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Rapid Auger recombination represents an important challenge faced by quasi-2D perovskites, which induces resulting perovskite light-emitting diodes’ (PeLEDs) efficiency roll-off. In principle, Auger recombination rate is proportional to materials’ exciton binding energy ( E b ). Thus, Auger recombination can be suppressed by reducing the corresponding materials’ E b . Here, a polar molecule, p -fluorophenethylammonium, is employed to generate quasi-2D perovskites with reduced E b . Recombination kinetics reveal the Auger recombination rate does decrease to one-order-of magnitude lower compared to its PEA + analogues. After effective passivation, nonradiative recombination is greatly suppressed, which enables resulting films to exhibit outstanding photoluminescence quantum yields in a broad range of excitation density. We herein demonstrate the very efficient PeLEDs with a peak external quantum efficiency of 20.36%. More importantly, devices exhibit a record luminance of 82,480 cd m −2 due to the suppressed efficiency roll-off, which represent one of the brightest visible PeLEDs yet. Designing efficient perovskite light-emitting diodes remains a challenge due to the strong Auger recombination and resulting Joule heating. Here, the authors propose polarizable p -fluorophenethylammonium to generate quasi-2D perovskites with reduced binding energy developing perovskite light-emitting diodes with a peak EQE of 20.36% and a maximum luminance of 82,480 cdm -2 .

The successful implementation of spin-wave devices requires efficient modulation of spin-wave propagation. Using cobalt/nickel multilayer films, we experimentally demonstrate that nanometer-wide magnetic domain walls can be applied to manipulate the phase and magnitude of coherent spin waves in a nonvolatile manner. We further show that a spin wave can, in turn, be used to change the position of magnetic domain walls by means of the spin-transfer torque effect generated from magnon spin current. This mutual interaction between spin waves and magnetic domain walls opens up the possibility of realizing all-magnon spintronic devices, in which one spin-wave signal can be used to control others by reconfiguring magnetic domain structures.

Widespread applications of magnetic devices require an efficient means to manipulate the local magnetization. One mechanism is the electrical spin-transfer torque associated with electron-mediated spin currents; however, this suffers from substantial energy dissipation caused by Joule heating. We experimentally demonstrated an alternative approach based on magnon currents and achieved magnon-torque–induced magnetization switching in Bi2Se3/antiferromagnetic insulator NiO/ferromagnet devices at room temperature. The magnon currents carry spin angular momentum efficiently without involving moving electrons through a 25-nanometer-thick NiO layer. The magnon torque is sufficient to control the magnetization, which is comparable with previously observed electrical spin torque ratios. This research, which is relevant to the energy-efficient control of spintronic devices, will invigorate magnon-based memory and logic devices.

Spin current–a flow of electron spins without a charge current–is an ideal information carrier free from Joule heating for electronic devices. The celebrated spin Hall effect, which arises from the relativistic spin-orbit coupling, enables us to generate and detect spin currents in inorganic materials and semiconductors, taking advantage of their constituent heavy atoms. In contrast, organic materials consisting of molecules with light elements have been believed to be unsuited for spin current generation. Here we show that a class of organic antiferromagnets with checker-plate type molecular arrangements can serve as a spin current generator by applying a thermal gradient or an electric field, even with vanishing spin-orbit coupling. Our findings provide another route to create a spin current distinct from the conventional spin Hall effect and open a new field of spintronics based on organic magnets having advantages of small spin scattering and long lifetime. Spin current generation in organic materials is hindered by the light elements in the molecules. Here the authors predict a class of organic antiferromagnets with checker-plate type molecular arrangements can be spin current generator under thermal gradient or an electric field, even without spin-orbit coupling.

Electrical manipulation of skyrmions attracts considerable attention for its rich physics and promising applications. To date, such a manipulation is realized mainly via spin-polarized current based on spin-transfer torque or spin–orbital torque effect. However, this scheme is energy consuming and may produce massive Joule heating. To reduce energy dissipation and risk of heightened temperatures of skyrmion-based devices, an effective solution is to use electric field instead of current as stimulus. Here, we realize an electric-field manipulation of skyrmions in a nanostructured ferromagnetic/ferroelectrical heterostructure at room temperature via an inverse magneto-mechanical effect. Intriguingly, such a manipulation is non-volatile and exhibits a multistate feature. Numerical simulations indicate that the electric-field manipulation of skyrmions originates from strain-mediated modification of effective magnetic anisotropy and Dzyaloshinskii–Moriya interaction. Our results open a direction for constructing low-energy-dissipation, non-volatile, and multistate skyrmion-based spintronic devices. Spin-polarized current manipulation of magnetic skyrmions is energy consuming. Here, the authors achieve an electric-field manipulation of individual skyrmions in a nanostructured ferromagnetic/ferroelectrical heterostructure at room temperature via an inverse magneto-mechanical effect.

