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The mandate of the Task Force Hemispheric Transport of Air Pollution (TF HTAP) under the Convention on Long-Range Transboundary Air Pollution (CLRTAP) is to improve the scientific understanding of the intercontinental air pollution transport, to quantify impacts on human health, vegetation and climate, to identify emission mitigation options across the regions of the Northern Hemisphere, and to guide future policies on these aspects. The harmonization and improvement of regional emission inventories is imperative to obtain consolidated estimates on the formation of global-scale air pollution. An emissions data set has been constructed using regional emission grid maps (annual and monthly) for SO2, NOx, CO, NMVOC, NH3, PM10, PM2.5, BC and OC for the years 2008 and 2010, with the purpose of providing consistent information to global and regional scale modelling efforts. This compilation of different regional gridded inventories – including that of the Environmental Protection Agency (EPA) for USA, the EPA and Environment Canada (for Canada), the European Monitoring and Evaluation Programme (EMEP) and Netherlands Organisation for Applied Scientific Research (TNO) for Europe, and the Model Inter-comparison Study for Asia (MICS-Asia III) for China, India and other Asian countries – was gap-filled with the emission grid maps of the Emissions Database for Global Atmospheric Research (EDGARv4.3) for the rest of the world (mainly South America, Africa, Russia and Oceania). Emissions from seven main categories of human activities (power, industry, residential, agriculture, ground transport, aviation and shipping) were estimated and spatially distributed on a common grid of 0.1° × 0.1° longitude-latitude, to yield monthly, global, sector-specific grid maps for each substance and year. The HTAP_v2.2 air pollutant grid maps are considered to combine latest available regional information within a complete global data set. The disaggregation by sectors, high spatial and temporal resolution and detailed information on the data sources and references used will provide the user the required transparency. Because HTAP_v2.2 contains primarily official and/or widely used regional emission grid maps, it can be recommended as a global baseline emission inventory, which is regionally accepted as a reference and from which different scenarios assessing emission reduction policies at a global scale could start. An analysis of country-specific implied emission factors shows a large difference between industrialised countries and developing countries for acidifying gaseous air pollutant emissions (SO2 and NOx) from the energy and industry sectors. This is not observed for the particulate matter emissions (PM10, PM2.5), which show large differences between countries in the residential sector instead. The per capita emissions of all world countries, classified from low to high income, reveal an increase in level and in variation for gaseous acidifying pollutants, but not for aerosols. For aerosols, an opposite trend is apparent with higher per capita emissions of particulate matter for low income countries.

Volatile chemical products (VCPs) are commonly used consumer and industrial items that are an important source of anthropogenic emissions. Organic compounds from VCPs evaporate on atmospherically relevant timescales and include many species that are secondary organic aerosol (SOA) precursors. However, the chemistry leading to SOA, particularly that of intermediate-volatility organic compounds (IVOCs), has not been fully represented in regional-scale models such as the Community Multiscale Air Quality (CMAQ) model, which tend to underpredict SOA concentrations in urban areas. Here we develop a model to represent SOA formation from VCP emissions. The model incorporates a new VCP emissions inventory and employs three new classes of emissions: siloxanes, oxygenated IVOCs, and nonoxygenated IVOCs. VCPs are estimated to produce 1.67 µg m−3 of noontime SOA, doubling the current model predictions and reducing the SOA mass concentration bias from −75 % to −58 % when compared to observations in Los Angeles in 2010. While oxygenated and nonoxygenated intermediate-volatility VCP species are emitted in similar quantities, SOA formation is dominated by the nonoxygenated IVOCs. Formaldehyde and SOA show similar relationships to temperature and bias signatures, indicating common sources and/or chemistry. This work suggests that VCPs contribute up to half of anthropogenic SOA in Los Angeles and models must better represent SOA precursors from VCPs to predict the urban enhancement of SOA.

It is widely accepted that future environmental changes will affect rainfall-induced shallow slides in high-mountain areas. In this study, the Val d’Aran region located in the Central Pyrenees was selected to analyze and quantify the impacts of land use and land cover (LULC) and climate changes on regional landslides susceptibility. We analyzed 26 climate models of the EURO-CORDEX database focussing on the future rainfall conditions. The IDRISI TerrSet software suite was used to create the future LULC maps. These two inputs were analyzed individually and in a combined way defining 20 different scenarios. All these scenarios were incorporated in a physically based stability model to compute landslides susceptibility maps. The results showed that both environmental conditions will considerably change in the future. The daily rainfall will increase between 14 and 26% assuming a return period of 100 years. This intensification of precipitation will produce an overall decrease of the stability condition in the study area. Regarding the LULC prediction, the forest area will significantly increase, while in particular grassland, but also shrubs decrease. As a consequence, the overall stability condition improves, because the root strength is higher in forest than in grassland and shrubs. When we analyzed the combined impacts, the results showed that the positive effect of LULC changes is larger than the negative influence of rainfall changes. Hence, when combining the two aspects in the future scenarios, the stability condition in the study area will improve.

