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"TK9001-9401"
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Feasibility Study on Production of High-Purity Rhenium-185 by Nuclear Transmutation of Natural Tantalum
2023
Rhenium-186 (Re-186) has attracted attention as a medical isotope. The feasibility of producing Re-185, the raw material for Re-186, using a fast reactor was evaluated using a continuous energy Monte Carlo code. The irradiation of natural tantalum (Ta) in the fast reactor can produce Re-185 with an isotopic purity of 99%. A two-step irradiation process with different moderators was found to improve the production rate of Re-185. Specifically, this can be achieved by using zirconium hydride (ZrH1.7) as a moderator in the first transmutation process from natural Ta to tungsten (W), and then zirconium deuteride (ZrD1.7) as a moderator in the second transmutation process from W to Re-185. Due to the two-step irradiation, the production rate of Re-185 from Ta can be increased up to a maximum of 470 times compared with irradiation without a moderator, and 2.3 g of Re-185 can be obtained from 1571 g of Ta in 1 year of irradiation. The proposed isotope production method is a new method that is different from the conventional electromagnetic enrichment process.
Journal Article
Core and safety design for France–Japan common concept on sodium-cooled fast reactor
by
Carluec, Bernard
,
Takano, Kazuya
,
Perrin, Benoit
in
[PHYS]Physics [physics]
,
Dispersion hardening steels
,
Heat
2022
France (CEA and FRAMATOME) and Japan (JAEA, MFBR, and MHI) teams have carried out collaborative works to have common technical views regarding a sodium-cooled fast reactor (SFR) concept. This paper mainly describes the capabilities of ASTRID 600 to demonstrate SFR technologies of both countries. Japan has studied the feasibility of an enhanced high burnup low-void effect (CFV) core and fuel using oxide dispersion-strengthened steel cladding in ASTRID 600, considering Japan’s target for core performance. The neutronics design of the core has satisfied most required design targets and conditions. Regarding passive shutdown capabilities, Japan team has performed a preliminary numerical analysis for ASTRID 600 using a complementary safety device (CSD), called a self-actuated shutdown system (SASS), one of the safest approaches in Japan. Japan’s team used the SASS in place of the hydraulically suspended absorber rod, called RBH, one of the safest approaches of France, to investigate the potential of the SASS as a design measure common to the countries. The preliminary analysis has shown that the SASS can satisfy the countries’ main requirements. This study has also revealed that the mitigation measures of ASTRID 600 against a severe accident are promising to achieve in-vessel retention for both countries.
Journal Article
Machine-Learning-Based Composition Analysis of the Stability of V–Cr–Ti Alloys
2023
Machine learning methods allow the prediction of material properties, potentially using only the elemental composition of a molecule or compound, without the knowledge of molecular or crystalline structures. Herein, a composition-based machine learning prediction of the material properties of V–Cr–Ti alloys is demonstrated. Our machine-learning-based prediction of the stability of the V–Cr–Ti alloys is qualitatively consistent with the composition-dependent experimental data of the ductile–brittle transition temperature and swelling. Furthermore, our computational results suggest the existence of a composition region, Cr+Ti ~ 60 wt.%, at a significantly low ductile–brittle transition temperature. This outcome contrasts with a reportedly low Cr+Ti content of less than 10 wt.% in conventional V–Cr–Ti alloys. Machine-learning-based numerical stability prediction is useful for the design and analysis of metal alloys, particularly for multicomponent alloys such as high-entropy alloys, to develop materials for nuclear fusion reactors.
Journal Article
Plant system study of France–Japan common concept on Sodium-cooled Fast Reactor
by
Ando, Masato
,
Carluec, Bernard
,
Oyama, Kazuhiro
in
[PHYS]Physics [physics]
,
Boilers
,
Chemical reactions
2022
This paper provides an overview of plant system studies to establish a common technical view for Sodium-cooled Fast Reactor (SFR) concept (the common SFR concept) between France and Japan based on ASTRID 600 and the new concept with downsized output (ASTRID150). One of important issues on a reactor structure design is to enhance seismic resistance to be tolerable against strong earthquake such that postulated in Japan. A concept of High Frequency Design (HFD) is shared, in which the natural frequency of the reactor structure should be higher than that of peak acceleration of vertical floor seismic response with a horizontal seismic isolation system. The design options related to HFD have been examined and design recommendations are established. ASTRID 600 adopted a gas power conversion system to strictly eliminate the chemical reaction risks due to the proximity of sodium and water in the steam generator units. On the other hand, a steam generator (SG) is thought to be a concept with high technical readiness level and is a reference option in Japan and a backup option in France. Then, design comparison of the SG with single-walled helical coil tubes was mainly conducted in this study from the viewpoint of safety and so on. A common concept of a decay heat removal system is discussed to achieve practical elimination of loss of decay heat removal function. A fuel handling system studies are performed to eliminate and ex-vessel storage of spent fuels in sodium to reduce a construction cost. An adequate confinement system is investigated to achieve practical mitigation of large radiological release to the environment even under the condition of core destructive accident.
