Explore the vast range of titles available.

Doppler-free saturated-absorption Lamb dips are observed for weak vibration-rotation transitions of C 2 H 2 between 7167 and 7217 cm −1 , using a frequency-comb assisted cavity ring-down spectrometer based on the use of a pair of phase-locked diode lasers. We measured the absolute center frequency of sixteen lines belonging to the 2 ν 3 + ν 5 1 band, targeting ortho and para states of the molecule. Line pairs of the P and Q branches were selected so as to form a ‘V’-scheme, sharing the lower energy level. Such a choice made it possible to determine the rotational energy separations of the excited vibrational state for J -values from 11 to 20. Line-center frequencies are determined with an overall uncertainty between 3 and 13 kHz. This is over three orders of magnitude more accurate than previous experimental studies in the spectral region around the wavelength of 1.4 μ m. The retrieved energy separations provide a stringent test of the so-called MARVEL method recently applied to acetylene.

Quantum cascade lasers (QCLs) are becoming a key tool for plenty of applications, from the mid-infrared (mid-IR) to the THz range. Progress in related areas, such as the development of ultra-low-loss crystalline microresonators, optical frequency standards, and optical fiber networks for time and frequency dissemination, is paving the way for unprecedented applications in many fields. For most demanding applications, a thorough control of QCLs emission must be achieved. In the last few years, QCLs’ unique spectral features have been unveiled, while multifrequency QCLs have been demonstrated. Ultra-narrow frequency linewidths are necessary for metrological applications, ranging from cold molecules interaction and ultra-high sensitivity spectroscopy to infrared/THz metrology. A review of the present status of research in this field is presented, with a view of perspectives and future applications.

We provide an overview on terahertz (THz) frequency metrology, starting from the nowadays available continuous wave THz sources, discussing their main features such as tunability, spectral purity, and frequency referencing to the primary frequency standards. A comparison on the achieved results in high-precision molecular spectroscopy is given and discussed, and finally, a special emphasis poses on the future developments of this upcoming field.

The realization of Coordinated Universal Time, one of the tasks of the International Bureau of Weights and Measures, relies on a network of international time links which currently is organized in a star-like scheme that links all contributing laboratories. GPS signal reception is the technique most widely employed by the laboratories. The PTB currently plays a unique role in the process due to its function as the central pivot in the time transfer between the participating laboratories. We discuss how the PTB meets its obligations to the international timekeeping community as well as to its users in Germany. In its role as an National Metrology Institute (NMI), PTB is entrusted with the realization and dissemination of legal time in Germany. The services were offered to the public support measurements and timing applications traceable to the national and international standards to be made in calibration laboratories and in many industrial sectors. We thus discuss the meaning and definition of traceability, how different GNSS systems can be used to establish traceability and their performance in doing so.

We review the progress made on the fabrication and applications of hollow-core photonic crystal fibres (HC-PCFs). The mechanism of the light guidance in these fibres is described along with their dispersion properties. We review the HC-PCF fabrication, the different results achieved in the fields of laser-induced particle guidance, low-threshold stimulated Raman scattering in hydrogen (vibrational and rotational), laser frequency metrology and quantum optics. Finally, we show the different new prospects opened up by these fibres.

Time and frequency metrology depends on stable oscillators in both radio-frequency and optical domains. With the increased complexity of the highly precise oscillators also came the demand for delivering the oscillators’ harmonic signals between delocalized sites for comparison, aggregation, or other purposes. Besides the traditional optical fiber networks, free-space optical links present an alternative tool for disseminating stable sources’ output. We present a pilot experiment of phase-coherent optical frequency transfer using a free-space optical link testbed. The experiment performed on a 30 m long link demonstrates the phase-noise parameters in a free-space optical channel under atmospheric turbulence conditions, and it studies the impact of active MEMS mirror stabilization of the received optical wave positioning on the resulting transfer’s performance. Our results indicate that a well-configured MEMS mirror beam stabilization significantly enhances fractional frequency stability, achieving the−14th-order level for integration times over 30 s.

We report the frequency stabilization of an external cavity diode laser (ECDL) to a reference molecular iodine (I2) transition at 13,531.18 cm−1 (739.03382 nm). Using the Modulation Transfer Spectroscopy (MTS) method for the highly sensitive detection of weak absorption signals, the Doppler-free absorption peaks of I2 corresponding to the hot band transition R(78) (1–11) are resolved. The ECDL’s frequency is stabilized with respect to one of the lines lying within the reference absorption band. For this, the iodine vapor cell is heated to 450 °C and the corresponding circularly polarized pump and probe beam powers are maintained at 10 mW and 1 mW, respectively, to avoid power broadening. The short (100 ms) and long-term (50 h) linewidths of the frequency stabilized laser are measured to be 0.75(3) MHz and 0.5(2) MHz, respectively, whereas the natural linewidth of the specific I2-transitions lie within a range of tens of MHz.

The appearance of the frequency comb technology, awarded the Nobel Prize in Physics 2005, has enormously revolutionized the metrology of optical frequencies, eliminating the need for complicated frequency chains. By direct linking to the unit of time, the second, through frequency standards (Cs, Rb), by using femtosecond mode-locked lasers and frequency comb technology, the Spanish Centre of Metrology (CEM) has established a new way of practical realisation of the National Standard of Length, the metre. By stabilising and characterising two free parameters – the repetition frequency fr and the offset frequency f0, the frequency comb generator thereby was successfully put into operation. After such realization, the accuracy of the length unit will be increased in two orders of magnitude, that is 2 × 10−13 instead of 2.1 × 10−11. In this paper we present the results of applying comb generator to the absolute measurement of the three Zeeman stabilized He–Ne lasers operating at 633 nm with a nominal frequency of 473.612 THz. A comparison of these results with those obtained by the current system based on standard iodine stabilized lasers is in good compatibility. A treatment for the evaluation of measurement uncertainty of laser frequency in calibration using a comb in accordance with Guide of Uncertainty Measurement ISO/BIPM is also presented.

A practical method for the absolute frequency measurement of continuous-wave terahertz (CW-THz) radiation uses a photocarrier terahertz frequency comb (PC-THz comb) because of its ability to realize real-time, precise measurement without the need for cryogenic cooling. However, the requirement for precise stabilization of the repetition frequency ( f rep ) and/or use of dual femtosecond lasers hinders its practical use. In this article, based on the fact that an equal interval between PC-THz comb modes is always maintained regardless of the fluctuation in f rep , the PC-THz comb induced by an unstabilized laser was used to determine the absolute frequency f THz of CW-THz radiation. Using an f rep -free-running PC-THz comb, the f THz of the frequency-fixed or frequency-fluctuated active frequency multiplier chain CW-THz source was determined at a measurement rate of 10 Hz with a relative accuracy of 8.2 × 10 −13 and a relative precision of 8.8 × 10 −12 to a rubidium frequency standard. Furthermore, f THz was correctly determined even when fluctuating over a range of 20 GHz. The proposed method enables the use of any commercial femtosecond laser for the absolute frequency measurement of CW-THz radiation.

Precision spectroscopy of the simple hydrogen atom has inspired dramatic advances in optical frequency metrology: femtosecond laser optical frequency comb synthesizers have revolutionized the precise measurement of optical frequencies, and they provide a reliable clock mechanism for optical atomic clocks. Precision spectroscopy of the hydrogen 1S-2S two-photon resonance has reached an accuracy of 1.4 parts in 1014, and considerable future improvements are envisioned. Such laboratory experiments are setting new limits for possible slow variations of the fine structure constant α and the magnetic moment of the caesium nucleus μ Cs in units of the Bohr magneton μ B.