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In this study, a model-free  PIφ-sliding mode control ( PIφ-SMC) methodology is proposed to synchronize a specific class of chaotic fractional-order memristive neural network systems (FOMNNSs) with delays and input saturation. The fractional-order Lyapunov stability theory is used to design a two-level  PIφ-SMC which can effectively manage the inherent chaotic behavior of delayed FOMNNSs and achieve finite-time synchronization. At the outset, an initial sliding surface is introduced. Subsequently, a robust  PIφ-sliding surface is designed as a second sliding surface, based on proportional–integral (PI) rules. The finite-time asymptotic stability of both surfaces is demonstrated. The final step involves the design of a dynamic-free control law that is robust against system uncertainties, input saturations, and delays. The independence of control rules from the functions of the system is accomplished through the application of the norm-boundedness property inherent in chaotic system states. The soft actor-critic (SAC) algorithm based deep Q-Learning is utilized to optimally adjust the coefficients embedded in the two-level  PIφ-SMC controller’s structure. By maximizing a reward signal, the optimal policy is found by the deep neural network of the SAC agent. This approach ensures that the sliding motion meets the reachability condition within a finite time. The validity of the proposed protocol is subsequently demonstrated through extensive simulation results and two numerical examples.