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result(s) for
"Polarons"
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Many-body quantum dynamics and induced correlations of Bose polarons
by
Katsimiga, G C
,
Schmelcher, P
,
Koutentakis, G M
in
Bose polarons
,
correlated dynamics
,
Correlation analysis
2020
We study the ground state properties and non-equilibrium dynamics of two spinor bosonic impurities immersed in a one-dimensional bosonic gas upon applying an interspecies interaction quench. For the ground state of two non-interacting impurities we reveal signatures of attractive induced interactions in both cases of attractive or repulsive interspecies interactions, while a weak impurity-impurity repulsion forces the impurities to stay apart. Turning to the quench dynamics we inspect the time-evolution of the contrast unveiling the existence, dynamical deformation and the orthogonality catastrophe of Bose polarons. We find that for an increasing postquench repulsion the impurities reside in a superposition of two distinct two-body configurations while at strong repulsions their corresponding two-body correlation patterns show a spatially delocalized behavior evincing the involvement of higher excited states. For attractive interspecies couplings, the impurities exhibit a tendency to localize at the origin and remarkably for strong attractions they experience a mutual attraction on the two-body level that is imprinted as a density hump on the bosonic bath.
Journal Article
Repulsive Fermi and Bose Polarons in Quantum Gases
by
Levinsen, Jesper
,
Zaccanti, Matteo
,
Massignan, Pietro
in
Atoms & subatomic particles
,
Bose polarons
,
Elementary excitations
2022
Polaron quasiparticles are formed when a mobile impurity is coupled to the elementary excitations of a many-particle background. In the field of ultracold atoms, the study of the associated impurity problem has attracted a growing interest over the last fifteen years. Polaron quasiparticle properties are essential to our understanding of a variety of paradigmatic quantum many-body systems realized in ultracold atomic gases and in the solid state, from imbalanced Bose–Fermi and Fermi–Fermi mixtures to fermionic Hubbard models. In this topical review, we focus on the so-called repulsive polaron branch, which emerges as an excited many-body state in systems with underlying attractive interactions such as ultracold atomic mixtures, and is characterized by an effective repulsion between the impurity and the surrounding medium. We give a brief account of the current theoretical and experimental understanding of repulsive polaron properties, for impurities embedded in both fermionic and bosonic media, and we highlight open issues deserving future investigations.
Journal Article
Bose polarons in ultracold atoms in one dimension: beyond the Fröhlich paradigm
by
Demler, Eugene
,
Grusdt, Fabian
,
Astrakharchik, Gregory E
in
Atomic physics
,
Bose polaron
,
Bose-Einstein condensates
2017
Mobile impurity atoms immersed in Bose-Einstein condensates provide a new platform for exploring Bose polarons. Recent experimental advances in the field of ultracold atoms make it possible to realize such systems with highly tunable microscopic parameters and to explore equilibrium and dynamical properties of polarons using a rich toolbox of atomic physics. In this paper we present a detailed theoretical analysis of Bose polarons in one-dimensional systems of ultracold atoms. By combining a non-perturbative renormalization group approach with numerically exact diffusion Monte Carlo calculations we obtain not only detailed numerical results over a broad range of parameters but also qualitative understanding of different regimes of the system. We find that an accurate description of Bose polarons requires the inclusion of two-phonon scattering terms which go beyond the commonly used Fröhlich model. Furthermore we show that when the Bose gas is in the strongly interacting regime, one needs to include interactions between the phonon modes. We use several theoretical approaches to calculate the polaron energy and its effective mass. The former can be measured using radio-frequency spectroscopy and the latter can be studied experimentally using impurity oscillations in a harmonic trapping potential. We compare our theoretical results for the effective mass to the experiments by Catani et al (2012 Phys. Rev. A 85 023623). In the weak-to-intermediate coupling regimes we obtain excellent quantitative agreement between theory and experiment, without any free fitting parameter. We supplement our analysis by full dynamical simulations of polaron oscillations in a shallow trapping potential. We also use our renormalization group approach to analyze the full phase diagram and identify regions that support repulsive and attractive polarons, as well as multi-particle bound states.
