the formation and modification of atmospheres and exospheres that consist of surface-related minerals. Magma ocean degassed silicate atmospheres or thin gaseous envelopes from planetary building blocks, airless bodies in the inner Solar System, and close-in magmatic rocky exoplanets such as CoRot-7b, HD 219134 b and 55 Cnc e are addressed. The depletion and fractionation of elements from planetary embryos, which act as the building blocks for proto-planets are also discussed. In this context the formation processes of the Moon and Mercury are briefly reviewed. The Lunar surface modification since its origin by micrometeoroids, plasma sputtering, plasma impingement as well as chemical surface alteration and the search of particles from the early Earth’s atmosphere that were collected by the Moon on its surface are also discussed. Finally, we address important questions on what can be learned from the study of Mercury’s environment and its solar wind interaction by MESSENGER and BepiColombo in comparison with the expected observations at exo-Mercurys by future space-observatories such as the JWST or ARIEL and ground-based telescopes and instruments like SPHERE and ESPRESSO on the VLT, and vice versa.

Volatiles and refractories represent the two end-members in the volatility range of species in any surface-bounded exosphere. Volatiles include elements that do not interact strongly with the surface, such as neon (detected on the Moon) and helium (detected both on the Moon and at Mercury), but also argon, a noble gas (detected on the Moon) that surprisingly adsorbs at the cold lunar nighttime surface. Refractories include species such as calcium, magnesium, iron, and aluminum, all of which have very strong bonds with the lunar surface and thus need energetic processes to be ejected into the exosphere. Here we focus on the properties of species that have been detected in the exospheres of inner Solar System bodies, specifically the Moon and Mercury, and how they provide important information to understand source and loss processes of these exospheres, as well as their dependence on variations in external drivers.

This manuscript represents a review on progress made over the past decade concerning our understanding of meteoroid bombardment on airless solar system bodies as one of the sources of the formation of their exospheres. Specifically, observations at Mercury by MESSENGER and at the Moon by LADEE, together with progress made in dynamical models of the meteoroid environment in the inner solar system, offer new tools to explore in detail the physical phenomena involved in this complex relationship. This progress is timely given the expected results during the next decade that will be provided by new missions such as DESTINY + , BepiColombo, the Artemis program or the Lunar Gateway.

The Moon has a magmatic and thermal history that is distinct from that of the terrestrial planets 1 . Radioisotope dating of lunar samples suggests that most lunar basaltic magmatism ceased by around 2.9–2.8 billion years ago (Ga) 2 , 3 , although younger basalts between 3 Ga and 1 Ga have been suggested by crater-counting chronology, which has large uncertainties owing to the lack of returned samples for calibration 4 , 5 . Here we report a precise lead–lead age of 2,030 ± 4 million years ago for basalt clasts returned by the Chang’e-5 mission, and a 238 U/ 204 Pb ratio ( µ value) 6 of about 680 for a source that evolved through two stages of differentiation. This is the youngest crystallization age reported so far for lunar basalts by radiometric dating, extending the duration of lunar volcanism by approximately 800–900 million years. The µ value of the Chang’e-5 basalt mantle source is within the range of low-titanium and high-titanium basalts from Apollo sites ( µ value of about 300–1,000), but notably lower than those of potassium, rare-earth elements and phosphorus (KREEP) and high-aluminium basalts 7 ( µ value of about 2,600–3,700), indicating that the Chang’e-5 basalts were produced by melting of a KREEP-poor source. This age provides a pivotal calibration point for crater-counting chronology in the inner Solar System and provides insight on the volcanic and thermal history of the Moon. Basalt samples returned from the Moon by the Chang’e-5 mission are revealed to be two billion years old by radioisotopic dating, providing insight on the volcanic history of the Moon.

Water ice may be allowed to accumulate in permanently shaded regions on airless bodies in the inner solar system such as Mercury, the Moon, and Ceres [Watson K, et al. (1961) J Geophys Res 66:3033–3045]. Unlike Mercury and Ceres, direct evidence for water ice exposed at the lunar surface has remained elusive. We utilize indirect lighting in regions of permanent shadow to report the detection of diagnostic near-infrared absorption features of water ice in reflectance spectra acquired by the Moon Mineralogy Mapper [M (3)] instrument. Several thousand M (3) pixels (∼280 × 280 m) with signatures of water ice at the optical surface (depth of less than a few millimeters) are identified within 20° latitude of both poles, including locations where independent measurements have suggested that water ice may be present. Most ice locations detected in M (3) data also exhibit lunar orbiter laser altimeter reflectance values and Lyman Alpha Mapping Project instrument UV ratio values consistent with the presence of water ice and also exhibit annual maximum temperatures below 110 K. However, only ∼3.5% of cold traps exhibit ice exposures. Spectral modeling shows that some ice-bearing pixels may contain ∼30 wt % ice that is intimately mixed with dry regolith. The patchy distribution and low abundance of lunar surface-exposed water ice might be associated with the true polar wander and impact gardening. The observation of spectral features of H₂O confirms that water ice is trapped and accumulates in permanently shadowed regions of the Moon, and in some locations, it is exposed at the modern optical surface.

