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2,423 result(s) for "Nuclides"
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Multiplicity of prompt fission neutron in the 239Pu(n,f) reaction and its energy dependence
Accurate multiplicities of prompt fission neutrons emitted in neutron-induced fission on a large energy range are essential for fundamental and applied nuclear physics. Measuring them to high precision for radioactive fissioning nuclides is, however, an experimental challenge. In this work, we extract the average prompt-neutron multiplicity emitted in the 239 Pu (n, f) reaction as a function of the incident-neutron energy, over the range 0.7-700 MeV. We used a novel technique, which allowed us to minimize and correct for the main sources of bias and thus achieve unprecedented precision. At low energies, our data validate, for the first time, the ENDF/B-VIII.0 nuclear data evaluation with an independent measurement and reduce the evaluated uncertainty by up to 60%. This work opens up the possibility of measuring, with high precision, prompt fission neutron multiplicities on highly radioactive nuclei relevant for energy production.
Research on the nuclear charge radius based on local interactions
Like physical quantities such as nuclear mass and electric quadrupole moment, the nuclear charge radius is one of the important physical quantities that constitute the essential properties of the atomic nucleus. This paper studies the evolution process of the nuclear charge radius. Based on the local interaction of the atomic nucleus, the original semi-empirical formula for calculating the nuclear charge radius has been improved. The accuracy and reliability of the formula are verified by combining experimental data, with the expectation of providing a reference for the accurate measurement of the nuclear charge radius of nuclides in the future.
Evaluation of covariance data in JENDL
Evaluation of covariance for JENDL was virtually started after the release of JENDL-3.2. The covariance data were obtained for 16 nuclides and compiled to the JENDL-3.2 Covariance File. At the time of the JENDL-4.0 development, covariances were much enhanced especially for actinides; covariance data were given for 99 nuclides in total. The latest version JENDL-5 includes covariance data for 105 nuclides by adding new evaluations for light nuclides and structure materials. An overview of the covariance evaluation for JENDL is presented.
Relative Atomic Solar System Abundances, Mass Fractions, and Atomic Masses of the Elements and Their Isotopes, Composition of the Solar Photosphere, and Compositions of the Major Chondritic Meteorite Groups
This brief special communications article gives data for atomic abundances and mass fractions for the elemental and isotopic solar system composition, the atomic masses of the elements and their isotopes, the composition of the solar photosphere, and the compositions of the major chondritic meteorite groups. This additional material is relevant for researchers who are interested in this Topical Collection on planetary evolution.
A kilonova as the electromagnetic counterpart to a gravitational-wave source
Observations and modelling of an optical transient counterpart to a gravitational-wave event and γ-ray burst reveal that neutron-star mergers produce gravitational waves and radioactively powered kilonovae, and are a source of heavy elements. When neutron stars collide Merging neutron stars are potential sources of gravitational waves and have long been predicted to produce jets of material as part of a low-luminosity transient known as a 'kilonova'. There is growing evidence that neutron-star mergers also give rise to short, hard gamma-ray bursts. A group of papers in this issue report observations of a transient associated with the gravitational-wave event GW170817—a signature of two neutron stars merging and a gamma-ray flash—that was detected in August 2017. The observed gamma-ray, X-ray, optical and infrared radiation signatures support the predictions of an outflow of matter from double neutron-star mergers and present a clear origin for gamma-ray bursts. Previous predictions differ over whether the jet material would combine to form light or heavy elements. These papers now show that the early part of the outflow was associated with lighter elements whereas the later observations can be explained by heavier elements, the origins of which have been uncertain. However, one paper (by Stephen Smartt and colleagues) argues that only light elements are needed for the entire event. Additionally, Eleonora Troja and colleagues report X-ray observations and radio emissions that suggest that the 'kilonova' jet was observed off-axis, which could explain why gamma-ray-burst detections are seen as dim. Gravitational waves were discovered with the detection of binary black-hole mergers 1 and they should also be detectable from lower-mass neutron-star mergers. These are predicted to eject material rich in heavy radioactive isotopes that can power an electromagnetic signal. This signal is luminous at optical and infrared wavelengths and is called a kilonova 2 , 3 , 4 , 5 . The gravitational-wave source GW170817 arose from a binary neutron-star merger in the nearby Universe with a relatively well confined sky position and distance estimate 6 . Here we report observations and physical modelling of a rapidly fading electromagnetic transient in the galaxy NGC 4993, which is spatially coincident with GW170817 and with a weak, short γ-ray burst 7 , 8 . The transient has physical parameters that broadly match the theoretical predictions of blue kilonovae from neutron-star mergers. The emitted electromagnetic radiation can be explained with an ejected mass of 0.04 ± 0.01 solar masses, with an opacity of less than 0.5 square centimetres per gram, at a velocity of 0.2 ± 0.1 times light speed. The power source is constrained to have a power-law slope of −1.2 ± 0.3, consistent with radioactive powering from r-process nuclides. (The r-process is a series of neutron capture reactions that synthesise many of the elements heavier than iron.) We identify line features in the spectra that are consistent with light r-process elements (atomic masses of 90–140). As it fades, the transient rapidly becomes red, and a higher-opacity, lanthanide-rich ejecta component may contribute to the emission. This indicates that neutron-star mergers produce gravitational waves and radioactively powered kilonovae, and are a nucleosynthetic source of the r-process elements.