Journal Article
Repulsive Fermi polarons and their induced interactions in binary mixtures of ultracold atoms
by
Katsimiga, G C
,
Schmelcher, P
,
Koutentakis, G M
in
Binary mixtures
,
correlations
,
Entanglement
2019
We explore repulsive Fermi polarons in one-dimensional harmonically trapped few-body mixtures of ultracold atoms using as a case example a 6Li-40K mixture. A characterization of these quasiparticle-like states, whose appearance is signaled in the impurity's radiofrequency spectrum, is achieved by extracting their lifetime and residua. Increasing the number of 40K impurities leads to the occurrence of both single and multiple polarons that are entangled with their environment. An interaction-dependent broadening of the spectral lines is observed suggesting the presence of induced interactions. We propose the relative distance between the impurities as an adequate measure to detect induced interactions independently of the specifics of the atomic mixture, a result that we showcase by considering also a 6Li-173Yb system. This distance is further shown to be indicative of the generation of entanglement independently of the size of the bath (6Li) and the atomic species of the impurity. The generation of entanglement and the importance of induced interactions are revealed with an emphasis on the regime of intermediate interaction strengths.
Journal Article
Many Fermi polarons at nonzero temperature
2018
An extremely polarized mixture of an ultracold Fermi gas is expected to reduce to a Fermi polaron system, which consists of a single impurity immersed in the Fermi sea of majority atoms. By developing a many-body T-matrix theory, we investigate spectral properties of the polarized mixture in experimentally relevant regimes in which the system of finite impurity concentration at nonzero temperature is concerned. We explicitly demonstrate presence of polaron physics in the polarized limit and discuss effects of many polarons in an intermediate regime in a selfconsistent manner. By analyzing the spectral function at finite impurity concentration, we extract the attractive and repulsive polaron energies. We find that a renormalization of majority atoms via an interaction with minority atoms and a thermal depletion of the impurity chemical potential are of significance to depict the many-polaron regime.
Journal Article
Dynamical formation of a magnetic polaron in a two-dimensional quantum antiferromagnet
2020
Tremendous recent progress in the quantum simulation of the Hubbard model paves the way to controllably study doped antiferromagnetic Mott insulators. Motivated by these experimental advancements, we numerically study the real-time dynamics of a single hole created in an antiferromagnet on a square lattice, as described by the t-J model. Initially, the hole spreads ballistically with a velocity proportional to the hopping matrix element. At intermediate to long times, the dimensionality as well as the spin background determine the hole dynamics. A hole created in the ground state of a two dimensional (2D) quantum antiferromagnet propagates again ballistically at long times but with a velocity proportional to the spin exchange coupling, showing the formation of a magnetic polaron. We provide an intuitive explanation of this dynamics in terms of a parton construction, which leads to a good quantitative agreement with the numerical tensor network state simulations. In the limit of infinite temperature and no spin exchange couplings, the dynamics can be approximated by a quantum random walk on a Bethe lattice with coordination number z ̃ = 4 . Adding Ising interactions corresponds to an effective disordered potential, which can dramatically slow down the hole propagation, consistent with subdiffusive dynamics. The study of the hole dynamics paves the way for understanding the microscopic constituents of this strongly correlated quantum state.
Journal Article
Evaluation of similarities and differences of LiTaO3 and LiNbO3 based on high-T-conductivity, nonlinear optical fs-spectroscopy and ab initio modeling of polaronic structures
2021
Different aspects of ferroelectric LiTaO3 (LT) such as polaronic defects, optical response and electrical conductivity are investigated by the most recent theoretical and experimental approaches. Comparing the results with the state-of-the-art knowledge of the widely studied LiNbO3 (LN), we evaluate the general assumption that there is little difference between the aforementioned properties of LT and LN. First-principles calculations reveal the existence of point defects in LT qualitatively compatible with the polaronic picture established in LN. Though, peculiar differences with respect to the individual binding energies and polaronic deformation can be revealed. Accordingly, (sub-)picosecond transient absorption measurements show pronounced differences in the kinetics in the sub-ps time domain of small polaron formation and, even more pronounced, in the long-term evolution identified with small polaron hopping. In contrast, (sub-)ps transient luminescence, attributed to the relaxation of self-trapped excitons in LN, shows very similar kinetics. Electrical conductivity measurements are performed in air as function of temperature. Up to about 600 °C they demonstrate similar temperature dependence for the two materials, from which rather comparable activation energies can be extracted. However, in the high-temperature range from about 600 °C to 920 °C both materials show noticeable differences. The results suggest that the fundamental microscopic understanding of LN can be in part transferred to LT. However, due to differences in structure, energetic landscape and temperature behavior, discrepancies between the two materials bear a striking potential for novel applications, even at high temperatures.