Dynamic models of the protoplanetary disk indicate there should be large-scale material transport in and out of the inner Solar System, but direct evidence for such transport is scarce. Here we show that the ε50Ti-ε54Cr-Δ17O systematics of large individual chondrules, which typically formed 2 to 3 My after the formation of the first solids in the Solar System, indicate certain meteorites (CV and CK chondrites) that formed in the outer Solar System accreted an assortment of both inner and outer Solar System materials, as well as material previously unidentified through the analysis of bulk meteorites. Mixing with primordial refractory components reveals a “missing reservoir” that bridges the gap between inner and outer Solar System materials. We also observe chondrules with positive ε50Ti and ε54Cr plot with a constant offset below the primitive chondrule mineral line (PCM), indicating that they are on the slope ∼1.0 in the oxygen three-isotope diagram. In contrast, chondrules with negative ε50Ti and ε54Cr increasingly deviate above from PCM line with increasing δ18O, suggesting that they are on a mixing trend with an ordinary chondrite-like isotope reservoir. Furthermore, the Δ17O-Mg# systematics of these chondrules indicate they formed in environments characterized by distinct abundances of dust and H₂O ice. We posit that large-scale outward transport of nominally inner Solar System materials most likely occurred along the midplane associated with a viscously evolving disk and that CV and CK chondrules formed in local regions of enhanced gas pressure and dust density created by the formation of Jupiter.

The bulk Earth composition contains probably less than 0.3% of water, but this trace amount of water can affect the long-term evolution of the Earth in a number of different ways. The foremost issue is the occurrence of plate tectonics, which governs almost all aspects of the Earth system, and the presence of water could either promote or hinder the operation of plate tectonics, depending on where water resides. The global water cycle, which circulates surface water into the deep mantle and back to the surface again, could thus have played a critical role in the Earth’s history. In this contribution, we first review the present-day water cycle and discuss its uncertainty as well as its secular variation. If the continental freeboard has been roughly constant since the Early Proterozoic, model results suggest long-term net water influx from the surface to the mantle, which is estimated to be 3−4.5×1014 g yr−1 on the billion years time scale. We survey geological and geochemical observations relevant to the emergence of continents above the sea level as well as the nature of Precambrian plate tectonics. The global water cycle is suggested to have been dominated by regassing, and its implications for geochemical cycles and atmospheric evolution are also discussed. This article is part of the themed issue ‘The origin, history and role of water in the evolution of the inner Solar System’.

The mass-independent calcium isotope composition of inner-Solar-System bodies is correlated with their masses and accretion ages, indicating a rapid growth for the precursors of Earth and the Moon during the protoplanetary disk’s lifetime. Like Earth, like moon Variation in the isotopic composition of material within the early inner Solar System is usually thought to reflect spatial heterogeneity in the protoplanetary disk. Martin Schiller and co-authors find that the calcium isotope composition of samples from the parent bodies of ureilite and angrite meteorites, as well as from Vesta, Mars and Earth, are correlated to the masses of their inferred parent asteroids and planets. This provides a proxy for their accretion timescales and implies a rapid 'secular' evolution of the bulk calcium isotope composition of the disk in the rocky-planet-forming region. The authors infer that this secular evolution reflects the introduction of pristine outer-Solar-System material to the thermally processed inner protoplanetary disk associated with the accretion of mass to the proto-Sun. They also conclude that the indistinguishable calcium isotope composition of the Earth and the Moon implies that the Moon-forming impact involved protoplanets that completed their accretion near the end of the disk's lifetime. Nucleosynthetic isotope variability among Solar System objects is often used to probe the genetic relationship between meteorite groups and the rocky planets (Mercury, Venus, Earth and Mars), which, in turn, may provide insights into the building blocks of the Earth–Moon system 1 , 2 , 3 , 4 , 5 . Using this approach, it has been inferred that no primitive meteorite matches the terrestrial composition and the protoplanetary disk material from which Earth and the Moon accreted is therefore largely unconstrained 6 . This conclusion, however, is based on the assumption that the observed nucleosynthetic variability of inner-Solar-System objects predominantly reflects spatial heterogeneity. Here we use the isotopic composition of the refractory element calcium to show that the nucleosynthetic variability in the inner Solar System primarily reflects a rapid change in the mass-independent calcium isotope composition of protoplanetary disk solids associated with early mass accretion to the proto-Sun. We measure the mass-independent 48 Ca/ 44 Ca ratios of samples originating from the parent bodies of ureilite and angrite meteorites, as well as from Vesta, Mars and Earth, and find that they are positively correlated with the masses of their parent asteroids and planets, which are a proxy of their accretion timescales. This correlation implies a secular evolution of the bulk calcium isotope composition of the protoplanetary disk in the terrestrial planet-forming region. Individual chondrules from ordinary chondrites formed within one million years of the collapse of the proto-Sun 7 reveal the full range of inner-Solar-System mass-independent 48 Ca/ 44 Ca ratios, indicating a rapid change in the composition of the material of the protoplanetary disk. We infer that this secular evolution reflects admixing of pristine outer-Solar-System material into the thermally processed inner protoplanetary disk associated with the accretion of mass to the proto-Sun. The identical calcium isotope composition of Earth and the Moon reported here is a prediction of our model if the Moon-forming impact involved protoplanets or precursors that completed their accretion near the end of the protoplanetary disk’s lifetime.