Purpose In this communication, a theoretical simulation is aimed to characterize the Darcy–Forchheimer flow of a magneto-couple stress fluid over an inclined exponentially stretching sheet. Stokes’ couple stress model is deployed to simulate non-Newtonian microstructural characteristics. Two different kinds of thermal boundary conditions, namely, the prescribed exponential order surface temperature (PEST) and prescribed exponential order heat flux, are considered in the heat transfer analysis. Joule heating (Ohmic dissipation), viscous dissipation and heat source/sink impacts are also included in the energy equation because these phenomena arise frequently in magnetic materials processing. Design/methodology/approach The governing partial differential equations are transformed into nonlinear ordinary differential equations (ODEs) by adopting suitable similar transformations. The resulting system of nonlinear ODEs is tackled numerically by using the Runge–Kutta fourth (RK4)-order numerical integration scheme based on the shooting technique. The impacts of sundry parameters on stream function, velocity and temperature profiles are viewed with the help of graphical illustrations. For engineering interests, the physical implication of the said parameters on skin friction coefficient, Nussult number and surface temperature are discussed numerically through tables. Findings As a key outcome, it is noted that the augmented Chandrasekhar number, porosity parameter and Forchhemeir parameter diminish the stream function as well as the velocity profile. The behavior of the Darcian drag force is similar to the magnetic field on fluid flow. Temperature profiles are generally upsurged with the greater magnetic field, couple stress parameter and porosity parameter, and are consistently higher for the PEST case. Practical implications The findings obtained from this analysis can be applied in magnetic material processing, metallurgy, casting, filtration of liquid metals, gas-cleaning filtration, cooling of metallic sheets, petroleum industries, geothermal operations, boundary layer resistors in aerodynamics, etc. Originality/value From the literature review, it has been found that the Darcy–Forchheimer flow of a magneto-couple stress fluid over an inclined exponentially stretching surface with heat flux conditions is still scarce. The numerical data of the present results are validated with the already existing studies under limited cases and inferred to have good concord.

It has been known for decades that the application of pulsed direct current can significantly enhance the formability of metals. However, the detailed mechanisms of this effect have been difficult to separate from simple Joule heating. Here, we study the electroplastic deformation of Ti–Al (7 at.% Al), an alloy that is uniquely suited for uncoupling this behaviour because, contrary to most metals, it has inherently lower ductility at higher temperature. We find that during mechanical deformation, electropulsing enhances cross-slip, producing a wavy dislocation morphology, and enhances twinning, which is similar to what occurs during cryogenic deformation. As a consequence, dislocations are prevented from localizing into planar slip bands that would lead to the early failure of the alloy under tension. Our results demonstrate that this macroscopic electroplastic behaviour originates from defect-level microstructural reconfiguration that cannot be rationalized by simple Joule heating. Transmission electron microscopy reveals the electroplastic effects in a Ti–Al alloy, which can be uncoupled from Joule heating effects. Electropulsing during deformation enhances wavy slip of dislocations, reconfiguring the dislocation pattern, and hence increases the ductility.

Solid-state spin sensors have the capacity to act as quantum microscopes for probing material properties and physical processes. However, so far, these tools have relied on quantum defects hosted in rigid, three-dimensional (3D) crystals such as diamond, limiting their ability to closely interface with the sample. Here we demonstrate a versatile quantum microscope using point defects embedded within a thin layer of the van der Waals material hexagonal boron nitride. To showcase the multi-modal capabilities of this platform, we assemble two different heterostructures of a van der Waals material in combination with a quantum-active boron nitride flake. We demonstrate time-resolved, simultaneous temperature and magnetic imaging near the Curie temperature of a van der Waals ferromagnet, as well as map out charge currents and Joule heating in an operating graphene device. The straightforward integration of the hexagonal boron nitride quantum sensor with other van der Waals materials will yield substantial practical benefits for the design and measurement of 2D devices.Hexagonal boron nitride is a common component of 2D heterostructures. Defects implanted in boron nitride crystals can be used to perform spatially resolved sensing of properties, including temperature, magnetism and current.

The flat bands that appear in some twisted van der Waals heterostructures provide a setting in which strong interactions between electrons lead to a variety of correlated phases1–20. In particular, heterostructures of twisted double bilayer graphene host correlated insulating states that can be tuned by both the twist angle and an external electric field11–14. Here, we report electrical transport measurements of twisted double bilayer graphene with which we examine the fundamental role of spontaneous symmetry breaking in its phase diagram. The metallic states near each of the correlated insulators exhibit abrupt drops in their resistivity as the temperature is lowered, along with associated nonlinear current–voltage characteristics. Despite qualitative similarities to superconductivity, the simultaneous reversals in the sign of the Hall coefficient point instead to spontaneous symmetry breaking as the origin of the abrupt resistivity drops, whereas Joule heating seems to underlie the nonlinear transport. Our results suggest that similar mechanisms are probably relevant across a broader class of semiconducting flat band van der Waals heterostructures.Transport measurements show that spontaneous symmetry breaking plays a crucial role in the correlated insulating and metallic states in twisted double bilayer graphene.

The advancement of laser-induced graphene (LIG) technology has streamlined the fabrications of flexible graphene devices. However, the ultrafast kinetics triggered by laser irradiation generates intrinsic amorphous characteristics, leading to high resistivity and compromised performance in electronic devices. Healing graphene defects in specific patterns is technologically challenging by conventional methods. Herein, we report the rapid rectification of LIG’s topological defects by flash Joule heating in milliseconds (referred to as F-LIG), whilst preserving its overall structure and porosity. The F-LIG exhibits a decreased I D / I G ratio from 0.84 – 0.33 and increased crystalline domain from Raman analysis, coupled with a 5-fold surge in conductivity. Pair distribution function and atomic-resolution imaging delineate a broader-range order of F-LIG with a shorter C-C bond of 1.425 Å. The improved crystallinity and conductivity of F-LIG with excellent flexibility enables its utilization in high-performance soft electronics and low-voltage disinfections. Notably, our F-LIG/polydimethylsiloxane strain sensor exhibits a gauge factor of 129.3 within 10% strain, which outperforms pristine LIG by 800%, showcasing significant potential for human-machine interfaces. Laser-induced graphene (LIG) can be obtained via a practically convenient approach, but its amorphous characteristics limit its applications. Here, the authors report a flash Joule heating strategy to improve the crystalline quality and conductivity of LIG, leading to strain sensors with enhanced sensitivity.