Journal Article
Diagrammatic Monte Carlo study of the acoustic and the Bose-Einstein condensate polaron
2015
We consider two large polaron systems that are described by a Fröhlich type of Hamiltonian, namely the Bose-Einstein condensate (BEC) polaron in the continuum and the acoustic polaron in a solid. We present ground-state energies of these two systems calculated with the Diagrammatic Monte Carlo (DiagMC) method and with a Feynman all-coupling approach. The DiagMC method evaluates up to very high order a diagrammatic series for the polaron's self-energy. The Feynman all-coupling approach is a variational method that has been used for a wide range of polaronic problems. For the acoustic and BEC polaron both methods provide remarkably similar non-renormalized ground-state energies that are obtained after introducing a finite momentum cutoff. For the renormalized ground-state energies of the BEC polaron, there are relatively large discrepancies between the DiagMC and the Feynman predictions. These differences can be attributed to the renormalization procedure for the contact interaction.
Journal Article
Quantum Dynamics of Attractive and Repulsive Polarons in a Doped MoSe2 Monolayer
by
Levinsen, Jesper
,
Taniguchi, Takashi
,
Sampson, Kevin
in
CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
,
Current carriers
,
Decay rate
2023
When mobile impurities are introduced and coupled to a Fermi sea, new quasiparticles known as Fermi polarons are formed. There are two interesting, yet drastically different regimes of the Fermi polaron problem: (i) the attractive polaron (AP) branch connected to pairing phenomena spanning the crossover from BCS superfluidity to the Bose-Einstein condensation of molecules and (ii) the repulsive branch (RP), which underlies the physics responsible for Stoner’s itinerant ferromagnetism. Here, we study Fermi polarons in two-dimensional systems, where many questions and debates regarding their nature persist. The model system we investigate is a dopedMoSe2monolayer. We find the observed AP-RP energy splitting and the quantum dynamics of attractive polarons agree with the predictions of polaron theory. As the doping density increases, the quantum dephasing of the attractive polarons remains constant, indicative of stable quasiparticles, while the repulsive polaron dephasing rate increases nearly quadratically. The dynamics of Fermi polarons are of critical importance for understanding the pairing and magnetic instabilities that lead to the formation of rich quantum phases found in a wide range of physical systems including nuclei, cold atomic gases, and solids.
Journal Article
Phonon signatures for polaron formation in an anharmonic semiconductor
2022
Mechanistic studies on lead halide perovskites (LHPs) in recent years have suggested charge carrier screening as partially responsible for long carrier diffusion lengths and lifetimes that are key to superior optoelectronic properties. These findings have led to the ferroelectric large polaron proposal, which attributes efficient charge carrier screening to the extended ordering of dipoles from symmetry-breaking unit cells that undergo local structural distortion and break inversion symmetry. It remains an open question whether this proposal applies in general to semiconductors with LHP-like anharmonic and dynamically disordered phonons. Here, we study electron-phonon coupling in Bi₂O₂Se, a semiconductor which bears resemblance to LHPs in ionic bonding, spin-orbit coupling, band transport with long carrier diffusion lengths and lifetimes, and phonon disorder as revealed by temperature-dependent Raman spectroscopy. Using coherent phonon spectroscopy, we show the strong coupling of an anharmonic phonon mode at 1.50 THz to photo-excited charge carriers, while the Raman excitation of this mode is symmetry-forbidden in the ground-state. Density functional theory calculations show that this mode, originating from the A1g phonon of out-of-plane Bi/Se motion, gains oscillator strength from symmetry-lowering in polaron formation. Specifically, lattice distortion upon ultrafast charge localization results in extended ordering of symmetry-breaking unit cells and a planar polaron wavefunction, namely a two-dimensional polaron in a three-dimensional lattice. This study provides experimental and theoretical insights into charge interaction with anharmonic phonons in Bi₂O₂Se and suggests ferroelectric polaron formation may be a general principle for efficient charge carrier screening and for defect-tolerant semiconductors.
Journal Article