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In research and engineering, short laser pulses are fundamental for metrology and communication. The generation of pulses by passive mode-locking is especially desirable due to the compact setup dimensions, without the need for active modulation requiring dedicated external circuitry. However, well-established models do not cover regular self-pulsing in gain media that recover faster than the cavity round trip time. For quantum cascade lasers (QCLs), this marked a significant limitation in their operation, as they exhibit picosecond gain dynamics associated with intersubband transitions. We present a model that gives detailed insights into the pulse dynamics of the first passively mode-locked QCL that was recently demonstrated. The presence of an incoherent saturable absorber, exemplarily realized by multilayer graphene distributed along the cavity, drives the laser into a pulsed state by exhibiting a similarly fast recovery time as the gain medium. This previously unstudied state of laser operation reveals a remarkable response of the gain medium on unevenly distributed intracavity intensity. We show that in presence of strong spatial hole burning in the laser gain medium, the pulse stabilizes itself by suppressing counter-propagating light and getting shortened again at the cavity facets. Finally, we study the robustness of passive mode-locking with respect to the saturable absorber properties and identify strategies for generating even shorter pulses. The obtained results may also have implications for other nanostructured mode-locked laser sources, for example, based on quantum dots.

Recent advances in perovskite crystals have highlighted their exceptional optical properties, making them promising candidates for a wide range of photonic applications. However, the exploration of high-repetition-rate laser systems based on these materials remains underdeveloped, hindering their potential in ultrafast laser technologies and related fields such as optical communications and precision metrology. In this study, we present, for the first time, the saturable absorption characteristics of a novel organic–inorganic hybrid perovskite incorporating the heavy metal bismuth (Bi), specifically N-methylbenzothiazoleBiI (BtzBiI ). The material was integrated as a saturable absorber (SA) into a passively mode-locking erbium-doped fiber laser. By harnessing the exceptional optical nonlinearity of BtzBiI -SA, we successfully achieved stable fundamental mode-locking, harmonic mode-locking, and bound-state soliton mode-locking within a single cavity. The fundamental mode-locking yielded pulses with a duration of 844 fs and a signal-to-noise ratio of 66.15 dB. Additionally, the 142nd-order harmonic solitons attained an impressive repetition rate of 1.3202 GHz. These results represent a significant step forward in the realization of high-repetition-rate fiber lasers utilizing perovskite materials. Our findings highlight the remarkable potential of BtzBiI as a high-performance nonlinear optical material, paving the way for next-generation ultrafast photonic devices.

An optoelectronic oscillator (OEO) is a microwave photonic system that produces microwave signals with ultralow phase noise using a high-quality-factor optical energy storage element. This type of oscillator is desired in various practical applications, such as communication links, signal processing, radar, metrology, radio astronomy, and reference clock distribution. Recently, new mode control and selection methods based on Fourier domain mode-locking and parity-time symmetry have been proposed and experimentally demonstrated in OEOs, which overcomes the long-existing mode building time and mode selection problems in a traditional OEO. Due to these mode control and selection methods, continuously chirped microwave waveforms can be generated directly from the OEO cavity and single-mode operation can be achieved without the need of ultranarrowband filters, which are not possible in a traditional OEO. Integrated OEOs with a compact size and low power consumption have also been demonstrated, which are key steps toward a new generation of compact and versatile OEOs for demanding applications. We review recent progress in the field of OEOs, with particular attention to new mode control and selection methods, as well as chip-scale integration of OEOs.

It is believed that passive mode locking is virtually impossible in quantum cascade lasers (QCLs) because of too fast carrier relaxation time. Here, we revisit this possibility and theoretically show that stable mode locking and pulse durations in the few cycle regime at terahertz (THz) frequencies are possible in suitably engineered bound-to-continuum QCLs. We achieve this by utilizing a multi-section cavity geometry with alternating gain and absorber sections. The critical ingredients are the very strong coupling of the absorber to both field and environment as well as a fast absorber carrier recovery dynamics. Under these conditions, even if the gain relaxation time is several times faster than the cavity round trip time, generation of few-cycle pulses is feasible. We investigate three different approaches for ultrashort pulse generation via THz quantum cascade lasers, namely passive, hybrid and colliding pulse mode locking.

Actively mode-locked fiber ring lasers (AMLLs) with loss modulators are used to generate approximately 100ps pulses with 100MHz repetition. RF detuning around the fundamental frequency, f0, causes a loss in phase lock (unlocking) of cavity modes and partial mode locking. Multiple RF inputs are shown, theoretically, to relock and extend the locking range of cavity modes in a detuned partially mode-locked AMLL. A custom-built Yb3+-doped AMLL with f0=26MHz, and operating wavelength of 1064nm, was used to experimentally verify the theoretical predictions. Two RF sinusoidal signals with constant phase and equal amplitude resulted in an extension of the range by Xn=6.4kHz in addition to the range Rn=14.34kHz with single input for the mode n=10. An increase in locking range was also observed for higher modes. Pulsewidth reduction to approximately 205ps from about 2ns was also observed in the AMLL.