Continental- to global-scale hydrologic and land surface models increasingly include representations of the groundwater system. Such large-scale models are essential for examining, communicating, and understanding the dynamic interactions between the Earth system above and below the land surface as well as the opportunities and limits of groundwater resources. We argue that both large-scale and regional-scale groundwater models have utility, strengths, and limitations, so continued modeling at both scales is essential and mutually beneficial. A crucial quest is how to evaluate the realism, capabilities, and performance of large-scale groundwater models given their modeling purpose of addressing large-scale science or sustainability questions as well as limitations in data availability and commensurability. Evaluation should identify if, when, or where large-scale models achieve their purpose or where opportunities for improvements exist so that such models better achieve their purpose. We suggest that reproducing the spatiotemporal details of regional-scale models and matching local data are not relevant goals. Instead, it is important to decide on reasonable model expectations regarding when a large-scale model is performing “well enough” in the context of its specific purpose. The decision of reasonable expectations is necessarily subjective even if the evaluation criteria are quantitative. Our objective is to provide recommendations for improving the evaluation of groundwater representation in continental- to global-scale models. We describe current modeling strategies and evaluation practices, and we subsequently discuss the value of three evaluation strategies: (1) comparing model outputs with available observations of groundwater levels or other state or flux variables (observation-based evaluation), (2) comparing several models with each other with or without reference to actual observations (model-based evaluation), and (3) comparing model behavior with expert expectations of hydrologic behaviors in particular regions or at particular times (expert-based evaluation). Based on evolving practices in model evaluation as well as innovations in observations, machine learning, and expert elicitation, we argue that combining observation-, model-, and expert-based model evaluation approaches, while accounting for commensurability issues, may significantly improve the realism of groundwater representation in large-scale models, thus advancing our ability for quantification, understanding, and prediction of crucial Earth science and sustainability problems. We encourage greater community-level communication and cooperation on this quest, including among global hydrology and land surface modelers, local to regional hydrogeologists, and hydrologists focused on model development and evaluation.

In climate and weather models, the quantitative description of aerosol and cloud processes relies on simplified assumptions. This contributes major uncertainties to the prediction of global and regional climate change. Therefore, models need good parameterizations for heterogeneous ice nucleation by atmospheric aerosols. Here the authors present a new parameterization of immersion freezing on desert dust particles derived from a large number of experiments carried out at the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) cloud chamber facility. The parameterization is valid in the temperature range between −12° and −36°C at or above water saturation and can be used in atmospheric models that include information about the dust surface area. The new parameterization was applied to calculate distribution maps of ice nuclei during a Saharan dust event based on model results from the regional-scale model Consortium for Small-Scale Modelling–Aerosols and Reactive Trace Gases (COSMO-ART). The results were then compared to measurements at the Taunus Observatory on Mount Kleiner Feldberg, Germany, and to three other parameterizations applied to the dust outbreak. The aerosol number concentration and surface area from the COSMO-ART model simulation were taken as input to different parameterizations. Although the surface area from the model agreed well with aerosol measurements during the dust event at Kleiner Feldberg, the ice nuclei (IN) number concentration calculated from the new surface-area-based parameterization was about a factor of 13 less than IN measurements during the same event. Systematic differences of more than a factor of 10 in the IN number concentration were also found among the different parameterizations. Uncertainties in the modeled and measured parameters probably both contribute to this discrepancy and should be addressed in future studies.