Practical realization and design of three-cascade prism mass analyzer for isotopic analysis of H-He mixtures using MS-platform technology
The paper presents the construction of a mass analyzer for the analysis of hydrogen-helium mixtures based on a magnetic prism using a three-stage circuit that includes two cylindrical capacitors. The choice of an ion-optical scheme that provides a high resolution of 3300, which is necessary for the separation of all nuclides formed during the analysis of hydrogen-helium mixtures, is justified. It is shown that the innovative «MS-Platform» technology makes it possible to ensure high assembly accuracy of the elements of the prism mass analyzer ion-optical circuit, which is necessary to realize all the advantages of a prism mass spectrometer compared to sector ones.
Nuclear waste from small modular reactors
Small modular reactors (SMRs; i.e., nuclear reactors that produce < 300 MWelec each) have garnered attention because of claims of inherent safety features and reduced cost. However, remarkably few studies have analyzed the management and disposal of their nuclear waste streams. Here, we compare three distinct SMR designs to an 1,100-MWelec pressurized water reactor in terms of the energy-equivalent volume, (radio-)chemistry, decay heat, and fissile isotope composition of (notional) high-, intermediate-, and low-level waste streams. Results reveal that water-, molten salt–, and sodium-cooled SMR designs will increase the volume of nuclear waste in need of management and disposal by factors of 2 to 30. The excess waste volume is attributed to the use of neutron reflectors and/or of chemically reactive fuels and coolants in SMR designs. That said, volume is not the most important evaluation metric; rather, geologic repository performance is driven by the decay heat power and the (radio-)chemistry of spent nuclear fuel, for which SMRs provide no benefit. SMRs will not reduce the generation of geochemically mobile 129I, 99Tc, and 79Se fission products, which are important dose contributors for most repository designs. In addition, SMR spent fuel will contain relatively high concentrations of fissile nuclides, which will demand novel approaches to evaluating criticality during storage and disposal. Since waste stream properties are influenced by neutron leakage, a basic physical process that is enhanced in small reactor cores, SMRs will exacerbate the challenges of nuclear waste management and disposal.
Comparison of post-activation performance enhancement
This study aimed to compare the post-activation performance enhancement (PAPE) induced by isometric and isotonic exercise on vertical jump performance. 18 healthy trained men (25.8±2.7 years; 78.4±8.2 kg; 175.7±6.1 cm; 25.4±1.8 BMI; 126.72±10.8 kg squat 1-RM) volunteered for this study. They randomly performed two different PAPE protocols: Isotonic squats (ISOTS), which consisted of 2 sets of 3 repetitions at 75% of one-maximum repetition (1-RM); and isometric squats (ISOMS), which consisted of 2 sets of 4 seconds of submaximal (75% of 1-RM) isometric contraction at 90°-knee flexion. Countermovement jump (CMJ) height was tested at baseline and 4 minutes after each conditioning set. CMJ height significantly increased after set 1 in both PAPE protocols (ISOMS: p <0.001; ES = 0.34; ISOTS: p 0.05) were found between both isometric and isotonic exercise conditions. Despite both protocols showed similar PAPE effects on CMJ height after set 1, none of the protocols demonstrated greater efficacy in increasing subsequent performance in healthy trained men.
Inductively coupled plasma mass spectrometry
Inductively coupled plasma mass spectrometry (ICP-MS) combines plasma chemistry, which produces singly charged elemental ions, with mass spectrometric detection. Unlike other mass spectrometry ionization sources, the ICP can efficiently handle liquid, solid and gaseous samples. Nuclides of metals, metalloids and some non-metals — such as sulfur, phosphorus and halogens — can be ionized, with an ionization degree that depends on the intrinsic properties of the element and sample matrix. As a stand-alone technique, ICP-MS excels in (ultra-)trace multi-elemental analysis and isotopic analysis. Combined with chromatographic separations, molecules are assessed as elemental species, whereas laser ablation-ICP-MS enables direct sampling from solid surfaces, either in the imaging modality or for bulk analysis. Scanning-type mass analysers, such as quadrupole-based mass spectrometers and sector field mass spectrometers, dominate the field. Time-of-flight ICP mass spectrometers are considered the go-to instruments for multi-elemental analysis of microscale and nanoscale particles and single cells as discrete entities in a time-resolved manner. This Primer covers the major analytical applications of ICP-MS — multi-element, single-particle, single-cell, laser ablation, speciation and isotopic analysis — and outlines the underlying measurement strategies, challenges and example applications.Inductively coupled plasma mass spectrometry (ICP-MS) uses a plasma to ionize samples, followed by detection with mass spectrometry. This Primer discusses the major analytical variants of ICP-MS and how they can be used for trace elemental and isotopic analysis.
CENDL-3.2: The new version of Chinese general purpose evaluated nuclear data library
A new version of Chinese Evaluated Nuclear Data Library, namely CENDL-3.2, has been completed under the joint efforts of CENDL working group. This library is constructed with the general purpose to provide high-quality nuclear data for the modern nuclear science and engineering. 272 nuclides from light to heavy are covered in CENDL-3.2 in total and the data for 134 nuclides are new or updated evaluations in energy region of 10 -5 eV-20 MeV. The data of most of the key nuclides in nuclear application like U, Pu, Th, Fe et al. have been revised and improved, and various evaluation techniques have been developed to produce the nuclear data with good quality. Moreover, model dependent covariances data for main reaction cross sections are added for 70 fission product nuclides. To assess the accuracy of CENDL-3.2 in application, the data have been tested with the criticality and shielding benchmarks collected in ENDITS-1.0.