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Waste-Derived Catalysts for Water Electrolysis: Circular Economy-Driven Sustainable Green Hydrogen Energy
HighlightsCritical strategies for converting wastes to catalysts are summarized.Applications of waste-derived catalysts in hydrogen evolution reaction, oxygen evolution reaction, and overall water electrolysis are comprehensively reviewed.Perspectives in the development of waste-derived catalysts are analyzed.The sustainable production of green hydrogen via water electrolysis necessitates cost-effective electrocatalysts. By following the circular economy principle, the utilization of waste-derived catalysts significantly promotes the sustainable development of green hydrogen energy. Currently, diverse waste-derived catalysts have exhibited excellent catalytic performance toward hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and overall water electrolysis (OWE). Herein, we systematically examine recent achievements in waste-derived electrocatalysts for water electrolysis. The general principles of water electrolysis and design principles of efficient electrocatalysts are discussed, followed by the illustration of current strategies for transforming wastes into electrocatalysts. Then, applications of waste-derived catalysts (i.e., carbon-based catalysts, transitional metal-based catalysts, and carbon-based heterostructure catalysts) in HER, OER, and OWE are reviewed successively. An emphasis is put on correlating the catalysts’ structure–performance relationship. Also, challenges and research directions in this booming field are finally highlighted. This review would provide useful insights into the design, synthesis, and applications of waste-derived electrocatalysts, and thus accelerate the development of the circular economy-driven green hydrogen energy scheme.
Journal Article
The hydrogen revolution : a blueprint for the future of clean energy
\"An energy expert shows why hydrogen can fight climate change and become the fuel of the future\"-- Provided by publisher
BOOK
Green hydrogen energy production: current status and potential
The technique of producing hydrogen by utilizing green and renewable energy sources is called green hydrogen production. Therefore, by implementing this technique, hydrogen will become a sustainable and clean energy source by lowering greenhouse gas emissions and reducing our reliance on fossil fuels. The key benefit of producing green hydrogen by utilizing green energy is that no harmful pollutants or greenhouse gases are directly released throughout the process. Hence, to guarantee all of the environmental advantages, it is crucial to consider the entire hydrogen supply chain, involving storage, transportation and end users. Hydrogen is a promising clean energy source and targets plan pathways towards decarbonization and net-zero emissions by 2050. This paper has highlighted the techniques for generating green hydrogen that are needed for a clean environment and sustainable energy solutions. Moreover, it summarizes an overview, outlook and energy transient of green hydrogen production. Consequently, its perspective provides new insights and research directions in order to accelerate the development and identify the potential of green hydrogen production.
Journal Article
Overview of hydrogen-resistant alloys for high-pressure hydrogen environment: on the hydrogen energy structural materials
With the progressive expansion of hydrogen fuel demand, hydrogen pipelines, hydrogen storage cylinders and hydrogen refuelling stations (HRSs) are the primary components of hydrogen energy systems that face high-pressure hydrogen environments. Hydrogen embrittlement (HE) is a typical phenomenon in metallic materials, particularly in the high-pressure hydrogen environment, that causes loss of ductility and potentially catastrophic failure. HE is associated with materials, the service environment and stress. The primary mechanisms for explaining the HE of materials are hydrogen-enhanced decohesion, hydrogen-induced phase transformation, hydrogen-enhanced local plasticity, adsorption-induced dislocation emission and hydrogen-enhanced strain-induced vacancy. To reduce the risk of HE for metallic structural materials used in hydrogen energy systems, it is crucial to reasonably select hydrogen-resistant materials for high-pressure hydrogen environments. This paper summarizes HE phenomena, mechanisms and current problems for the metallic structural materials of hydrogen energy systems. A research perspective is also proposed, mainly focusing on metal structural materials for hydrogen pipelines, hydrogen storage cylinders and hydrogen compressors in HRSs from an application perspective.