We present the collective evaluation of the regional-scale models that took part in the fourth edition of the Air Quality Model Evaluation International Initiative (AQMEII). The activity consists of the evaluation and intercomparison of regional-scale air quality models run over North American (NA) and European (EU) domains for 2016 (NA) and 2010 (EU). The focus of the paper is ozone dry deposition. Dry deposition is among the most important processes of removal of chemical compounds from the atmosphere and an important contributor to the overall chemical budget of the latter. Furthermore ozone dry deposition is very important as it can be severely detrimental to vegetation physiology. The collective evaluation begins with an operational evaluation, namely a direct comparison of model-simulated predictions with monitoring data aiming at assessing model performance (Dennis et al., 2010). Following the AQMEII protocol and Dennis et al. (2010), we also perform a probabilistic evaluation in the form of ensemble analyses and an introductory diagnostic evaluation. The latter analyzes the role of dry deposition in comparison with dynamic and radiative processes and land use/land cover (LULC) types in determining surface ozone variability. Important differences are found across dry deposition results when the same LULC is considered. Furthermore, we found that models use very different LULC masks, thus introducing an additional level of diversity in the model results. The study stresses that, as for other kinds of prior and problem-defining information (emissions, topography, or land–water masks), the choice of LULC mask should not be at modeler discretion. Furthermore, LULC should be considered as a variable to be evaluated in any future model intercomparison, unless set as common input information. The differences in LULC selection can have a substantial impact on model results, making the task of evaluating dry deposition modules across different regional-scale models very difficult.

The fourth phase of the Air Quality Model Evaluation International Initiative (AQMEII4) is conducting a diagnostic intercomparison and evaluation of deposition simulated by regional-scale air quality models over North America and Europe. In this study, we analyze annual AQMEII4 simulations performed with the Community Multiscale Air Quality Model (CMAQ) version 5.3.1 over North America. These simulations were configured with both the M3Dry and Surface Tiled Aerosol and Gas Exchange (STAGE) dry deposition schemes available in CMAQ. A comparison of observed and modeled concentrations and wet deposition fluxes shows that the AQMEII4 CMAQ simulations perform similarly to other contemporary regional-scale modeling studies. During summer, M3Dry has higher ozone (O3) deposition velocities (Vd) and lower mixing ratios than STAGE for much of the eastern US, while the reverse is the case over eastern Canada and along the US West Coast. In contrast, during winter STAGE has higher O3 Vd and lower mixing ratios than M3Dry over most of the southern half of the modeling domain, while the reverse is the case for much of the northern US and southern Canada. Analysis of the diagnostic variables defined for the AQMEII4 project, i.e., grid-scale and land-use-specific effective conductances and deposition fluxes for the major dry deposition pathways, reveals generally higher summertime stomatal and wintertime cuticular grid-scale effective conductances for M3Dry and generally higher soil grid-scale effective conductances (for both vegetated and bare soil) for STAGE in both summer and winter. On a domain-wide basis, the stomatal grid-scale effective conductances account for about half of the total O3 Vd during daytime hours in summer for both schemes. Employing land-use-specific diagnostics, results show that daytime Vd varies by a factor of 2 between land use (LU) categories. Furthermore, M3Dry vs. STAGE differences are most pronounced for the stomatal and vegetated soil pathway for the forest LU categories, with M3Dry estimating larger effective conductances for the stomatal pathway and STAGE estimating larger effective conductances for the vegetated soil pathway for these LU categories. Annual domain total O3 deposition fluxes differ only slightly between M3Dry (74.4 Tg yr−1) and STAGE (76.2 Tg yr−1), but pathway-specific fluxes to individual LU types can vary more substantially on both annual and seasonal scales, which would affect estimates of O3 damage to sensitive vegetation. A comparison of two simulations differing only in their LU classification scheme shows that the differences in LU cause seasonal mean O3 mixing ratio differences on the order of 1 ppb across large portions of the domain, with the differences generally being largest during summer and in areas characterized by the largest differences in the fractional coverages of the forest, planted and cultivated, and grassland LU categories. These differences are generally smaller than the M3Dry vs. STAGE differences outside the summer season but have a similar magnitude during summer. Results indicate that the deposition impacts of LU differences are caused by differences in the fractional coverages and spatial distributions of different LU categories and the characterization of these categories through variables like surface roughness and vegetation fraction in lookup tables used in the land surface model and deposition schemes. Overall, the analyses and results presented in this study illustrate how the diagnostic grid-scale and LU-specific dry deposition variables adopted for AQMEII4 can provide insights into similarities and differences between the CMAQ M3Dry and STAGE dry deposition schemes that affect simulated pollutant budgets and ecosystem impacts from atmospheric pollution.