Journal Article
France–Japan synthesis concept on sodium-cooled fast reactor review of a joint collaborative work
by
Christophe Venard
,
Yumi Yamada
,
Denis Verrier
in
[PHYS]Physics [physics]
,
Agreements
,
Collaboration
2021
In the frame of the France-Japan agreement on nuclear collaboration, a bilateral collaboration agreement on nuclear energy was signed on March 21st, 2017, including a topic dedicated to Sodium-cooled Fast Reactor (SFR). This agreement has set the framework to start a bilateral discussion on a joint view of an SFR concept. France (CEA and FRAMATOME) and Japan (JAEA, MHI and MFBR) have carried out these studies from 2017 to 2019. Based on the beginning of the basic design phase of ASTRID project − ASTRID − 600 MWe (ASTRID for Advanced Sodium Technological Reactor for Industrial Demonstration), the two countries performed a common work to examine ways to develop a feasible common design concept, which could be realized both in France and in Japan. The subject was then extended and extrapolated with the ASTRID − 150 MWe data (reduced power reactor and enhanced experimental capabilities) in a second phase of this study. France and Japan first focused on design requirements. Common requirements were identified, as well as differences in the safety approach and the structural design requirements, according to national standards and respective site conditions, in particular considering seismic hazards. The teams developed common Top-Level design Requirements (TLRs) to allow common specification data, then joint design. This collaborative work was carried out through the implementation of twelve France-Japan Working Groups, working jointly. This paper is providing a review of this joint synthesis on Sodium Fast Reactor design concept. It is summarizing the context and objectives, then the definition and approaches of the Top Level Requirements. This paper is then dealing with the major design features: the core design and their related safety aspects, and the nuclear island design. Thus, this paper is providing a comprehensive review of this joint work gathering French and Japan nuclear design teams during two full years.
Journal Article
NMB4.0: development of integrated nuclear fuel cycle simulator from the front to back-end
2021
Nuclear Material Balance code version 4.0 (NMB4.0) has been developed through collaborative R&D between TokyoTech&JAEA. Conventional nuclear fuel cycle simulation codes mainly analyze actinides and are specialized for front-end mass balance analysis. However, quantitative back-end simulation has recently become necessary for considering R&D strategies and sustainable nuclear energy utilization. Therefore, NMB4.0 was developed to realize the integrated nuclear fuel cycle simulation from front- to back-end. There are three technical features in NMB4.0: 179 nuclides are tracked, more than any other code, throughout the nuclear fuel cycle; the Okamura explicit method is implemented, which contributes to reducing the numerical cost while maintaining the accuracy of depletion calculations on nuclides with a shorter half-life; and flexibility of back-end simulation is achieved. The main objective of this paper is to show the newly developed functions, made for integrated back-end simulation, and verify NMB4.0 through a benchmark study to show the computational performance.
Journal Article
Thermal decomposition analysis of simulated high-level liquid waste in cold-cap
2016
The cold cap floating on top of the molten glass pool in liquid fed joule-heated ceramic melter plays an important role for operation of the vitrification process. A series of such phenomena as evaporation, melting and thermal decomposition of HLLW (high-level liquid waste) takes place within the cold-cap. An understanding of the varied thermal decomposition behavior of various nitrates constituting HLLW is necessary to elucidate a series of phenomena occurring within the cold-cap. In this study, reaction rates of the thermal decomposition reaction of 13 kinds of nitrates, which are main constituents of simulated HLLW (sHLLW), were investigated using thermogravimetrical instrument in a range of room temperature to 1000 °C. The reaction rates of the thermal decompositions of 13 kinds of nitrates were depicted according to composition ratio (wt%) of each nitrate in sHLLW. It was found that the thermal decomposition of sHLLW could be predicted by the reaction rates and reaction temperatures of individual nitrates. The thermal decomposition of sHLLW with borosilicate glass system was also investigated. The above mentioned results will be able to provide a useful knowledge for understanding the phenomena occurring within the cold-cap.
Journal Article
Single Event Effect cross section calibration and application to quasi-monoenergetic and spallation facilities
2018
We describe an approach to calibrate Single Event Effect (SEE)-based detectors in monoenergetic fields and apply the resulting semi-empiric responses to more general mixed-field cases in which a broad variety of particle species and energy spectra are present. The calibration of the response functions is based both on experimental proton (30–200 MeV) and neutron (5–300 MeV) data and considerations derived from Monte Carlo simulations using the FLUKA Monte Carlo code. The application environments include the quasi-monoenergetic neutrons at RCNP, the atmospheric-like VESUVIO spallation spectrum and the CHARM high-energy accelerator test facility. The agreement between the mixed-field response and that predicted through the mono-energetic calibration is within ±30% for the broad variety of cases considered and thus regarded as highly successful for mixed-field monitoring applications.
Journal Article