Journal Article
Transition to hydrogen : pathways toward clean transportation
\"This book is a comprehensive and objective guide to understanding hydrogen as a transportation fuel. The effects that pursuing different vehicle technology development paths will have on the economy, the environment, public safety and human health are presented with implications for policy makers, industrial stakeholders and researchers alike. Using hydrogen as a fuel offers a possible solution to satisfying global mobility needs, including sustainability of supply and the potential reduction of greenhouse gas emissions. This book focuses on research issues that are at the intersection of hydrogen and transportation, since the study of vehicles and energy-carriers is inseparable. It concentrates on light duty vehicles (cars and light trucks), set in the context of other competing technologies, the larger energy sector and the overall economy. The book is invaluable for researchers and policy makers in transportation policy, energy economics, systems dynamics, vehicle powertrain modeling and simulation, environmental science and environmental engineering\"-- Provided by publisher.
Book
Controlled growth of a high selectivity interface for seawater electrolysis
Overall seawater electrolysis is an important direction for the development of hydrogen energy conversion. The key issues include how to achieve high selectivity, activity, and stability in seawater electrolysis reactions. In this report, the heterostructures of graphdiyne-RhOₓ-graphdiyne (GDY/RhOₓ/GDY) were constructed by in situ-controlled growth of GDY on RhOx nanocrystals. A double layer interface of sp-hybridized carbon-oxide-Rhodium (sp-C∼O-Rh) was formed in this system. The microstructures at the interface are composed of active sites of sp-C∼O-Rh. The obvious electron-withdrawing surface enhances the catalytic activity with orders of magnitude, while the GDY outer of the metal oxides guarantees the stability. The electron-donating and withdrawing sp-C∼O-Rh structures enhance the catalytic activity, achieving high-performance overall seawater electrolysis with very small cell voltages of 1.42 and 1.52 V at large current densities of 10 and 500 mA cm−2 at room temperatures and ambient pressures, respectively. The compositional and structural superiority of the GDY-derived sp-C-metal-oxide active center offers great opportunities to engineer tunable redox properties and catalytic performance for seawater electrolysis and beyond. This is a typical successful example of the rational design of catalytic systems.
Journal Article
Innovations and techno-ecological transition
\"This book aims to present a systemic perspective to energetic transition to a discarbonated society implying an increase of energetic efficiency of current production process, new way of energy production -- integration of renewable energies, re-use of wastes. Main societal functions are analyzed in order to highlight the ongoing process of technological and non-technological innovations: transport and mobility, food, building. The purpose of this book is to analyze from a global perspective the energetic innovative system on building and to understand the limits of its development and potential new actions.\" -- Publisher's website.
Book
Self-Consistent Multi-Energy Flow Coordination Optimization for Hydrogen Energy Railway with Tank Car in Hydrogen Energy Parks
The multi-energy flow coordination optimization of the self-sufficient hydrogen energy park is becoming a research focus. However, without explicit consideration of tank car, the optimization remains incomplete, thereby undermining practical applicability. In this paper, a Dynamic Adaptive Grey Wolf Optimization (DA-GWO) algorithm is proposed for self-consistent multi-energy flow coordination optimization, considering hydrogen energy-based tank cars in hydrogen railway energy parks. First, a foundational model of the hydrogen-based railway energy system was constructed that integrates green non-dispatchable units such as wind power and photovoltaics, as well as dispatchable units such as fuel cells, gas boilers, and cogeneration units. Given the diversity and complexity of in-service hydrogen railway tank cars, a probabilistic model of daily charging behaviour was constructed using a Monte Carlo method to simulate real-world operating conditions of tank cars, thereby enhancing the reliability of the hydrogen-powered railway model. Considering the diverse and complex units in the self-consistent hydrogen energy park for hydrogen-powered railways, a DA-GWO algorithm was constructed for the multi-energy flow optimization. Through a self-adaptive parameter adjustment, the algorithm’s global optimization performance is improved. Finally, the model parameters were further adjusted with data from a coastal Chinese city, and the optimization experimental tests were conducted to validate the proposed method. From the results, the proposed method can save at least 6.7% cost compared with the grey wolf optimization method and the PSO (Particle Swarm Optimization) optimization method.
Journal Article