Currently, about 12 %–13 % of High Mountain Asia’s glacier area is debris-covered, which alters its surface mass balance. However, in regional-scale modelling approaches, debris-covered glaciers are typically treated as clean-ice glaciers, leading to a bias when modelling their future evolution. Here, we present a new approach for modelling debris area and thickness evolution, applicable from single glaciers to the global scale. We derive a parameterization and implement it as a module into the Global Glacier Evolution Model (GloGEMflow), a combined mass-balance ice-flow model. The module is initialized with both glacier-specific observations of the debris' spatial distribution and estimates of debris thickness. These data sets account for the fact that debris can either enhance or reduce surface melt depending on thickness. Our model approach also enables representing the spatiotemporal evolution of debris extent and thickness. We calibrate and evaluate the module on a selected subset of glaciers and apply GloGEMflow using different climate scenarios to project the future evolution of all glaciers in High Mountain Asia until 2100. Explicitly accounting for debris cover has only a minor effect on the projected mass loss, which is in line with previous projections. Despite this small effect, we argue that the improved process representation is of added value when aiming at capturing intra-glacier scales, i.e. spatial mass-balance distribution. Depending on the climate scenario, the mean debris-cover fraction is expected to increase, while mean debris thickness is projected to show only minor changes, although large local thickening is expected. To isolate the influence of explicitly accounting for supraglacial debris cover, we re-compute glacier evolution without the debris-cover module. We show that glacier geometry, area, volume, and flow velocity evolve differently, especially at the level of individual glaciers. This highlights the importance of accounting for debris cover and its spatiotemporal evolution when projecting future glacier changes.

An intercomparison of climate change impacts projected by nine regional-scale hydrological models for 12 large river basins on all continents was performed, and sources of uncertainty were quantified in the framework of the ISIMIP project. The models ECOMAG, HBV, HYMOD, HYPE, mHM, SWAT, SWIM, VIC and WaterGAP3 were applied in the following basins: Rhine and Tagus in Europe, Niger and Blue Nile in Africa, Ganges, Lena, Upper Yellow and Upper Yangtze in Asia, Upper Mississippi, MacKenzie and Upper Amazon in America, and Darling in Australia. The model calibration and validation was done using WATCH climate data for the period 1971-2000. The results, evaluated with 14 criteria, are mostly satisfactory, except for the low flow. Climate change impacts were analyzed using projections from five global climate models under four representative concentration pathways. Trends in the period 2070-2099 in relation to the reference period 1975-2004 were evaluated for three variables: the long-term mean annual flow and high and low flow percentiles Q10 and Q90, as well as for flows in three months high- and low-flow periods denoted as HF and LF. For three river basins: the Lena, MacKenzie and Tagus strong trends in all five variables were found (except for Q10 in the MacKenzie); trends with moderate certainty for three to five variables were confirmed for the Rhine, Ganges and Upper Mississippi; and increases in HF and LF were found for the Upper Amazon, Upper Yangtze and Upper Yellow. The analysis of projected streamflow seasonality demonstrated increasing streamflow volumes during the high-flow period in four basins influenced by monsoonal precipitation (Ganges, Upper Amazon, Upper Yangtze and Upper Yellow), an amplification of the snowmelt flood peaks in the Lena and MacKenzie, and a substantial decrease of discharge in the Tagus (all months). The overall average fractions of uncertainty for the annual mean flow projections in the multi-model ensemble applied for all basins were 57% for GCMs, 27% for RCPs, and 16% for hydrological models.

This study features a cohesive modelling approach of human-caused wildfire ignitions applied to a set of representative regions in terms of fire activity across Europe (pilot sites, PS). Our main goal was to develop a common approach to model human-caused ignition probability at a fine-grained spatial resolution (100 m) and identify the main drivers of ignitions. Specifically, we (i) ascertain which factors influence ignitions in each PS; (ii) deliver a spatial-explicit representation of ignition probability, and (iii) provide a framework for comparison with regional-scale models among PS. To do so, we calibrated Random Forest models from historical fire records compiled by local fire agencies, and geospatial layers of land cover, accessibility, population density and dead fine-fuel moisture content (DFMC). Models were built individually for each PS, comparing them with a full model constructed from all PS. Furthermore, special attention was given to the effect of spatial autocorrelation in model performance. All models achieved sufficient predictive performance (Areas Under the Receiver Operating Characteristic Curve (AUCs) from 0.70 to 0.89). For all PS models, the yearly anomaly in DFMC was the most influential variable. Among human-related factors, distance to the Wildland Urban Interface emerged as the most relevant variable, followed by proximity to roads, population density, and the fraction of wildland coverage. The performance of the full model achieved an AUC value of 0.81, with mean DFMC and anomaly being the main ignition factors, modulated by distance to roads and population density. The local performance of the full model dropped by 0.10 for AUC in both Southern Sweden and Attica (Greece) regions. The wildfire occurrence models developed in this study are essential for understanding wildfire ignition hazard and may help implement integrated wildfire risk management strategies and mitigation policies in fire-prone EU landscapes.