We demonstrate absorber-free passive and hybrid mode-locking at sub-GHz repetition rates, using a hybrid integrated extended cavity diode laser operating near 1550 nm. The laser is based on InP as a gain medium and a Si3N4 waveguide feedback circuit. Absorber-free Fourier domain mode-locking with ≈15 comb lines at around 0.2 mW total power is achieved with repetition rates around 500 MHz, using three highly frequency-selective micro-ring resonators that extend the on-chip cavity length to 0.6 m. To stabilize the repetition rate, hybrid mode-locking is demonstrated by weak RF modulation of the diode current. The RF injection reduces the Lorentzian linewidth component from 8.9 kHz to a detection-limited value of around 300 mHz. To measure the locking range of the repetition rate, the injected RF frequency is tuned with regard to the passive mode-locking frequency and the injected RF power is varied. The locking range increases approximately as a square-root function of the injected RF power. At 1 mW injection, a wide locking range of about 80 MHz is obtained. We also observe the laser maintaining stable mode-locking when the DC diode pump current is increased from 40 mA to 190 mA, provided that the cavity length is maintained constant with thermo-refractive tuning.

We provide a perspective review over the recent development of short-pulsed Raman fiber lasers (RFLs), which can provide laser emissions with flexible wavelengths for a variety of applications as well as an excellent platform to investigate various nonlinear pulse dynamics behaviors that cannot be captured in conventional rare-earth (RE) doped counterparts. Various pulse generation techniques have been explored in RFLs. However, the output pulse performance in terms of the pulse energy, duration and stability from short-pulsed RFLs is still inferior to their RE-doped counterparts despite significant advances made over the past few decades. Therefore, more efforts are required to improve these targets. In this review, we present a detailed overview of the short-pulsed RFLs based on different mechanisms from the principle to the experiment, including the Q-switching, gain-switching, mode-locking, synchronous pumping and other innovative techniques. In addition, Raman-induced pulse dynamics in ultrafast RFLs and RE-doped mode-locked fiber lasers (MLFLs) are briefly reviewed. Finally, a perspective outlook for the future ultrafast RFLs is provided based on their potential applications in industrial and scientific research areas.

Optically pumped semiconductor disk lasers—known as vertical-external-cavity surface-emitting lasers (VECSELs)—are promising devices for ultrashort pulse formation. For it, a “SESAM-free” approach labeled “self-mode-locking” received considerable attention in the past decade, relying solely on a chip-related nonlinear optical property which can establish adequate pulsing conditions—thereby suggesting a reduced reliance on a semiconductor saturable-absorber mirror (the SESAM) in the cavity. Self-mode-locked (SML) VECSELs with sub-ps pulse durations were reported repeatedly. This motivated investigations on a Kerr-lensing type effect acting as an artificial saturable absorber. So-called Z-scan and ultrafast beam-deflection experiments were conducted to emphasize the role of nonlinear lensing in the chip for pulse formation. Recently, in addition to allowing stable ultrashort pulsed operation, self-starting mode-locked operation gave rise to another emission regime related to frequency comb formation. While amplitude-modulated combs relate to signal peaks in time, providing a so-called pulse train, a frequency-modulated comb is understood to cause quasi continuous-wave output with its sweep of instantaneous frequency over the range of phase-locked modes. With gain-bandwidth-enhanced chips, as well as with an improved understanding of the impacts of dispersion and nonlinear lensing properties and cavity configurations on the device output, an enhanced employment of SML VECSELs is to be expected.

We show that the mode-locking region of the family of quasi-periodically forced Arnold circle maps with a topologically generic forcing function is dense. This gives a rigorous verification of certain numerical observations in [M. Ding, C. Grebogi and E. Ott. Evolution of attractors in quasiperiodically forced systems: from quasiperiodic to strange nonchaotic to chaotic. Phys. Rev. A 39(5) (1989), 2593–2598] for such forcing functions. More generally, under some general conditions on the base map, we show the density of the mode-locking property among dynamically forced maps (defined in [Z. Zhang. On topological genericity of the mode-locking phenomenon. Math. Ann. 376 (2020), 707–72]) equipped with a topology that is much stronger than the $C^0$ topology, compatible with smooth fiber maps. For quasi-periodic base maps, our result generalizes the main results in [A. Avila, J. Bochi and D. Damanik. Cantor spectrum for Schrödinger operators with potentials arising from generalized skew-shifts. Duke Math. J. 146 (2009), 253–280], [J. Wang, Q. Zhou and T. Jäger. Genericity of mode-locking for quasiperiodically forced circle maps. Adv. Math. 348 (2019), 353–377] and Zhang (2020).

The mode-locked fluoride fiber laser (MLFFL) is an exciting platform for directly generating ultrashort pulses in the mid-infrared (mid-IR). However, owing to difficulty in managing the dispersion in fluoride fiber lasers, MLFFLs are restricted to the soliton regime, hindering pulse-energy scaling. We overcame the problem of dispersion management by utilizing the huge normal dispersion generated near the absorption edge of an infrared-bandgap semiconductor and promoted MLFFL from soliton to breathing-pulse mode-locking. In the breathing-pulse regime, the accumulated nonlinear phase shift can be significantly reduced in the cavity, and the pulse-energy-limitation effect is mitigated. The breathing-pulse MLFFL directly produced a pulse energy of 9.3 nJ and pulse duration of 215 fs, with a record peak power of 43.3 kW at 2.8  μm. Our work paves the way for the pulse-energy and peak-power scaling of mid-IR fluoride fiber lasers, enabling a wide range of applications.